Research article
13 Apr 2018
Research article
| 13 Apr 2018
Continuous non-marine inputs of per- and polyfluoroalkyl substances to the High Arctic: a multi-decadal temporal record
Heidi M. Pickard et al.
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Total article views: 2,869 (including HTML, PDF, and XML)
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Cited
39 citations as recorded by crossref.
- Gas-Phase Detection of Fluorotelomer Alcohols and Other Oxygenated Per- and Polyfluoroalkyl Substances by Chemical Ionization Mass Spectrometry T. Riedel et al. 10.1021/acs.estlett.9b00196
- Wastewater sources of per- and polyfluorinated alkyl substances (PFAS) and pharmaceuticals in four Canadian Arctic communities K. Stroski et al. 10.1016/j.scitotenv.2019.134494
- Atmospheric perfluoroalkyl acid occurrence and isomer profiles in Beijing, China J. Wu et al. 10.1016/j.envpol.2019.113129
- A global atmospheric chemistry model for the fate and transport of PFCAs and their precursors C. Thackray et al. 10.1039/C9EM00326F
- Perfluoroalkyl acids in pregnant women from Nunavik (Quebec, Canada): Trends in exposure and associations with country foods consumption É. Caron-Beaudoin et al. 10.1016/j.envint.2020.106169
- The fate of poly- and perfluoroalkyl substances in a marine food web influenced by land-based sources in the Norwegian Arctic A. Ali et al. 10.1039/D0EM00510J
- PFAS Exposure Pathways for Humans and Wildlife: A Synthesis of Current Knowledge and Key Gaps in Understanding A. De Silva et al. 10.1002/etc.4935
- Legacy and Novel Per- and Polyfluoroalkyl Substances in Juvenile Seabirds from the U.S. Atlantic Coast A. Robuck et al. 10.1021/acs.est.0c01951
- Climate change influence on the levels and trends of persistent organic pollutants (POPs) and chemicals of emerging Arctic concern (CEACs) in the Arctic physical environment – a review H. Hung et al. 10.1039/D1EM00485A
- Investigating the Uptake and Fate of Poly- and Perfluoroalkylated Substances (PFAS) in Sea Ice Using an Experimental Sea Ice Chamber J. Garnett et al. 10.1021/acs.est.1c01645
- Ice Core Record of Persistent Short‐Chain Fluorinated Alkyl Acids: Evidence of the Impact From Global Environmental Regulations H. Pickard et al. 10.1029/2020GL087535
- Levels and trends of poly- and perfluoroalkyl substances in the Arctic environment – An update D. Muir et al. 10.1016/j.emcon.2019.06.002
- Transport of Legacy Perfluoroalkyl Substances and the Replacement Compound HFPO-DA through the Atlantic Gateway to the Arctic Ocean—Is the Arctic a Sink or a Source? H. Joerss et al. 10.1021/acs.est.0c00228
- Occurrence and source apportionment of perfluoroalkyl acids (PFAAs) in the atmosphere in China D. Han et al. 10.5194/acp-19-14107-2019
- Occurrence and sources of per- and polyfluoroalkyl substances in the ice-melting lakes of Larsemann Hills, East Antarctica G. Shan et al. 10.1016/j.scitotenv.2021.146747
- High Concentrations of Perfluoroalkyl Acids in Arctic Seawater Driven by Early Thawing Sea Ice J. Garnett et al. 10.1021/acs.est.1c01676
- Per‐ and polyfluoroalkyl substances and their alternatives in paper food packaging G. Glenn et al. 10.1111/1541-4337.12726
- Perfluoroalkyl substances in precipitation from the Tibetan Plateau during monsoon season: Concentrations, source regions and mass fluxes M. Chen et al. 10.1016/j.chemosphere.2021.131105
- Side-chain fluorotelomer-based polymers in children car seats Y. Wu et al. 10.1016/j.envpol.2020.115477
- Understanding PFAAs exposure in a generalist seabird species breeding in the vicinity of a fluorochemical plant: Influence of maternal transfer and diet A. Lopez-Antia et al. 10.1016/j.envpol.2020.116355
- Per- and polyfluoroalkyl substances in surface water, gas and particle in open ocean and coastal environment E. Yamazaki et al. 10.1016/j.chemosphere.2021.129869
- Occurrence and toxicity of perfluoroalkyl acids along the estuarine and coastal regions under varied environmental factors R. Avellán-Llaguno et al. 10.1016/j.scitotenv.2020.144584
- A review of the pathways of human exposure to poly- and perfluoroalkyl substances (PFASs) and present understanding of health effects E. Sunderland et al. 10.1038/s41370-018-0094-1
- Snow buntings (Plectrophenax nivealis) as bio-indicators for exposure differences to legacy and emerging persistent organic pollutants from the Arctic terrestrial environment on Svalbard N. Warner et al. 10.1016/j.scitotenv.2019.02.351
- Legacy and Emerging Persistent Organic Pollutants (POPs) in Terrestrial Compartments in the High Arctic: Sorption and Secondary Sources A. Cabrerizo et al. 10.1021/acs.est.8b05011
- Atmospheric Deposition and Annual Flux of Legacy Perfluoroalkyl Substances and Replacement Perfluoroalkyl Ether Carboxylic Acids in Wilmington, NC, USA M. Shimizu et al. 10.1021/acs.estlett.1c00251
- Fluorine Mass Balance and Suspect Screening in Marine Mammals from the Northern Hemisphere K. Spaan et al. 10.1021/acs.est.9b06773
- Fate and Transport of Perfluoroalkyl Substances from Snowpacks into a Lake in the High Arctic of Canada J. MacInnis et al. 10.1021/acs.est.9b03372
