Articles | Volume 19, issue 2
https://doi.org/10.5194/acp-19-1241-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-1241-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
31 Jan 2019
Research article |
| 31 Jan 2019
| 31 Jan 2019
Modeling the effect of non-ideality, dynamic mass transfer and viscosity on SOA formation in a 3-D air quality model
CEREA, Joint Laboratory École des Ponts ParisTech/EDF R&D,
Université Paris-Est, 77455 Champs-sur-Marne, France
Karine Sartelet
CEREA, Joint Laboratory École des Ponts ParisTech/EDF R&D,
Université Paris-Est, 77455 Champs-sur-Marne, France
Florian Couvidat
Institut National de l'Environnement Industriel et des Risques, 60550 Verneuil-en-Halatte, France
Viewed
Total article views: 2,583 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 06 Jun 2018)
| HTML | XML | Total | BibTeX | EndNote | |
|---|---|---|---|---|---|
| 1,867 | 666 | 50 | 2,583 | 50 | 48 |
- HTML: 1,867
- PDF: 666
- XML: 50
- Total: 2,583
- BibTeX: 50
- EndNote: 48
Total article views: 1,933 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 31 Jan 2019)
| HTML | XML | Total | BibTeX | EndNote | |
|---|---|---|---|---|---|
| 1,441 | 454 | 38 | 1,933 | 40 | 40 |
- HTML: 1,441
- PDF: 454
- XML: 38
- Total: 1,933
- BibTeX: 40
- EndNote: 40
Total article views: 650 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 06 Jun 2018)
| HTML | XML | Total | BibTeX | EndNote | |
|---|---|---|---|---|---|
| 426 | 212 | 12 | 650 | 10 | 8 |
- HTML: 426
- PDF: 212
- XML: 12
- Total: 650
- BibTeX: 10
- EndNote: 8
Viewed (geographical distribution)
Total article views: 2,583 (including HTML, PDF, and XML)
Thereof 2,402 with geography defined
and 181 with unknown origin.
Total article views: 1,933 (including HTML, PDF, and XML)
Thereof 1,762 with geography defined
and 171 with unknown origin.
Total article views: 650 (including HTML, PDF, and XML)
Thereof 640 with geography defined
and 10 with unknown origin.
| Country | # | Views | % |
|---|
| Country | # | Views | % |
|---|
| Country | # | Views | % |
|---|
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
Cited
21 citations as recorded by crossref.
- Global Distribution of the Phase State and Mixing Times within Secondary Organic Aerosol Particles in the Troposphere Based on Room-Temperature Viscosity Measurements A. Maclean et al. 10.1021/acsearthspacechem.1c00296
- SSH-Aerosol v1.1: A Modular Box Model to Simulate the Evolution of Primary and Secondary Aerosols K. Sartelet et al. 10.3390/atmos11050525
- Modeling Secondary Organic Aerosols in China: State of the Art and Perspectives J. Li et al. 10.1007/s40726-022-00246-3
- Impacts of water partitioning and polarity of organic compounds on secondary organic aerosol over eastern China J. Li et al. 10.5194/acp-20-7291-2020
- GENerator of reduced Organic Aerosol mechanism (GENOA v1.0): an automatic generation tool of semi-explicit mechanisms Z. Wang et al. 10.5194/gmd-15-8957-2022
- Diffusion of Organic Molecules as a Function of Temperature in a Sucrose Matrix (a Proxy for Secondary Organic Aerosol) K. Kiland et al. 10.1021/acs.jpclett.9b02182
- The CHIMERE v2020r1 online chemistry-transport model L. Menut et al. 10.5194/gmd-14-6781-2021
- Diffusion Coefficients and Mixing Times of Organic Molecules in β-Caryophyllene Secondary Organic Aerosol (SOA) and Biomass Burning Organic Aerosol (BBOA) E. Evoy et al. 10.1021/acsearthspacechem.1c00317
- Effects of volatility, viscosity, and non-ideality on particle–particle mixing timescales of secondary organic aerosols M. Schervish et al. 10.1080/02786826.2023.2256827
- A new hot-stage microscopy technique for measuring temperature-dependent viscosities of aerosol particles and its application to farnesene secondary organic aerosol K. Kiland et al. 10.5194/amt-15-5545-2022
- Insights into the aging of biomass burning aerosol from satellite observations and 3D atmospheric modeling: evolution of the aerosol optical properties in Siberian wildfire plumes I. Konovalov et al. 10.5194/acp-21-357-2021
- Ion-molecule interactions enable unexpected phase transitions in organic-inorganic aerosol D. Richards et al. 10.1126/sciadv.abb5643
- Liquid–liquid phase separation and viscosity within secondary organic aerosol generated from diesel fuel vapors M. Song et al. 10.5194/acp-19-12515-2019
- Impact of the Atmospheric Photochemical Evolution of the Organic Component of Biomass Burning Aerosol on Its Radiative Forcing Efficiency: A Box Model Analysis T. Zhuravleva et al. 10.3390/atmos12121555
- Unified Description of Diffusion Coefficients from Small to Large Molecules in Organic–Water Mixtures E. Evoy et al. 10.1021/acs.jpca.9b11271
- Viscosity and phase state of aerosol particles consisting of sucrose mixed with inorganic salts Y. Song et al. 10.5194/acp-21-10215-2021
- Relative-humidity-dependent organic aerosol thermodynamics via an efficient reduced-complexity model K. Gorkowski et al. 10.5194/acp-19-13383-2019
- Precursors and formation of secondary organic aerosols from wildfires in the Euro-Mediterranean region M. Majdi et al. 10.5194/acp-19-5543-2019
- Humidity-Dependent Viscosity of Secondary Organic Aerosol from Ozonolysis of β-Caryophyllene: Measurements, Predictions, and Implications A. Maclean et al. 10.1021/acsearthspacechem.0c00296
- Viscosity, Glass Formation, and Mixing Times within Secondary Organic Aerosol from Biomass Burning Phenolics K. Kiland et al. 10.1021/acsearthspacechem.3c00039
- Morphology and phase state of PM2.5 in urban and coastal-rural areas during summer S. Gaikwad et al. 10.3389/fenvs.2023.1142941
21 citations as recorded by crossref.
