Articles | Volume 20, issue 13
https://doi.org/10.5194/acp-20-7875-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-20-7875-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
08 Jul 2020
Research article |
| 08 Jul 2020
| 08 Jul 2020
A 1-year characterization of organic aerosol composition and sources using an extractive electrospray ionization time-of-flight mass spectrometer (EESI-TOF)
Lu Qi
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI),
5232 Villigen, Switzerland
Collaborative Innovation Center of Atmospheric Environment and
Equipment Technology, Nanjing University of Information Science &
Technology, Nanjing, 210044, China
Alexander L. Vogel
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI),
5232 Villigen, Switzerland
now at: Institute for Atmospheric and Environmental Sciences, Goethe
University, Frankfurt am Main, Germany
Sepideh Esmaeilirad
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI),
5232 Villigen, Switzerland
Liming Cao
Key Laboratory for Urban Habitat Environmental Science and Technology,
School of Environment and Energy, Peking University Shenzhen Graduate
School, Shenzhen, 518055, China
Jing Zheng
State Key Joint Laboratory of Environmental Simulation and Pollution
Control, College of Environmental Sciences and Engineering, Peking
University, Beijing, 100871, China
Jean-Luc Jaffrezo
University Grenoble Alpes, CNRS, IGE, 38000 Grenoble, France
Paola Fermo
Department of Chemistry, University of Milan, 20133 Milan, Italy
Anne Kasper-Giebl
Institute of Chemical Technologies and Analytics, Vienna University of
Technology, 1060 Vienna, Austria
Kaspar R. Daellenbach
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI),
5232 Villigen, Switzerland
now at: Institute for Atmospheric and Earth System Research,
University of Helsinki, Helsinki, Finland
Mindong Chen
Collaborative Innovation Center of Atmospheric Environment and
Equipment Technology, Nanjing University of Information Science &
Technology, Nanjing, 210044, China
Xinlei Ge
Collaborative Innovation Center of Atmospheric Environment and
Equipment Technology, Nanjing University of Information Science &
Technology, Nanjing, 210044, China
Urs Baltensperger
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI),
5232 Villigen, Switzerland
André S. H. Prévôt
CORRESPONDING AUTHOR
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI),
5232 Villigen, Switzerland
Jay G. Slowik
CORRESPONDING AUTHOR
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI),
5232 Villigen, Switzerland
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Cited
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- A multi-instrumental approach for calibrating real-time mass spectrometers using high-performance liquid chromatography and positive matrix factorization M. Schueneman et al. 10.5194/ar-2-59-2024
- Chemical Characterization of Rural Organic Aerosol in the North China Plain Using Ultrahigh-Resolution Mass Spectrometry Y. Zhang et al. 10.3390/atmos14111636
- Seasonal characterization of chemical and optical properties of water-soluble organic aerosol in Beijing B. You et al. 10.1016/j.scitotenv.2024.172508
- Organic aerosol sources in the Milan metropolitan area – Receptor modelling based on field observations and air quality modelling K. Daellenbach et al. 10.1016/j.atmosenv.2023.119799
- Long-Term Studies of Biological Components of Atmospheric Aerosol: Trends and Variability A. Safatov et al. 10.3390/atmos13050651
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- Characterizing the Sources of Ambient PM10 Organic Aerosol in Urban and Rural Catalonia, Spain M. in 't Veld et al. 10.2139/ssrn.4463228
- Characterizing the sources of ambient PM10 organic aerosol in urban and rural Catalonia, Spain M. in 't Veld et al. 10.1016/j.scitotenv.2023.166440
- Composition and Sources of Organic Aerosol in Two Megacities in Western China Using Complementary Mass Spectrometric and Statistical Techniques T. Cui et al. 10.1021/acsestair.4c00051
- Identification and semi-quantification of nitrooxy organosulfates in aerosol particles by HPLC-MS/MS W. Li et al. 10.1039/D2AY00460G
- Variations and Sources of Organic Aerosol in Winter Beijing under Markedly Reduced Anthropogenic Activities During COVID-2019 R. Hu et al. 10.1021/acs.est.1c05125
- Singlet Oxygen Seasonality in Aqueous PM10 is Driven by Biomass Burning and Anthropogenic Secondary Organic Aerosol S. Bogler et al. 10.1021/acs.est.2c04554
- Applications of environmental mass spectrometry in atmospheric haze chemistry T. Chen et al. 10.1016/j.trac.2024.117614
- Highly time-resolved chemical speciation and source apportionment of organic aerosol components in Delhi, India, using extractive electrospray ionization mass spectrometry V. Kumar et al. 10.5194/acp-22-7739-2022
- Chemical ionization mass spectrometry: Developments and applications for on-line characterization of atmospheric aerosols and trace gases Y. Zhang et al. 10.1016/j.trac.2023.117353
- Mass spectrometry-based Aerosolomics: a new approach to resolve sources, composition, and partitioning of secondary organic aerosol M. Thoma et al. 10.5194/amt-15-7137-2022
- A 1-year aerosol chemical speciation monitor (ACSM) source analysis of organic aerosol particle contributions from anthropogenic sources after long-range transport at the TROPOS research station Melpitz S. Atabakhsh et al. 10.5194/acp-23-6963-2023
- Chemical composition and sources of organic aerosol on the Adriatic coast in Croatia R. Casotto et al. 10.1016/j.aeaoa.2022.100159
- Molecular Characterization of Water-Soluble Brown Carbon Chromophores in Snowpack from Northern Xinjiang, China Y. Zhou et al. 10.1021/acs.est.1c07972
- Composition and sources of carbonaceous aerosol in the European Arctic at Zeppelin Observatory, Svalbard (2017 to 2020) K. Yttri et al. 10.5194/acp-24-2731-2024
22 citations as recorded by crossref.
