Articles | Volume 18, issue 10
https://doi.org/10.5194/acp-18-7313-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-7313-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
25 May 2018
Research article |
| 25 May 2018
| 25 May 2018
Cloud droplet size distribution broadening during diffusional growth: ripening amplified by deactivation and reactivation
Environmental and Climate Sciences Department, Brookhaven National Laboratory, Upton, New York, USA
Pavlos Kollias
Environmental and Climate Sciences Department, Brookhaven National Laboratory, Upton, New York, USA
School of Marine and Atmospheric Sciences, Stony Brook University, Stony Brook, New York, USA
Raymond A. Shaw
Department of Physics, Michigan Technological University, Houghton, Michigan, USA
Andrew M. Vogelmann
Environmental and Climate Sciences Department, Brookhaven National Laboratory, Upton, New York, USA
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Madison L. Ghiz, Ryan C. Scott, Andrew M. Vogelmann, Jan T. M. Lenaerts, Matthew Lazzara, and Dan Lubin
The Cryosphere, 15, 3459–3494, https://doi.org/10.5194/tc-15-3459-2021, https://doi.org/10.5194/tc-15-3459-2021, 2021
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We investigate how melt occurs over the vulnerable ice shelves of West Antarctica and determine that the three primary mechanisms can be evaluated using archived numerical weather prediction model data and satellite imagery. We find examples of each mechanism: thermal blanketing by a warm atmosphere, radiative heating by thin clouds, and downslope winds. Our results signify the potential to make a multi-decadal assessment of atmospheric stress on West Antarctic ice shelves in a warming climate.
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Multi-wavelength radar measurements provide capabilities to identify ice particle types and growth processes in clouds beyond the capabilities of single-frequency radar measurements. This study introduces Doppler velocity and polarimetric radar observables into the multi-wavelength radar reflectivity measurement to improve identification analysis. The analysis clearly discerns snowflake aggregation and riming processes and even early stages of riming.
Katia Lamer, Mariko Oue, Alessandro Battaglia, Richard J. Roy, Ken B. Cooper, Ranvir Dhillon, and Pavlos Kollias
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Observations collected during the 25 February 2020 deployment of the VIPR at the Stony Brook Radar Observatory clearly demonstrate the potential of G-band radars for cloud and precipitation research. The field experiment, which coordinated an X-, Ka-, W- and G-band radar, revealed that the differential reflectivity from Ka–G band pair provides larger signals than the traditional Ka–W pairing underpinning an increased sensitivity to smaller amounts of liquid and ice water mass and sizes.
Marek Jacob, Pavlos Kollias, Felix Ament, Vera Schemann, and Susanne Crewell
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Sonja Drueke, Daniel J. Kirshbaum, and Pavlos Kollias
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According to ground-based radar observations, 50 % of liquid low-level clouds over the Atlantic extend below 1.2 km and are thinner than 400 m, thus limiting their detection from space. Using an emulator, we estimate that a 250 m resolution radar would capture cloud base better than the CloudSat radar which misses about 52 %. The more sensitive EarthCARE radar is expected to capture cloud cover but stretch cloud. This calls for the operation of interlaced pulse modes for future space missions.
Mariko Oue, Aleksandra Tatarevic, Pavlos Kollias, Dié Wang, Kwangmin Yu, and Andrew M. Vogelmann
Geosci. Model Dev., 13, 1975–1998, https://doi.org/10.5194/gmd-13-1975-2020, https://doi.org/10.5194/gmd-13-1975-2020, 2020
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We developed the Cloud-resolving model Radar SIMulator (CR-SIM) capable of apples-to-apples comparisons between the multiwavelength, zenith-pointing, and scanning radar and multi-remote-sensing (radar and lidar) observations and the high-resolution atmospheric model output. Applications of CR-SIM as a virtual observatory operator aid interpretation of the differences and improve understanding of the representativeness errors due to the sampling limitations of the ground-based measurements.
Dennis Niedermeier, Jens Voigtländer, Silvio Schmalfuß, Daniel Busch, Jörg Schumacher, Raymond A. Shaw, and Frank Stratmann
Atmos. Meas. Tech., 13, 2015–2033, https://doi.org/10.5194/amt-13-2015-2020, https://doi.org/10.5194/amt-13-2015-2020, 2020
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In this paper, we present the new moist-air wind tunnel LACIS-T (Turbulent Leipzig Aerosol Cloud Interaction Simulator). It is used to study cloud physical processes in general and interactions between turbulence and cloud microphysical processes in particular. The operating principle of LACIS-T is explained, and the first results are depicted from deliquescence and droplet formation experiments observing clear indications on the effect of turbulence on these microphysical processes.
Fan Yang, Robert McGraw, Edward P. Luke, Damao Zhang, Pavlos Kollias, and Andrew M. Vogelmann
Atmos. Meas. Tech., 12, 5817–5828, https://doi.org/10.5194/amt-12-5817-2019, https://doi.org/10.5194/amt-12-5817-2019, 2019
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In-cloud supersaturation is crucial for droplet activation, growth, and drizzle initiation but is poorly known and hardly measured. Here we provide a novel method to estimate supersaturation fluctuation in stratocumulus clouds using remote-sensing measurements, and results show that our estimated supersaturation agrees reasonably well with in situ measurements. Our method provides a unique way to estimate supersaturation in stratocumulus clouds from long-term ground-based observations.
Mario Mech, Leif-Leonard Kliesch, Andreas Anhäuser, Thomas Rose, Pavlos Kollias, and Susanne Crewell
Atmos. Meas. Tech., 12, 5019–5037, https://doi.org/10.5194/amt-12-5019-2019, https://doi.org/10.5194/amt-12-5019-2019, 2019
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An improved understanding of Arctic mixed-phase clouds and their contribution to Arctic warming can be achieved by observations from airborne platforms with remote sensing instruments. Such an instrument is MiRAC combining active and passive techniques to gain information on the distribution of clouds, the occurrence of precipitation, and the amount of liquid and ice within the cloud. Operated during a campaign in Arctic summer, it could observe lower clouds often not seen by spaceborne radars.
Pavlos Kollias, Bernat Puigdomènech Treserras, and Alain Protat
Atmos. Meas. Tech., 12, 4949–4964, https://doi.org/10.5194/amt-12-4949-2019, https://doi.org/10.5194/amt-12-4949-2019, 2019
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Profiling millimeter-wavelength radars are the cornerstone instrument of surface-based observatories. Calibrating these radars is important for establishing a long record of observations suitable for model evaluation and improvement. Here, the CloudSat CPR is used to assess the calibration of a record over 10 years long of ARM cloud radar observations (a total of 44 years). The results indicate that correction coefficients are needed to improve record reliability and usability.
Katia Lamer, Bernat Puigdomènech Treserras, Zeen Zhu, Bradley Isom, Nitin Bharadwaj, and Pavlos Kollias
Atmos. Meas. Tech., 12, 4931–4947, https://doi.org/10.5194/amt-12-4931-2019, https://doi.org/10.5194/amt-12-4931-2019, 2019
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This article describes the three newly deployed second-generation radar of the Atmospheric Radiation Measurement program. Techniques to retrieve precipitation rate from their measurements are presented: noise and clutter filtering, gas and liquid attenuation correction, and radar reflectivity calibration. Rain rate for a 40 km radius domain around Graciosa estimated from all three radar differ, which highlights the need to consider sensor capabilities when interpreting radar measurements.
Alessandro Battaglia and Pavlos Kollias
Atmos. Meas. Tech., 12, 3335–3349, https://doi.org/10.5194/amt-12-3335-2019, https://doi.org/10.5194/amt-12-3335-2019, 2019
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This work investigates the potential of an innovative differential absorption radar for retrieving relative humidity inside ice clouds. The radar exploits the strong spectral dependence of the water vapour absorption for frequencies close to the 183 GHz water vapour band.
Results show that observations from a system with 4–6 frequencies can provide
novel information for understanding the formation and growth of ice crystals.
Katarzyna Karpińska, Jonathan F. E. Bodenschatz, Szymon P. Malinowski, Jakub L. Nowak, Steffen Risius, Tina Schmeissner, Raymond A. Shaw, Holger Siebert, Hengdong Xi, Haitao Xu, and Eberhard Bodenschatz
Atmos. Chem. Phys., 19, 4991–5003, https://doi.org/10.5194/acp-19-4991-2019, https://doi.org/10.5194/acp-19-4991-2019, 2019
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Observations of clouds at a mountain-top laboratory revealed for the first time the presence of “voids”, i.e., elongated volumes inside a cloud that are devoid of droplets. Theoretical and numerical analyses suggest that these voids are a result of strong and long-lasting vortex presence in turbulent air. If this is confirmed in further investigation, the effect may become an important part of models describing cloud evolution and rain formation.
Mariko Oue, Pavlos Kollias, Alan Shapiro, Aleksandra Tatarevic, and Toshihisa Matsui
Atmos. Meas. Tech., 12, 1999–2018, https://doi.org/10.5194/amt-12-1999-2019, https://doi.org/10.5194/amt-12-1999-2019, 2019
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This study investigated impacts of the selected radar volume coverage pattern, the sampling time period, the number of radars used, and the added value of advection correction on the retrieval of vertical air motion from a multi-Doppler-radar technique. The results suggest that the use of rapid-scan radars can substantially improve the quality of wind retrievals and that the retrieved wind field needs to be carefully used considering the limitations of the radar observing system.
Guangjie Zheng, Yang Wang, Allison C. Aiken, Francesca Gallo, Michael P. Jensen, Pavlos Kollias, Chongai Kuang, Edward Luke, Stephen Springston, Janek Uin, Robert Wood, and Jian Wang
Atmos. Chem. Phys., 18, 17615–17635, https://doi.org/10.5194/acp-18-17615-2018, https://doi.org/10.5194/acp-18-17615-2018, 2018
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Here, we elucidate the key processes that drive marine boundary layer (MBL) aerosol size distribution in the eastern North Atlantic (ENA) using long-term measurements. The governing equations of particle concentration are established for different modes. Particles entrained from the free troposphere represent the major source of MBL cloud condensation nuclei (CCN), contributing both directly to CCN population and indirectly by supplying Aitken-mode particles that grow to CCN in the MBL.
