Articles | Volume 20, issue 10
https://doi.org/10.5194/acp-20-6115-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-20-6115-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
26 May 2020
Research article |
| 26 May 2020
| 26 May 2020
Molecular composition and photochemical evolution of water-soluble organic carbon (WSOC) extracted from field biomass burning aerosols using high-resolution mass spectrometry
Jing Cai
State Key Laboratory of Organic Geochemistry, Guangdong Key Laboratory of Environment and Resources, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou, 510640, China
University of Chinese Academy of Sciences, Beijing, 100049, China
Xiangying Zeng
State Key Laboratory of Organic Geochemistry, Guangdong Key Laboratory of Environment and Resources, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou, 510640, China
Guorui Zhi
State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Sciences, Beijing, 100012, China
Sasho Gligorovski
State Key Laboratory of Organic Geochemistry, Guangdong Key Laboratory of Environment and Resources, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou, 510640, China
Guoying Sheng
State Key Laboratory of Organic Geochemistry, Guangdong Key Laboratory of Environment and Resources, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou, 510640, China
Zhiqiang Yu
CORRESPONDING AUTHOR
State Key Laboratory of Organic Geochemistry, Guangdong Key Laboratory of Environment and Resources, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou, 510640, China
Xinming Wang
State Key Laboratory of Organic Geochemistry, Guangdong Key Laboratory of Environment and Resources, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou, 510640, China
Ping'an Peng
State Key Laboratory of Organic Geochemistry, Guangdong Key Laboratory of Environment and Resources, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou, 510640, China
Viewed
Total article views: 3,150 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 14 Oct 2019)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 2,161 | 935 | 54 | 3,150 | 663 | 59 | 101 |
- HTML: 2,161
- PDF: 935
- XML: 54
- Total: 3,150
- Supplement: 663
- BibTeX: 59
- EndNote: 101
Total article views: 2,481 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 26 May 2020)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 1,764 | 671 | 46 | 2,481 | 439 | 52 | 93 |
- HTML: 1,764
- PDF: 671
- XML: 46
- Total: 2,481
- Supplement: 439
- BibTeX: 52
- EndNote: 93
Total article views: 669 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 14 Oct 2019)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 397 | 264 | 8 | 669 | 224 | 7 | 8 |
- HTML: 397
- PDF: 264
- XML: 8
- Total: 669
- Supplement: 224
- BibTeX: 7
- EndNote: 8
Viewed (geographical distribution)
Total article views: 3,150 (including HTML, PDF, and XML)
Thereof 3,059 with geography defined
and 91 with unknown origin.
Total article views: 2,481 (including HTML, PDF, and XML)
Thereof 2,452 with geography defined
and 29 with unknown origin.
Total article views: 669 (including HTML, PDF, and XML)
Thereof 607 with geography defined
and 62 with unknown origin.
| Country | # | Views | % |
|---|
| Country | # | Views | % |
|---|
| Country | # | Views | % |
|---|
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
Cited
30 citations as recorded by crossref.
- Research progress on the characteristics, sources, and environmental and potential health effects of water-soluble organic compounds in atmospheric particulate matter L. Wang et al. 10.1007/s11356-023-31723-x
- Characterizing water-soluble brown carbon in fine particles in four typical cities in northwestern China during wintertime: integrating optical properties with chemical processes M. Zhong et al. 10.5194/acp-23-12609-2023
- Investigation of the Mechanism of Oxidative Potential Increase in Atmospheric Particulate Matter during Photoaging: Important Role of Aromatic Nitrogenous Compounds Q. Wang et al. 10.1021/acs.est.4c03199
- Molecular characterization of nitrogen-containing organic compounds in the winter North China Plain J. Mao et al. 10.1016/j.scitotenv.2022.156189
- Impact of combustion-derived black carbon oxidation states on optical properties and cellular metabolomics in HeLa cells: Insights into soot organics J. Yan et al. 10.1016/j.atmosenv.2023.120118
