Articles | Volume 19, issue 22
https://doi.org/10.5194/acp-19-14311-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue:
https://doi.org/10.5194/acp-19-14311-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Sulfate formation during heavy winter haze events and the potential contribution from heterogeneous SO2 + NO2 reactions in the Yangtze River Delta region, China
Ling Huang
School of Environmental and Chemical Engineering, Shanghai University,
Shanghai, 200444, China
Jingyu An
State Environmental Protection Key Laboratory of the Cause and
Prevention of Urban Air Pollution Complex, Shanghai Academy of Environmental
Sciences, Shanghai, 200233, China
Bonyoung Koo
Bay Area Air Quality Management District, San Francisco, CA 94105, USA
Greg Yarwood
Ramboll, Novato, CA 95995, USA
Rusha Yan
State Environmental Protection Key Laboratory of the Cause and
Prevention of Urban Air Pollution Complex, Shanghai Academy of Environmental
Sciences, Shanghai, 200233, China
Yangjun Wang
School of Environmental and Chemical Engineering, Shanghai University,
Shanghai, 200444, China
State Environmental Protection Key Laboratory of the Cause and
Prevention of Urban Air Pollution Complex, Shanghai Academy of Environmental
Sciences, Shanghai, 200233, China
School of Environmental and Chemical Engineering, Shanghai University,
Shanghai, 200444, China
Viewed
Total article views: 2,856 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 29 Apr 2019)
HTML | XML | Total | Supplement | BibTeX | EndNote | |
---|---|---|---|---|---|---|
1,880 | 912 | 64 | 2,856 | 338 | 67 | 89 |
- HTML: 1,880
- PDF: 912
- XML: 64
- Total: 2,856
- Supplement: 338
- BibTeX: 67
- EndNote: 89
Total article views: 2,149 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 27 Nov 2019)
HTML | XML | Total | Supplement | BibTeX | EndNote | |
---|---|---|---|---|---|---|
1,511 | 593 | 45 | 2,149 | 194 | 59 | 78 |
- HTML: 1,511
- PDF: 593
- XML: 45
- Total: 2,149
- Supplement: 194
- BibTeX: 59
- EndNote: 78
Total article views: 707 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 29 Apr 2019)
HTML | XML | Total | Supplement | BibTeX | EndNote | |
---|---|---|---|---|---|---|
369 | 319 | 19 | 707 | 144 | 8 | 11 |
- HTML: 369
- PDF: 319
- XML: 19
- Total: 707
- Supplement: 144
- BibTeX: 8
- EndNote: 11
Viewed (geographical distribution)
Total article views: 2,856 (including HTML, PDF, and XML)
Thereof 2,759 with geography defined
and 97 with unknown origin.
Total article views: 2,149 (including HTML, PDF, and XML)
Thereof 2,074 with geography defined
and 75 with unknown origin.
Total article views: 707 (including HTML, PDF, and XML)
Thereof 685 with geography defined
and 22 with unknown origin.
Country | # | Views | % |
---|
Country | # | Views | % |
---|
Country | # | Views | % |
---|
Total: | 0 |
HTML: | 0 |
PDF: | 0 |
XML: | 0 |
- 1
1
Total: | 0 |
HTML: | 0 |
PDF: | 0 |
XML: | 0 |
- 1
1
Total: | 0 |
HTML: | 0 |
PDF: | 0 |
XML: | 0 |
- 1
1
Cited
36 citations as recorded by crossref.
