Articles | Volume 19, issue 24
https://doi.org/10.5194/acp-19-15609-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-15609-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
20 Dec 2019
Research article |
| 20 Dec 2019
| 20 Dec 2019
Sources and formation of carbonaceous aerosols in Xi'an, China: primary emissions and secondary formation constrained by radiocarbon
Haiyan Ni
State Key Laboratory of Loess and Quaternary Geology, Key Laboratory of Aerosol Chemistry and Physics, Center for Excellence in Quaternary Science and Global Change, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an, 710061, China
Centre for Isotope Research (CIO), Energy and Sustainability Research Institute Groningen (ESRIG), University of Groningen, Groningen, 9747 AG, the Netherlands
University of Chinese Academy of Sciences, Beijing, 100049, China
Ru-Jin Huang
CORRESPONDING AUTHOR
State Key Laboratory of Loess and Quaternary Geology, Key Laboratory of Aerosol Chemistry and Physics, Center for Excellence in Quaternary Science and Global Change, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an, 710061, China
Institute of Global Environmental Change, Xi’an Jiaotong University, Xi’an, 710049, China
Junji Cao
State Key Laboratory of Loess and Quaternary Geology, Key Laboratory of Aerosol Chemistry and Physics, Center for Excellence in Quaternary Science and Global Change, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an, 710061, China
Jie Guo
State Key Laboratory of Loess and Quaternary Geology, Key Laboratory of Aerosol Chemistry and Physics, Center for Excellence in Quaternary Science and Global Change, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an, 710061, China
Haoyue Deng
Centre for Isotope Research (CIO), Energy and Sustainability Research Institute Groningen (ESRIG), University of Groningen, Groningen, 9747 AG, the Netherlands
Ulrike Dusek
Centre for Isotope Research (CIO), Energy and Sustainability Research Institute Groningen (ESRIG), University of Groningen, Groningen, 9747 AG, the Netherlands
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Cited
17 citations as recorded by crossref.
- Source apportionment of carbonaceous aerosols in diverse atmospheric environments of China by dual-carbon isotope method M. Li et al. 10.1016/j.scitotenv.2021.150654
- 13C signatures of aerosol organic and elemental carbon from major combustion sources in China compared to worldwide estimates P. Yao et al. 10.1016/j.scitotenv.2021.151284
- Non‐Fossil Origin Explains the Large Seasonal Variation of Highly Processed Organic Aerosol in the Northeastern Tibetan Plateau (3,200 m a.s.l.) H. Ni et al. 10.1029/2023GL104710
- Quantification of fossil and non-fossil sources to the reduction of carbonaceous aerosols in the Yangtze River Delta, China: Insights from radiocarbon analysis during 2014–2019 M. Yu et al. 10.1016/j.atmosenv.2022.119421
- Trends in the development and utilization of agricultural wastes as heterogeneous catalyst for biodiesel production O. Awogbemi et al. 10.1016/j.joei.2021.06.017
- An automated method for thermal-optical separation of aerosol organic/elemental carbon for 13C analysis at the sub-μgC level: A comprehensive assessment P. Yao et al. 10.1016/j.scitotenv.2021.150031
- Distinctive Sources Govern Organic Aerosol Fractions with Different Degrees of Oxygenation in the Urban Atmosphere R. Zhou et al. 10.1021/acs.est.0c08604
- Sediment Soot Radiocarbon Indicates that Recent Pollution Controls Slowed Fossil Fuel Emissions in Southeastern China Y. Han et al. 10.1021/acs.est.1c05424
- First Measurements of Carbonaceous Aerosol across Urban, Rural and Residential Areas in Jeddah City, Saudi Arabia I. Ismail et al. 10.5572/ajae.2021.021
- The outflow of Asian biomass burning carbonaceous aerosol into the upper troposphere and lower stratosphere in spring: radiative effects seen in a global model P. Chavan et al. 10.5194/acp-21-14371-2021
- A Novel Apportionment Method Utilizing Particle Mass Size Distribution across Multiple Particle Size Ranges P. Wang et al. 10.3390/atmos15080955
- Weak transport of atmospheric water-insoluble particulate carbon from South Asia to the inner Tibetan Plateau in the monsoon season C. Li et al. 10.1016/j.scitotenv.2024.171321
- Characterization of aerosol composition: Insights from SEM-EDX analysis and CALIPSO overpasses R. Rajan et al. 10.1016/j.asr.2024.07.058
- Measurement report: dual-carbon isotopic characterization of carbonaceous aerosol reveals different primary and secondary sources in Beijing and Xi'an during severe haze events H. Ni et al. 10.5194/acp-20-16041-2020
- Organic aerosol formation and aging processes in Beijing constrained by size-resolved measurements of radiocarbon and stable isotopic 13C H. Ni et al. 10.1016/j.envint.2021.106890
- Significant Contribution of Primary Sources to Water-Soluble Organic Carbon During Spring in Beijing, China Y. Jin et al. 10.3390/atmos11040395
- Optical properties and potential sources of water-soluble and methanol-soluble organic aerosols in Taipei, Taiwan Y. Ting et al. 10.1016/j.atmosenv.2022.119364
17 citations as recorded by crossref.