Katia Lamer, Ann M. Fridlind, Andrew S. Ackerman, Pavlos Kollias, Eugene E. Clothiaux, and Maxwell Kelley
Geosci. Model Dev., 11, 4195–4214, https://doi.org/10.5194/gmd-11-4195-2018, https://doi.org/10.5194/gmd-11-4195-2018, 2018
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Weather and climate predictions of cloud, rain, and snow occurrence remain uncertain, in part because guidance from observation is incomplete. We present a tool that transforms predictions into observations from ground-based remote sensors. Liquid water and ice occurrence errors associated with the transformation are below 8 %, with ~ 3 % uncertainty. This (GO)2-SIM forward-simulator tool enables better evaluation of cloud, rain, and snow occurrence predictions using available observations.
Michael L. Larsen and Raymond A. Shaw
Atmos. Meas. Tech., 11, 4261–4272, https://doi.org/10.5194/amt-11-4261-2018, https://doi.org/10.5194/amt-11-4261-2018, 2018
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A statistical tool frequently utilized to measure scale-dependent departures from perfect randomness is the radial distribution function. This tool has many strengths, but it is not easy to calculate for particle detections within a three-dimensional sample volume. In this manuscript, we introduce and test a new method to estimate the three-dimensional radial distribution function in realistic measurement volumes.
Damao Zhang, Zhien Wang, Pavlos Kollias, Andrew M. Vogelmann, Kang Yang, and Tao Luo
Atmos. Chem. Phys., 18, 4317–4327, https://doi.org/10.5194/acp-18-4317-2018, https://doi.org/10.5194/acp-18-4317-2018, 2018
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Ice production in atmospheric clouds is important for global water cycle and radiation budget. Active satellite remote sensing measurements are analyzed to quantitatively study primary ice particle production in stratiform mixed-phase clouds on a global scale. We quantify the geographic and seasonal variations of ice production and their correlations with aerosol, especially mineral dust activities. The results can be used to evaluate mixed-phased clouds simulations by global climate models.
Xiaoli Zhou, Andrew S. Ackerman, Ann M. Fridlind, Robert Wood, and Pavlos Kollias
Atmos. Chem. Phys., 17, 12725–12742, https://doi.org/10.5194/acp-17-12725-2017, https://doi.org/10.5194/acp-17-12725-2017, 2017
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Shallow maritime clouds make a well-known transition from stratocumulus to trade cumulus with flow from the subtropics equatorward. Three-day large-eddy simulations that investigate the potential influence of overlying African biomass burning plumes during that transition indicate that cloud-related impacts are likely substantially cooling to negligible at the top of the atmosphere, with magnitude sensitive to background and perturbation aerosol and cloud properties.
Kirk W. North, Mariko Oue, Pavlos Kollias, Scott E. Giangrande, Scott M. Collis, and Corey K. Potvin
Atmos. Meas. Tech., 10, 2785–2806, https://doi.org/10.5194/amt-10-2785-2017, https://doi.org/10.5194/amt-10-2785-2017, 2017
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Vertical air motion retrievals from 3DVAR multiple distributed scanning Doppler radars are compared against collocated profiling radars and retrieved from an upward iteration integration iterative technique to characterize their veracity. The retrieved vertical air motions are generally within 1–2 m s−1 of agreement with profiling radars and better solution than the upward integration technique, and therefore can be used as a means to improve parameterizations in numerical models moving forward.
Claudia Acquistapace, Stefan Kneifel, Ulrich Löhnert, Pavlos Kollias, Maximilian Maahn, and Matthias Bauer-Pfundstein
Atmos. Meas. Tech., 10, 1783–1802, https://doi.org/10.5194/amt-10-1783-2017, https://doi.org/10.5194/amt-10-1783-2017, 2017
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The goal of the paper is to understand what the optimal cloud radar settings for drizzle detection are. The number of cloud radars in the world has increased in the last 10 years and it is important to develop strategies to derive optimal settings which can be applied to all radar systems. The study is part of broader research focused on better understanding the microphysical process of drizzle growth using ground-based observations.
Fan Yang, Raymond Shaw, and Huiwen Xue
Atmos. Chem. Phys., 16, 9421–9433, https://doi.org/10.5194/acp-16-9421-2016, https://doi.org/10.5194/acp-16-9421-2016, 2016
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When dry air is mixed into a cloud, droplets evaporate. If the diluted cloud mixture continues to rise, the remaining droplets will grow. In this work we show theoretically and computationally that a critical height exists, above which the droplets in a mixed, diluted cloud volume become larger than those in an undiluted volume. An environment that is humid and aerosol free is most favorable for producing such large droplets, which may contribute to the onset of precipitation formation.
B. Wehner, F. Werner, F. Ditas, R. A. Shaw, M. Kulmala, and H. Siebert
Atmos. Chem. Phys., 15, 11701–11711, https://doi.org/10.5194/acp-15-11701-2015, https://doi.org/10.5194/acp-15-11701-2015, 2015
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During the CARRIBA campaign on Barbados, 91 cases with increased aerosol particle number concentrations near clouds were detected from helicopter-borne measurements. Most of these cases are correlated with enhanced irradiance in the ultraviolet range. The events have a mean length of 100m, corresponding to a lifetime of 300s, meaning a growth of several nm/h. Such high values cannot be explained by sulfuric acid alone; thus extremely low volatility organic compounds are probably involved here.
S. Risius, H. Xu, F. Di Lorenzo, H. Xi, H. Siebert, R. A. Shaw, and E. Bodenschatz
Atmos. Meas. Tech., 8, 3209–3218, https://doi.org/10.5194/amt-8-3209-2015, https://doi.org/10.5194/amt-8-3209-2015, 2015
Related subject area
Subject: Clouds and Precipitation | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
The impact of the mesh size and microphysics scheme on the representation of mid-level clouds in the ICON model in hilly and complex terrain
The role of ascent timescales for warm conveyor belt (WCB) moisture transport into the upper troposphere and lower stratosphere (UTLS)
Estimating the concentration of silver iodide needed to detect unambiguous signatures of glaciogenic cloud seeding
Ice-nucleating particle concentration impacts cloud properties over Dronning Maud Land, East Antarctica, in COSMO-CLM2
Numerical simulation of aerosol concentration effects on cloud droplet size spectrum evolutions of warm stratiform clouds in Jiangxi, China
The impact of aerosol on cloud water: a heuristic perspective
The presence of clouds lowers climate sensitivity in the MPI-ESM1.2 climate model
Diurnal variation in an amplified canopy urban heat island during heat wave periods in the megacity of Beijing: roles of mountain–valley breeze and urban morphology
Diurnal evolution of non-precipitating marine stratocumuli in a large-eddy simulation ensemble
High ice water content in tropical mesoscale convective systems (a conceptual model)
Evolution of cloud droplet temperature and lifetime in spatiotemporally varying subsaturated environments with implications for ice nucleation at cloud edges
Effect of secondary ice production processes on the simulation of ice pellets using the Predicted Particle Properties microphysics scheme
Simulated particle evolution within a winter storm: contributions of riming to radar moments and precipitation fallout
A thermal-driven graupel generation process to explain dry-season convective vigor over the Amazon
Modeling homogeneous ice nucleation from drop-freezing experiments: impact of droplet volume dispersion and cooling rates
Cloud water adjustments to aerosol perturbations are buffered by solar heating in non-precipitating marine stratocumuli
Glaciation of mixed-phase clouds: insights from bulk model and bin-microphysics large-eddy simulation informed by laboratory experiment
Microphysical processes involving the vapour phase dominate in simulated low-level Arctic clouds
Understanding aerosol–cloud interactions using a single-column model for a cold-air outbreak case during the ACTIVATE campaign
On the sensitivity of aerosol–cloud interactions to changes in sea surface temperature in radiative–convective equilibrium
Exploring aerosol–cloud interactions in liquid-phase clouds over eastern China and its adjacent ocean using the WRF-Chem–SBM model
How the representation of microphysical processes affects tropical condensate in a global storm-resolving model
Impact of secondary ice production on thunderstorm electrification under different aerosol conditions
Finite domains cause bias in measured and modeled distributions of cloud sizes
A systematic evaluation of high-cloud controlling factors
Tracking precipitation features and associated large-scale environments over southeastern Texas
Revisiting the evolution of downhill thunderstorms over Beijing: a new perspective from a radar wind profiler mesonet
How well can persistent contrails be predicted? An update
Model analysis of biases in satellite diagnosed aerosol effect on cloud liquid water path
Dynamical imprints on precipitation cluster statistics across a hierarchy of high-resolution simulations
Potential impacts of marine fuel regulations on Arctic clouds and radiative feedbacks
Present-day correlations are insufficient to predict cloud albedo change by anthropogenic aerosols in E3SM v2
Simulations of primary and secondary ice production during an Arctic mixed-phase cloud case from the Ny-Ålesund Aerosol Cloud Experiment (NASCENT) campaign
Microphysical characteristics of precipitation within convective overshooting over East China observed by GPM DPR and ERA5
Effects of radiative cooling on advection fog over the northwest Pacific Ocean: observations and large-eddy simulations
Evaluating the Wegener–Bergeron–Findeisen process in ICON in large-eddy mode with in situ observations from the CLOUDLAB project
Aerosol-induced closure of marine cloud cells: enhanced effects in the presence of precipitation
Impact of ice multiplication on the cloud electrification of a cold-season thunderstorm: a numerical case study
Developing a climatological simplification of aerosols to enter the cloud microphysics of a global climate model
Interactions between trade wind clouds and local forcings over the Great Barrier Reef: a case study using convection-permitting simulations
Variability in the properties of the distribution of the relative humidity with respect to ice: implications for contrail formation
Simulating the seeder–feeder impacts on cloud ice and precipitation over the Alps
Can pollen affect precipitation?