- 基于WRF-Chem/DART的硫酸盐化学反应速率同化研究 丛. 黄 et al. 10.1360/SSTe-2023-0057
- Unveiling the Role of Carbonate Radical Anions in Dust‐Driven SO2 Oxidation Y. Liu et al. 10.1029/2023JD040017
- Exploring dust heterogeneous chemistry over China: Insights from field observation and GEOS-Chem simulation R. Tian et al. 10.1016/j.scitotenv.2021.149307
- Sensitivity analysis of the surface ozone and fine particulate matter to meteorological parameters in China Z. Shi et al. 10.5194/acp-20-13455-2020
- Global estimates of ambient reactive nitrogen components during 2000–2100 based on the multi-stage model R. Li et al. 10.5194/acp-24-7623-2024
- A novel pathway of atmospheric sulfate formation through carbonate radicals Y. Liu et al. 10.5194/acp-22-9175-2022
- Incorporation and improvement of a heterogeneous chemistry mechanism in the atmospheric chemistry model GRAPES_Meso5.1/CUACE and its impacts on secondary inorganic aerosol and PM2.5 simulations in Middle-Eastern China Z. Liu et al. 10.1016/j.scitotenv.2022.157530
- Significant formation of sulfate aerosols contributed by the heterogeneous drivers of dust surface T. Wang et al. 10.5194/acp-22-13467-2022
- Key Factors Determining the Formation of Sulfate Aerosols Through Multiphase Chemistry—A Kinetic Modeling Study Based on Beijing Conditions T. Wang et al. 10.1029/2022JD038382
- Improvement and Uncertainties of Global Simulation of Sulfate Concentration and Radiative Forcing in CESM2 W. Ge et al. 10.1029/2022JD037623
- Aerosol water content enhancement leads to changes in the major formation mechanisms of nitrate and secondary organic aerosols in winter over the North China Plain C. Chen et al. 10.1016/j.envpol.2021.117625
- A Novel Hybrid Machine Learning Method (OR-ELM-AR) Used in Forecast of PM2.5 Concentrations and Its Forecast Performance Evaluation G. Lu et al. 10.3390/atmos12010078
- Strategies towards PM2.5 attainment for non-compliant cities in China: A case study H. Ling et al. 10.1016/j.jenvman.2021.113529
- Study on the assimilation of the sulphate reaction rates based on WRF-Chem/DART C. Huang et al. 10.1007/s11430-023-1153-9
- Improvement of inorganic aerosol component in PM2.5 by constraining aqueous-phase formation of sulfate in cloud with satellite retrievals: WRF-Chem simulations T. Sha et al. 10.1016/j.scitotenv.2021.150229
- Characteristics of air pollution episodes influenced by biomass burning pollution in Shanghai, China S. Tong et al. 10.1016/j.atmosenv.2020.117756
- Influence of atmospheric in-cloud aqueous-phase chemistry on the global simulation of SO<sub>2</sub> in CESM2 W. Ge et al. 10.5194/acp-21-16093-2021
- Recommendations on benchmarks for photochemical air quality model applications in China — NO2, SO2, CO and PM10 H. Zhai et al. 10.1016/j.atmosenv.2023.120290
- Evaluation and Bias Correction of the Secondary Inorganic Aerosol Modeling over North China Plain in Autumn and Winter Q. Wu et al. 10.3390/atmos12050578
- Assessment of the impacts of cloud chemistry on surface SO2 and sulfate levels in typical regions of China J. Lu et al. 10.5194/acp-23-8021-2023
- PM2.5 and O3 relationships affected by the atmospheric oxidizing capacity in the Yangtze River Delta, China M. Qin et al. 10.1016/j.scitotenv.2021.152268
- Secondary PM2.5 dominates aerosol pollution in the Yangtze River Delta region: Environmental and health effects of the Clean air Plan N. Li et al. 10.1016/j.envint.2022.107725
- Recommendations on benchmarks for numerical air quality model applications in China – Part 1: PM<sub>2.5</sub> and chemical species L. Huang et al. 10.5194/acp-21-2725-2021
- Air quality changes during the COVID-19 lockdown over the Yangtze River Delta Region: An insight into the impact of human activity pattern changes on air pollution variation L. Li et al. 10.1016/j.scitotenv.2020.139282
- Assessment of the effects of straw burning bans in China: Emissions, air quality, and health impacts L. Huang et al. 10.1016/j.scitotenv.2021.147935
- Response of PM2.5 chemical composition to the emission reduction and meteorological variation during the COVID-19 lockdown Y. Gong et al. 10.1016/j.chemosphere.2024.142844
