Articles | Volume 20, issue 20
https://doi.org/10.5194/acp-20-11747-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-20-11747-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
19 Oct 2020
Research article |
| 19 Oct 2020
Sources and sinks driving sulfuric acid concentrations in contrasting environments: implications on proxy calculations
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology, 100029 Beijing, China
Institute for Atmospheric and Earth System Research INAR/Physics, Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Ilona Ylivinkka
Institute for Atmospheric and Earth System Research INAR/Physics, Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
SMEAR II station, University of Helsinki, 35500 Korkeakoski, Finland
Rima Baalbaki
Institute for Atmospheric and Earth System Research INAR/Physics, Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Chang Li
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology, 100029 Beijing, China
Yishuo Guo
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology, 100029 Beijing, China
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology, 100029 Beijing, China
Institute for Atmospheric and Earth System Research INAR/Physics, Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology, 100029 Beijing, China
Institute for Atmospheric and Earth System Research INAR/Physics, Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Nina Sarnela
Institute for Atmospheric and Earth System Research INAR/Physics, Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Tuija Jokinen
Institute for Atmospheric and Earth System Research INAR/Physics, Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Kaspar R. Daellenbach
Institute for Atmospheric and Earth System Research INAR/Physics, Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Rujing Yin
State Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Tsinghua University, 100084 Beijing, China
Chenjuan Deng
State Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Tsinghua University, 100084 Beijing, China
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology, 100029 Beijing, China
Institute for Atmospheric and Earth System Research INAR/Physics, Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Tuomo Nieminen
Institute for Atmospheric and Earth System Research INAR/Physics, Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Institute for Atmospheric and Earth System Research INAR/Forest Sciences, Faculty of Agriculture and Forestry, University of Helsinki, 00014, Helsinki, Finland
Yonghong Wang
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology, 100029 Beijing, China
Institute for Atmospheric and Earth System Research INAR/Physics, Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Zhuohui Lin
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology, 100029 Beijing, China
Roseline C. Thakur
Institute for Atmospheric and Earth System Research INAR/Physics, Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Jenni Kontkanen
Institute for Atmospheric and Earth System Research INAR/Physics, Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Dominik Stolzenburg
Institute for Atmospheric and Earth System Research INAR/Physics, Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Mikko Sipilä
Institute for Atmospheric and Earth System Research INAR/Physics, Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Tareq Hussein
Institute for Atmospheric and Earth System Research INAR/Physics, Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Department of Physics, The University of Jordan, Amman 11942, Jordan
Department Material Analysis and Indoor Chemistry, Fraunhofer WKI, 38108 Braunschweig, Germany
Pauli Paasonen
Institute for Atmospheric and Earth System Research INAR/Physics, Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Federico Bianchi
Institute for Atmospheric and Earth System Research INAR/Physics, Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Imre Salma
Institute of Chemistry, Eötvös University, P.O. Box 32, 1518 Budapest, Hungary
Tamás Weidinger
Department of Meteorology, Eötvös University, P.O. Box 32, 1518 Budapest, Hungary
Michael Pikridas
The Cyprus Institute, Climate & Atmosphere Research Centre (CARE-C), 20 Konstantinou Kavafi Street, 2121 Nicosia, Cyprus
Jean Sciare
The Cyprus Institute, Climate & Atmosphere Research Centre (CARE-C), 20 Konstantinou Kavafi Street, 2121 Nicosia, Cyprus
Jingkun Jiang
State Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Tsinghua University, 100084 Beijing, China
Yongchun Liu
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology, 100029 Beijing, China
Tuukka Petäjä
Institute for Atmospheric and Earth System Research INAR/Physics, Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Veli-Matti Kerminen
Institute for Atmospheric and Earth System Research INAR/Physics, Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Markku Kulmala
CORRESPONDING AUTHOR
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology, 100029 Beijing, China
Institute for Atmospheric and Earth System Research INAR/Physics, Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
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Cited
16 citations as recorded by crossref.
