Articles | Volume 19, issue 4
https://doi.org/10.5194/acp-19-2327-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-2327-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Quantifying primary and secondary humic-like substances in urban aerosol based on emission source characterization and a source-oriented air quality model
Xinghua Li
CORRESPONDING AUTHOR
School of Space and Environment, Beihang University, Beijing, 100191,
China
Junzan Han
School of Space and Environment, Beihang University, Beijing, 100191,
China
Philip K. Hopke
Center for Air Resources Engineering and Science, Clarkson University,
Potsdam, NY, USA
Jingnan Hu
State Environmental Protection Key Laboratory of Vehicle Emission
Control and Simulation, Chinese Research Academy of Environmental Sciences,
Beijing 100012, China
Qi Shu
School of Space and Environment, Beihang University, Beijing, 100191,
China
Qing Chang
School of Space and Environment, Beihang University, Beijing, 100191,
China
Qi Ying
CORRESPONDING AUTHOR
Zachry Department of Civil Engineering, Texas A&M University,
College Station, TX 77843, USA
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Cited
29 citations as recorded by crossref.
- Characteristics, primary sources and secondary formation of water-soluble organic aerosols in downtown Beijing Q. Yu et al. 10.5194/acp-21-1775-2021
- Molecular composition and optical property of humic-like substances (HULIS) in winter-time PM2.5 in the rural area of North China Plain H. Sun et al. 10.1016/j.atmosenv.2021.118316
- Concentration, optical characteristics, and emission factors of brown carbon emitted by on-road vehicles R. Huang et al. 10.1016/j.scitotenv.2021.151307
- Atmospheric “HULIS” in Different Environments: Polarities, Molecular Sizes, and Sources Suggest More Than 50% Are Not “Humic-like” T. Spranger et al. 10.1021/acsearthspacechem.9b00299
- Light absorption and source apportionment of water soluble humic-like substances (HULIS) in PM2.5 at Nanjing, China M. Bao et al. 10.1016/j.envres.2021.112554
- Brown carbon: An underlying driving force for rapid atmospheric sulfate formation and haze event Y. Liu et al. 10.1016/j.scitotenv.2020.139415
- Significant seasonal changes in optical properties of brown carbon in the midlatitude atmosphere H. Han et al. 10.5194/acp-20-2709-2020
- Estimating mean molecular weight, carbon number, and OM∕OC with mid-infrared spectroscopy in organic particulate matter samples from a monitoring network A. Yazdani et al. 10.5194/amt-14-4805-2021
- Temporal and Spatial Trends in Particulate Matter and the Responses to Meteorological Conditions and Environmental Management in Xi’an, China Y. Tian et al. 10.3390/atmos12091112
- Seasonal and diurnal variation of PM2.5 HULIS over Xi'an in Northwest China: Optical properties, chemical functional group, and relationship with reactive oxygen species (ROS) T. Zhang et al. 10.1016/j.atmosenv.2021.118782
- Improving apportionment of PM2.5 using multisite PMF by constraining G-values with a prioriinformation Q. Dai et al. 10.1016/j.scitotenv.2020.139657
- Light absorption properties and molecular profiles of HULIS in PM2.5 emitted from biomass burning in traditional “Heated Kang” in Northwest China T. Zhang et al. 10.1016/j.scitotenv.2021.146014
- Associations between ambient fine particulate matter and child respiratory infection: The role of particulate matter source composition in Dhaka, Bangladesh A. Sherris et al. 10.1016/j.envpol.2021.118073
- Chemical Fingerprinting of HULIS in Particulate Matters Emitted from Residential Coal and Biomass Combustion Y. Huo et al. 10.1021/acs.est.0c08518
- Theoretical equilibration time is supported by measurement study of residence time at dilution sampling on fine particulate matter emissions from household biofuel burning X. Li et al. 10.1016/j.chemosphere.2020.129178