- Global Distribution of the Phase State and Mixing Times within Secondary Organic Aerosol Particles in the Troposphere Based on Room-Temperature Viscosity Measurements A. Maclean et al. 10.1021/acsearthspacechem.1c00296
- SSH-Aerosol v1.1: A Modular Box Model to Simulate the Evolution of Primary and Secondary Aerosols K. Sartelet et al. 10.3390/atmos11050525
- Modeling Secondary Organic Aerosols in China: State of the Art and Perspectives J. Li et al. 10.1007/s40726-022-00246-3
- Impacts of water partitioning and polarity of organic compounds on secondary organic aerosol over eastern China J. Li et al. 10.5194/acp-20-7291-2020
- GENerator of reduced Organic Aerosol mechanism (GENOA v1.0): an automatic generation tool of semi-explicit mechanisms Z. Wang et al. 10.5194/gmd-15-8957-2022
- Diffusion of Organic Molecules as a Function of Temperature in a Sucrose Matrix (a Proxy for Secondary Organic Aerosol) K. Kiland et al. 10.1021/acs.jpclett.9b02182
- The CHIMERE v2020r1 online chemistry-transport model L. Menut et al. 10.5194/gmd-14-6781-2021
- Diffusion Coefficients and Mixing Times of Organic Molecules in β-Caryophyllene Secondary Organic Aerosol (SOA) and Biomass Burning Organic Aerosol (BBOA) E. Evoy et al. 10.1021/acsearthspacechem.1c00317
- Effects of volatility, viscosity, and non-ideality on particle–particle mixing timescales of secondary organic aerosols M. Schervish et al. 10.1080/02786826.2023.2256827
- A new hot-stage microscopy technique for measuring temperature-dependent viscosities of aerosol particles and its application to farnesene secondary organic aerosol K. Kiland et al. 10.5194/amt-15-5545-2022
- Insights into the aging of biomass burning aerosol from satellite observations and 3D atmospheric modeling: evolution of the aerosol optical properties in Siberian wildfire plumes I. Konovalov et al. 10.5194/acp-21-357-2021
- Ion-molecule interactions enable unexpected phase transitions in organic-inorganic aerosol D. Richards et al. 10.1126/sciadv.abb5643
- Liquid–liquid phase separation and viscosity within secondary organic aerosol generated from diesel fuel vapors M. Song et al. 10.5194/acp-19-12515-2019
- Impact of the Atmospheric Photochemical Evolution of the Organic Component of Biomass Burning Aerosol on Its Radiative Forcing Efficiency: A Box Model Analysis T. Zhuravleva et al. 10.3390/atmos12121555
- Unified Description of Diffusion Coefficients from Small to Large Molecules in Organic–Water Mixtures E. Evoy et al. 10.1021/acs.jpca.9b11271
- Viscosity and phase state of aerosol particles consisting of sucrose mixed with inorganic salts Y. Song et al. 10.5194/acp-21-10215-2021
- Relative-humidity-dependent organic aerosol thermodynamics via an efficient reduced-complexity model K. Gorkowski et al. 10.5194/acp-19-13383-2019
- Precursors and formation of secondary organic aerosols from wildfires in the Euro-Mediterranean region M. Majdi et al. 10.5194/acp-19-5543-2019
- Humidity-Dependent Viscosity of Secondary Organic Aerosol from Ozonolysis of β-Caryophyllene: Measurements, Predictions, and Implications A. Maclean et al. 10.1021/acsearthspacechem.0c00296
- Viscosity, Glass Formation, and Mixing Times within Secondary Organic Aerosol from Biomass Burning Phenolics K. Kiland et al. 10.1021/acsearthspacechem.3c00039
- Morphology and phase state of PM2.5 in urban and coastal-rural areas during summer S. Gaikwad et al. 10.3389/fenvs.2023.1142941
Latest update: 18 Apr 2024
Short summary
Assumptions (ideality and thermodynamic equilibrium) commonly made in 3-dimensional air quality models were reconsidered to evaluate their impacts on secondary organic aerosol (SOA) formation. Non-ideality (short-, medium- and long-range interactions of organics and inorganics) influences SOA concentrations by about 30 % over Europe. If SOA are highly viscous rather than inviscid, hydrophobic SOA concentrations increase by 6 % but can increase by an order of magnitude for volatile compounds.
Assumptions (ideality and thermodynamic equilibrium) commonly made in 3-dimensional air quality...
Altmetrics
Final-revised paper
Preprint