- Response of particle number concentrations to the clean air action plan: lessons from the first long-term aerosol measurements in a typical urban valley in western China S. Zhao et al. 10.5194/acp-21-14959-2021
- Influence of vegetation on occurrence and time distributions of regional new aerosol particle formation and growth I. Salma et al. 10.5194/acp-21-2861-2021
- Measurement report: New particle formation characteristics at an urban and a mountain station in northern China Y. Zhou et al. 10.5194/acp-21-17885-2021
- Chemistry of new particle formation and growth events during wintertime in suburban area of Beijing: Insights from highly polluted atmosphere S. Yang et al. 10.1016/j.atmosres.2021.105553
- Condensation sink of atmospheric vapors: the effect of vapor properties and the resulting uncertainties S. Tuovinen et al. 10.1039/D1EA00032B
- Formation of nighttime sulfuric acid from the ozonolysis of alkenes in Beijing Y. Guo et al. 10.5194/acp-21-5499-2021
- Toward Building a Physical Proxy for Gas-Phase Sulfuric Acid Concentration Based on Its Budget Analysis in Polluted Yangtze River Delta, East China L. Yang et al. 10.1021/acs.est.1c00738
- New particle formation event detection with Mask R-CNN P. Su et al. 10.5194/acp-22-1293-2022
- A modelling study of OH, NO3 and H2SO4 in 2007–2018 at SMEAR II, Finland: analysis of long-term trends D. Chen et al. 10.1039/D1EA00020A
- Decennial time trends and diurnal patterns of particle number concentrations in a central European city between 2008 and 2018 S. Mikkonen et al. 10.5194/acp-20-12247-2020
- Observation of sub-3nm particles and new particle formation at an urban location in India M. Sebastian et al. 10.1016/j.atmosenv.2021.118460
- Aerosol number concentrations and new particle formation events over a polluted megacity during the COVID-19 lockdown S. Yadav et al. 10.1016/j.atmosenv.2021.118526
- Wintertime subarctic new particle formation from Kola Peninsula sulfur emissions M. Sipilä et al. 10.5194/acp-21-17559-2021
- Observed coupling between air mass history, secondary growth of nucleation mode particles and aerosol pollution levels in Beijing S. Hakala et al. 10.1039/D1EA00089F
- Investigation of several proxies to estimate sulfuric acid concentration under volcanic plume conditions C. Rose et al. 10.5194/acp-21-4541-2021
- Towards understanding the characteristics of new particle formation in the Eastern Mediterranean R. Baalbaki et al. 10.5194/acp-21-9223-2021
16 citations as recorded by crossref.
- Response of particle number concentrations to the clean air action plan: lessons from the first long-term aerosol measurements in a typical urban valley in western China S. Zhao et al. 10.5194/acp-21-14959-2021
- Influence of vegetation on occurrence and time distributions of regional new aerosol particle formation and growth I. Salma et al. 10.5194/acp-21-2861-2021
- Measurement report: New particle formation characteristics at an urban and a mountain station in northern China Y. Zhou et al. 10.5194/acp-21-17885-2021
- Chemistry of new particle formation and growth events during wintertime in suburban area of Beijing: Insights from highly polluted atmosphere S. Yang et al. 10.1016/j.atmosres.2021.105553
- Condensation sink of atmospheric vapors: the effect of vapor properties and the resulting uncertainties S. Tuovinen et al. 10.1039/D1EA00032B
- Formation of nighttime sulfuric acid from the ozonolysis of alkenes in Beijing Y. Guo et al. 10.5194/acp-21-5499-2021
- Toward Building a Physical Proxy for Gas-Phase Sulfuric Acid Concentration Based on Its Budget Analysis in Polluted Yangtze River Delta, East China L. Yang et al. 10.1021/acs.est.1c00738
- New particle formation event detection with Mask R-CNN P. Su et al. 10.5194/acp-22-1293-2022
- A modelling study of OH, NO3 and H2SO4 in 2007–2018 at SMEAR II, Finland: analysis of long-term trends D. Chen et al. 10.1039/D1EA00020A
- Decennial time trends and diurnal patterns of particle number concentrations in a central European city between 2008 and 2018 S. Mikkonen et al. 10.5194/acp-20-12247-2020
- Observation of sub-3nm particles and new particle formation at an urban location in India M. Sebastian et al. 10.1016/j.atmosenv.2021.118460
- Aerosol number concentrations and new particle formation events over a polluted megacity during the COVID-19 lockdown S. Yadav et al. 10.1016/j.atmosenv.2021.118526
- Wintertime subarctic new particle formation from Kola Peninsula sulfur emissions M. Sipilä et al. 10.5194/acp-21-17559-2021
- Observed coupling between air mass history, secondary growth of nucleation mode particles and aerosol pollution levels in Beijing S. Hakala et al. 10.1039/D1EA00089F
- Investigation of several proxies to estimate sulfuric acid concentration under volcanic plume conditions C. Rose et al. 10.5194/acp-21-4541-2021
- Towards understanding the characteristics of new particle formation in the Eastern Mediterranean R. Baalbaki et al. 10.5194/acp-21-9223-2021
Latest update: 29 Mar 2023
Short summary
We rely on sulfuric acid measurements in four contrasting environments, Hyytiälä, Finland; Agia Marina, Cyprus; Budapest, Hungary; and Beijing, China, representing semi-pristine boreal forest, rural environment in the Mediterranean area, urban environment, and heavily polluted megacity, respectively, in order to define the sources and sinks of sulfuric acid in these environments and to derive a new sulfuric acid proxy to be utilized in locations and during periods when it is not measured.
We rely on sulfuric acid measurements in four contrasting environments, Hyytiälä, Finland; Agia...
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