Articles | Volume 19, issue 19
https://doi.org/10.5194/acp-19-12221-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue:
https://doi.org/10.5194/acp-19-12221-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
02 Oct 2019
Research article |
| 02 Oct 2019
| 02 Oct 2019
Isotopic constraints on the atmospheric sources and formation of nitrogenous species in clouds influenced by biomass burning
Yunhua Chang
KLME & CIC-FEMD, Yale-NUIST Center on Atmospheric Environment, Nanjing University of
Information Science & Technology, Nanjing 210044, China
Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention (LAP), Department of Environmental Science &
Engineering, Institute of Atmospheric Sciences, Fudan University, Shanghai
200433, China
KLME & CIC-FEMD, Yale-NUIST Center on Atmospheric Environment, Nanjing University of
Information Science & Technology, Nanjing 210044, China
Jiarong Li
Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention (LAP), Department of Environmental Science &
Engineering, Institute of Atmospheric Sciences, Fudan University, Shanghai
200433, China
Chongguo Tian
Key Laboratory of Coastal Environmental Processes and Ecological
Remediation, Yantai Institute of Coastal Zone Research, Chinese Academy of
Sciences, Yantai 264003, China
Linlin Song
CAS Key Laboratory of Forest Ecology and Management, Institute of
Applied Ecology, Chinese Academy of Sciences, Shenyang 110016, China
Xiaoyao Zhai
KLME & CIC-FEMD, Yale-NUIST Center on Atmospheric Environment, Nanjing University of
Information Science & Technology, Nanjing 210044, China
Wenqi Zhang
KLME & CIC-FEMD, Yale-NUIST Center on Atmospheric Environment, Nanjing University of
Information Science & Technology, Nanjing 210044, China
Tong Huang
KLME & CIC-FEMD, Yale-NUIST Center on Atmospheric Environment, Nanjing University of
Information Science & Technology, Nanjing 210044, China
Yu-Chi Lin
KLME & CIC-FEMD, Yale-NUIST Center on Atmospheric Environment, Nanjing University of
Information Science & Technology, Nanjing 210044, China
Chao Zhu
Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention (LAP), Department of Environmental Science &
Engineering, Institute of Atmospheric Sciences, Fudan University, Shanghai
200433, China
Yunting Fang
CAS Key Laboratory of Forest Ecology and Management, Institute of
Applied Ecology, Chinese Academy of Sciences, Shenyang 110016, China
Moritz F. Lehmann
Aquatic and Isotope Biogeochemistry, Department of Environmental
Sciences, University of Basel, Basel 4056, Switzerland
Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention (LAP), Department of Environmental Science &
Engineering, Institute of Atmospheric Sciences, Fudan University, Shanghai
200433, China
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Cited
20 citations as recorded by crossref.
- Importance of NO3 radical in particulate nitrate formation in a southeast Chinese urban city: New constraints by δ15N-δ18O space of NO3- Z. Zhang et al. 10.1016/j.atmosenv.2021.118387
- Nitrate Isotopic Composition in Precipitation at a Chinese Megacity: Seasonal Variations, Atmospheric Processes, and Implications for Sources Z. Li et al. 10.1029/2019EA000759
- Key biogeochemical processes and source apportionment of nitrate in the Bohai Sea based on nitrate stable isotopes K. Yu et al. 10.1016/j.marpolbul.2024.116617
- Sources and transformation of nitrate aerosol in winter 2017–2018 of megacity Beijing: Insights from an alternative approach Z. Zhang et al. 10.1016/j.atmosenv.2020.117842
- Biomass burning related ammonia emissions promoted a self-amplifying loop in the urban environment in Kunming (SW China) Y. Zhou et al. 10.1016/j.atmosenv.2020.118138
- Oxidation and sources of atmospheric NOx during winter in Beijing based on δ18O-δ15N space of particulate nitrate Z. Zhang et al. 10.1016/j.envpol.2021.116708
- Isotopic Evidence for the High Contribution of Wintertime Photochemistry to Particulate Nitrate Formation in Northern China Z. Zhang et al. 10.1029/2021JD035324
- Nitrate chemistry in the northeast US – Part 1: Nitrogen isotope seasonality tracks nitrate formation chemistry C. Bekker et al. 10.5194/acp-23-4185-2023
- Nitrate Regeneration and Loss in the Central Yellow Sea Bottom Water Revealed by Nitrogen Isotopes S. Tian et al. 10.3389/fmars.2022.834953
- Fog event is possibly a source rather than a sink of atmospheric nitrate aerosols: Insights from isotopic measurements in Nanjing, China H. Yu et al. 10.1016/j.apgeochem.2023.105721
- The evolution of cloud and aerosol microphysics at the summit of Mt. Tai, China J. Li et al. 10.5194/acp-20-13735-2020
- A nitrate budget of the Bohai Sea based on an isotope mass balance model S. Tian et al. 10.5194/bg-19-2397-2022
- Recent Isotopic Evidence for Elevated Vehicular NOx Emission to Atmospheric Nitrate Formation in Chinese Megacities Z. Zhang et al. 10.1021/acsearthspacechem.1c00166
- Formation pathways and source apportionments of inorganic nitrogen-containing aerosols in urban environment: Insights from nitrogen and oxygen isotopic compositions in Guangzhou, China D. Xi et al. 10.1016/j.atmosenv.2023.119888
- Formation pathway of secondary inorganic aerosol and its influencing factors in Northern China: Comparison between urban and rural sites S. Wang et al. 10.1016/j.scitotenv.2022.156404
- Response of fine aerosol nitrate chemistry to Clean Air Action in winter Beijing: Insights from the oxygen isotope signatures Z. Zhang et al. 10.1016/j.scitotenv.2020.141210
- Enhanced biomass burning as a source of aerosol ammonium over cities in central China in autumn H. Xiao et al. 10.1016/j.envpol.2020.115278
- Convergent evidence for the pervasive but limited contribution of biomass burning to atmospheric ammonia in peninsular Southeast Asia Y. Chang et al. 10.5194/acp-21-7187-2021
- Chemical and isotopic characteristics of PM2.5 over New Delhi from September 2014 to May 2015: Evidences for synergy between air-pollution and meteorological changes R. Sawlani et al. 10.1016/j.scitotenv.2020.142966
- The importance of coal combustion and heterogeneous reaction for atmospheric nitrate pollution in a cold metropolis in China: Insights from isotope fractionation and Bayesian mixing model X. Sun et al. 10.1016/j.atmosenv.2020.117730
20 citations as recorded by crossref.