Cloud response to co-condensation of water and organic vapors over the boreal forest
Distribution and morphology of non-persistent contrail and persistent contrail formation areas in ERA5
Connection of Surface Snowfall Bias to Cloud Phase Bias – Satellite Observations, ERA5, and CMIP6
Above-cloud concentrations of cloud condensation nuclei help to sustain some Arctic low-level clouds
Contrail formation on ambient aerosol particles for aircraft with hydrogen combustion: a box model trajectory study
Effects of intermittent aerosol forcing on the stratocumulus-to-cumulus transition
Cloud properties and their projected changes in CMIP models with low to high climate sensitivity
Nadja Omanovic, Brigitta Goger, and Ulrike Lohmann
Atmos. Chem. Phys., 24, 14145–14175, https://doi.org/10.5194/acp-24-14145-2024, https://doi.org/10.5194/acp-24-14145-2024, 2024
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We evaluated the numerical weather model ICON in two horizontal resolutions with two bulk microphysics schemes over hilly and complex terrain in Switzerland and Austria, respectively. We focused on the model's ability to simulate mid-level clouds in summer and winter. By combining observational data from two different field campaigns, we show that an increase in the horizontal resolution and a more advanced cloud microphysics scheme is strongly beneficial for cloud representation.
Cornelis Schwenk and Annette Miltenberger
Atmos. Chem. Phys., 24, 14073–14099, https://doi.org/10.5194/acp-24-14073-2024, https://doi.org/10.5194/acp-24-14073-2024, 2024
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Warm conveyor belts (WCBs) transport moisture into the upper atmosphere, where it acts as a greenhouse gas. This transport is not well understood, and the role of rapidly rising air is unclear. We simulate a WCB and look at fast- and slow-rising air to see how moisture is (differently) transported. We find that for fast-ascending air more ice particles reach higher into the atmosphere and that frozen cloud particles are removed differently than during slow ascent, which has more water vapour.
Jing Yang, Jiaojiao Li, Meilian Chen, Xiaoqin Jing, Yan Yin, Bart Geerts, Zhien Wang, Yubao Liu, Baojun Chen, Shaofeng Hua, Hao Hu, Xiaobo Dong, Ping Tian, Qian Chen, and Yang Gao
Atmos. Chem. Phys., 24, 13833–13848, https://doi.org/10.5194/acp-24-13833-2024, https://doi.org/10.5194/acp-24-13833-2024, 2024
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Detecting unambiguous signatures is vital for examining cloud-seeding impacts, but often, seeding signatures are immersed in natural variability. In this study, reflectivity changes induced by glaciogenic seeding using different AgI concentrations are investigated under various conditions, and a method is developed to estimate the AgI concentration needed to detect unambiguous seeding signatures. The results aid in operational seeding-based decision-making regarding the amount of AgI dispersed.
Florian Sauerland, Niels Souverijns, Anna Possner, Heike Wex, Preben Van Overmeiren, Alexander Mangold, Kwinten Van Weverberg, and Nicole van Lipzig
Atmos. Chem. Phys., 24, 13751–13768, https://doi.org/10.5194/acp-24-13751-2024, https://doi.org/10.5194/acp-24-13751-2024, 2024
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We use a regional climate model, COSMO-CLM², enhanced with a module resolving aerosol processes, to study Antarctic clouds. We prescribe different concentrations of ice-nucleating particles to our model to assess how these clouds respond to concentration changes, validating results with cloud and aerosol observations from the Princess Elisabeth Antarctica station. Our results show that aerosol–cloud interactions vary with temperature, providing valuable insights into Antarctic cloud dynamics.
Yi Li, Xiaoli Liu, and Hengjia Cai
Atmos. Chem. Phys., 24, 13525–13540, https://doi.org/10.5194/acp-24-13525-2024, https://doi.org/10.5194/acp-24-13525-2024, 2024
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The influence of different aerosol modes on cloud processes remains controversial. We modified the aerosol spectra and concentrations to simulate a warm stratiform cloud process in Jiangxi, China, using the WRF-SBM scheme. Research shows that different aerosol spectra have diverse effects on cloud droplet spectra, cloud development, and the correlation between dispersion (ε) and cloud physics quantities. Compared to cloud droplet concentration, ε is more sensitive to the volume radius.
Fabian Hoffmann, Franziska Glassmeier, and Graham Feingold
Atmos. Chem. Phys., 24, 13403–13412, https://doi.org/10.5194/acp-24-13403-2024, https://doi.org/10.5194/acp-24-13403-2024, 2024
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Clouds constitute a major cooling influence on Earth's climate system by reflecting a large fraction of the incident solar radiation back to space. This ability is controlled by the number of cloud droplets, which is governed by the number of aerosol particles in the atmosphere, laying the foundation for so-called aerosol–cloud–climate interactions. In this study, a simple model to understand the effect of aerosol on cloud water is developed and applied.
Andrea Mosso, Thomas Hocking, and Thorsten Mauritsen
Atmos. Chem. Phys., 24, 12793–12806, https://doi.org/10.5194/acp-24-12793-2024, https://doi.org/10.5194/acp-24-12793-2024, 2024
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Clouds play a crucial role in the Earth's energy balance, as they can either warm up or cool down the area they cover depending on their height and depth. They are expected to alter their behaviour under climate change, affecting the warming generated by greenhouse gases. This paper proposes a new method to estimate their overall effect on this warming by simulating a climate where clouds are transparent. Results show that with the model used, clouds have a stabilising effect on climate.
Tao Shi, Yuanjian Yang, Ping Qi, and Simone Lolli
Atmos. Chem. Phys., 24, 12807–12822, https://doi.org/10.5194/acp-24-12807-2024, https://doi.org/10.5194/acp-24-12807-2024, 2024
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This paper explored the formation mechanisms of the amplified canopy urban heat island intensity (ΔCUHII) during heat wave (HW) periods in the megacity of Beijing from the perspectives of mountain–valley breeze and urban morphology. During the mountain breeze phase, high-rise buildings with lower sky view factors (SVFs) had a pronounced effect on the ΔCUHII. During the valley breeze phase, high-rise buildings exerted a dual influence on the ΔCUHII.
Yao-Sheng Chen, Jianhao Zhang, Fabian Hoffmann, Takanobu Yamaguchi, Franziska Glassmeier, Xiaoli Zhou, and Graham Feingold
Atmos. Chem. Phys., 24, 12661–12685, https://doi.org/10.5194/acp-24-12661-2024, https://doi.org/10.5194/acp-24-12661-2024, 2024
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Marine stratocumulus cloud is a type of shallow cloud that covers the vast areas of Earth's surface. It plays an important role in Earth's energy balance by reflecting solar radiation back to space. We used numerical models to simulate a large number of marine stratocumuli with different characteristics. We found that how the clouds develop throughout the day is affected by the level of humidity in the air above the clouds and how closely the clouds connect to the ocean surface.
Alexei Korolev, Zhipeng Qu, Jason Milbrandt, Ivan Heckman, Mélissa Cholette, Mengistu Wolde, Cuong Nguyen, Greg M. McFarquhar, Paul Lawson, and Ann M. Fridlind
Atmos. Chem. Phys., 24, 11849–11881, https://doi.org/10.5194/acp-24-11849-2024, https://doi.org/10.5194/acp-24-11849-2024, 2024
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The phenomenon of high ice water content (HIWC) occurs in mesoscale convective systems (MCSs) when a large number of small ice particles with typical sizes of a few hundred micrometers is found at high altitudes. It was found that secondary ice production in the vicinity of the melting layer plays a key role in the formation and maintenance of HIWC. This study presents a conceptual model of the formation of HIWC in tropical MCSs based on in situ observations and numerical simulation.
Puja Roy, Robert M. Rauber, and Larry Di Girolamo
Atmos. Chem. Phys., 24, 11653–11678, https://doi.org/10.5194/acp-24-11653-2024, https://doi.org/10.5194/acp-24-11653-2024, 2024
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Cloud droplet temperature and lifetime impact cloud microphysical processes such as the activation of ice-nucleating particles. We investigate the thermal and radial evolution of supercooled cloud droplets and their surrounding environments with an aim to better understand observed enhanced ice formation at supercooled cloud edges. This analysis shows that the magnitude of droplet cooling during evaporation is greater than estimated from past studies, especially for drier environments.
Mathieu Lachapelle, Mélissa Cholette, and Julie M. Thériault
Atmos. Chem. Phys., 24, 11285–11304, https://doi.org/10.5194/acp-24-11285-2024, https://doi.org/10.5194/acp-24-11285-2024, 2024
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Hazardous precipitation types such as ice pellets and freezing rain are difficult to predict because they are associated with complex microphysical processes. Using Predicted Particle Properties (P3), this work shows that secondary ice production processes increase the amount of ice pellets simulated while decreasing the amount of freezing rain. Moreover, the properties of the simulated precipitation compare well with those that were measured.
Andrew DeLaFrance, Lynn A. McMurdie, Angela K. Rowe, and Andrew J. Heymsfield
Atmos. Chem. Phys., 24, 11191–11206, https://doi.org/10.5194/acp-24-11191-2024, https://doi.org/10.5194/acp-24-11191-2024, 2024
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Using a numerical model, the process whereby falling ice crystals accumulate supercooled liquid water droplets is investigated to elucidate its effects on radar-based measurements and surface precipitation. We demonstrate that this process accounted for 55% of the precipitation during a wintertime storm and is uniquely discernable from other ice crystal growth processes in Doppler velocity measurements. These results have implications for measurements from airborne and spaceborne platforms.
Toshi Matsui, Daniel Hernandez-Deckers, Scott E. Giangrande, Thiago S. Biscaro, Ann Fridlind, and Scott Braun
Atmos. Chem. Phys., 24, 10793–10814, https://doi.org/10.5194/acp-24-10793-2024, https://doi.org/10.5194/acp-24-10793-2024, 2024
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Using computer simulations and real measurements, we discovered that storms over the Amazon were narrower but more intense during the dry periods, producing heavier rain and more ice particles in the clouds. Our research showed that cumulus bubbles played a key role in creating these intense storms. This study can improve the representation of the effect of continental and ocean environments on tropical regions' rainfall patterns in simulations.