- Why it makes sense that increased PM 2.5 was correlated with anthropogenic combustion-derived water P. Hopke & Q. Dai 10.1073/pnas.2102255118
- Relative effects of open biomass burning and open crop straw burning on haze formation over central and eastern China: modeling study driven by constrained emissions K. Mehmood et al. 10.5194/acp-20-2419-2020
- Global review of recent source apportionments for airborne particulate matter P. Hopke et al. 10.1016/j.scitotenv.2020.140091
- Evaluation of regional transport of PM2.5 during severe atmospheric pollution episodes in the western Yangtze River Delta, China I. Sulaymon et al. 10.1016/j.jenvman.2021.112827
- Fluorescence characteristics of water-soluble organic carbon in atmospheric aerosol☆ G. Wu et al. 10.1016/j.envpol.2020.115906
- Carbonaceous aerosols emission reduction by using red mud additive in coal briquette Y. Zhang et al. 10.1016/j.fuproc.2019.106290
- Increased secondary aerosol contribution and possible processing on polluted winter days in China Y. Wang et al. 10.1016/j.envint.2019.03.021
- Approval Research for Carcinogen Humic-Like Substances (HULIS) Emitted from Residential Coal Combustion in High Lung Cancer Incidence Areas of China K. Xiao et al. 10.3390/pr9071254
- Chemical composition, optical properties, and oxidative potential of water- and methanol-soluble organic compounds emitted from the combustion of biomass materials and coal T. Cao et al. 10.5194/acp-21-13187-2021
- Changing Emissions Results in Changed PM2.5 Composition and Health Impacts P. Hopke & G. Hidy 10.3390/atmos13020193
- Distinctive Sources Govern Organic Aerosol Fractions with Different Degrees of Oxygenation in the Urban Atmosphere R. Zhou et al. 10.1021/acs.est.0c08604
- Aqueous-phase reactive species formed by fine particulate matter from remote forests and polluted urban air H. Tong et al. 10.5194/acp-21-10439-2021
- Sources of humic-like substances (HULIS) in PM2.5 in Beijing: Receptor modeling approach X. Li et al. 10.1016/j.scitotenv.2019.03.333
- Concentrations, optical properties and sources of humic-like substances (HULIS) in fine particulate matter in Xi'an, Northwest China W. Yuan et al. 10.1016/j.scitotenv.2021.147902
29 citations as recorded by crossref.
- Characteristics, primary sources and secondary formation of water-soluble organic aerosols in downtown Beijing Q. Yu et al. 10.5194/acp-21-1775-2021
- Molecular composition and optical property of humic-like substances (HULIS) in winter-time PM2.5 in the rural area of North China Plain H. Sun et al. 10.1016/j.atmosenv.2021.118316
- Concentration, optical characteristics, and emission factors of brown carbon emitted by on-road vehicles R. Huang et al. 10.1016/j.scitotenv.2021.151307
- Atmospheric “HULIS” in Different Environments: Polarities, Molecular Sizes, and Sources Suggest More Than 50% Are Not “Humic-like” T. Spranger et al. 10.1021/acsearthspacechem.9b00299
- Light absorption and source apportionment of water soluble humic-like substances (HULIS) in PM2.5 at Nanjing, China M. Bao et al. 10.1016/j.envres.2021.112554
- Brown carbon: An underlying driving force for rapid atmospheric sulfate formation and haze event Y. Liu et al. 10.1016/j.scitotenv.2020.139415
- Significant seasonal changes in optical properties of brown carbon in the midlatitude atmosphere H. Han et al. 10.5194/acp-20-2709-2020
- Estimating mean molecular weight, carbon number, and OM∕OC with mid-infrared spectroscopy in organic particulate matter samples from a monitoring network A. Yazdani et al. 10.5194/amt-14-4805-2021
- Temporal and Spatial Trends in Particulate Matter and the Responses to Meteorological Conditions and Environmental Management in Xi’an, China Y. Tian et al. 10.3390/atmos12091112
- Seasonal and diurnal variation of PM2.5 HULIS over Xi'an in Northwest China: Optical properties, chemical functional group, and relationship with reactive oxygen species (ROS) T. Zhang et al. 10.1016/j.atmosenv.2021.118782
