Articles | Volume 20, issue 17
https://doi.org/10.5194/acp-20-10331-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-20-10331-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
07 Sep 2020
Research article |
| 07 Sep 2020
| 07 Sep 2020
Vertical distribution of particle-phase dicarboxylic acids, oxoacids and α-dicarbonyls in the urban boundary layer based on the 325 m tower in Beijing
Wanyu Zhao
State Key Laboratory of Atmospheric Boundary Layer Physics and
Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China
Institute of Surface-Earth System Science, School of Earth System
Science, Tianjin University, Tianjin 300072, China
Institute of Low Temperature Science, Hokkaido University, Sapporo
060-0819, Japan
College of Earth and Planetary Sciences, University of Chinese Academy of Sciences, Beijing 100049, China
Hong Ren
Institute of Surface-Earth System Science, School of Earth System
Science, Tianjin University, Tianjin 300072, China
Kimitaka Kawamura
Institute of Low Temperature Science, Hokkaido University, Sapporo
060-0819, Japan
Chubu Institute for Advanced Studies, Chubu University, Kasugai
487–8501, Japan
Huiyun Du
State Key Laboratory of Atmospheric Boundary Layer Physics and
Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China
College of Earth and Planetary Sciences, University of Chinese Academy of Sciences, Beijing 100049, China
Xueshun Chen
State Key Laboratory of Atmospheric Boundary Layer Physics and
Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China
College of Earth and Planetary Sciences, University of Chinese Academy of Sciences, Beijing 100049, China
Siyao Yue
State Key Laboratory of Atmospheric Boundary Layer Physics and
Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China
College of Earth and Planetary Sciences, University of Chinese Academy of Sciences, Beijing 100049, China
Qiaorong Xie
State Key Laboratory of Atmospheric Boundary Layer Physics and
Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China
College of Earth and Planetary Sciences, University of Chinese Academy of Sciences, Beijing 100049, China
Lianfang Wei
State Key Laboratory of Atmospheric Boundary Layer Physics and
Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China
College of Earth and Planetary Sciences, University of Chinese Academy of Sciences, Beijing 100049, China
Ping Li
State Key Laboratory of Atmospheric Boundary Layer Physics and
Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China
College of Earth and Planetary Sciences, University of Chinese Academy of Sciences, Beijing 100049, China
Xin Zeng
Department of Atmospheric Science, School of Environmental Sciences, China University of Geosciences, Wuhan 430074, China
Shaofei Kong
Department of Atmospheric Science, School of Environmental Sciences, China University of Geosciences, Wuhan 430074, China
State Key Laboratory of Atmospheric Boundary Layer Physics and
Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China
Zifa Wang
State Key Laboratory of Atmospheric Boundary Layer Physics and
Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China
Institute of Surface-Earth System Science, School of Earth System
Science, Tianjin University, Tianjin 300072, China
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Cited
13 citations as recorded by crossref.
- Atmospheric Chemistry of Oxalate: Insight Into the Role of Relative Humidity and Aerosol Acidity From High‐Resolution Observation C. Yang et al. 10.1029/2021JD035364
- Vertically Resolved Aerosol Chemistry in the Low Boundary Layer of Beijing in Summer Y. Li et al. 10.1021/acs.est.2c02861
- Contrasting molecular characteristics and formation mechanisms of biogenic and anthropogenic secondary organic aerosols at the summit and foot of Mt. Huang, East China Y. Wang et al. 10.1016/j.scitotenv.2023.165116
- Characterization of dicarboxylic acids, oxoacids, and α-dicarbonyls in PM2.5 within the urban boundary layer in southern China: Sources and formation pathways J. Liu et al. 10.1016/j.envpol.2021.117185
- Molecular distributions of dicarboxylic acids, oxocarboxylic acids, and α-dicarbonyls in aerosols over Tuoji Island in the Bohai Sea: Effects of East Asian continental outflow Y. Zhu et al. 10.1016/j.atmosres.2022.106154
- Seasonal distributions and possible sources of low molecular weight organic acids in PM2.5 from a typical mining city after decade green mining developing in Southeastern Hubei, Central China S. Liu et al. 10.1016/j.atmosenv.2024.120455
- Characteristics of fine particle matter at the top of Shanghai Tower C. Yin et al. 10.5194/acp-23-1329-2023
- Measurement Report: Investigation on the sources and formation processes of dicarboxylic acids and related species in urban aerosols before and during the COVID-19 lockdown in Jinan, East China J. Meng et al. 10.5194/acp-23-14481-2023
- Photochemical Degradation of Organic Matter in the Atmosphere W. Hu et al. 10.1002/adsu.202100027
- Molecular characterization and spatial distribution of dicarboxylic acids and related compounds in fresh snow in China Z. Zhang et al. 10.1016/j.envpol.2021.118114
- Measurement report: Vertical distribution of biogenic and anthropogenic secondary organic aerosols in the urban boundary layer over Beijing during late summer H. Ren et al. 10.5194/acp-21-12949-2021
- Influence of vertical transport on chemical evolution of dicarboxylic acids and related secondary organic aerosol from surface emission to the top of Mount Hua, Northwest China M. Shen et al. 10.1016/j.scitotenv.2022.159892
- Diurnal Variations in High Time-Resolved Molecular Distributions and Formation Mechanisms of Biogenic Secondary Organic Aerosols at Mt. Huang, East China Y. Li et al. 10.3390/molecules28165939
13 citations as recorded by crossref.