- Heterogeneous interactions between SO<sub>2</sub> and organic peroxides in submicron aerosol S. Wang et al. 10.5194/acp-21-6647-2021
- The combined effects of heterogeneous chemistry and aerosol-radiation interaction on severe haze simulation by atmospheric chemistry model in Middle-Eastern China Z. Liu et al. 10.1016/j.atmosenv.2023.119729
- Wintertime Formation of Large Sulfate Particles in China and Implications for Human Health Q. Zhang et al. 10.1021/acs.est.3c05645
- Hourly organic tracers-based source apportionment of PM2.5 before and during the Covid-19 lockdown in suburban Shanghai, China: Insights into regional transport influences and response to urban emission reductions S. Wang et al. 10.1016/j.atmosenv.2022.119308
- Air pollutant variations in Suzhou during the 2019 novel coronavirus (COVID-19) lockdown of 2020: High time-resolution measurements of aerosol chemical compositions and source apportionment H. Wang et al. 10.1016/j.envpol.2020.116298
- Ammonium nitrate promotes sulfate formation through uptake kinetic regime Y. Liu et al. 10.5194/acp-21-13269-2021
- Estimation of secondary PM<sub>2.5</sub> in China and the United States using a multi-tracer approach H. Zhang et al. 10.5194/acp-22-5495-2022
- Bias in ammonia emission inventory and implications on emission control of nitrogen oxides over North China Plain Q. Zhang et al. 10.1016/j.atmosenv.2019.116869
- Estimation of interannual trends of ammonia emissions from agriculture in Jiangsu Province from 2000 to 2017 J. HUANG et al. 10.1080/16742834.2020.1736499
- Efficient control of atmospheric sulfate production based on three formation regimes J. Xue et al. 10.1038/s41561-019-0485-5
33 citations as recorded by crossref.
- 基于WRF-Chem/DART的硫酸盐化学反应速率同化研究 丛. 黄 et al. 10.1360/SSTe-2023-0057
- Unveiling the Role of Carbonate Radical Anions in Dust‐Driven SO2 Oxidation Y. Liu et al. 10.1029/2023JD040017
- Exploring dust heterogeneous chemistry over China: Insights from field observation and GEOS-Chem simulation R. Tian et al. 10.1016/j.scitotenv.2021.149307
- Sensitivity analysis of the surface ozone and fine particulate matter to meteorological parameters in China Z. Shi et al. 10.5194/acp-20-13455-2020
- Global estimates of ambient reactive nitrogen components during 2000–2100 based on the multi-stage model R. Li et al. 10.5194/acp-24-7623-2024
- A novel pathway of atmospheric sulfate formation through carbonate radicals Y. Liu et al. 10.5194/acp-22-9175-2022
- Incorporation and improvement of a heterogeneous chemistry mechanism in the atmospheric chemistry model GRAPES_Meso5.1/CUACE and its impacts on secondary inorganic aerosol and PM2.5 simulations in Middle-Eastern China Z. Liu et al. 10.1016/j.scitotenv.2022.157530
- Significant formation of sulfate aerosols contributed by the heterogeneous drivers of dust surface T. Wang et al. 10.5194/acp-22-13467-2022
- Key Factors Determining the Formation of Sulfate Aerosols Through Multiphase Chemistry—A Kinetic Modeling Study Based on Beijing Conditions T. Wang et al. 10.1029/2022JD038382
- Improvement and Uncertainties of Global Simulation of Sulfate Concentration and Radiative Forcing in CESM2 W. Ge et al. 10.1029/2022JD037623
- Aerosol water content enhancement leads to changes in the major formation mechanisms of nitrate and secondary organic aerosols in winter over the North China Plain C. Chen et al. 10.1016/j.envpol.2021.117625
- A Novel Hybrid Machine Learning Method (OR-ELM-AR) Used in Forecast of PM2.5 Concentrations and Its Forecast Performance Evaluation G. Lu et al. 10.3390/atmos12010078
- Strategies towards PM2.5 attainment for non-compliant cities in China: A case study H. Ling et al. 10.1016/j.jenvman.2021.113529
- Study on the assimilation of the sulphate reaction rates based on WRF-Chem/DART C. Huang et al. 10.1007/s11430-023-1153-9
- Improvement of inorganic aerosol component in PM2.5 by constraining aqueous-phase formation of sulfate in cloud with satellite retrievals: WRF-Chem simulations T. Sha et al. 10.1016/j.scitotenv.2021.150229
- Characteristics of air pollution episodes influenced by biomass burning pollution in Shanghai, China S. Tong et al. 10.1016/j.atmosenv.2020.117756
