Articles | Volume 19, issue 7
https://doi.org/10.5194/acp-19-5033-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue:
https://doi.org/10.5194/acp-19-5033-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
12 Apr 2019
Research article |
| 12 Apr 2019
| 12 Apr 2019
New particle formation from sulfuric acid and ammonia: nucleation and growth model based on thermodynamics derived from CLOUD measurements for a wide range of conditions
Andreas Kürten
CORRESPONDING AUTHOR
Institute for Atmospheric and Environmental Sciences, Goethe University
Frankfurt, 60438 Frankfurt am Main, Germany
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37 citations as recorded by crossref.
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- Role of iodine oxoacids in atmospheric aerosol nucleation X. He et al. 10.1126/science.abe0298
- Enhanced growth rate of atmospheric particles from sulfuric acid D. Stolzenburg et al. 10.5194/acp-20-7359-2020
- Neutral Sulfuric Acid–Water Clustering Rates: Bridging the Gap between Molecular Simulation and Experiment P. Carlsson et al. 10.1021/acs.jpclett.0c01045
- A consistent formation free energy definition for multicomponent clusters in quantum thermochemistry R. Halonen 10.1016/j.jaerosci.2022.105974
- What chemical species are responsible for new particle formation and growth in the Netherlands? A hybrid positive matrix factorization (PMF) analysis using aerosol composition (ACSM) and size (SMPS) F. Nursanto et al. 10.5194/acp-23-10015-2023
- Influence of vegetation on occurrence and time distributions of regional new aerosol particle formation and growth I. Salma et al. 10.5194/acp-21-2861-2021
- Modeling the formation and growth of atmospheric molecular clusters: A review J. Elm et al. 10.1016/j.jaerosci.2020.105621
- Real-time monitoring of aerosol particle formation from sulfuric acid vapor at elevated concentrations and temperatures D. Becker et al. 10.1039/D1CP04580F
- Boundary layer versus free tropospheric submicron particle formation: A case study from NASA DC-8 observations in the Asian continental outflow during the KORUS-AQ campaign D. Park et al. 10.1016/j.atmosres.2021.105857
- Chemistry of new particle formation and growth events during wintertime in suburban area of Beijing: Insights from highly polluted atmosphere S. Yang et al. 10.1016/j.atmosres.2021.105553
- Diurnal evolution of negative atmospheric ions above the boreal forest: from ground level to the free troposphere L. Beck et al. 10.5194/acp-22-8547-2022
- Atmospheric new particle formation from the CERN CLOUD experiment J. Kirkby et al. 10.1038/s41561-023-01305-0
- Investigation of new particle formation mechanisms and aerosol processes at Marambio Station, Antarctic Peninsula L. Quéléver et al. 10.5194/acp-22-8417-2022
- An extraction method for nitrogen isotope measurement of ammonium in a low-concentration environment A. Lamothe et al. 10.5194/amt-16-4015-2023
- Atmospheric nanoparticle growth D. Stolzenburg et al. 10.1103/RevModPhys.95.045002
- Technical note: Emission factors, chemical composition, and morphology of particles emitted from Euro 5 diesel and gasoline light-duty vehicles during transient cycles E. Kostenidou et al. 10.5194/acp-21-4779-2021
- H<sub>2</sub>SO<sub>4</sub> and particle production in a photolytic flow reactor: chemical modeling, cluster thermodynamics and contamination issues D. Hanson et al. 10.5194/acp-19-8999-2019
- The driving factors of new particle formation and growth in the polluted boundary layer M. Xiao et al. 10.5194/acp-21-14275-2021
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- In situ observation of new particle formation (NPF) in the tropical tropopause layer of the 2017 Asian monsoon anticyclone – Part 1: Summary of StratoClim results R. Weigel et al. 10.5194/acp-21-11689-2021
- Clustering of HClO4 with Brønsted (H2SO4, HClO4, HNO3) and Lewis acids BX3 (X = H, F, Cl, Br, OH): a DFT study Y. Valadbeigi & T. Kurtén 10.1039/C9NJ04694A
- Structural Diversity of Protonated Citric Acid-Ammonia Clusters and Its Atmospheric Implication S. Zhou et al. 10.1021/acs.jpca.3c05160
- Exploring the hydrogen-bonded interactions of vanillic acid with atmospheric bases: a DFT study T. de Oliveira et al. 10.1007/s11224-024-02307-3
- Measurement report: Sulfuric acid nucleation and experimental conditions in a photolytic flow reactor D. Hanson et al. 10.5194/acp-21-1987-2021
- Measurement of ammonia, amines and iodine compounds using protonated water cluster chemical ionization mass spectrometry J. Pfeifer et al. 10.5194/amt-13-2501-2020
- Quantum Machine Learning Approach for Studying Atmospheric Cluster Formation J. Kubečka et al. 10.1021/acs.estlett.1c00997
- Reduction of anthropogenic emissions enhanced atmospheric new particle formation: Observational evidence during the Beijing 2022 Winter Olympics W. Zhu et al. 10.1016/j.atmosenv.2023.120094
- Evidence of nitrate-based nighttime atmospheric nucleation driven by marine microorganisms in the South Pacific G. Chamba et al. 10.1073/pnas.2308696120
- Potential enhancement in atmospheric new particle formation by amine-assisted nitric acid condensation at room temperature K. Chen et al. 10.1016/j.atmosenv.2022.119252
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Short summary
New particle formation and growth are important processes affecting climate and air quality. A significant fraction of newly formed particles originates from sulfuric acid, water, and ammonia. The present study introduces a new process model for the calculation of aerosol nucleation and growth rates for the sulfuric acid–ammonia system. The thermodynamic parameters enabling these calculations are derived from laboratory (CLOUD chamber) measurements.
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