Ravi Kumar Reddy Addula, Ingrid de Almeida Ribeiro, Valeria Molinero, and Baron Peters
Atmos. Chem. Phys., 24, 10833–10848, https://doi.org/10.5194/acp-24-10833-2024, https://doi.org/10.5194/acp-24-10833-2024, 2024
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Ice nucleation from supercooled droplets is important in many weather and climate modeling efforts. For experiments where droplets are steadily supercooled from the freezing point, our work combines nucleation theory and survival probability analysis to predict the nucleation spectrum, i.e., droplet freezing probabilities vs. temperature. We use the new framework to extract approximately consistent rate parameters from experiments with different cooling rates and droplet sizes.
Jianhao Zhang, Yao-Sheng Chen, Takanobu Yamaguchi, and Graham Feingold
Atmos. Chem. Phys., 24, 10425–10440, https://doi.org/10.5194/acp-24-10425-2024, https://doi.org/10.5194/acp-24-10425-2024, 2024
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Quantifying cloud response to aerosol perturbations presents a major challenge in understanding the human impact on climate. Using a large number of process-resolving simulations of marine stratocumulus, we show that solar heating drives a negative feedback mechanism that buffers the persistent negative trend in cloud water adjustment after sunrise. This finding has implications for the dependence of the cloud cooling effect on the timing of deliberate aerosol perturbations.
Aaron Wang, Steve Krueger, Sisi Chen, Mikhail Ovchinnikov, Will Cantrell, and Raymond A. Shaw
Atmos. Chem. Phys., 24, 10245–10260, https://doi.org/10.5194/acp-24-10245-2024, https://doi.org/10.5194/acp-24-10245-2024, 2024
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We employ two methods to examine a laboratory experiment on clouds with both ice and liquid phases. The first assumes well-mixed properties; the second resolves the spatial distribution of turbulence and cloud particles. Results show that while the trends in mean properties generally align, when turbulence is resolved, liquid droplets are not fully depleted by ice due to incomplete mixing. This underscores the threshold of ice mass fraction in distinguishing mixed-phase clouds from ice clouds.
Theresa Kiszler, Davide Ori, and Vera Schemann
Atmos. Chem. Phys., 24, 10039–10053, https://doi.org/10.5194/acp-24-10039-2024, https://doi.org/10.5194/acp-24-10039-2024, 2024
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Microphysical processes impact the phase-partitioning of clouds. In this study we evaluate these processes while focusing on low-level Arctic clouds. To achieve this we used an extensive simulation set in combination with a new diagnostic tool. This study presents our findings on the relevance of these processes and their behaviour under different thermodynamic regimes.
Shuaiqi Tang, Hailong Wang, Xiang-Yu Li, Jingyi Chen, Armin Sorooshian, Xubin Zeng, Ewan Crosbie, Kenneth L. Thornhill, Luke D. Ziemba, and Christiane Voigt
Atmos. Chem. Phys., 24, 10073–10092, https://doi.org/10.5194/acp-24-10073-2024, https://doi.org/10.5194/acp-24-10073-2024, 2024
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We examined marine boundary layer clouds and their interactions with aerosols in the E3SM single-column model (SCM) for a case study. The SCM shows good agreement when simulating the clouds with high-resolution models. It reproduces the relationship between cloud droplet and aerosol particle number concentrations as produced in global models. However, the relationship between cloud liquid water and droplet number concentration is different, warranting further investigation.
Suf Lorian and Guy Dagan
Atmos. Chem. Phys., 24, 9323–9338, https://doi.org/10.5194/acp-24-9323-2024, https://doi.org/10.5194/acp-24-9323-2024, 2024
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We examine the combined effect of aerosols and sea surface temperature (SST) on clouds under equilibrium conditions in cloud-resolving radiative–convective equilibrium simulations. We demonstrate that the aerosol–cloud interaction's effect on top-of-atmosphere energy gain strongly depends on the underlying SST, while the shortwave part of the spectrum is significantly more sensitive to SST. Furthermore, increasing aerosols influences upper-troposphere stability and thus anvil cloud fraction.
Jianqi Zhao, Xiaoyan Ma, Johannes Quaas, and Hailing Jia
Atmos. Chem. Phys., 24, 9101–9118, https://doi.org/10.5194/acp-24-9101-2024, https://doi.org/10.5194/acp-24-9101-2024, 2024
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We explore aerosol–cloud interactions in liquid-phase clouds over eastern China and its adjacent ocean in winter based on the WRF-Chem–SBM model, which couples a spectral-bin microphysics scheme and an online aerosol module. Our study highlights the differences in aerosol–cloud interactions between land and ocean and between precipitation clouds and non-precipitation clouds, and it differentiates and quantifies their underlying mechanisms.
Ann Kristin Naumann, Monika Esch, and Bjorn Stevens
EGUsphere, https://doi.org/10.5194/egusphere-2024-2268, https://doi.org/10.5194/egusphere-2024-2268, 2024
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This study explores how uncertainties in the representation of microphysical processes affect the tropical condensate distribution in the global storm-resolving model ICON. The results point to the importance of the fall speed of hydrometeor particles and to a simple relationship: the faster a condensate falls, the less there is of it. Implications for the energy balance and precipitation properties are discussed.
Shiye Huang, Jing Yang, Qian Chen, Jiaojiao Li, Qilin Zhang, and Fengxia Guo
EGUsphere, https://doi.org/10.5194/egusphere-2024-2013, https://doi.org/10.5194/egusphere-2024-2013, 2024
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Aerosol and secondary ice production are both vital to charge separation in thunderstorms, but the relative importance of different SIP processes to cloud electrification under different aerosol conditions is not well understood. In this study, we show in a clean environment, the shattering of freezing drops has the greatest effect on the charging rate, while in a polluted environment, both rime splintering and the shattering of freezing drops have a significant effect on cloud electrification.
Thomas D. DeWitt and Timothy J. Garrett
Atmos. Chem. Phys., 24, 8457–8472, https://doi.org/10.5194/acp-24-8457-2024, https://doi.org/10.5194/acp-24-8457-2024, 2024
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There is considerable disagreement on mathematical parameters that describe the number of clouds of different sizes as well as the size of the largest clouds. Both are key defining characteristics of Earth's atmosphere. A previous study provided an incorrect explanation for the disagreement. Instead, the disagreement may be explained by prior studies not properly accounting for the size of their measurement domain. We offer recommendations for how the domain size can be accounted for.
Sarah Wilson Kemsley, Paulo Ceppi, Hendrik Andersen, Jan Cermak, Philip Stier, and Peer Nowack
Atmos. Chem. Phys., 24, 8295–8316, https://doi.org/10.5194/acp-24-8295-2024, https://doi.org/10.5194/acp-24-8295-2024, 2024
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Aiming to inform parameter selection for future observational constraint analyses, we incorporate five candidate meteorological drivers specifically targeting high clouds into a cloud controlling factor framework within a range of spatial domain sizes. We find a discrepancy between optimal domain size for predicting locally and globally aggregated cloud radiative anomalies and identify upper-tropospheric static stability as an important high-cloud controlling factor.
Ye Liu, Yun Qian, Larry K. Berg, Zhe Feng, Jianfeng Li, Jingyi Chen, and Zhao Yang
Atmos. Chem. Phys., 24, 8165–8181, https://doi.org/10.5194/acp-24-8165-2024, https://doi.org/10.5194/acp-24-8165-2024, 2024
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Deep convection under various large-scale meteorological patterns (LSMPs) shows distinct precipitation features. In southeastern Texas, mesoscale convective systems (MCSs) contribute significantly to precipitation year-round, while isolated deep convection (IDC) is prominent in summer and fall. Self-organizing maps (SOMs) reveal convection can occur without large-scale lifting or moisture convergence. MCSs and IDC events have distinct life cycles influenced by specific LSMPs.
Xiaoran Guo, Jianping Guo, Tianmeng Chen, Ning Li, Fan Zhang, and Yuping Sun
Atmos. Chem. Phys., 24, 8067–8083, https://doi.org/10.5194/acp-24-8067-2024, https://doi.org/10.5194/acp-24-8067-2024, 2024
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The prediction of downhill thunderstorms (DSs) remains elusive. We propose an objective method to identify DSs, based on which enhanced and dissipated DSs are discriminated. A radar wind profiler (RWP) mesonet is used to derive divergence and vertical velocity. The mid-troposphere divergence and prevailing westerlies enhance the intensity of DSs, whereas low-level divergence is observed when the DS dissipates. The findings highlight the key role that an RWP mesonet plays in the evolution of DSs.
Sina Hofer, Klaus Gierens, and Susanne Rohs
Atmos. Chem. Phys., 24, 7911–7925, https://doi.org/10.5194/acp-24-7911-2024, https://doi.org/10.5194/acp-24-7911-2024, 2024
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We try to improve the forecast of ice supersaturation (ISS) and potential persistent contrails using data on dynamical quantities in addition to temperature and relative humidity in a modern kind of regression model. Although the results are improved, they are not good enough for flight routing. The origin of the problem is the strong overlap of probability densities conditioned on cases with and without ice-supersaturated regions (ISSRs) in the important range of 70–100 %.
Harri Kokkola, Juha Tonttila, Silvia Calderón, Sami Romakkaniemi, Antti Lipponen, Aapo Peräkorpi, Tero Mielonen, Edward Gryspeerdt, Timo H. Virtanen, Pekka Kolmonen, and Antti Arola
EGUsphere, https://doi.org/10.5194/egusphere-2024-1964, https://doi.org/10.5194/egusphere-2024-1964, 2024
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Understanding how atmospheric aerosols affect clouds is a scientific challenge. One question is how aerosols affects the amount cloud water. We used a cloud-scale model to study these effects on marine clouds. The study showed that variations in cloud properties and instrument noise can cause bias in satellite derived cloud water content. However, our results suggest that for similar weather conditions with well-defined aerosol concentrations, satellite data can reliably track these effects.