- Humic-like Substances (HULIS) in Ship Engine Emissions: Molecular Composition Effected by Fuel Type, Engine Mode, and Wet Scrubber Usage E. Schneider et al. 10.1021/acs.est.3c04390
- Photochemical Reduction of Particle Bound Mercury in Atmospheric Aerosol Water D. Han et al. 10.1021/acsestair.3c00070
- An observation-constrained estimation of brown carbon aerosol direct radiative effects Y. Cheng et al. 10.5194/acp-24-3065-2024
- Characterization of Organosulfates (OSs) in typical urban areas in Eastern China: Source, Process, and Volatility Y. Du et al. 10.1016/j.atmosres.2024.107258
- Investigation of water-soluble organic constituents and their spatio-temporal heterogeneity over the Tibetan Plateau H. Niu et al. 10.1016/j.envpol.2022.119093
- A review of physicochemical properties of dissolved organic carbon and its impact over mountain glaciers H. Niu et al. 10.1007/s11629-023-8437-3
- Molecular compositions and optical properties of water-soluble brown carbon during the autumn and winter in Guangzhou, China T. He et al. 10.1016/j.atmosenv.2022.119573
- Pm2.5-Mediated Photochemical Reaction of Typical Toluene in Real Air Matrix with Identification of Products by Isotopic Tracing and Ft-Icr Ms Q. Li et al. 10.2139/ssrn.4157123
- Impact of fossil and non-fossil fuel sources on the molecular compositions of water-soluble humic-like substances in PM2.5 at a suburban site of Yangtze River Delta, China M. Bao et al. 10.5194/acp-23-8305-2023
- Light absorption properties and molecular profiles of HULIS in PM2.5 emitted from biomass burning in traditional “Heated Kang” in Northwest China T. Zhang et al. 10.1016/j.scitotenv.2021.146014
- Characterization of Products from the Aqueous-Phase Photochemical Oxidation of Benzene-Diols Y. Ou et al. 10.3390/atmos12050534
- Measurement report: Particle-size-dependent fluorescence properties of water-soluble organic compounds (WSOCs) and their atmospheric implications for the aging of WSOCs J. Qin et al. 10.5194/acp-22-465-2022
- Compositional and optical characteristics of aqueous brown carbon and HULIS in the eastern Indo-Gangetic Plain using a coupled EEM PARAFAC, FT-IR and 1H NMR approach S. Dey & S. Sarkar 10.1016/j.scitotenv.2024.171084
- Source apportionment and elevational gradient of dissolved organic matter over the Tibetan plateau H. Niu et al. 10.1016/j.catena.2022.106372
- Multidimensional Analytical Characterization of Water-Soluble Organic Aerosols: Challenges and New Perspectives R. Duarte et al. 10.3390/app11062539
- PM2.5-mediated photochemical reaction of typical toluene in real air matrix with identification of products by isotopic tracing and FT-ICR MS Q. Li et al. 10.1016/j.envpol.2022.120181
- Chemical Signatures of Seasonally Unique Anthropogenic Influences on Organic Aerosol Composition in the Central Amazon E. Franklin et al. 10.1021/acs.est.2c07260
- Water-soluble organic compounds (WSOC) from atmospheric aerosols in Bou-Ismail (Algeria) B. Cherfaoui et al. 10.1007/s11356-024-34520-2
- Overcoming the lack of authentic standards for the quantification of biogenic secondary organic aerosol markers D. Bryant et al. 10.1039/D2EA00074A
- Effect of photooxidation on size distribution, light absorption, and molecular compositions of smoke particles from rice straw combustion R. Zhao et al. 10.1016/j.envpol.2022.119950
- Molecular Characterization of Water-Soluble Brown Carbon Chromophores in Snowpack from Northern Xinjiang, China Y. Zhou et al. 10.1021/acs.est.1c07972
- Factors Influencing the Molecular Compositions and Distributions of Atmospheric Nitrogen‐Containing Compounds H. Jiang et al. 10.1029/2021JD036284
- Photolytic aging of organic aerosol from pyrolyzed urban materials K. Hopstock et al. 10.1039/D3EA00078H
- New insights into the influences of firework combustion on molecular composition and formation of sulfur- and halogen-containing organic compounds C. Yan et al. 10.1016/j.scitotenv.2024.172929
- Amplification of black carbon light absorption induced by atmospheric aging: temporal variation at seasonal and diel scales in urban Guangzhou J. Sun et al. 10.5194/acp-20-2445-2020
29 citations as recorded by crossref.
