Articles | Volume 20, issue 11
https://doi.org/10.5194/acp-20-6357-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-20-6357-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Photochemical transformation of residential wood combustion emissions: dependence of organic aerosol composition on OH exposure
Department of Environmental and Biological Sciences, University of
Eastern Finland, Kuopio, 70211, Finland
Petri Tiitta
Department of Environmental and Biological Sciences, University of
Eastern Finland, Kuopio, 70211, Finland
currently at: Finnish Meteorological Institute, Atmospheric Research Centre of Eastern Finland, P.O. Box 1627, 70211 Kuopio
Mika Ihalainen
Department of Environmental and Biological Sciences, University of
Eastern Finland, Kuopio, 70211, Finland
Pasi Yli-Pirilä
Department of Environmental and Biological Sciences, University of
Eastern Finland, Kuopio, 70211, Finland
Jürgen Orasche
Joint Mass Spectrometry Centre, Comprehensive Molecular Analytics,
Helmholtz Zentrum München, 85764 Neuherberg, Germany
Hendryk Czech
Department of Environmental and Biological Sciences, University of
Eastern Finland, Kuopio, 70211, Finland
Joint Mass Spectrometry Centre, Comprehensive Molecular Analytics,
Helmholtz Zentrum München, 85764 Neuherberg, Germany
Joint Mass Spectrometry Centre, Institute of Chemistry, University of Rostock, 18059 Rostock, Germany
Miika Kortelainen
Department of Environmental and Biological Sciences, University of
Eastern Finland, Kuopio, 70211, Finland
Heikki Lamberg
Department of Environmental and Biological Sciences, University of
Eastern Finland, Kuopio, 70211, Finland
Heikki Suhonen
Department of Environmental and Biological Sciences, University of
Eastern Finland, Kuopio, 70211, Finland
Hanna Koponen
Department of Environmental and Biological Sciences, University of
Eastern Finland, Kuopio, 70211, Finland
Liqing Hao
Department of Applied Physics, University of Eastern Finland,
Kuopio, 70211, Finland
Ralf Zimmermann
Joint Mass Spectrometry Centre, Comprehensive Molecular Analytics,
Helmholtz Zentrum München, 85764 Neuherberg, Germany
Joint Mass Spectrometry Centre, Institute of Chemistry, University of Rostock, 18059 Rostock, Germany
Jorma Jokiniemi
Department of Environmental and Biological Sciences, University of
Eastern Finland, Kuopio, 70211, Finland
Jarkko Tissari
Department of Environmental and Biological Sciences, University of
Eastern Finland, Kuopio, 70211, Finland
Olli Sippula
Department of Environmental and Biological Sciences, University of
Eastern Finland, Kuopio, 70211, Finland
Department of Chemistry, University of Eastern Finland, Joensuu,
80101, Finland
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Short summary
Residential wood combustion emits large amounts of organic compounds, which are transformed in the atmosphere via photochemical ageing reactions. We assessed this organic emission at various stages of exposure with an oxidation flow reactor. Ageing led to major changes in both gaseous and particulate phases including increased acidic compounds and transformation of the polycyclic aromatic compounds. Such changes have serious implications for the health- and climate-related effects of combustion.
Residential wood combustion emits large amounts of organic compounds, which are transformed in...
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