Articles | Volume 20, issue 10
https://doi.org/10.5194/acp-20-5977-2020
https://doi.org/10.5194/acp-20-5977-2020
Research article
 | 
20 May 2020
Research article |  | 20 May 2020

Characterization of carbonaceous aerosols in Singapore: insight from black carbon fragments and trace metal ions detected by a soot particle aerosol mass spectrometer

Laura-Hélèna Rivellini, Max Gerrit Adam, Nethmi Kasthuriarachchi, and Alex King Yin Lee

Related authors

Elemental analysis of oxygenated organic coating on black carbon particles using a soot-particle aerosol mass spectrometer
Mutian Ma, Laura-Hélèna Rivellini, YuXi Cui, Megan D. Willis, Rio Wilkie, Jonathan P. D. Abbatt, Manjula R. Canagaratna, Junfeng Wang, Xinlei Ge, and Alex K. Y. Lee
Atmos. Meas. Tech., 14, 2799–2812, https://doi.org/10.5194/amt-14-2799-2021,https://doi.org/10.5194/amt-14-2799-2021, 2021
Short summary

Cited articles

Achad, M., Caumo, S., de Castro Vasconcellos, P., Bajano, H., Gómez, D., and Smichowski, P.: Chemical markers of biomass burning: Determination of levoglucosan, and potassium in size-classified atmospheric aerosols collected in Buenos Aires, Argentina by different analytical techniques, Microchem. J., 139, 181–187, https://doi.org/10.1016/j.microc.2018.02.016, 2018. 
Agrawal, H., Eden, R., Zhang, X., Fine, P. M., Katzenstein, A., Miller, J. W., Ospital, J., Teffera, S., and Cocker, D. R.: Primary Particulate Matter from Ocean-Going Engines in the Southern California Air Basin, Environ. Sci. Technol., 43, 5398–5402, https://doi.org/10.1021/es8035016, 2009. 
Allan, J. D., Bower, K. N., Coe, H., Boudries, H., Jayne, J. T., Caragaratna, M. R., Millet, D. B., Goldstein, A. H., Quinn, P. K., Weber, R. J. C. G. L., and Worsnop, D. R.: Submicron aerosol composition at Trinidad Head, California, during ITCT 2K2: Its relationship with gas phase volatile organic carbon and assessment of instrument performance, J. Aerosol Sci., 35, 909–922, https://doi.org/10.1016/j.jaerosci.2004.02.007, 2004. 
Allan, J. D., Williams, P. I., Morgan, W. T., Martin, C. L., Flynn, M. J., Lee, J., Nemitz, E., Phillips, G. J., Gallagher, M. W., and Coe, H.: Contributions from transport, solid fuel burning and cooking to primary organic aerosols in two UK cities, Atmos. Chem. Phys., 10, 647–668, https://doi.org/10.5194/acp-10-647-2010, 2010. 
Artaxo, P., Gerab, F., and Rabello, M. L.: Elemental composition of aerosol particles from two atmospheric monitoring stations in the Amazon Basin, Nucl. Instrum. Methods Phys. Res. Sect. B, 75, 277–281, 1993. 
Download
Short summary
This work highlights that trace metals and refractory black carbon (rBC), and their inclusion in a source–receptor model, can provide important insight into the source apportionment of carbonaceous aerosols. In Singapore, we evidenced that 90 % of rBC originated from traffic/industrial emissions. The association of aged OA with K and Rb underlines the influence of regional biomass burning sources, while rBC fragmentation patterns and V/Ni were used to identify industrial and shipping pollutants.
Share
Altmetrics
Final-revised paper
Preprint