Claudia Christine Stephan and Bjorn Stevens
EGUsphere, https://doi.org/10.5194/egusphere-2024-2020, https://doi.org/10.5194/egusphere-2024-2020, 2024
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Tropical precipitation cluster area and intensity distributions follow power laws, but the physical processes responsible for this behavior remain unknown. We analyze global simulations that realistically represent precipitation processes. We consider Earth-like planets as well as virtual planets to realize different types of large-scale dynamics. Our finding is that power laws in Earth’s precipitation cluster statistics stem from the robust power laws in Earth’s atmospheric wind field.
Luís Filipe Escusa dos Santos, Hannah C. Frostenberg, Alejandro Baró Pérez, Annica M. L. Ekman, Luisa Ickes, and Erik S. Thomson
EGUsphere, https://doi.org/10.5194/egusphere-2024-1891, https://doi.org/10.5194/egusphere-2024-1891, 2024
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The Arctic is experiencing enhanced surface warming. The observed decline in Arctic sea-ice extent is projected to lead to an increase in Arctic shipping activity which may lead to further climatic feedbacks. We investigate, using an atmospheric model and results from marine engine experiments which focused on fuel sulfur content reduction and exhaust wet scrubbing, how ship exhaust particles influence the properties of Arctic clouds. Implications for radiative surface processes are discussed.
Naser Mahfouz, Johannes Mülmenstädt, and Susannah Burrows
Atmos. Chem. Phys., 24, 7253–7260, https://doi.org/10.5194/acp-24-7253-2024, https://doi.org/10.5194/acp-24-7253-2024, 2024
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Climate models are our primary tool to probe past, present, and future climate states unlike the more recent observation record. By constructing a hypothetical model configuration, we show that present-day correlations are insufficient to predict a persistent uncertainty in climate projection (how much sun because clouds will reflect in a changing climate). We hope our result will contribute to the scholarly conversation on better utilizing observations to constrain climate uncertainties.
Britta Schäfer, Robert Oscar David, Paraskevi Georgakaki, Julie Thérèse Pasquier, Georgia Sotiropoulou, and Trude Storelvmo
Atmos. Chem. Phys., 24, 7179–7202, https://doi.org/10.5194/acp-24-7179-2024, https://doi.org/10.5194/acp-24-7179-2024, 2024
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Mixed-phase clouds, i.e., clouds consisting of ice and supercooled water, are very common in the Arctic. However, how these clouds form is often not correctly represented in standard weather models. We show that both ice crystal concentrations in the cloud and precipitation from the cloud can be improved in the model when aerosol concentrations are prescribed from observations and when more processes for ice multiplication, i.e., the production of new ice particles from existing ice, are added.
Nan Sun, Gaopeng Lu, and Yunfei Fu
Atmos. Chem. Phys., 24, 7123–7135, https://doi.org/10.5194/acp-24-7123-2024, https://doi.org/10.5194/acp-24-7123-2024, 2024
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Microphysical characteristics of convective overshooting are essential but poorly understood, and we examine them by using the latest data. (1) Convective overshooting events mainly occur over NC (Northeast China) and northern MEC (Middle and East China). (2) Radar reflectivity of convective overshooting over NC accounts for a higher proportion below the zero level, while the opposite is the case for MEC and SC (South China). (3) Droplets of convective overshooting are large but sparse.
Liu Yang, Saisai Ding, Jing-Wu Liu, and Su-Ping Zhang
Atmos. Chem. Phys., 24, 6809–6824, https://doi.org/10.5194/acp-24-6809-2024, https://doi.org/10.5194/acp-24-6809-2024, 2024
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Advection fog occurs when warm and moist air moves over a cold sea surface. In this situation, the temperature of the foggy air usually drops below the sea surface temperature (SST), particularly at night. High-resolution simulations show that the cooling effect of longwave radiation from the top of the fog layer permeates through the fog, resulting in a cooling of the surface air below SST. This study emphasizes the significance of monitoring air temperature to enhance sea fog forecasting.
Nadja Omanovic, Sylvaine Ferrachat, Christopher Fuchs, Jan Henneberger, Anna J. Miller, Kevin Ohneiser, Fabiola Ramelli, Patric Seifert, Robert Spirig, Huiying Zhang, and Ulrike Lohmann
Atmos. Chem. Phys., 24, 6825–6844, https://doi.org/10.5194/acp-24-6825-2024, https://doi.org/10.5194/acp-24-6825-2024, 2024
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We present simulations with a high-resolution numerical weather prediction model to study the growth of ice crystals in low clouds following glaciogenic seeding. We show that the simulated ice crystals grow slower than observed and do not consume as many cloud droplets as measured in the field. This may have implications for forecasting precipitation, as the ice phase is crucial for precipitation at middle and high latitudes.
Matthew W. Christensen, Peng Wu, Adam C. Varble, Heng Xiao, and Jerome D. Fast
Atmos. Chem. Phys., 24, 6455–6476, https://doi.org/10.5194/acp-24-6455-2024, https://doi.org/10.5194/acp-24-6455-2024, 2024
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Clouds are essential to keep Earth cooler by reflecting sunlight back to space. We show that an increase in aerosol concentration suppresses precipitation in clouds, causing them to accumulate water and expand in a polluted environment with stronger turbulence and radiative cooling. This process enhances their reflectance by 51 %. It is therefore prudent to account for cloud fraction changes in assessments of aerosol–cloud interactions to improve predictions of climate change.
Jing Yang, Shiye Huang, Tianqi Yang, Qilin Zhang, Yuting Deng, and Yubao Liu
Atmos. Chem. Phys., 24, 5989–6010, https://doi.org/10.5194/acp-24-5989-2024, https://doi.org/10.5194/acp-24-5989-2024, 2024
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This study contributes to filling the dearth of understanding the impacts of different secondary ice production (SIP) processes on the cloud electrification in cold-season thunderstorms. The results suggest that SIP, especially the rime-splintering process and the shattering of freezing drops, has significant impacts on the charge structure of the storm. In addition, the modeled radar composite reflectivity and flash rate are improved after implementing the SIP processes in the model.
Ulrike Proske, Sylvaine Ferrachat, and Ulrike Lohmann
Atmos. Chem. Phys., 24, 5907–5933, https://doi.org/10.5194/acp-24-5907-2024, https://doi.org/10.5194/acp-24-5907-2024, 2024
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Climate models include treatment of aerosol particles because these influence clouds and radiation. Over time their representation has grown increasingly detailed. This complexity may hinder our understanding of model behaviour. Thus here we simplify the aerosol representation of our climate model by prescribing mean concentrations, which saves run time and helps to discover unexpected model behaviour. We conclude that simplifications provide a new perspective for model study and development.
Wenhui Zhao, Yi Huang, Steven Siems, Michael Manton, and Daniel Harrison
Atmos. Chem. Phys., 24, 5713–5736, https://doi.org/10.5194/acp-24-5713-2024, https://doi.org/10.5194/acp-24-5713-2024, 2024
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We studied how shallow clouds and rain behave over the Great Barrier Reef (GBR) using a detailed weather model. We found that the shape of the land, especially mountains, and particles in the air play big roles in influencing these clouds. Surprisingly, the sea's temperature had a smaller effect. Our research helps us understand the GBR's climate and how various factors can influence it, where the importance of the local cloud in thermal coral bleaching has recently been identified.
Sidiki Sanogo, Olivier Boucher, Nicolas Bellouin, Audran Borella, Kevin Wolf, and Susanne Rohs
Atmos. Chem. Phys., 24, 5495–5511, https://doi.org/10.5194/acp-24-5495-2024, https://doi.org/10.5194/acp-24-5495-2024, 2024
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Relative humidity relative to ice (RHi) is a key variable in the formation of cirrus clouds and contrails. This study shows that the properties of the probability density function of RHi differ between the tropics and higher latitudes. In line with RHi and temperature variability, aircraft are likely to produce more contrails with bioethanol and liquid hydrogen as fuel. The impact of this fuel change decreases with decreasing pressure levels but increases from high latitudes to the tropics.
Zane Dedekind, Ulrike Proske, Sylvaine Ferrachat, Ulrike Lohmann, and David Neubauer
Atmos. Chem. Phys., 24, 5389–5404, https://doi.org/10.5194/acp-24-5389-2024, https://doi.org/10.5194/acp-24-5389-2024, 2024
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Ice particles precipitating into lower clouds from an upper cloud, the seeder–feeder process, can enhance precipitation. A numerical modeling study conducted in the Swiss Alps found that 48 % of observed clouds were overlapping, with the seeder–feeder process occurring in 10 % of these clouds. Inhibiting the seeder–feeder process reduced the surface precipitation and ice particle growth rates, which were further reduced when additional ice multiplication processes were included in the model.
Marje Prank, Juha Tonttila, Xiaoxia Shang, Sami Romakkaniemi, and Tomi Raatikainen
EGUsphere, https://doi.org/10.5194/egusphere-2024-876, https://doi.org/10.5194/egusphere-2024-876, 2024
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Large primary bioparticles such as pollen can be abundant in the atmosphere. In humid conditions pollens can rupture and release a large number of fine sub-pollen particles (SPPs). The paper investigates what kind of birch pollen concentrations are needed for the pollen and SPPs to start playing a noticeable role in cloud processes and alter precipitation formation. In the studied cases only the largest observed pollen concentrations were able to noticeably alter the precipitation formation.
Liine Heikkinen, Daniel G. Partridge, Sara Blichner, Wei Huang, Rahul Ranjan, Paul Bowen, Emanuele Tovazzi, Tuukka Petäjä, Claudia Mohr, and Ilona Riipinen
Atmos. Chem. Phys., 24, 5117–5147, https://doi.org/10.5194/acp-24-5117-2024, https://doi.org/10.5194/acp-24-5117-2024, 2024
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The organic vapor condensation with water vapor (co-condensation) in rising air below clouds is modeled in this work over the boreal forest because the forest air is rich in organic vapors. We show that the number of cloud droplets can increase by 20 % if considering co-condensation. The enhancements are even larger if the air contains many small, naturally produced aerosol particles. Such conditions are most frequently met in spring in the boreal forest.
