Articles | Volume 20, issue 11
https://doi.org/10.5194/acp-20-6357-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-20-6357-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
03 Jun 2020
Research article |
| 03 Jun 2020
| 03 Jun 2020
Photochemical transformation of residential wood combustion emissions: dependence of organic aerosol composition on OH exposure
Department of Environmental and Biological Sciences, University of
Eastern Finland, Kuopio, 70211, Finland
Petri Tiitta
Department of Environmental and Biological Sciences, University of
Eastern Finland, Kuopio, 70211, Finland
currently at: Finnish Meteorological Institute, Atmospheric Research Centre of Eastern Finland, P.O. Box 1627, 70211 Kuopio
Mika Ihalainen
Department of Environmental and Biological Sciences, University of
Eastern Finland, Kuopio, 70211, Finland
Pasi Yli-Pirilä
Department of Environmental and Biological Sciences, University of
Eastern Finland, Kuopio, 70211, Finland
Jürgen Orasche
Joint Mass Spectrometry Centre, Comprehensive Molecular Analytics,
Helmholtz Zentrum München, 85764 Neuherberg, Germany
Hendryk Czech
Department of Environmental and Biological Sciences, University of
Eastern Finland, Kuopio, 70211, Finland
Joint Mass Spectrometry Centre, Comprehensive Molecular Analytics,
Helmholtz Zentrum München, 85764 Neuherberg, Germany
Joint Mass Spectrometry Centre, Institute of Chemistry, University of Rostock, 18059 Rostock, Germany
Miika Kortelainen
Department of Environmental and Biological Sciences, University of
Eastern Finland, Kuopio, 70211, Finland
Heikki Lamberg
Department of Environmental and Biological Sciences, University of
Eastern Finland, Kuopio, 70211, Finland
Heikki Suhonen
Department of Environmental and Biological Sciences, University of
Eastern Finland, Kuopio, 70211, Finland
Hanna Koponen
Department of Environmental and Biological Sciences, University of
Eastern Finland, Kuopio, 70211, Finland
Liqing Hao
Department of Applied Physics, University of Eastern Finland,
Kuopio, 70211, Finland
Ralf Zimmermann
Joint Mass Spectrometry Centre, Comprehensive Molecular Analytics,
Helmholtz Zentrum München, 85764 Neuherberg, Germany
Joint Mass Spectrometry Centre, Institute of Chemistry, University of Rostock, 18059 Rostock, Germany
Jorma Jokiniemi
Department of Environmental and Biological Sciences, University of
Eastern Finland, Kuopio, 70211, Finland
Jarkko Tissari
Department of Environmental and Biological Sciences, University of
Eastern Finland, Kuopio, 70211, Finland
Olli Sippula
Department of Environmental and Biological Sciences, University of
Eastern Finland, Kuopio, 70211, Finland
Department of Chemistry, University of Eastern Finland, Joensuu,
80101, Finland
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Cited
17 citations as recorded by crossref.
- Interfacial Dark Aging Is an Overlooked Source of Aqueous Secondary Organic Aerosol F. Zhang et al. 10.3390/atmos13020188
- Modeling atmospheric aging of small-scale wood combustion emissions: distinguishing causal effects from non-causal associations V. Leinonen et al. 10.1039/D2EA00048B
- Technical note: Emission factors, chemical composition, and morphology of particles emitted from Euro 5 diesel and gasoline light-duty vehicles during transient cycles E. Kostenidou et al. 10.5194/acp-21-4779-2021
- Chemical source profiles of particulate matter and gases emitted from solid fuels for residential cooking and heating scenarios in Qinghai-Tibetan Plateau J. Sun et al. 10.1016/j.envpol.2021.117503
- Carbonaceous aerosol composition in air masses influenced by large-scale biomass burning: a case study in northwestern Vietnam D. Nguyen et al. 10.5194/acp-21-8293-2021
- Effect of Atmospheric Aging on Soot Particle Toxicity in Lung Cell Models at the Air–Liquid Interface: Differential Toxicological Impacts of Biogenic and Anthropogenic Secondary Organic Aerosols (SOAs) S. Offer et al. 10.1289/EHP9413
- Contribution of brown carbon to light absorption in emissions of European residential biomass combustion appliances S. Basnet et al. 10.5194/acp-24-3197-2024
- Cyclic Ion Mobility Spectrometry Coupled to High-Resolution Time-of-Flight Mass Spectrometry Equipped with Atmospheric Solid Analysis Probe for the Molecular Characterization of Combustion Particulate Matter C. Rüger et al. 10.1021/jasms.0c00274
- Highly oxidized organic aerosols in Beijing: Possible contribution of aqueous-phase chemistry Z. Feng et al. 10.1016/j.atmosenv.2022.118971
- Chemical composition of PM<sub>2.5</sub> in October 2017 Northern California wildfire plumes Y. Liang et al. 10.5194/acp-21-5719-2021
- Hyper-fast gas chromatography and single-photon ionisation time-of-flight mass spectrometry with integrated electrical modulator-based sampling for headspace and online VOC analyses C. Gehm et al. 10.1039/D1AN00114K
- Photochemical Aging Induces Changes in the Effective Densities, Morphologies, and Optical Properties of Combustion Aerosol Particles J. Leskinen et al. 10.1021/acs.est.2c04151
- Photochemical aging process on PM2.5 bound PAHs emission from solid fuel combustion in traditional and improved stoves Y. Zhang et al. 10.1016/j.atmosres.2021.105807
- Novel fine particle reduction method for wood stoves based on high-temperature electric collection of naturally charged soot particles H. Suhonen et al. 10.1016/j.jclepro.2021.127831
- A new oxidation flow reactor for the measurements of secondary aerosol formation: Characterisation and a case study C. Wu et al. 10.1016/j.atmosenv.2023.119886
- Wildfire plume ageing in the Photochemical Large Aerosol Chamber (PHOTO-LAC) H. Czech et al. 10.1039/D3EM00280B
- Volatility Measurements of Oxygenated Volatile Organics from Fresh and Aged Residential Wood Burning Emissions M. Priestley et al. 10.1021/acsearthspacechem.3c00066
16 citations as recorded by crossref.
