Articles | Volume 20, issue 22
https://doi.org/10.5194/acp-20-14063-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-20-14063-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
20 Nov 2020
Research article |
| 20 Nov 2020
| 20 Nov 2020
Impact of in-cloud aqueous processes on the chemical compositions and morphology of individual atmospheric aerosols
Yuzhen Fu
State Key Laboratory of Organic Geochemistry and Guangdong Key Laboratory of Environmental Protection and Resources Utilization, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, PR China
University of Chinese Academy of Sciences, Beijing 100049, PR China
Qinhao Lin
State Key Laboratory of Organic Geochemistry and Guangdong Key Laboratory of Environmental Protection and Resources Utilization, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, PR China
now at: Guangdong Key Laboratory of Environmental Catalysis and
Health Risk Control, Guangzhou Key Laboratory Environmental Catalysis and
Pollution Control, School of Environmental Science and Engineering,
Institute of Environmental Health and Pollution Control, Guangdong
University of Technology, Guangzhou 510006, PR China
State Key Laboratory of Organic Geochemistry and Guangdong Key Laboratory of Environmental Protection and Resources Utilization, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, PR China
Guangdong-Hong Kong-Macao Joint Laboratory for Environmental
Pollution and Control, Guangzhou 510640, PR China
Yuxiang Yang
State Key Laboratory of Organic Geochemistry and Guangdong Key Laboratory of Environmental Protection and Resources Utilization, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, PR China
University of Chinese Academy of Sciences, Beijing 100049, PR China
Yiping Yang
University of Chinese Academy of Sciences, Beijing 100049, PR China
CAS Key Laboratory of Mineralogy and Metallogeny & Guangdong
Provincial Key Laboratory of Mineral Physics and Materials, Guangzhou
Institute of Geochemistry, CAS, Guangzhou 510640, PR China
Xiufeng Lian
State Key Laboratory of Organic Geochemistry and Guangdong Key Laboratory of Environmental Protection and Resources Utilization, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, PR China
University of Chinese Academy of Sciences, Beijing 100049, PR China
Long Peng
State Key Laboratory of Organic Geochemistry and Guangdong Key Laboratory of Environmental Protection and Resources Utilization, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, PR China
University of Chinese Academy of Sciences, Beijing 100049, PR China
Feng Jiang
State Key Laboratory of Organic Geochemistry and Guangdong Key Laboratory of Environmental Protection and Resources Utilization, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, PR China
University of Chinese Academy of Sciences, Beijing 100049, PR China
now at: Institute of Meteorology and Climate Research,
Karlsruhe Institute of Technology, 76344 Eggenstein-Leopoldshafen, Germany
State Key Laboratory of Organic Geochemistry and Guangdong Key Laboratory of Environmental Protection and Resources Utilization, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, PR China
Guangdong-Hong Kong-Macao Joint Laboratory for Environmental
Pollution and Control, Guangzhou 510640, PR China
Institute of Mass Spectrometer and Atmosphere Environment, Jinan
University, Guangzhou 510632, PR China
Yuanyuan Wang
Department of Atmospheric Science, School of Earth Science, Zhejiang University, Hangzhou 310027, PR China
Duohong Chen
State Environmental Protection Key Laboratory of Regional Air Quality Monitoring, Guangdong Environmental Monitoring Center, Guangzhou 510308, PR China
Jie Ou
Shaoguan Environmental Monitoring Center, Shaoguan 512026, PR
China
Xinming Wang
State Key Laboratory of Organic Geochemistry and Guangdong Key Laboratory of Environmental Protection and Resources Utilization, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, PR China
Guangdong-Hong Kong-Macao Joint Laboratory for Environmental
Pollution and Control, Guangzhou 510640, PR China
Ping'an Peng
State Key Laboratory of Organic Geochemistry and Guangdong Key Laboratory of Environmental Protection and Resources Utilization, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, PR China
Guangdong-Hong Kong-Macao Joint Laboratory for Environmental
Pollution and Control, Guangzhou 510640, PR China
Jianxi Zhu
CAS Key Laboratory of Mineralogy and Metallogeny & Guangdong
Provincial Key Laboratory of Mineral Physics and Materials, Guangzhou
Institute of Geochemistry, CAS, Guangzhou 510640, PR China
Guoying Sheng
State Key Laboratory of Organic Geochemistry and Guangdong Key Laboratory of Environmental Protection and Resources Utilization, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, PR China
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Cited
15 citations as recorded by crossref.
