Articles | Volume 20, issue 12
https://doi.org/10.5194/acp-20-7259-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue:
https://doi.org/10.5194/acp-20-7259-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Importance of gas-particle partitioning of ammonia in haze formation in the rural agricultural environment
Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention (LAP3), Department of Environmental Science and Engineering,
Fudan University, Shanghai, 200433, China
Jia Chen
Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention (LAP3), Department of Environmental Science and Engineering,
Fudan University, Shanghai, 200433, China
Na Zhao
Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention (LAP3), Department of Environmental Science and Engineering,
Fudan University, Shanghai, 200433, China
Guochen Wang
Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention (LAP3), Department of Environmental Science and Engineering,
Fudan University, Shanghai, 200433, China
Guangyuan Yu
Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention (LAP3), Department of Environmental Science and Engineering,
Fudan University, Shanghai, 200433, China
Hao Li
Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention (LAP3), Department of Environmental Science and Engineering,
Fudan University, Shanghai, 200433, China
Juntao Huo
Shanghai Environmental Monitoring Center, Shanghai, 200030, China
Yanfen Lin
Shanghai Environmental Monitoring Center, Shanghai, 200030, China
Qingyan Fu
Shanghai Environmental Monitoring Center, Shanghai, 200030, China
Hongyu Guo
Cooperative Institute for Research in Environmental Sciences and
Department of Chemistry, University of Colorado, Boulder, Colorado 80309,
USA
Congrui Deng
Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention (LAP3), Department of Environmental Science and Engineering,
Fudan University, Shanghai, 200433, China
Shan-Hu Lee
Department of Atmospheric Science, University of Alabama in
Huntsville, Huntsville, Alabama 35758, USA
Jianmin Chen
Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention (LAP3), Department of Environmental Science and Engineering,
Fudan University, Shanghai, 200433, China
Kan Huang
CORRESPONDING AUTHOR
Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention (LAP3), Department of Environmental Science and Engineering,
Fudan University, Shanghai, 200433, China
Institute of Eco-Chongming (IEC), No.20 Cuiniao Road, Chen Jiazhen,
Shanghai, 202162, China
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37 citations as recorded by crossref.
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- Secondary inorganic aerosols and aerosol acidity at different PM2.5 pollution levels during winter haze episodes in the Sichuan Basin, China X. Fu et al. 10.1016/j.scitotenv.2024.170512
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- Identifying the reaction network complexity and structure sensitivity of selective catalytic oxidation of ammonia over Ag surfaces K. Yang & B. Yang 10.1016/j.apsusc.2022.152584
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- Formation of droplet-mode secondary inorganic aerosol dominated the increased PM2.5 during both local and transport haze episodes in Zhengzhou, China S. Wang et al. 10.1016/j.chemosphere.2020.128744
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- Nitrate formation and iron dissolution in the heterogeneous reactions of NH3 on nano α-Fe2O3 R. Wang et al. 10.1039/D3EN00494E
- Precipitation frequency controls nitrogenous aerosol in a tropical coastal city and its implications for plant carbon sequestration X. Zhou et al. 10.1016/j.chemosphere.2023.138473
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36 citations as recorded by crossref.
- Contribution of chemical composition to oxidative potential of atmospheric particles at a rural and an urban site in the Po Valley: Influence of high ammonia agriculture emissions M. Pietrogrande et al. 10.1016/j.atmosenv.2023.120203
- Quantitative Decomposition of Influencing Factors to Aerosol pH Variation over the Coasts of the South China Sea, East China Sea, and Bohai Sea G. Wang et al. 10.1021/acs.estlett.2c00527
- Atmospheric Pollution of Agriculture-Dominated Cities L. Guo & W. Chen 10.3390/atmos13060900
- Thermodynamical framework for effective mitigation of high aerosol loading in the Indo-Gangetic Plain during winter P. Acharja et al. 10.1038/s41598-023-40657-w
- Mechanism-based structure-activity relationship investigation on hydrolysis kinetics of atmospheric organic nitrates Q. Zhao et al. 10.1038/s41612-023-00517-w
- New insights into the formation of ammonium nitrate from a physical and chemical level perspective Y. Wei et al. 10.1007/s11783-023-1737-6
- Biomass burning related ammonia emissions promoted a self-amplifying loop in the urban environment in Kunming (SW China) Y. Zhou et al. 10.1016/j.atmosenv.2020.118138
- Secondary inorganic aerosols and aerosol acidity at different PM2.5 pollution levels during winter haze episodes in the Sichuan Basin, China X. Fu et al. 10.1016/j.scitotenv.2024.170512
- Measurement report: Elevated atmospheric ammonia may promote particle pH and HONO formation – insights from the COVID-19 pandemic X. Zhang et al. 10.5194/acp-24-9885-2024