- Importance of NO3 radical in particulate nitrate formation in a southeast Chinese urban city: New constraints by δ15N-δ18O space of NO3- Z. Zhang et al. 10.1016/j.atmosenv.2021.118387
- Nitrate Isotopic Composition in Precipitation at a Chinese Megacity: Seasonal Variations, Atmospheric Processes, and Implications for Sources Z. Li et al. 10.1029/2019EA000759
- Key biogeochemical processes and source apportionment of nitrate in the Bohai Sea based on nitrate stable isotopes K. Yu et al. 10.1016/j.marpolbul.2024.116617
- Sources and transformation of nitrate aerosol in winter 2017–2018 of megacity Beijing: Insights from an alternative approach Z. Zhang et al. 10.1016/j.atmosenv.2020.117842
- Biomass burning related ammonia emissions promoted a self-amplifying loop in the urban environment in Kunming (SW China) Y. Zhou et al. 10.1016/j.atmosenv.2020.118138
- Oxidation and sources of atmospheric NOx during winter in Beijing based on δ18O-δ15N space of particulate nitrate Z. Zhang et al. 10.1016/j.envpol.2021.116708
- Isotopic Evidence for the High Contribution of Wintertime Photochemistry to Particulate Nitrate Formation in Northern China Z. Zhang et al. 10.1029/2021JD035324
- Nitrate chemistry in the northeast US – Part 1: Nitrogen isotope seasonality tracks nitrate formation chemistry C. Bekker et al. 10.5194/acp-23-4185-2023
- Nitrate Regeneration and Loss in the Central Yellow Sea Bottom Water Revealed by Nitrogen Isotopes S. Tian et al. 10.3389/fmars.2022.834953
- Fog event is possibly a source rather than a sink of atmospheric nitrate aerosols: Insights from isotopic measurements in Nanjing, China H. Yu et al. 10.1016/j.apgeochem.2023.105721
- The evolution of cloud and aerosol microphysics at the summit of Mt. Tai, China J. Li et al. 10.5194/acp-20-13735-2020
- A nitrate budget of the Bohai Sea based on an isotope mass balance model S. Tian et al. 10.5194/bg-19-2397-2022
- Recent Isotopic Evidence for Elevated Vehicular NOx Emission to Atmospheric Nitrate Formation in Chinese Megacities Z. Zhang et al. 10.1021/acsearthspacechem.1c00166
- Formation pathways and source apportionments of inorganic nitrogen-containing aerosols in urban environment: Insights from nitrogen and oxygen isotopic compositions in Guangzhou, China D. Xi et al. 10.1016/j.atmosenv.2023.119888
- Formation pathway of secondary inorganic aerosol and its influencing factors in Northern China: Comparison between urban and rural sites S. Wang et al. 10.1016/j.scitotenv.2022.156404
- Response of fine aerosol nitrate chemistry to Clean Air Action in winter Beijing: Insights from the oxygen isotope signatures Z. Zhang et al. 10.1016/j.scitotenv.2020.141210
- Enhanced biomass burning as a source of aerosol ammonium over cities in central China in autumn H. Xiao et al. 10.1016/j.envpol.2020.115278
- Convergent evidence for the pervasive but limited contribution of biomass burning to atmospheric ammonia in peninsular Southeast Asia Y. Chang et al. 10.5194/acp-21-7187-2021
- Chemical and isotopic characteristics of PM2.5 over New Delhi from September 2014 to May 2015: Evidences for synergy between air-pollution and meteorological changes R. Sawlani et al. 10.1016/j.scitotenv.2020.142966
- The importance of coal combustion and heterogeneous reaction for atmospheric nitrate pollution in a cold metropolis in China: Insights from isotope fractionation and Bayesian mixing model X. Sun et al. 10.1016/j.atmosenv.2020.117730
Latest update: 08 Jul 2025
Short summary
The present work underscores the value of cloud water dissolved inorganic nitrogen isotopes as carriers of quantitative information on regional NOx and NH3 emissions. It sheds light on the origin and production pathways of nitrogenous species in clouds and emphasizes the importance of biomass-burning-derived nitrogenous species as cloud condensation nuclei in China’s troposphere. Moreover, it highlights the rapid evolution of NOx emissions in China.
The present work underscores the value of cloud water dissolved inorganic nitrogen isotopes as...
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