- Atmospheric Chemistry of Oxalate: Insight Into the Role of Relative Humidity and Aerosol Acidity From High‐Resolution Observation C. Yang et al. 10.1029/2021JD035364
- Vertically Resolved Aerosol Chemistry in the Low Boundary Layer of Beijing in Summer Y. Li et al. 10.1021/acs.est.2c02861
- Contrasting molecular characteristics and formation mechanisms of biogenic and anthropogenic secondary organic aerosols at the summit and foot of Mt. Huang, East China Y. Wang et al. 10.1016/j.scitotenv.2023.165116
- Characterization of dicarboxylic acids, oxoacids, and α-dicarbonyls in PM2.5 within the urban boundary layer in southern China: Sources and formation pathways J. Liu et al. 10.1016/j.envpol.2021.117185
- Molecular distributions of dicarboxylic acids, oxocarboxylic acids, and α-dicarbonyls in aerosols over Tuoji Island in the Bohai Sea: Effects of East Asian continental outflow Y. Zhu et al. 10.1016/j.atmosres.2022.106154
- Seasonal distributions and possible sources of low molecular weight organic acids in PM2.5 from a typical mining city after decade green mining developing in Southeastern Hubei, Central China S. Liu et al. 10.1016/j.atmosenv.2024.120455
- Characteristics of fine particle matter at the top of Shanghai Tower C. Yin et al. 10.5194/acp-23-1329-2023
- Measurement Report: Investigation on the sources and formation processes of dicarboxylic acids and related species in urban aerosols before and during the COVID-19 lockdown in Jinan, East China J. Meng et al. 10.5194/acp-23-14481-2023
- Photochemical Degradation of Organic Matter in the Atmosphere W. Hu et al. 10.1002/adsu.202100027
- Molecular characterization and spatial distribution of dicarboxylic acids and related compounds in fresh snow in China Z. Zhang et al. 10.1016/j.envpol.2021.118114
- Measurement report: Vertical distribution of biogenic and anthropogenic secondary organic aerosols in the urban boundary layer over Beijing during late summer H. Ren et al. 10.5194/acp-21-12949-2021
- Influence of vertical transport on chemical evolution of dicarboxylic acids and related secondary organic aerosol from surface emission to the top of Mount Hua, Northwest China M. Shen et al. 10.1016/j.scitotenv.2022.159892
- Diurnal Variations in High Time-Resolved Molecular Distributions and Formation Mechanisms of Biogenic Secondary Organic Aerosols at Mt. Huang, East China Y. Li et al. 10.3390/molecules28165939
Latest update: 25 Apr 2024
Short summary
Our observations provide detailed information on the abundance and vertical distribution of dicarboxylic acids, oxoacids and α-dicarbonyls in PM2.5 collected at three heights based on a 325 m meteorological tower in Beijing in summer. Our results demonstrate that organic acids at the ground surface are largely associated with local traffic emissions, while long-range atmospheric transport followed by photochemical ageing contributes more in the urban boundary layer than the ground surface.
Our observations provide detailed information on the abundance and vertical distribution of...
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