Articles | Volume 19, issue 5
https://doi.org/10.5194/acp-19-3137-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-3137-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
12 Mar 2019
Research article |
| 12 Mar 2019
| 12 Mar 2019
The potential role of methanesulfonic acid (MSA) in aerosol formation and growth and the associated radiative forcings
Anna L. Hodshire
CORRESPONDING AUTHOR
Department of Atmospheric Science, Colorado State University, Fort
Collins, CO 80523, USA
Pedro Campuzano-Jost
Department of Chemistry, University of Colorado, Boulder, CO, USA
Cooperative Institute for Research in Environmental Sciences,
University of Colorado, Boulder, CO, USA
John K. Kodros
Department of Atmospheric Science, Colorado State University, Fort
Collins, CO 80523, USA
Betty Croft
Dalhousie University, Department of Physics and Atmospheric Science,
Halifax, NS, B3H 4R2, Canada
Benjamin A. Nault
Department of Chemistry, University of Colorado, Boulder, CO, USA
Cooperative Institute for Research in Environmental Sciences,
University of Colorado, Boulder, CO, USA
Jason C. Schroder
Department of Chemistry, University of Colorado, Boulder, CO, USA
Cooperative Institute for Research in Environmental Sciences,
University of Colorado, Boulder, CO, USA
Jose L. Jimenez
Department of Chemistry, University of Colorado, Boulder, CO, USA
Cooperative Institute for Research in Environmental Sciences,
University of Colorado, Boulder, CO, USA
Jeffrey R. Pierce
Department of Atmospheric Science, Colorado State University, Fort
Collins, CO 80523, USA
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- Investigation of new particle formation mechanisms and aerosol processes at Marambio Station, Antarctic Peninsula L. Quéléver et al. 10.5194/acp-22-8417-2022
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- Emissions and radiative impacts of sub-10 nm particles from biofuel and fossil fuel cookstoves S. Jathar et al. 10.1080/02786826.2020.1769837
- Structural Effects of Amines in Enhancing Methanesulfonic Acid-Driven New Particle Formation J. Shen et al. 10.1021/acs.est.0c05358
- Modification of the Conversion of Dimethylsulfide to Methanesulfonic Acid by Anthropogenic Pollution as Revealed by Long-Term Observations B. Jiang et al. 10.1021/acsearthspacechem.1c00222
- Atmospheric Gas-Phase Formation of Methanesulfonic Acid J. Chen et al. 10.1021/acs.est.3c07120
- Oxygenated Aromatic Compounds are Important Precursors of Secondary Organic Aerosol in Biomass-Burning Emissions A. Akherati et al. 10.1021/acs.est.0c01345
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Discussed (final revised paper)
Latest update: 20 Nov 2024
Short summary
A global chemical-transport model is used to determine the impact of methanesulfonic acid (MSA) on the aerosol size distribution and associated radiative effects, testing varying assumptions of MSA’s effective volatility and nucleating ability. We find that MSA mass best matches the ATom airborne measurements when volatility varies as a function of temperature, relative humidity, and available gas-phase bases, and the MSA radiative forcing is on the order of -50 mW m-2 over the Southern Ocean.
A global chemical-transport model is used to determine the impact of methanesulfonic acid (MSA)...
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Final-revised paper
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