- Secondary aerosol formation during a special dust transport event: impacts from unusually enhanced ozone and dust backflows over the ocean D. Lu et al. 10.5194/acp-23-13853-2023
- Modeling of reducing NH4NO3 in PM2.5 under high ammonia emission in urban areas: Based on high-resolution data N. Jiang et al. 10.1016/j.jclepro.2022.131499
- Monitoring ammonia concentrations in more than 10 stations in the Po Valley for the period 2007–2022 in relation to the evolution of different sources C. Colombi et al. 10.3389/fenvh.2024.1249457
- Chloride (HCl ∕ Cl−) dominates inorganic aerosol formation from ammonia in the Indo-Gangetic Plain during winter: modeling and comparison with observations P. Pawar et al. 10.5194/acp-23-41-2023
- Role of gas-particle conversion of ammonia in haze pollution under ammonia-rich environment in Northern China and prospects of effective emission reduction X. Zou et al. 10.1016/j.scitotenv.2024.173277
- Distribution of Air pollutant Concentration and Ammonium conversion rate in Livestock Areas: Focusing on Boryeong J. Kim et al. 10.4491/KSEE.2024.46.10.559
- Ammonia and PM2.5 Air Pollution in Paris during the 2020 COVID Lockdown C. Viatte et al. 10.3390/atmos12020160
- δ15N-stable isotope analysis of NHx: An overview on analytical measurements, source sampling and its source apportionment N. Bhattarai et al. 10.1007/s11783-021-1414-6
- Identifying the reaction network complexity and structure sensitivity of selective catalytic oxidation of ammonia over Ag surfaces K. Yang & B. Yang 10.1016/j.apsusc.2022.152584
- Atmospheric Processing at the Sea‐Land Interface Over the South China Sea: Secondary Aerosol Formation, Aerosol Acidity, and Role of Sea Salts G. Wang et al. 10.1029/2021JD036255
- Potential Impacts of Energy and Vehicle Transformation Through 2050 on Oxidative Stress‐Inducing PM2.5 Metals Concentration in Japan S. Kayaba & M. Kajino 10.1029/2023GH000789
- Continuous Measurement and Molecular Compositions of Atmospheric Water‐Soluble Brown Carbon in the Nearshore Marine Boundary Layer of Northern China: Secondary Formation and Influencing Factors H. Li et al. 10.1029/2023JD038565
- Insights into high concentrations of particle-bound imidazoles in the background atmosphere of southern China: Potential sources and influencing factors C. He et al. 10.1016/j.scitotenv.2021.150804
- PM2.5 and water-soluble inorganic ion concentrations decreased faster in urban than rural areas in China Y. Zhang et al. 10.1016/j.jes.2021.09.031
- Strategic control of combustion-induced ammonia emissions: A key initiative for substantial PM2.5 reduction in Tianjin, North China Plain H. Xiao et al. 10.1016/j.scitotenv.2024.172328
- Comparative multi-model study of PM2.5 acidity trend changes in ammonia-rich regions in winter: Based on a new ammonia concentration assessment method Y. Wei et al. 10.1016/j.jhazmat.2023.131970
- Characteristics and sources of atmospheric ammonia at the SORPES station in the western Yangtze river delta of China R. Liu et al. 10.1016/j.atmosenv.2023.120234
- Investigating the convective transport possibilities of lower-atmospheric pollutants to the UTLS region using rainwater and aerosol chemical characterization C. Jain et al. 10.1016/j.apr.2024.102225
- Formation of droplet-mode secondary inorganic aerosol dominated the increased PM2.5 during both local and transport haze episodes in Zhengzhou, China S. Wang et al. 10.1016/j.chemosphere.2020.128744
- Atmospheric ammonia and its effect on PM2.5 pollution in urban Chengdu, Sichuan Basin, China X. Huang et al. 10.1016/j.envpol.2021.118195
- Evaluation of the ammonia emission sensitivity of secondary inorganic aerosol concentrations measured by the national reference method J. Lim et al. 10.1016/j.atmosenv.2021.118903
- May SARS-CoV-2 Diffusion Be Favored by Alkaline Aerosols and Ammonia Emissions? M. Manigrasso et al. 10.3390/atmos11090995
- Impact of Gaseous Pollutants Reduction on Fine Particulate Matter and Its Secondary Inorganic Aerosols in Beijing–Tianjin–Hebei Region Z. Wei & N. Mohamed Tahrin 10.3390/atmos14061027
- Daytime and nighttime aerosol soluble iron formation in clean and slightly polluted moist air in a coastal city in eastern China W. Li et al. 10.5194/acp-24-6495-2024
- Role of ammonia in secondary inorganic aerosols formation at an ammonia-rich city in winter in north China: A comparative study among industry, urban, and rural sites X. Duan et al. 10.1016/j.envpol.2021.118151
- Nitrate formation and iron dissolution in the heterogeneous reactions of NH3 on nano α-Fe2O3 R. Wang et al. 10.1039/D3EN00494E
- Precipitation frequency controls nitrogenous aerosol in a tropical coastal city and its implications for plant carbon sequestration X. Zhou et al. 10.1016/j.chemosphere.2023.138473
Latest update: 20 Nov 2024
Short summary
This study provided evidence that gas-particle partitioning of ammonia, as opposed to ammonia concentration, plays a critical role in the haze formation. A reduction in ammonia emissions alone may not reduce air pollution effectively, at least at rural agricultural sites in China.
This study provided evidence that gas-particle partitioning of ammonia, as opposed to ammonia...
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