- Improving apportionment of PM2.5 using multisite PMF by constraining G-values with a prioriinformation Q. Dai et al. 10.1016/j.scitotenv.2020.139657
- Light absorption properties and molecular profiles of HULIS in PM2.5 emitted from biomass burning in traditional “Heated Kang” in Northwest China T. Zhang et al. 10.1016/j.scitotenv.2021.146014
- Associations between ambient fine particulate matter and child respiratory infection: The role of particulate matter source composition in Dhaka, Bangladesh A. Sherris et al. 10.1016/j.envpol.2021.118073
- Chemical Fingerprinting of HULIS in Particulate Matters Emitted from Residential Coal and Biomass Combustion Y. Huo et al. 10.1021/acs.est.0c08518
- Theoretical equilibration time is supported by measurement study of residence time at dilution sampling on fine particulate matter emissions from household biofuel burning X. Li et al. 10.1016/j.chemosphere.2020.129178
- Why it makes sense that increased PM 2.5 was correlated with anthropogenic combustion-derived water P. Hopke & Q. Dai 10.1073/pnas.2102255118
- Relative effects of open biomass burning and open crop straw burning on haze formation over central and eastern China: modeling study driven by constrained emissions K. Mehmood et al. 10.5194/acp-20-2419-2020
- Global review of recent source apportionments for airborne particulate matter P. Hopke et al. 10.1016/j.scitotenv.2020.140091
- Evaluation of regional transport of PM2.5 during severe atmospheric pollution episodes in the western Yangtze River Delta, China I. Sulaymon et al. 10.1016/j.jenvman.2021.112827
- Fluorescence characteristics of water-soluble organic carbon in atmospheric aerosol☆ G. Wu et al. 10.1016/j.envpol.2020.115906
- Carbonaceous aerosols emission reduction by using red mud additive in coal briquette Y. Zhang et al. 10.1016/j.fuproc.2019.106290
- Increased secondary aerosol contribution and possible processing on polluted winter days in China Y. Wang et al. 10.1016/j.envint.2019.03.021
- Approval Research for Carcinogen Humic-Like Substances (HULIS) Emitted from Residential Coal Combustion in High Lung Cancer Incidence Areas of China K. Xiao et al. 10.3390/pr9071254
- Chemical composition, optical properties, and oxidative potential of water- and methanol-soluble organic compounds emitted from the combustion of biomass materials and coal T. Cao et al. 10.5194/acp-21-13187-2021
- Changing Emissions Results in Changed PM2.5 Composition and Health Impacts P. Hopke & G. Hidy 10.3390/atmos13020193
- Distinctive Sources Govern Organic Aerosol Fractions with Different Degrees of Oxygenation in the Urban Atmosphere R. Zhou et al. 10.1021/acs.est.0c08604
- Aqueous-phase reactive species formed by fine particulate matter from remote forests and polluted urban air H. Tong et al. 10.5194/acp-21-10439-2021
- Sources of humic-like substances (HULIS) in PM2.5 in Beijing: Receptor modeling approach X. Li et al. 10.1016/j.scitotenv.2019.03.333
- Concentrations, optical properties and sources of humic-like substances (HULIS) in fine particulate matter in Xi'an, Northwest China W. Yuan et al. 10.1016/j.scitotenv.2021.147902
Latest update: 21 Mar 2023
Short summary
HULIS are widely distributed in atmospheric aerosol. Their sources are rarely studied quantitatively. Biomass burning is generally accepted as a major primary source with additional secondary material formed in the atmosphere. The present study provides direct evidence that residential coal burning is also a significant source of ambient HULIS in northern China based on source measurements, ambient sampling and analysis, and apportionment with source-oriented CMAQ modeling.
HULIS are widely distributed in atmospheric aerosol. Their sources are rarely studied...
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