Articles | Volume 19, issue 19
https://doi.org/10.5194/acp-19-12175-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-12175-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
01 Oct 2019
Research article |
| 01 Oct 2019
| 01 Oct 2019
Laboratory study of the heterogeneous ice nucleation on black-carbon-containing aerosol
Leonid Nichman
CORRESPONDING AUTHOR
Department of Chemistry, Boston College, Chestnut Hill, MA 02467, USA
Aerodyne Research, Inc., Billerica, MA 01821, USA
now at: Flight Research Laboratory, National Research Council of Canada, Ottawa, ON, K1V 9B4, Canada
Martin Wolf
Department of Earth, Atmospheric and Planetary Sciences, Massachusetts Institute of Technology, Cambridge, MA 02139, USA
Paul Davidovits
Department of Chemistry, Boston College, Chestnut Hill, MA 02467, USA
Timothy B. Onasch
Department of Chemistry, Boston College, Chestnut Hill, MA 02467, USA
Aerodyne Research, Inc., Billerica, MA 01821, USA
Yue Zhang
Department of Chemistry, Boston College, Chestnut Hill, MA 02467, USA
Aerodyne Research, Inc., Billerica, MA 01821, USA
Department of Environmental Sciences and Engineering, Gillings School of Global Public Health, University of North Carolina at Chapel Hill, Chapel Hill, NC 27599, USA
Doug R. Worsnop
Aerodyne Research, Inc., Billerica, MA 01821, USA
Janarjan Bhandari
Department of Physics and Atmospheric Sciences, Michigan
Technological University, Houghton, MI 49931, USA
Claudio Mazzoleni
Department of Physics and Atmospheric Sciences, Michigan
Technological University, Houghton, MI 49931, USA
Daniel J. Cziczo
Department of Earth, Atmospheric and Planetary Sciences, Massachusetts Institute of Technology, Cambridge, MA 02139, USA
Department of Civil and Environmental Engineering, Massachusetts
Institute of Technology, Cambridge, MA 02139, USA
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Latest update: 23 Nov 2024
Short summary
Previous studies showed widespread ice nucleation activity of soot. In this systematic study we investigated the factors that affect the heterogeneous ice nucleation activity of soot surrogates in the cirrus cloud regime. Our observations are consistent with an ice nucleation mechanism of pore condensation followed by freezing. The results show significant variations in ice nucleation activity as a function of size, morphology, and surface chemistry of the black-carbon-containing particles.
Previous studies showed widespread ice nucleation activity of soot. In this systematic study we...
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