Articles | Volume 19, issue 24
https://doi.org/10.5194/acp-19-15673-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-15673-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
20 Dec 2019
Research article |
| 20 Dec 2019
| 20 Dec 2019
Detection of tar brown carbon with a single particle soot photometer (SP2)
Joel C. Corbin
CORRESPONDING AUTHOR
Metrology Research Centre, 1200 Montreal Road, National Research Council Canada, Ottawa, ON K1A 0R6, Canada
Martin Gysel-Beer
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232 Villigen PSI, Switzerland
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Cited
29 citations as recorded by crossref.
- Relating the single particle soot photometer (SP2) signal response to soot maturity L. Nilsson et al. 10.1080/02786826.2024.2341057
- Intercomparison of equivalent black carbon (eBC) and elemental carbon (EC) concentrations with three-year continuous measurement in Beijing, China X. Liu et al. 10.1016/j.envres.2022.112791
- A dominant contribution to light absorption by methanol-insoluble brown carbon produced in the combustion of biomass fuels typically consumed in wildland fires in the United States K. Atwi et al. 10.1039/D1EA00065A
- Concentration and Physical Characteristics of Black Carbon in Winter Snow of Beijing in 2015 D. Zhao et al. 10.3390/atmos12070816
- Gaseous and particulate pollutant emissions from ocean-going tankers in the context of carbon reduction: Main engine, auxiliary engine, and auxiliary boiler S. Zhou et al. 10.1016/j.energy.2024.133831
- Undersizing of aged African biomass burning aerosol by an ultra-high-sensitivity aerosol spectrometer S. Howell et al. 10.5194/amt-14-7381-2021
- Detailed characterization of the CAPS single-scattering albedo monitor (CAPS PMssa) as a field-deployable instrument for measuring aerosol light absorption with the extinction-minus-scattering method R. Modini et al. 10.5194/amt-14-819-2021
- Evaluating emissions and air quality implications of residential waste incineration D. Mentes et al. 10.1038/s41598-024-72173-w
- Comparison of co-located refractory black carbon (rBC) and elemental carbon (EC) mass concentration measurements during field campaigns at several European sites R. Pileci et al. 10.5194/amt-14-1379-2021
- An overview of optical and thermal methods for the characterization of carbonaceous aerosol D. Massabò & P. Prati 10.1007/s40766-021-00017-8
- Overview of methods to characterize the mass, size, and morphology of soot T. Sipkens et al. 10.1016/j.jaerosci.2023.106211
- Shortwave absorption by wildfire smoke dominated by dark brown carbon R. Chakrabarty et al. 10.1038/s41561-023-01237-9
- Microphysical properties of atmospheric soot and organic particles: measurements, modeling, and impacts W. Li et al. 10.1038/s41612-024-00610-8
- Reduction in greenhouse gas and other emissions from ship engines: Current trends and future options P. Aakko-Saksa et al. 10.1016/j.pecs.2022.101055
- Suitability of Different Methods for Measuring Black Carbon Emissions from Marine Engines P. Aakko-Saksa et al. 10.3390/atmos13010031
- Rapid evolution of aerosol particles and their optical properties downwind of wildfires in the western US L. Kleinman et al. 10.5194/acp-20-13319-2020
- Ash-Decorated and Ash-Painted Soot from Residual and Distillate-Fuel Combustion in Four Marine Engines and One Aviation Engine S. Gagné et al. 10.1021/acs.est.0c07130
- Mass and Light Absorption Properties of Atmospheric Carbonaceous Aerosols over the Outflow Regions of Indo-Gangetic Plain A. Soni et al. 10.1016/j.atmosenv.2024.120413
- Occurrence, abundance, and formation of atmospheric tarballs from a wide range of wildfires in the western US K. Adachi et al. 10.5194/acp-24-10985-2024
- Closure between particulate matter concentrations measured ex situ by thermal–optical analysis and in situ by the CPMA–electrometer reference mass system J. Corbin et al. 10.1080/02786826.2020.1788710
- Dark brown carbon from wildfires: a potent snow radiative forcing agent? G. Chelluboyina et al. 10.1038/s41612-024-00738-7
- Carbonaceous Nanoparticle Air Pollution: Toxicity and Detection in Biological Samples I. Aslam & M. Roeffaers 10.3390/nano12223948
- Comparison of the LEO and CPMA-SP2 techniques for black-carbon mixing-state measurements A. Naseri et al. 10.5194/amt-17-3719-2024
- A 2-year intercomparison of three methods for measuring black carbon concentration at a high-altitude research station in Europe S. Tinorua et al. 10.5194/amt-17-3897-2024
- Climate-relevant properties of black carbon aerosols revealed by in situ measurements: a review N. Moteki 10.1186/s40645-023-00544-4
- Evidence for Large Amounts of Brown Carbonaceous Tarballs in the Himalayan Atmosphere Q. Yuan et al. 10.1021/acs.estlett.0c00735
- Water/Methanol-Insoluble Brown Carbon Can Dominate Aerosol-Enhanced Light Absorption in Port Cities Z. Bai et al. 10.1021/acs.est.0c03844
- Comparison of black carbon measurement techniques for marine engine emissions using three marine fuel types A. Momenimovahed et al. 10.1080/02786826.2021.1967281
- Review of Brown Carbon Aerosols in China: Pollution Level, Optical Properties, and Emissions Q. Wang et al. 10.1029/2021JD035473
29 citations as recorded by crossref.