- Interfacial Dark Aging Is an Overlooked Source of Aqueous Secondary Organic Aerosol F. Zhang et al. 10.3390/atmos13020188
- Modeling atmospheric aging of small-scale wood combustion emissions: distinguishing causal effects from non-causal associations V. Leinonen et al. 10.1039/D2EA00048B
- Technical note: Emission factors, chemical composition, and morphology of particles emitted from Euro 5 diesel and gasoline light-duty vehicles during transient cycles E. Kostenidou et al. 10.5194/acp-21-4779-2021
- Chemical source profiles of particulate matter and gases emitted from solid fuels for residential cooking and heating scenarios in Qinghai-Tibetan Plateau J. Sun et al. 10.1016/j.envpol.2021.117503
- Carbonaceous aerosol composition in air masses influenced by large-scale biomass burning: a case study in northwestern Vietnam D. Nguyen et al. 10.5194/acp-21-8293-2021
- Effect of Atmospheric Aging on Soot Particle Toxicity in Lung Cell Models at the Air–Liquid Interface: Differential Toxicological Impacts of Biogenic and Anthropogenic Secondary Organic Aerosols (SOAs) S. Offer et al. 10.1289/EHP9413
- Contribution of brown carbon to light absorption in emissions of European residential biomass combustion appliances S. Basnet et al. 10.5194/acp-24-3197-2024
- Cyclic Ion Mobility Spectrometry Coupled to High-Resolution Time-of-Flight Mass Spectrometry Equipped with Atmospheric Solid Analysis Probe for the Molecular Characterization of Combustion Particulate Matter C. Rüger et al. 10.1021/jasms.0c00274
- Highly oxidized organic aerosols in Beijing: Possible contribution of aqueous-phase chemistry Z. Feng et al. 10.1016/j.atmosenv.2022.118971
- Chemical composition of PM<sub>2.5</sub> in October 2017 Northern California wildfire plumes Y. Liang et al. 10.5194/acp-21-5719-2021
- Hyper-fast gas chromatography and single-photon ionisation time-of-flight mass spectrometry with integrated electrical modulator-based sampling for headspace and online VOC analyses C. Gehm et al. 10.1039/D1AN00114K
- Photochemical Aging Induces Changes in the Effective Densities, Morphologies, and Optical Properties of Combustion Aerosol Particles J. Leskinen et al. 10.1021/acs.est.2c04151
- Photochemical aging process on PM2.5 bound PAHs emission from solid fuel combustion in traditional and improved stoves Y. Zhang et al. 10.1016/j.atmosres.2021.105807
- Novel fine particle reduction method for wood stoves based on high-temperature electric collection of naturally charged soot particles H. Suhonen et al. 10.1016/j.jclepro.2021.127831
- A new oxidation flow reactor for the measurements of secondary aerosol formation: Characterisation and a case study C. Wu et al. 10.1016/j.atmosenv.2023.119886
- Wildfire plume ageing in the Photochemical Large Aerosol Chamber (PHOTO-LAC) H. Czech et al. 10.1039/D3EM00280B
Latest update: 24 Apr 2024
Short summary
Residential wood combustion emits large amounts of organic compounds, which are transformed in the atmosphere via photochemical ageing reactions. We assessed this organic emission at various stages of exposure with an oxidation flow reactor. Ageing led to major changes in both gaseous and particulate phases including increased acidic compounds and transformation of the polycyclic aromatic compounds. Such changes have serious implications for the health- and climate-related effects of combustion.
Residential wood combustion emits large amounts of organic compounds, which are transformed in...
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