Articles | Volume 20, issue 21
https://doi.org/10.5194/acp-20-12549-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-20-12549-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| Highlight paper
| 
02 Nov 2020
Research article | Highlight paper |
| 02 Nov 2020
| 02 Nov 2020
The Aarhus Chamber Campaign on Highly Oxygenated Organic Molecules and Aerosols (ACCHA): particle formation, organic acids, and dimer esters from α-pinene ozonolysis at different temperatures
Kasper Kristensen
CORRESPONDING AUTHOR
Department of Engineering, Aarhus University, 8000 Aarhus C, Denmark
Louise N. Jensen
Department of Chemistry and iCLIMATE, Aarhus University, 8000 Aarhus
C, Denmark
Lauriane L. J. Quéléver
Institute for Atmospheric and Earth System Research – INAR/Physics,
University of Helsinki, P.O. Box 64, 00014, Helsinki, Finland
Sigurd Christiansen
Department of Chemistry and iCLIMATE, Aarhus University, 8000 Aarhus
C, Denmark
Bernadette Rosati
Department of Chemistry and iCLIMATE, Aarhus University, 8000 Aarhus
C, Denmark
Department of Physics and Astronomy, Aarhus University, 8000 Aarhus C,
Denmark
Jonas Elm
Department of Chemistry and iCLIMATE, Aarhus University, 8000 Aarhus
C, Denmark
Ricky Teiwes
Department of Physics and Astronomy, Aarhus University, 8000 Aarhus C,
Denmark
Henrik B. Pedersen
Department of Physics and Astronomy, Aarhus University, 8000 Aarhus C,
Denmark
Marianne Glasius
Department of Chemistry and iCLIMATE, Aarhus University, 8000 Aarhus
C, Denmark
Mikael Ehn
Institute for Atmospheric and Earth System Research – INAR/Physics,
University of Helsinki, P.O. Box 64, 00014, Helsinki, Finland
Department of Chemistry and iCLIMATE, Aarhus University, 8000 Aarhus
C, Denmark
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Cited
28 citations as recorded by crossref.
- Isoprene versus Monoterpenes as Gas-Phase Organic Acid Precursors in the Atmosphere M. Link et al. 10.1021/acsearthspacechem.1c00093
- Methodological advances to improve repeatability of SOA generation in environmental chambers A. Flueckiger & G. Petrucci 10.1080/02786826.2023.2223688
- Organic Peroxides in Aerosol: Key Reactive Intermediates for Multiphase Processes in the Atmosphere S. Wang et al. 10.1021/acs.chemrev.2c00430
- Formation and temperature dependence of highly oxygenated organic molecules (HOMs) from Δ3-carene ozonolysis Y. Luo et al. 10.5194/acp-24-9459-2024
- Review of Smog Chamber Experiments for Secondary Organic Aerosol Formation H. Kim et al. 10.3390/atmos15010115
- Assessing pH- and temperature-dependence in the aqueous phase partitioning of organic acids and bases in the atmosphere O. Driessen & J. Murphy 10.1039/D5EA00034C
- Comparison of saturation vapor pressures of α-pinene + O3 oxidation products derived from COSMO-RS computations and thermal desorption experiments N. Hyttinen et al. 10.5194/acp-22-1195-2022
- Development of the low-temperature hygroscopicity tandem differential mobility analyzer (Low-T HTDMA) and its application to (NH4)2SO4 and NaCl particles M. Cheng & M. Kuwata 10.1016/j.jaerosci.2022.106111
- Isomer-Resolved Reactivity of Organic Peroxides in Monoterpene-Derived Secondary Organic Aerosol M. Yao et al. 10.1021/acs.est.2c01297
- Large Discrepancy in the Formation of Secondary Organic Aerosols from Structurally Similar Monoterpenes D. Thomsen et al. 10.1021/acsearthspacechem.0c00332
- Temperature effects on SOA formation of n-dodecane reaction initiated by Cl atoms C. Fan et al. 10.1016/j.atmosenv.2025.121070
- Ozonolysis of α-Pinene and Δ3-Carene Mixtures: Formation of Dimers with Two Precursors D. Thomsen et al. 10.1021/acs.est.2c04786
- Relative Humidity Impact on Organic New Particle Formation from Ozonolysis of α- and β-Pinene at Atmospherically Relevant Mixing Ratios C. Snyder et al. 10.3390/atmos14010173