- Relating the single particle soot photometer (SP2) signal response to soot maturity L. Nilsson et al. 10.1080/02786826.2024.2341057
- Intercomparison of equivalent black carbon (eBC) and elemental carbon (EC) concentrations with three-year continuous measurement in Beijing, China X. Liu et al. 10.1016/j.envres.2022.112791
- A dominant contribution to light absorption by methanol-insoluble brown carbon produced in the combustion of biomass fuels typically consumed in wildland fires in the United States K. Atwi et al. 10.1039/D1EA00065A
- Concentration and Physical Characteristics of Black Carbon in Winter Snow of Beijing in 2015 D. Zhao et al. 10.3390/atmos12070816
- Gaseous and particulate pollutant emissions from ocean-going tankers in the context of carbon reduction: Main engine, auxiliary engine, and auxiliary boiler S. Zhou et al. 10.1016/j.energy.2024.133831
- Undersizing of aged African biomass burning aerosol by an ultra-high-sensitivity aerosol spectrometer S. Howell et al. 10.5194/amt-14-7381-2021
- Detailed characterization of the CAPS single-scattering albedo monitor (CAPS PMssa) as a field-deployable instrument for measuring aerosol light absorption with the extinction-minus-scattering method R. Modini et al. 10.5194/amt-14-819-2021
- Evaluating emissions and air quality implications of residential waste incineration D. Mentes et al. 10.1038/s41598-024-72173-w
- Comparison of co-located refractory black carbon (rBC) and elemental carbon (EC) mass concentration measurements during field campaigns at several European sites R. Pileci et al. 10.5194/amt-14-1379-2021
- An overview of optical and thermal methods for the characterization of carbonaceous aerosol D. Massabò & P. Prati 10.1007/s40766-021-00017-8
- Overview of methods to characterize the mass, size, and morphology of soot T. Sipkens et al. 10.1016/j.jaerosci.2023.106211
- Shortwave absorption by wildfire smoke dominated by dark brown carbon R. Chakrabarty et al. 10.1038/s41561-023-01237-9
- Microphysical properties of atmospheric soot and organic particles: measurements, modeling, and impacts W. Li et al. 10.1038/s41612-024-00610-8
- Reduction in greenhouse gas and other emissions from ship engines: Current trends and future options P. Aakko-Saksa et al. 10.1016/j.pecs.2022.101055
- Suitability of Different Methods for Measuring Black Carbon Emissions from Marine Engines P. Aakko-Saksa et al. 10.3390/atmos13010031
- Rapid evolution of aerosol particles and their optical properties downwind of wildfires in the western US L. Kleinman et al. 10.5194/acp-20-13319-2020
- Ash-Decorated and Ash-Painted Soot from Residual and Distillate-Fuel Combustion in Four Marine Engines and One Aviation Engine S. Gagné et al. 10.1021/acs.est.0c07130
- Mass and Light Absorption Properties of Atmospheric Carbonaceous Aerosols over the Outflow Regions of Indo-Gangetic Plain A. Soni et al. 10.1016/j.atmosenv.2024.120413
- Occurrence, abundance, and formation of atmospheric tarballs from a wide range of wildfires in the western US K. Adachi et al. 10.5194/acp-24-10985-2024
- Closure between particulate matter concentrations measured ex situ by thermal–optical analysis and in situ by the CPMA–electrometer reference mass system J. Corbin et al. 10.1080/02786826.2020.1788710
- Dark brown carbon from wildfires: a potent snow radiative forcing agent? G. Chelluboyina et al. 10.1038/s41612-024-00738-7
- Carbonaceous Nanoparticle Air Pollution: Toxicity and Detection in Biological Samples I. Aslam & M. Roeffaers 10.3390/nano12223948
- Comparison of the LEO and CPMA-SP2 techniques for black-carbon mixing-state measurements A. Naseri et al. 10.5194/amt-17-3719-2024
- A 2-year intercomparison of three methods for measuring black carbon concentration at a high-altitude research station in Europe S. Tinorua et al. 10.5194/amt-17-3897-2024
- Climate-relevant properties of black carbon aerosols revealed by in situ measurements: a review N. Moteki 10.1186/s40645-023-00544-4
- Evidence for Large Amounts of Brown Carbonaceous Tarballs in the Himalayan Atmosphere Q. Yuan et al. 10.1021/acs.estlett.0c00735
- Water/Methanol-Insoluble Brown Carbon Can Dominate Aerosol-Enhanced Light Absorption in Port Cities Z. Bai et al. 10.1021/acs.est.0c03844
- Comparison of black carbon measurement techniques for marine engine emissions using three marine fuel types A. Momenimovahed et al. 10.1080/02786826.2021.1967281
- Review of Brown Carbon Aerosols in China: Pollution Level, Optical Properties, and Emissions Q. Wang et al. 10.1029/2021JD035473
Latest update: 14 Dec 2024
Short summary
We review the literature to refine the definition of "tar balls" (or tar particles). Then, using a marine-engine data set, we show that a standard SP2 can identify tar particles in two ways, as evaporating and non-incandescing (30 % of tar particles by number) or incandescing particles which scatter more light than soot at incandescence (70 % of tar particles by number). To our knowledge, no other technique can provide in situ, real-time evidence for the presence of tar particles in an aerosol.
We review the literature to refine the definition of "tar balls" (or tar particles). Then, using...
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