- Research progress on the characteristics, sources, and environmental and potential health effects of water-soluble organic compounds in atmospheric particulate matter L. Wang et al. 10.1007/s11356-023-31723-x
- Characterizing water-soluble brown carbon in fine particles in four typical cities in northwestern China during wintertime: integrating optical properties with chemical processes M. Zhong et al. 10.5194/acp-23-12609-2023
- Investigation of the Mechanism of Oxidative Potential Increase in Atmospheric Particulate Matter during Photoaging: Important Role of Aromatic Nitrogenous Compounds Q. Wang et al. 10.1021/acs.est.4c03199
- Molecular characterization of nitrogen-containing organic compounds in the winter North China Plain J. Mao et al. 10.1016/j.scitotenv.2022.156189
- Impact of combustion-derived black carbon oxidation states on optical properties and cellular metabolomics in HeLa cells: Insights into soot organics J. Yan et al. 10.1016/j.atmosenv.2023.120118
- Humic-like Substances (HULIS) in Ship Engine Emissions: Molecular Composition Effected by Fuel Type, Engine Mode, and Wet Scrubber Usage E. Schneider et al. 10.1021/acs.est.3c04390
- Photochemical Reduction of Particle Bound Mercury in Atmospheric Aerosol Water D. Han et al. 10.1021/acsestair.3c00070
- An observation-constrained estimation of brown carbon aerosol direct radiative effects Y. Cheng et al. 10.5194/acp-24-3065-2024
- Characterization of Organosulfates (OSs) in typical urban areas in Eastern China: Source, Process, and Volatility Y. Du et al. 10.1016/j.atmosres.2024.107258
- Investigation of water-soluble organic constituents and their spatio-temporal heterogeneity over the Tibetan Plateau H. Niu et al. 10.1016/j.envpol.2022.119093
- A review of physicochemical properties of dissolved organic carbon and its impact over mountain glaciers H. Niu et al. 10.1007/s11629-023-8437-3
- Molecular compositions and optical properties of water-soluble brown carbon during the autumn and winter in Guangzhou, China T. He et al. 10.1016/j.atmosenv.2022.119573
- Pm2.5-Mediated Photochemical Reaction of Typical Toluene in Real Air Matrix with Identification of Products by Isotopic Tracing and Ft-Icr Ms Q. Li et al. 10.2139/ssrn.4157123
- Impact of fossil and non-fossil fuel sources on the molecular compositions of water-soluble humic-like substances in PM2.5 at a suburban site of Yangtze River Delta, China M. Bao et al. 10.5194/acp-23-8305-2023
- Light absorption properties and molecular profiles of HULIS in PM2.5 emitted from biomass burning in traditional “Heated Kang” in Northwest China T. Zhang et al. 10.1016/j.scitotenv.2021.146014
- Characterization of Products from the Aqueous-Phase Photochemical Oxidation of Benzene-Diols Y. Ou et al. 10.3390/atmos12050534
- Measurement report: Particle-size-dependent fluorescence properties of water-soluble organic compounds (WSOCs) and their atmospheric implications for the aging of WSOCs J. Qin et al. 10.5194/acp-22-465-2022
- Compositional and optical characteristics of aqueous brown carbon and HULIS in the eastern Indo-Gangetic Plain using a coupled EEM PARAFAC, FT-IR and 1H NMR approach S. Dey & S. Sarkar 10.1016/j.scitotenv.2024.171084
- Source apportionment and elevational gradient of dissolved organic matter over the Tibetan plateau H. Niu et al. 10.1016/j.catena.2022.106372
- Multidimensional Analytical Characterization of Water-Soluble Organic Aerosols: Challenges and New Perspectives R. Duarte et al. 10.3390/app11062539
- PM2.5-mediated photochemical reaction of typical toluene in real air matrix with identification of products by isotopic tracing and FT-ICR MS Q. Li et al. 10.1016/j.envpol.2022.120181
- Chemical Signatures of Seasonally Unique Anthropogenic Influences on Organic Aerosol Composition in the Central Amazon E. Franklin et al. 10.1021/acs.est.2c07260
- Water-soluble organic compounds (WSOC) from atmospheric aerosols in Bou-Ismail (Algeria) B. Cherfaoui et al. 10.1007/s11356-024-34520-2
- Overcoming the lack of authentic standards for the quantification of biogenic secondary organic aerosol markers D. Bryant et al. 10.1039/D2EA00074A
- Effect of photooxidation on size distribution, light absorption, and molecular compositions of smoke particles from rice straw combustion R. Zhao et al. 10.1016/j.envpol.2022.119950
- Molecular Characterization of Water-Soluble Brown Carbon Chromophores in Snowpack from Northern Xinjiang, China Y. Zhou et al. 10.1021/acs.est.1c07972
- Factors Influencing the Molecular Compositions and Distributions of Atmospheric Nitrogen‐Containing Compounds H. Jiang et al. 10.1029/2021JD036284
- Photolytic aging of organic aerosol from pyrolyzed urban materials K. Hopstock et al. 10.1039/D3EA00078H
- New insights into the influences of firework combustion on molecular composition and formation of sulfur- and halogen-containing organic compounds C. Yan et al. 10.1016/j.scitotenv.2024.172929
Latest update: 23 Nov 2024
Short summary
The composition and light-induced evolution of a water-soluble organic carbon mixture from fresh biomass burning aerosols was investigated with direct infusion electrospray ionisation high-resolution mass spectrometry (HRMS) and liquid chromatography coupled with HRMS. Our findings indicate that the water-soluble organic fraction of combustion-derived aerosols has the potential to form more oxidised organic matter, contributing to the highly oxygenated nature of atmospheric organic aerosols.
The composition and light-induced evolution of a water-soluble organic carbon mixture from fresh...
Altmetrics
Final-revised paper
Preprint