Kevin Wolf, Nicolas Bellouin, and Olivier Boucher
Atmos. Chem. Phys., 24, 5009–5024, https://doi.org/10.5194/acp-24-5009-2024, https://doi.org/10.5194/acp-24-5009-2024, 2024
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The contrail formation potential and its tempo-spatial distribution are estimated for the North Atlantic flight corridor. Meteorological conditions of temperature and relative humidity are taken from the ERA5 re-analysis and IAGOS. Based on IAGOS flight tracks, crossing length, size, orientation, frequency of occurrence, and overlap of persistent contrail formation areas are determined. The presented conclusions might provide a guide for statistical flight track optimization to reduce contrails.
Franziska Hellmuth, Tim Carlsen, Anne Sophie Daloz, Robert Oscar David, and Trude Storelvmo
EGUsphere, https://doi.org/10.5194/egusphere-2024-754, https://doi.org/10.5194/egusphere-2024-754, 2024
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This article compares the occurrence of supercooled liquid-containing clouds (sLCCs) and their link to surface snowfall in CloudSat-CALIPSO, ERA5, and CMIP6 models. Significant discrepancies were found, with ERA5 and CMIP6 consistently overestimating sLCC and snowfall frequency. This bias is likely due to cloud microphysics parameterization. This conclusion has implications for accurately representing cloud phase and snowfall in future climate projections.
Lucas J. Sterzinger and Adele L. Igel
Atmos. Chem. Phys., 24, 3529–3540, https://doi.org/10.5194/acp-24-3529-2024, https://doi.org/10.5194/acp-24-3529-2024, 2024
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Using idealized large eddy simulations, we find that clouds forming in the Arctic in environments with low concentrations of aerosol particles may be sustained by mixing in new particles through the cloud top. Observations show that higher concentrations of these particles regularly exist above cloud top in concentrations that are sufficient to promote this sustenance.
Andreas Bier, Simon Unterstrasser, Josef Zink, Dennis Hillenbrand, Tina Jurkat-Witschas, and Annemarie Lottermoser
Atmos. Chem. Phys., 24, 2319–2344, https://doi.org/10.5194/acp-24-2319-2024, https://doi.org/10.5194/acp-24-2319-2024, 2024
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Using hydrogen as aviation fuel affects contrails' climate impact. We study contrail formation behind aircraft with H2 combustion. Due to the absence of soot emissions, contrail ice crystals are assumed to form only on ambient particles mixed into the plume. The ice crystal number, which strongly varies with temperature and aerosol number density, is decreased by more than 80 %–90 % compared to kerosene contrails. However H2 contrails can form at lower altitudes due to higher H2O emissions.
Prasanth Prabhakaran, Fabian Hoffmann, and Graham Feingold
Atmos. Chem. Phys., 24, 1919–1937, https://doi.org/10.5194/acp-24-1919-2024, https://doi.org/10.5194/acp-24-1919-2024, 2024
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In this study, we explore the impact of deliberate aerosol perturbation in the northeast Pacific region using large-eddy simulations. Our results show that cloud reflectivity is sensitive to the aerosol sprayer arrangement in the pristine system, whereas in the polluted system it is largely proportional to the total number of aerosol particles injected. These insights would aid in assessing the efficiency of various aerosol injection strategies for climate intervention applications.
Lisa Bock and Axel Lauer
Atmos. Chem. Phys., 24, 1587–1605, https://doi.org/10.5194/acp-24-1587-2024, https://doi.org/10.5194/acp-24-1587-2024, 2024
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Climate model simulations still show a large range of effective climate sensitivity (ECS) with high uncertainties. An important contribution to ECS is cloud climate feedback. We investigate the representation of cloud physical and radiative properties from Coupled Model Intercomparison Project models grouped by ECS. We compare the simulated cloud properties of today’s climate from three ECS groups and quantify how the projected changes in cloud properties and cloud radiative effects differ.
Cited articles
Andrejczuk, M., Reisner, J., Henson, B., Dubey, M., and Jeffery, C.: The
potential impacts of pollution on a nondrizzling stratus deck: Does aerosol
number matter more than type?, J. Geophys. Res.-Atmos., 113, D19204,
https://doi.org/10.1029/2007JD009445, 2008. a, b, c
Andrejczuk, M., Grabowski, W., Reisner, J., and Gadian, A.: Cloud-aerosol
interactions for boundary layer stratocumulus in the Lagrangian Cloud Model,
J. Geophys. Res.-Atmos., 115, D22214, https://doi.org/10.1029/2010JD014248, 2010. a
Arabas, S. and Shima, S.-I.: On the CCN (de)activation nonlinearities, Nonlin. Processes Geophys., 24, 535–542, https://doi.org/10.5194/npg-24-535-2017, 2017. a
Beals, M. J., Fugal, J. P., Shaw, R. A., Lu, J., Spuler, S. M., and Stith,
J. L.: Holographic measurements of inhomogeneous cloud mixing at the
centimeter scale, Science, 350, 87–90, https://doi.org/10.1126/science.aab0751, 2015. a
Boucher, O., Randall, D., Artaxo, P., Bretherton, C., Feingold, G., Forster,
P., Kerminen, V.-M., Kondo, Y., Liao, H., Lohmann, U., Rasch, P., Satheesh, S., Sherwood, S., Stevens, B., and Zhang, X.: Clouds and
aerosols, in: Climate change 2013: the physical science basis, Contribution
of Working Group I to the Fifth Assessment Report of the Intergovernmental
Panel on Climate Change, Cambridge University Press,
571–657, https://doi.org/10.1017/CBO9781107415324, 2013. a
Brenguier, J.-L., Burnet, F., and Geoffroy, O.: Cloud optical thickness and liquid water path – does the k coefficient vary with droplet
concentration?, Atmos. Chem. Phys., 11, 9771–9786, https://doi.org/10.5194/acp-11-9771-2011, 2011. a
Brown, P. N., Byrne, G. D., and Hindmarsh, A. C.: VODE: A variable-coefficient
ODE solver, SIAM J. Sci. Stat. Comp., 10, 1038–1051, https://doi.org/10.1137/0910062,
1989. a
Çelik, F. and Marwitz, J. D.: Droplet Spectra Broadening by Ripening
Process. Part I: Roles of Curvature and Salinity of Cloud Droplets, J. Atmos.
Sci., 56, 3091–3105, https://doi.org/10.1175/1520-0469(1999)056<3091:DSBBRP>2.0.CO;2,
1999. a, b
Chandrakar, K. K., Cantrell, W., Chang, K., Ciochetto, D., Niedermeier, D.,
Ovchinnikov, M., Shaw, R. A., and Yang, F.: Aerosol indirect effect from
turbulence-induced broadening of cloud-droplet size distributions, P. Natl.
Acad. Sci. USA, 113, 14243–14248, https://doi.org/10.1073/pnas.1612686113, 2016. a, b, c
Chen, J., Liu, Y., Zhang, M., and Peng, Y.: Height Dependency of Aerosol-Cloud
Interaction Regimes, J. Geophys. Res.-Atmos., 123, 491–506,
https://doi.org/10.1002/2017JD027431, 2018. a, b, c, d
Cheng, W. Y., Carrió, G. G., Cotton, W. R., and Saleeby, S. M.: Influence
of cloud condensation and giant cloud condensation nuclei on the development
of precipitating trade wind cumuli in a large eddy simulation, J. Geophys. Res.-Atmos., 114, D08201, https://doi.org/10.1029/2008JD011011, 2009. a
Chuang, P., Charlson, R. J., and Seinfeld, J.: Kinetic limitations on droplet
formation in clouds, Nature, 390, 594–596, https://doi.org/10.1038/37576, 1997. a
Cooper, W. A.: Effects of variable droplet growth histories on droplet size
distributions. Part I: Theory, J. Atmos. Sci., 46, 1301–1311,
https://doi.org/10.1175/1520-0469(1989)046<1301:EOVDGH>2.0.CO;2, 1989. a
Cooper, W. A., Lasher-Trapp, S. G., and Blyth, A. M.: The Influence of
Entrainment and Mixing on the Initial Formation of Rain in a Warm Cumulus
Cloud, J. Atmos. Sci., 70, 1727–1743, https://doi.org/10.1175/JAS-D-12-0128.1, 2013. a
de Lozar, A. and Muessle, L.: Long-resident droplets at the stratocumulus top, Atmos. Chem. Phys., 16, 6563–6576, https://doi.org/10.5194/acp-16-6563-2016, 2016. a
Desai, N., Chandrakar, K., Chang, K., Cantrell, W., and Shaw, R.: Influence of
Microphysical Variability on Stochastic Condensation in a Turbulent
Laboratory Cloud, J. Atmos. Sci., 75, 189–201,
https://doi.org/10.1175/JAS-D-17-0158.1, 2018. a
Devenish, B., Bartello, P., Brenguier, J.-L., Collins, L., Grabowski, W.,
IJzermans, R., Malinowski, S., Reeks, M., Vassilicos, J., Wang, L.-P.,
and Warhaft, Z.: Droplet growth in warm turbulent clouds, Q. J. Roy. Meteor. Soc.,