- Influence of atmospheric in-cloud aqueous-phase chemistry on the global simulation of SO<sub>2</sub> in CESM2 W. Ge et al. 10.5194/acp-21-16093-2021
- Recommendations on benchmarks for photochemical air quality model applications in China — NO2, SO2, CO and PM10 H. Zhai et al. 10.1016/j.atmosenv.2023.120290
- Evaluation and Bias Correction of the Secondary Inorganic Aerosol Modeling over North China Plain in Autumn and Winter Q. Wu et al. 10.3390/atmos12050578
- Assessment of the impacts of cloud chemistry on surface SO2 and sulfate levels in typical regions of China J. Lu et al. 10.5194/acp-23-8021-2023
- PM2.5 and O3 relationships affected by the atmospheric oxidizing capacity in the Yangtze River Delta, China M. Qin et al. 10.1016/j.scitotenv.2021.152268
- Secondary PM2.5 dominates aerosol pollution in the Yangtze River Delta region: Environmental and health effects of the Clean air Plan N. Li et al. 10.1016/j.envint.2022.107725
- Recommendations on benchmarks for numerical air quality model applications in China – Part 1: PM<sub>2.5</sub> and chemical species L. Huang et al. 10.5194/acp-21-2725-2021
- Air quality changes during the COVID-19 lockdown over the Yangtze River Delta Region: An insight into the impact of human activity pattern changes on air pollution variation L. Li et al. 10.1016/j.scitotenv.2020.139282
- Assessment of the effects of straw burning bans in China: Emissions, air quality, and health impacts L. Huang et al. 10.1016/j.scitotenv.2021.147935
- Response of PM2.5 chemical composition to the emission reduction and meteorological variation during the COVID-19 lockdown Y. Gong et al. 10.1016/j.chemosphere.2024.142844
- Heterogeneous interactions between SO<sub>2</sub> and organic peroxides in submicron aerosol S. Wang et al. 10.5194/acp-21-6647-2021
- The combined effects of heterogeneous chemistry and aerosol-radiation interaction on severe haze simulation by atmospheric chemistry model in Middle-Eastern China Z. Liu et al. 10.1016/j.atmosenv.2023.119729
- Wintertime Formation of Large Sulfate Particles in China and Implications for Human Health Q. Zhang et al. 10.1021/acs.est.3c05645
- Hourly organic tracers-based source apportionment of PM2.5 before and during the Covid-19 lockdown in suburban Shanghai, China: Insights into regional transport influences and response to urban emission reductions S. Wang et al. 10.1016/j.atmosenv.2022.119308
- Air pollutant variations in Suzhou during the 2019 novel coronavirus (COVID-19) lockdown of 2020: High time-resolution measurements of aerosol chemical compositions and source apportionment H. Wang et al. 10.1016/j.envpol.2020.116298
- Ammonium nitrate promotes sulfate formation through uptake kinetic regime Y. Liu et al. 10.5194/acp-21-13269-2021
- Estimation of secondary PM<sub>2.5</sub> in China and the United States using a multi-tracer approach H. Zhang et al. 10.5194/acp-22-5495-2022
3 citations as recorded by crossref.
- Bias in ammonia emission inventory and implications on emission control of nitrogen oxides over North China Plain Q. Zhang et al. 10.1016/j.atmosenv.2019.116869
- Estimation of interannual trends of ammonia emissions from agriculture in Jiangsu Province from 2000 to 2017 J. HUANG et al. 10.1080/16742834.2020.1736499
- Efficient control of atmospheric sulfate production based on three formation regimes J. Xue et al. 10.1038/s41561-019-0485-5
Latest update: 14 Dec 2024
Short summary
Severe haze events characterized by extremely high concentrations of particulate matter occurred frequently in the Yangtze River Delta (YRD) region, China. Rapid sulfate production during these severe haze episodes was observed via atmospheric measurements but air quality models tend to underestimated sulfate. Our study suggests that the SO2+NO2 heterogeneous reactions could be potentially important for sulfate formation in the YRD region and ammonia emissions need to be carefully estimated.
Severe haze events characterized by extremely high concentrations of particulate matter occurred...
Altmetrics
Final-revised paper
Preprint