- Recent advances in mass spectrometry techniques for atmospheric chemistry research on molecular‐level W. Zhang et al. 10.1002/mas.21857
- A multi-instrumental approach for calibrating real-time mass spectrometers using high-performance liquid chromatography and positive matrix factorization M. Schueneman et al. 10.5194/ar-2-59-2024
- Chemical Characterization of Rural Organic Aerosol in the North China Plain Using Ultrahigh-Resolution Mass Spectrometry Y. Zhang et al. 10.3390/atmos14111636
- Seasonal characterization of chemical and optical properties of water-soluble organic aerosol in Beijing B. You et al. 10.1016/j.scitotenv.2024.172508
- Organic aerosol sources in the Milan metropolitan area – Receptor modelling based on field observations and air quality modelling K. Daellenbach et al. 10.1016/j.atmosenv.2023.119799
- Long-Term Studies of Biological Components of Atmospheric Aerosol: Trends and Variability A. Safatov et al. 10.3390/atmos13050651
- Quantification of primary and secondary organic aerosol sources by combined factor analysis of extractive electrospray ionisation and aerosol mass spectrometer measurements (EESI-TOF and AMS) Y. Tong et al. 10.5194/amt-15-7265-2022
- Influence of organic aerosol molecular composition on particle absorptive properties in autumn Beijing J. Cai et al. 10.5194/acp-22-1251-2022
- Characterizing the Sources of Ambient PM10 Organic Aerosol in Urban and Rural Catalonia, Spain M. in 't Veld et al. 10.2139/ssrn.4463228
- Characterizing the sources of ambient PM10 organic aerosol in urban and rural Catalonia, Spain M. in 't Veld et al. 10.1016/j.scitotenv.2023.166440
- Composition and Sources of Organic Aerosol in Two Megacities in Western China Using Complementary Mass Spectrometric and Statistical Techniques T. Cui et al. 10.1021/acsestair.4c00051
- Identification and semi-quantification of nitrooxy organosulfates in aerosol particles by HPLC-MS/MS W. Li et al. 10.1039/D2AY00460G
- Variations and Sources of Organic Aerosol in Winter Beijing under Markedly Reduced Anthropogenic Activities During COVID-2019 R. Hu et al. 10.1021/acs.est.1c05125
- Singlet Oxygen Seasonality in Aqueous PM10 is Driven by Biomass Burning and Anthropogenic Secondary Organic Aerosol S. Bogler et al. 10.1021/acs.est.2c04554
- Applications of environmental mass spectrometry in atmospheric haze chemistry T. Chen et al. 10.1016/j.trac.2024.117614
- Highly time-resolved chemical speciation and source apportionment of organic aerosol components in Delhi, India, using extractive electrospray ionization mass spectrometry V. Kumar et al. 10.5194/acp-22-7739-2022
- Chemical ionization mass spectrometry: Developments and applications for on-line characterization of atmospheric aerosols and trace gases Y. Zhang et al. 10.1016/j.trac.2023.117353
- Mass spectrometry-based Aerosolomics: a new approach to resolve sources, composition, and partitioning of secondary organic aerosol M. Thoma et al. 10.5194/amt-15-7137-2022
- A 1-year aerosol chemical speciation monitor (ACSM) source analysis of organic aerosol particle contributions from anthropogenic sources after long-range transport at the TROPOS research station Melpitz S. Atabakhsh et al. 10.5194/acp-23-6963-2023
- Chemical composition and sources of organic aerosol on the Adriatic coast in Croatia R. Casotto et al. 10.1016/j.aeaoa.2022.100159
- Molecular Characterization of Water-Soluble Brown Carbon Chromophores in Snowpack from Northern Xinjiang, China Y. Zhou et al. 10.1021/acs.est.1c07972
- Composition and sources of carbonaceous aerosol in the European Arctic at Zeppelin Observatory, Svalbard (2017 to 2020) K. Yttri et al. 10.5194/acp-24-2731-2024
Latest update: 20 Nov 2024
Short summary
We present the first application of this online and offline strategy using the new extractive electrospray ionization time-of-flight mass spectrometer (EESI-TOF), which achieves increased chemical specificity relative to other online techniques. Measurement and source apportionment of 1 year of filter samples collected in Zurich, Switzerland, show seasonal contributions from fresh and aged wood combustion in winter and biogenic emission-derived SOA in summer, as well as other sources.
We present the first application of this online and offline strategy using the new extractive...
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