138, 1401–1429, https://doi.org/10.1002/qj.1897, 2012. a, b, c, d
Ditas, F., Shaw, R. A., Siebert, H., Simmel, M., Wehner, B., and Wiedensohler, A.: Aerosols-cloud microphysics-thermodynamics-turbulence:
evaluating supersaturation in a marine stratocumulus cloud, Atmos. Chem. Phys., 12, 2459–2468, https://doi.org/10.5194/acp-12-2459-2012, 2012. a, b
Ervens, B. and Feingold, G.: On the representation of immersion and condensation freezing in cloud models using different
nucleation schemes, Atmos. Chem. Phys., 12, 5807–5826, https://doi.org/10.5194/acp-12-5807-2012, 2012. a
Falkovich, G. and Pumir, A.: Sling effect in collisions of water droplets in
turbulent clouds, J. Atmos. Sci., 64, 4497–4505,
https://doi.org/10.1175/2007JAS2371.1, 2007. a
Feingold, G. and Heymsfield, A. J.: Parameterizations of Condensational Growth
of Droplets for Use in General Circulation Models, J. Atmos. Sci., 49,
2325–2342, https://doi.org/10.1175/1520-0469(1992)049<2325:POCGOD>2.0.CO;2, 1992. a
Feingold, G. and Kreidenweis, S.: Does cloud processing of aerosol enhance
droplet concentrations?, J. Geophys. Res.-Atmos., 105, 24351–24361,
https://doi.org/10.1029/2000JD900369, 2000. a, b
Feingold, G. and Siebert, H.: Cloud-Aerosol Interactions from the Micro to the
Cloud Scale, in: Clouds in the Perturbed Climate System: Their Relationship
to Energy Balance, Atmospheric Dynamics, and Precipitation, MIT
Press, 319–338, https://doi.org/10.7551/mitpress/9780262012874.001.0001, 2009. a
Feingold, G., Cotton, W., Stevens, B., and Frisch, A.: The relationship between
drop in-cloud residence time and drizzle production in numerically simulated
stratocumulus clouds, J. Atmos. Sci., 53, 1108–1122,
https://doi.org/10.1175/1520-0469(1996)053<1108:TRBDIC>2.0.CO;2, 1996. a
Feingold, G., Boers, R., Stevens, B., and Cotton, W. R.: A modeling study of
the effect of drizzle on cloud optical depth and susceptibility, J. Geophys. Res.-Atmos., 102, 13527–13534, https://doi.org/10.1029/97JD00963, 1997. a
Feingold, G., Kreidenweis, S. M., and Zhang, Y.: Stratocumulus processing of
gases and cloud condensation nuclei: 1. Trajectory ensemble model, J. Geophys. Res.-Atmos., 103, 19527–19542, https://doi.org/10.1029/98JD01750, 1998. a, b
Feingold, G., Cotton, W. R., Kreidenweis, S. M., and Davis, J. T.: The Impact
of Giant Cloud Condensation Nuclei on Drizzle Formation in Stratocumulus:
Implications for Cloud Radiative Properties, J. Atmos. Sci., 56, 4100–4117,
https://doi.org/10.1175/1520-0469(1999)056<4100:TIOGCC>2.0.CO;2, 1999. a
Feingold, G., Remer, L. A., Ramaprasad, J., and Kaufman, Y. J.: Analysis of
smoke impact on clouds in Brazilian biomass burning regions: An extension of
Twomey's approach, J. Geophys. Res.-Atmos., 106, 22907–22922,
https://doi.org/10.1029/2001JD000732, 2001. a
Ghan, S. J., Guzman, G., and Abdul-Razzak, H.: Competition between Sea Salt and
Sulfate Particles as Cloud Condensation Nuclei, J. Atmos. Sci., 55,
3340–3347, https://doi.org/10.1175/1520-0469(1998)055<3340:CBSSAS>2.0.CO;2, 1998. a
Glienke, S., Kostinski, A., Fugal, J., Shaw, R., Borrmann, S., and Stith, J.:
Cloud droplets to drizzle: contribution of transition drops to microphysical
and optical properties of marine stratocumulus clouds, Geophys. Res. Lett.,
44, 8002–8010, https://doi.org/10.1002/2017GL074430, 2017. a, b
Göke, S., Ochs III, H. T., and Rauber, R. M.: Radar Analysis of
Precipitation Initiation in Maritime versus Continental Clouds near the
Florida Coast: Inferences Concerning the Role of CCN and Giant Nuclei, J.
Atmos. Sci., 64, 3695–3707, https://doi.org/10.1175/JAS3961.1, 2007. a
Grabowski, W. W. and Abade, G. C.: Broadening of Cloud Droplet Spectra Through
Eddy Hopping: Turbulent Adiabatic Parcel Simulations, J. Atmos. Sci., 74,
1485–1493, https://doi.org/10.1175/JAS-D-17-0043.1, 2017. a
Grabowski, W. W. and Wang, L.-P.: Growth of Cloud Droplets in a Turbulent
Environment, Annu. Rev. Fluid Mech., 45, 293–324,
https://doi.org/10.1146/annurev-fluid-011212-140750, 2013. a
Grabowski, W. W., Dziekan, P., and Pawlowska, H.: Lagrangian condensation microphysics with Twomey CCN activation,
Geosci. Model Dev., 11, 103–120, https://doi.org/10.5194/gmd-11-103-2018, 2018. a, b
Hagen, D. E.: A numerical cloud model for the support of laboratory
experimentation, J. Appl. Meteorol., 18, 1035–1043,
https://doi.org/10.1175/1520-0450(1979)018<1035:ANCMFT>2.0.CO;2, 1979. a
Hammer, E., Bukowiecki, N., Luo, B. P., Lohmann, U., Marcolli, C., Weingartner, E., Baltensperger, U., and Hoyle, C. R.:
Sensitivity estimations for cloud droplet formation in the vicinity of the high-alpine research station
Jungfraujoch (3580 m a.s.l.), Atmos. Chem. Phys., 15, 10309–10323, https://doi.org/10.5194/acp-15-10309-2015, 2015. a
Heymsfield, A. J. and Sabin, R. M.: Cirrus Crystal Nucleation by Homogeneous
Freezing of Solution Droplets, J. Atmos. Sci., 46, 2252–2264,
https://doi.org/10.1175/1520-0469(1989)046<2252:CCNBHF>2.0.CO;2, 1989. a, b
Hoffmann, F.: On the limits of Köhler activation theory: how do collision and coalescence affect the activation of aerosols?,
Atmos. Chem. Phys., 17, 8343–8356, https://doi.org/10.5194/acp-17-8343-2017, 2017. a
Hoffmann, F., Raasch, S., and Noh, Y.: Entrainment of aerosols and their
activation in a shallow cumulus cloud studied with a coupled LCM–LES
approach, Atmos. Res., 156, 43–57, https://doi.org/10.1016/j.atmosres.2014.12.008,
2015. a
Howell, W. E.: The growth of cloud drops in uniformly cooled air, J. Meteorol.,
6, 134–149, https://doi.org/10.1175/1520-0469(1949)006<0134:TGOCDI>2.0.CO;2, 1949. a
Jensen, J. B. and Lee, S.: Giant Sea-Salt Aerosols and Warm Rain Formation in
Marine Stratocumulus, J. Atmos. Sci., 65, 3678–3694,
https://doi.org/10.1175/2008JAS2617.1, 2008. a
Johnson, D. B.: The Role of Giant and Ultragiant Aerosol Particles in Warm Rain
Initiation, J. Atmos. Sci., 39, 448–460,
https://doi.org/10.1175/1520-0469(1982)039<0448:TROGAU>2.0.CO;2, 1982. a
Katzwinkel, J., Siebert, H., Heus, T., and Shaw, R. A.: Measurements of
Turbulent Mixing and Subsiding Shells in Trade Wind Cumuli, J. Atmos. Sci.,
71, 2810–2822, https://doi.org/10.1175/JAS-D-13-0222.1, 2014. a
Khain, A., Ovtchinnikov, M., Pinsky, M., Pokrovsky, A., and Krugliak, H.: Notes
on the state-of-the-art numerical modeling of cloud microphysics, Atmos.
Res., 55, 159–224, https://doi.org/10.1016/S0169-8095(00)00064-8, 2000. a, b
Khain, A., Beheng, K., Heymsfield, A., Korolev, A., Krichak, S., Levin, Z.,
Pinsky, M., Phillips, V., Prabhakaran, T., Teller, A., van de Heever, S., and Yano, J.: Representation
of microphysical processes in cloud-resolving models: Spectral (bin)
microphysics versus bulk parameterization, Rev. Geophys., 53, 247–322,
https://doi.org/10.1002/2014RG000468, 2015. a
Khvorostyanov, V. I. and Curry, J. A.: Toward the Theory of Stochastic
Condensation in Clouds. Part I: A General Kinetic Equation, J. Atmos. Sci.,
56, 3985–3996, https://doi.org/10.1175/1520-0469(1999)056<3985:TTTOSC>2.0.CO;2, 1999. a
Kogan, Y. L.: Large-eddy simulation of air parcels in stratocumulus clouds:
Time scales and spatial variability, J. Atmos. Sci., 63, 952–967,
https://doi.org/10.1175/JAS3665.1, 2006. a
Korolev, A. V. and Mazin, I. P.: Supersaturation of Water Vapor in Clouds, J.
Atmos. Sci., 60, 2957–2974,
https://doi.org/10.1175/1520-0469(2003)060<2957:SOWVIC>2.0.CO;2, 2003. a, b
Kostinski, A. B. and Shaw, R. A.: Fluctuations and luck in droplet growth by
coalescence, B. Am. Meteorol. Soc., 86, 235–244,
https://doi.org/10.1175/BAMS-86-2-235, 2005. a
Kreidenweis, S. M., Walcek, C. J., Feingold, G., Gong, W., Jacobson, M. Z.,
Kim, C.-H., Liu, X., Penner, J. E., Nenes, A., and Seinfeld, J. H.:
Modification of aerosol mass and size distribution due to aqueous-phase
SO2 oxidation in clouds: Comparisons of several models, J. Geophys. Res.-Atmos., 108, 4213, https://doi.org/10.1029/2002JD002697, 2003. a, b
Laird, N. F., Ochs III, H. T., Rauber, R. M., and Miller, L. J.: Initial
Precipitation Formation in Warm Florida Cumulus, J. Atmos. Sci., 57,
3740–3751, https://doi.org/10.1175/1520-0469(2000)057<3740:IPFIWF>2.0.CO;2, 2000. a
Lamb, D. and Verlinde, J.: Physics and Chemistry of Clouds, Cambridge
University Press, https://doi.org/10.1017/CBO9780511976377, 2011. a, b, c
Lasher-Trapp, S. G., Cooper, W. A., and Blyth, A. M.: Broadening of droplet
size distributions from entrainment and mixing in a cumulus cloud, Q. J. Roy.