- Gaseous and Particle Products Formation from α-Pinene Ozonolysis under Conditions of Different Relative Humidities and Particle Seeds J. Wang et al. 10.1021/acsearthspacechem.4c00368
- Particle-Bound Highly Oxidized Organic Molecules Derived from Aromatic Hydrocarbons in an Urban Atmosphere M. Zhu et al. 10.1021/acs.estlett.2c00841
- Acylperoxy Radicals as Key Intermediates in the Formation of Dimeric Compounds in α-Pinene Secondary Organic Aerosol Y. Zhao et al. 10.1021/acs.est.2c02090
- Nontrivial Impact of Relative Humidity on Organic New Particle Formation from Ozonolysis of cis-3-Hexenyl Acetate A. Flueckiger et al. 10.3390/air1040017
- Large Gas-Phase Source of Esters and Other Accretion Products in the Atmosphere O. Peräkylä et al. 10.1021/jacs.2c10398
- Particle-phase accretion forms dimer esters in pinene secondary organic aerosol C. Kenseth et al. 10.1126/science.adi0857
- Impact of temperature on the role of Criegee intermediates and peroxy radicals in dimer formation from β-pinene ozonolysis Y. Gong et al. 10.5194/acp-24-167-2024
- Real-Time Identification of Aerosol-Phase Carboxylic Acid Production Using Extractive Electrospray Ionization Mass Spectrometry M. Surdu et al. 10.1021/acs.est.4c01605
- Effect of Relative Humidity on the Rate of New Particle Formation for Different VOCs A. Flueckiger & G. Petrucci 10.3390/atmos15040480
- A comprehensive evaluation of enhanced temperature influence on gas and aerosol chemistry in the lamp-enclosed oxidation flow reactor (OFR) system T. Pan et al. 10.5194/amt-17-4915-2024
- Temperature and volatile organic compound concentrations as controlling factors for chemical composition of α-pinene-derived secondary organic aerosol L. Jensen et al. 10.5194/acp-21-11545-2021
- The effect of temperature and relative humidity on secondary organic aerosol formation from ozonolysis of Δ3-carene D. Thomsen et al. 10.1039/D3EA00128H
- A neglected pathway for the accretion products formation in the atmosphere X. Shi et al. 10.1016/j.scitotenv.2022.157494
- A combined gas- and particle-phase analysis of highly oxygenated organic molecules (HOMs) from α-pinene ozonolysis J. Zhao et al. 10.5194/acp-23-3707-2023
- Differences in Secondary Organic Aerosol Formation from α-Pinene Photooxidation in a Chamber with Purified Air and Ambient Air as Matrices: Preliminary Results X. Li et al. 10.3390/atmos15020204
28 citations as recorded by crossref.
- Isoprene versus Monoterpenes as Gas-Phase Organic Acid Precursors in the Atmosphere M. Link et al. 10.1021/acsearthspacechem.1c00093
- Methodological advances to improve repeatability of SOA generation in environmental chambers A. Flueckiger & G. Petrucci 10.1080/02786826.2023.2223688
- Organic Peroxides in Aerosol: Key Reactive Intermediates for Multiphase Processes in the Atmosphere S. Wang et al. 10.1021/acs.chemrev.2c00430
- Formation and temperature dependence of highly oxygenated organic molecules (HOMs) from Δ3-carene ozonolysis Y. Luo et al. 10.5194/acp-24-9459-2024
- Review of Smog Chamber Experiments for Secondary Organic Aerosol Formation H. Kim et al. 10.3390/atmos15010115
- Assessing pH- and temperature-dependence in the aqueous phase partitioning of organic acids and bases in the atmosphere O. Driessen & J. Murphy 10.1039/D5EA00034C
- Comparison of saturation vapor pressures of α-pinene + O3 oxidation products derived from COSMO-RS computations and thermal desorption experiments N. Hyttinen et al. 10.5194/acp-22-1195-2022
- Development of the low-temperature hygroscopicity tandem differential mobility analyzer (Low-T HTDMA) and its application to (NH4)2SO4 and NaCl particles M. Cheng & M. Kuwata 10.1016/j.jaerosci.2022.106111