- Source apportionment of carbonaceous aerosols in diverse atmospheric environments of China by dual-carbon isotope method M. Li et al. 10.1016/j.scitotenv.2021.150654
- 13C signatures of aerosol organic and elemental carbon from major combustion sources in China compared to worldwide estimates P. Yao et al. 10.1016/j.scitotenv.2021.151284
- Non‐Fossil Origin Explains the Large Seasonal Variation of Highly Processed Organic Aerosol in the Northeastern Tibetan Plateau (3,200 m a.s.l.) H. Ni et al. 10.1029/2023GL104710
- Quantification of fossil and non-fossil sources to the reduction of carbonaceous aerosols in the Yangtze River Delta, China: Insights from radiocarbon analysis during 2014–2019 M. Yu et al. 10.1016/j.atmosenv.2022.119421
- Trends in the development and utilization of agricultural wastes as heterogeneous catalyst for biodiesel production O. Awogbemi et al. 10.1016/j.joei.2021.06.017
- An automated method for thermal-optical separation of aerosol organic/elemental carbon for 13C analysis at the sub-μgC level: A comprehensive assessment P. Yao et al. 10.1016/j.scitotenv.2021.150031
- Distinctive Sources Govern Organic Aerosol Fractions with Different Degrees of Oxygenation in the Urban Atmosphere R. Zhou et al. 10.1021/acs.est.0c08604
- Sediment Soot Radiocarbon Indicates that Recent Pollution Controls Slowed Fossil Fuel Emissions in Southeastern China Y. Han et al. 10.1021/acs.est.1c05424
- First Measurements of Carbonaceous Aerosol across Urban, Rural and Residential Areas in Jeddah City, Saudi Arabia I. Ismail et al. 10.5572/ajae.2021.021
- The outflow of Asian biomass burning carbonaceous aerosol into the upper troposphere and lower stratosphere in spring: radiative effects seen in a global model P. Chavan et al. 10.5194/acp-21-14371-2021
- A Novel Apportionment Method Utilizing Particle Mass Size Distribution across Multiple Particle Size Ranges P. Wang et al. 10.3390/atmos15080955
- Weak transport of atmospheric water-insoluble particulate carbon from South Asia to the inner Tibetan Plateau in the monsoon season C. Li et al. 10.1016/j.scitotenv.2024.171321
- Characterization of aerosol composition: Insights from SEM-EDX analysis and CALIPSO overpasses R. Rajan et al. 10.1016/j.asr.2024.07.058
- Measurement report: dual-carbon isotopic characterization of carbonaceous aerosol reveals different primary and secondary sources in Beijing and Xi'an during severe haze events H. Ni et al. 10.5194/acp-20-16041-2020
- Organic aerosol formation and aging processes in Beijing constrained by size-resolved measurements of radiocarbon and stable isotopic 13C H. Ni et al. 10.1016/j.envint.2021.106890
- Significant Contribution of Primary Sources to Water-Soluble Organic Carbon During Spring in Beijing, China Y. Jin et al. 10.3390/atmos11040395
- Optical properties and potential sources of water-soluble and methanol-soluble organic aerosols in Taipei, Taiwan Y. Ting et al. 10.1016/j.atmosenv.2022.119364
Latest update: 01 Nov 2024
Short summary
We present a 1-year source apportionment record of carbonaceous aerosols in Xi'an, China. Biomass burning strongly increases in winter, while seasonal changes of coal and liquid fossil fuel combustion are moderate. We find strong evidence for fossil secondary OC formation during the warm period that is further enhanced in stagnant, polluted conditions due to longer atmospheric residence times. At the same time we find that water-insoluble (primary) fossil is lost due to photochemical processing.
We present a 1-year source apportionment record of carbonaceous aerosols in Xi'an, China....
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