Meteor. Soc., 131, 195–220, https://doi.org/10.1256/qj.03.199, 2005. a
Lebo, Z. J. and Seinfeld, J. H.: A continuous spectral aerosol-droplet microphysics model,
Atmos. Chem. Phys., 11, 12297–12316, https://doi.org/10.5194/acp-11-12297-2011, 2011. a
Li, Z., Xue, H., and Yang, F.: A modeling study of ice formation affected by
aerosols, J. Geophys. Res.-Atmos., 118, 11213–11227,
https://doi.org/10.1002/jgrd.50861, 2013. a
Liu, Y. and Daum, P. H.: Anthropogenic aerosols: Indirect warming effect from
dispersion forcing, Nature, 419, 580–581, https://doi.org/10.1038/419580a, 2002. a, b
Lu, M.-L. and Seinfeld, J. H.: Effect of aerosol number concentration on cloud
droplet dispersion: A large-eddy simulation study and implications for
aerosol indirect forcing, J. Geophys. Res.-Atmos., 111, D02207,
https://doi.org/10.1029/2005JD006419, 2006. a
McFiggans, G., Artaxo, P., Baltensperger, U., Coe, H., Facchini, M. C., Feingold, G., Fuzzi, S., Gysel, M., Laaksonen, A.,
Lohmann, U., Mentel, T. F., Murphy, D. M., O'Dowd, C. D., Snider, J. R., and Weingartner, E.: The effect of
physical and chemical aerosol properties on warm cloud droplet activation, Atmos. Chem. Phys., 6, 2593–2649, https://doi.org/10.5194/acp-6-2593-2006, 2006. a, b
McGraw, R. and Liu, Y.: Brownian drift-diffusion model for evolution of droplet
size distributions in turbulent clouds, Geophys. Res. Lett., 33,
L03802, https://doi.org/10.1029/2005GL023545, 2006. a
Miles, N. L., Verlinde, J., and Clothiaux, E. E.: Cloud Droplet Size
Distributions in Low-Level Stratiform Clouds, J. Atmos. Sci., 57, 295–311,
https://doi.org/10.1175/1520-0469(2000)057<0295:CDSDIL>2.0.CO;2, 2000. a, b
Mordy, W.: Computations of the Growth by Condensation of a Population of Cloud
Droplets, Tellus, 11, 16–44, https://doi.org/10.1111/j.2153-3490.1959.tb00003.x, 1959. a, b
Murphy, D., Thomson, D., and Mahoney, M.: In situ measurements of organics,
meteoritic material, mercury, and other elements in aerosols at 5 to 19
kilometers, Science, 282, 1664–1669, https://doi.org/10.1126/science.282.5394.1664,
1998. a
Naumann, A. K. and Seifert, A.: A Lagrangian drop model to study warm rain
microphysical processes in shallow cumulus, J. Adv. Model Earth Sy., 7,
1136–1154, https://doi.org/10.1002/2015MS000456, 2015. a
Ovchinnikov, M. and Easter, R. C.: Modeling aerosol growth by aqueous chemistry
in a nonprecipitating stratiform cloud, J. Geophys. Res.-Atmos., 115,
D14210, https://doi.org/10.1029/2009JD012816, 2010. a, b
Paluch, I. R.: Theoretical collision efficiencies of charged cloud droplets, J.
Geophys. Res., 75, 1633–1640, https://doi.org/10.1029/JC075i009p01633, 1970. a
Politovich, M. K. and Cooper, W. A.: Variability of the Supersaturation in
Cumulus Clouds, J. Atmos. Sci., 45, 1651–1664,
https://doi.org/10.1175/1520-0469(1988)045<1651:VOTSIC>2.0.CO;2, 1988. a
Pöschl, U., Rose, D., and Andreae, M.: Climatologies of Cloud-related
Aerosols. Part 2: Particle Hygroscopicity and Cloud Condensation Nucleus
Activity, in: Clouds in the Perturbed Climate System: Their Relationship to
Energy Balance, Atmospheric Dynamics, and Precipitation, MIT
Press, 58–72, https://doi.org/10.7551/mitpress/9780262012874.001.0001, 2009. a
Pruppacher, H. R. and Klett, J. D.: Microphysics of Clouds and Precipitation,
Springer Science & Business Media, https://doi.org/10.1007/978-0-306-48100-0, 2010. a, b, c, d
Reutter, P., Su, H., Trentmann, J., Simmel, M., Rose, D., Gunthe, S. S., Wernli, H., Andreae, M. O., and Pöschl, U.: Aerosol- and updraft-limited
regimes of cloud droplet formation: influence of particle number, size and hygroscopicity on the activation of cloud condensation nuclei (CCN),
Atmos. Chem. Phys., 9, 7067–7080, https://doi.org/10.5194/acp-9-7067-2009, 2009. a, b
Romakkaniemi, S., McFiggans, G., Bower, K., Brown, P., Coe, H., and Choularton,
T.: A comparison between trajectory ensemble and adiabatic parcel modeled
cloud properties and evaluation against airborne measurements, J. Geophys. Res.-Atmos., 114, D06214, https://doi.org/10.1029/2008JD011286, 2009. a
Sardina, G., Picano, F., Brandt, L., and Caballero, R.: Continuous growth of
droplet size variance due to condensation in turbulent clouds, Phys. Rev.
Lett., 115, 184501, https://doi.org/10.1103/PhysRevLett.115.184501, 2015. a
Sardina, G., Poulain, S., Brandt, L., and Caballero, R.: Broadening of Cloud
Droplet Size Spectra by Stochastic Condensation: Effects of Mean Updraft
Velocity and CCN Activation, J. Atmos. Sci., 75, 451–467,
https://doi.org/10.1175/JAS-D-17-0241.1, 2018. a
Shaw, R. A.: Particle-turbulence interactions in atmospheric clouds, Annu. Rev.
Fluid Mech., 35, 183–227, https://doi.org/10.1146/annurev.fluid.35.101101.161125,
2003. a, b
Shaw, R. A. and Lamb, D.: Experimental determination of the thermal
accommodation and condensation coefficients of water, J. Chem. Phys., 111,
10659–10663, https://doi.org/10.1063/1.480419, 1999. a
Siebert, H. and Shaw, R. A.: Supersaturation Fluctuations during the Early
Stage of Cumulus Formation, J. Atmos. Sci., 74, 975–988,
https://doi.org/10.1175/JAS-D-16-0115.1, 2017.
a, b
Siewert, C., Bec, J., and Krstulovic, G.: Statistical steady state in turbulent
droplet condensation, J. Fluid Mech., 810, 254–280,
https://doi.org/10.1017/jfm.2016.712, 2017. a
Squires, P.: The growth of cloud drops by condensation. I. General
characteristics, Aust. J. Chem., 5, 59–86, https://doi.org/10.1071/CH9520059, 1952. a
Srivastava, R.: Growth of Cloud Drops by Condensation: Effect of Surface
Tension on the Dispersion of Drop Sizes, J. Atmos. Sci., 48, 1596–1599,
https://doi.org/10.1175/1520-0469(1991)048<1596:GOCDBC>2.0.CO;2, 1991. a, b, c
Takeda, T. and Kuba, N.: Numerical study of the effect of CCN on the size
distribution of cloud droplets, J. Meteorol. Soc. Jpn., 60, 978–993,
https://doi.org/10.2151/jmsj1965.60.4_978, 1982. a
Tang, I. and Munkelwitz, H.: Water activities, densities, and refractive
indices of aqueous sulfates and sodium nitrate droplets of atmospheric
importance, J. Geophys. Res.-Atmos., 99, 18801–18808,
https://doi.org/10.1029/94JD01345, 1994. a
Wood, R.: Stratocumulus Clouds, Mon. Weather Rev., 140, 2373–2423,
https://doi.org/10.1175/MWR-D-11-00121.1, 2012. a, b
Xue, H. and Feingold, G.: A modeling study of the effect of nitric acid on
cloud properties, J. Geophys. Res.-Atmos., 109, D18204,
https://doi.org/10.1029/2004JD004750, 2004. a, b, c
Yang, F., Xue, H., Deng, Z., Zhao, C., and Zhang, Q.: A closure study of cloud condensation nuclei in the North China
Plain using droplet kinetic condensational growth model, Atmos. Chem. Phys., 12, 5399–5411, https://doi.org/10.5194/acp-12-5399-2012, 2012. a
Yang, F., Ovchinnikov, M., and Shaw, R. A.: Long-lifetime ice particles in
mixed-phase stratiform clouds: Quasi-steady and recycled growth, J. Geophys. Res.-Atmos., 120, 11617–11635, https://doi.org/10.1002/2015JD023679, 2015. a
Yang, F., Shaw, R., and Xue, H.: Conditions for super-adiabatic droplet growth after entrainment mixing,
Atmos. Chem. Phys., 16, 9421–9433, https://doi.org/10.5194/acp-16-9421-2016, 2016. a, b, c, d
Yin, Y., Levin, Z., Reisin, T. G., and Tzivion, S.: The effects of giant cloud
condensation nuclei on the development of precipitation in convective
clouds – A numerical study, Atmos. Res., 53, 91–116,
https://doi.org/10.1016/S0169-8095(99)00046-0, 2000. a
Short summary
Cloud droplet size distribution (CDSD), which is related to cloud albedo and lifetime, is usually observed broader than predicted from adiabatic parcel calculations. Results in this study show that the CDSD can be broadened during condensational growth as a result of Ostwald ripening amplified by droplet deactivation and reactivation. Our results suggest that it is important to consider both curvature and solute effects before and after cloud droplet activation in a 3-D cloud model.
Cloud droplet size distribution (CDSD), which is related to cloud albedo and lifetime, is...
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