- Characteristics and Aging of Traffic-Emitted Particles with Sulfate and Organic Compound Formation in Urban Air J. Xing et al. 10.3390/atmos13040608
- Impact of in-cloud aqueous processes on the chemical compositions and morphology of individual atmospheric aerosols Y. Fu et al. 10.5194/acp-20-14063-2020
- Stage-resolved in-cloud scavenging of submicron and BC-containing particles: A case study Y. Yang et al. 10.1016/j.atmosenv.2020.117883
- Molecular characteristics, sources and transformation of water-insoluble organic matter in cloud water W. Sun et al. 10.1016/j.envpol.2023.121430
- Fog/cloud processing of atmospheric aerosols from a single particle perspective: A review of field observations G. Zhang et al. 10.1016/j.atmosenv.2024.120536
- Vertical Gradient of Size-Resolved Aerosol Compositions over the Arctic Reveals Cloud Processed Aerosol in-Cloud and above Cloud N. Lata et al. 10.1021/acs.est.2c09498
- The optical properties and in-situ observational evidence for the formation of brown carbon in clouds Z. Guo et al. 10.5194/acp-22-4827-2022
- Updated In-Cloud Secondary Aerosol Production in the Northern Hemisphere Predicted by the Community Multiscale Air Quality Modeling System K. Fahey et al. 10.1021/acsearthspacechem.4c00370
- Air pollution in the operating room: A case study of characteristics of airborne particles, PAHs and environmentally persistent free radicals X. Yu et al. 10.1016/j.apr.2021.101257
- Impacts of Cloud‐Processing on Ice Nucleation of Soot Particles Internally Mixed With Sulfate and Organics K. Gao & Z. Kanji 10.1029/2022JD037146
- Variability in morphology of soot particles during non-cloud and in-cloud processes Y. Wang et al. 10.1016/j.atmosenv.2024.120489
- Impact of Cloud Process in the Mixing State and Microphysical Properties of Soot Particles: Implications in Light Absorption Enhancement Y. Fu et al. 10.1029/2022JD037169
- Characterization of Microplastics in Clouds over Eastern China X. Xu et al. 10.1021/acs.estlett.3c00729
- Light absorption and scattering of core–shell aerosol particles G. David & R. Signorell 10.1364/AO.555468
- Constructing Shapes and Mixing Structures of Black Carbon Particles With Applications to Optical Calculations Y. Wang et al. 10.1029/2021JD034620
15 citations as recorded by crossref.
- Characteristics and Aging of Traffic-Emitted Particles with Sulfate and Organic Compound Formation in Urban Air J. Xing et al. 10.3390/atmos13040608
- Impact of in-cloud aqueous processes on the chemical compositions and morphology of individual atmospheric aerosols Y. Fu et al. 10.5194/acp-20-14063-2020
- Stage-resolved in-cloud scavenging of submicron and BC-containing particles: A case study Y. Yang et al. 10.1016/j.atmosenv.2020.117883
- Molecular characteristics, sources and transformation of water-insoluble organic matter in cloud water W. Sun et al. 10.1016/j.envpol.2023.121430
- Fog/cloud processing of atmospheric aerosols from a single particle perspective: A review of field observations G. Zhang et al. 10.1016/j.atmosenv.2024.120536
- Vertical Gradient of Size-Resolved Aerosol Compositions over the Arctic Reveals Cloud Processed Aerosol in-Cloud and above Cloud N. Lata et al. 10.1021/acs.est.2c09498
- The optical properties and in-situ observational evidence for the formation of brown carbon in clouds Z. Guo et al. 10.5194/acp-22-4827-2022
- Updated In-Cloud Secondary Aerosol Production in the Northern Hemisphere Predicted by the Community Multiscale Air Quality Modeling System K. Fahey et al. 10.1021/acsearthspacechem.4c00370
- Air pollution in the operating room: A case study of characteristics of airborne particles, PAHs and environmentally persistent free radicals X. Yu et al. 10.1016/j.apr.2021.101257
- Impacts of Cloud‐Processing on Ice Nucleation of Soot Particles Internally Mixed With Sulfate and Organics K. Gao & Z. Kanji 10.1029/2022JD037146
- Variability in morphology of soot particles during non-cloud and in-cloud processes Y. Wang et al. 10.1016/j.atmosenv.2024.120489
- Impact of Cloud Process in the Mixing State and Microphysical Properties of Soot Particles: Implications in Light Absorption Enhancement Y. Fu et al. 10.1029/2022JD037169
- Characterization of Microplastics in Clouds over Eastern China X. Xu et al. 10.1021/acs.estlett.3c00729
- Light absorption and scattering of core–shell aerosol particles G. David & R. Signorell 10.1364/AO.555468
- Constructing Shapes and Mixing Structures of Black Carbon Particles With Applications to Optical Calculations Y. Wang et al. 10.1029/2021JD034620
Latest update: 30 May 2025
Short summary
Based on the analysis of the morphology and mixing structure of the activated and unactivated particles, our results emphasize the role of in-cloud processes in the chemistry and microphysical properties of individual activated particles. Given that organic coatings may determine the particle hygroscopicity and heterogeneous chemical reactivity, the increase of OM-shelled particles upon in-cloud processes should have considerable implications for their evolution and climate impact.
Based on the analysis of the morphology and mixing structure of the activated and unactivated...
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