- Isomer-Resolved Reactivity of Organic Peroxides in Monoterpene-Derived Secondary Organic Aerosol M. Yao et al. 10.1021/acs.est.2c01297
- Large Discrepancy in the Formation of Secondary Organic Aerosols from Structurally Similar Monoterpenes D. Thomsen et al. 10.1021/acsearthspacechem.0c00332
- Temperature effects on SOA formation of n-dodecane reaction initiated by Cl atoms C. Fan et al. 10.1016/j.atmosenv.2025.121070
- Ozonolysis of α-Pinene and Δ3-Carene Mixtures: Formation of Dimers with Two Precursors D. Thomsen et al. 10.1021/acs.est.2c04786
- Relative Humidity Impact on Organic New Particle Formation from Ozonolysis of α- and β-Pinene at Atmospherically Relevant Mixing Ratios C. Snyder et al. 10.3390/atmos14010173
- Gaseous and Particle Products Formation from α-Pinene Ozonolysis under Conditions of Different Relative Humidities and Particle Seeds J. Wang et al. 10.1021/acsearthspacechem.4c00368
- Particle-Bound Highly Oxidized Organic Molecules Derived from Aromatic Hydrocarbons in an Urban Atmosphere M. Zhu et al. 10.1021/acs.estlett.2c00841
- Acylperoxy Radicals as Key Intermediates in the Formation of Dimeric Compounds in α-Pinene Secondary Organic Aerosol Y. Zhao et al. 10.1021/acs.est.2c02090
- Nontrivial Impact of Relative Humidity on Organic New Particle Formation from Ozonolysis of cis-3-Hexenyl Acetate A. Flueckiger et al. 10.3390/air1040017
- Large Gas-Phase Source of Esters and Other Accretion Products in the Atmosphere O. Peräkylä et al. 10.1021/jacs.2c10398
- Particle-phase accretion forms dimer esters in pinene secondary organic aerosol C. Kenseth et al. 10.1126/science.adi0857
- Impact of temperature on the role of Criegee intermediates and peroxy radicals in dimer formation from β-pinene ozonolysis Y. Gong et al. 10.5194/acp-24-167-2024
- Real-Time Identification of Aerosol-Phase Carboxylic Acid Production Using Extractive Electrospray Ionization Mass Spectrometry M. Surdu et al. 10.1021/acs.est.4c01605
- Effect of Relative Humidity on the Rate of New Particle Formation for Different VOCs A. Flueckiger & G. Petrucci 10.3390/atmos15040480
- A comprehensive evaluation of enhanced temperature influence on gas and aerosol chemistry in the lamp-enclosed oxidation flow reactor (OFR) system T. Pan et al. 10.5194/amt-17-4915-2024
- Temperature and volatile organic compound concentrations as controlling factors for chemical composition of α-pinene-derived secondary organic aerosol L. Jensen et al. 10.5194/acp-21-11545-2021
- The effect of temperature and relative humidity on secondary organic aerosol formation from ozonolysis of Δ3-carene D. Thomsen et al. 10.1039/D3EA00128H
- A neglected pathway for the accretion products formation in the atmosphere X. Shi et al. 10.1016/j.scitotenv.2022.157494
- A combined gas- and particle-phase analysis of highly oxygenated organic molecules (HOMs) from α-pinene ozonolysis J. Zhao et al. 10.5194/acp-23-3707-2023
- Differences in Secondary Organic Aerosol Formation from α-Pinene Photooxidation in a Chamber with Purified Air and Ambient Air as Matrices: Preliminary Results X. Li et al. 10.3390/atmos15020204
Latest update: 22 Jul 2025
Short summary
Atmospheric particles are important in relation to human health and the global climate. As the global temperature changes, so may the atmospheric chemistry controlling the formation of particles from reactions of naturally emitted volatile organic compounds (VOCs). In the current work, we show how temperatures influence the formation and chemical composition of atmospheric particles from α-pinene: a biogenic VOC largely emitted in high-latitude environments such as the boreal forests.
Atmospheric particles are important in relation to human health and the global climate. As the...
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