- Influence of Water Concentrations of Perfluoroalkyl Acids (PFAAs) on Their Size-Resolved Enrichment in Nascent Sea Spray Aerosols B. Sha et al. 10.1021/acs.est.0c03804
- A Bad Start in Life? Maternal Transfer of Legacy and Emerging Poly- and Perfluoroalkyl Substances to Eggs in an Arctic Seabird W. Jouanneau et al. 10.1021/acs.est.1c03773
- Influence of atmospheric conditions on the role of trifluoroacetic acid in atmospheric sulfuric acid–dimethylamine nucleation L. Liu et al. 10.5194/acp-21-6221-2021
- Investigation of perfluoroalkyl substances in proglacial rivers and permafrost seep in a high Arctic watershed J. MacInnis et al. 10.1039/D1EM00349F
- A closer look into the contribution of atmospheric gas-phase pathways in the formation of perfluorocarboxylic acids M. Altarawneh 10.1016/j.apr.2021.101255
- Levels and Seasonal Trends of C1–C4 Perfluoroalkyl Acids and the Discovery of Trifluoromethane Sulfonic Acid in Surface Snow in the Arctic M. Björnsdotter et al. 10.1021/acs.est.1c04776
- Assessing the contribution of atmospheric transport and tourism activities to the occurrence of perfluoroalkyl acids (PFAAs) in an Alpine Nature Reserve C. Wang et al. 10.1016/j.scitotenv.2019.133851
- Lethal and sublethal toxicity of perfluorooctanoic acid (PFOA) in chronic tests with Hyalella azteca (amphipod) and early-life stage tests with Pimephales promelas (fathead minnow) A. Bartlett et al. 10.1016/j.ecoenv.2020.111250
- Poly- and Perfluoroalkyl Substances in Seawater and Plankton from the Northwestern Atlantic Margin X. Zhang et al. 10.1021/acs.est.9b03230
- Sea Spray Aerosol (SSA) as a Source of Perfluoroalkyl Acids (PFAAs) to the Atmosphere: Field Evidence from Long-Term Air Monitoring B. Sha et al. 10.1021/acs.est.1c04277
- Characterization of perfluoroalkyl substances in sediment cores from High and Low Arctic lakes in Canada J. MacInnis et al. 10.1016/j.scitotenv.2019.02.210
38 citations as recorded by crossref.
- Gas-Phase Detection of Fluorotelomer Alcohols and Other Oxygenated Per- and Polyfluoroalkyl Substances by Chemical Ionization Mass Spectrometry T. Riedel et al. 10.1021/acs.estlett.9b00196
- Wastewater sources of per- and polyfluorinated alkyl substances (PFAS) and pharmaceuticals in four Canadian Arctic communities K. Stroski et al. 10.1016/j.scitotenv.2019.134494
- Atmospheric perfluoroalkyl acid occurrence and isomer profiles in Beijing, China J. Wu et al. 10.1016/j.envpol.2019.113129
- A global atmospheric chemistry model for the fate and transport of PFCAs and their precursors C. Thackray et al. 10.1039/C9EM00326F
- Perfluoroalkyl acids in pregnant women from Nunavik (Quebec, Canada): Trends in exposure and associations with country foods consumption É. Caron-Beaudoin et al. 10.1016/j.envint.2020.106169
- The fate of poly- and perfluoroalkyl substances in a marine food web influenced by land-based sources in the Norwegian Arctic A. Ali et al. 10.1039/D0EM00510J
- PFAS Exposure Pathways for Humans and Wildlife: A Synthesis of Current Knowledge and Key Gaps in Understanding A. De Silva et al. 10.1002/etc.4935
- Legacy and Novel Per- and Polyfluoroalkyl Substances in Juvenile Seabirds from the U.S. Atlantic Coast A. Robuck et al. 10.1021/acs.est.0c01951
- Climate change influence on the levels and trends of persistent organic pollutants (POPs) and chemicals of emerging Arctic concern (CEACs) in the Arctic physical environment – a review H. Hung et al. 10.1039/D1EM00485A
- Investigating the Uptake and Fate of Poly- and Perfluoroalkylated Substances (PFAS) in Sea Ice Using an Experimental Sea Ice Chamber J. Garnett et al. 10.1021/acs.est.1c01645
- Ice Core Record of Persistent Short‐Chain Fluorinated Alkyl Acids: Evidence of the Impact From Global Environmental Regulations H. Pickard et al. 10.1029/2020GL087535
- Levels and trends of poly- and perfluoroalkyl substances in the Arctic environment – An update D. Muir et al. 10.1016/j.emcon.2019.06.002
- Transport of Legacy Perfluoroalkyl Substances and the Replacement Compound HFPO-DA through the Atlantic Gateway to the Arctic Ocean—Is the Arctic a Sink or a Source? H. Joerss et al. 10.1021/acs.est.0c00228
- Occurrence and source apportionment of perfluoroalkyl acids (PFAAs) in the atmosphere in China D. Han et al. 10.5194/acp-19-14107-2019
- Occurrence and sources of per- and polyfluoroalkyl substances in the ice-melting lakes of Larsemann Hills, East Antarctica G. Shan et al. 10.1016/j.scitotenv.2021.146747
- High Concentrations of Perfluoroalkyl Acids in Arctic Seawater Driven by Early Thawing Sea Ice J. Garnett et al. 10.1021/acs.est.1c01676
- Per‐ and polyfluoroalkyl substances and their alternatives in paper food packaging G. Glenn et al. 10.1111/1541-4337.12726
- Perfluoroalkyl substances in precipitation from the Tibetan Plateau during monsoon season: Concentrations, source regions and mass fluxes M. Chen et al. 10.1016/j.chemosphere.2021.131105
- Side-chain fluorotelomer-based polymers in children car seats Y. Wu et al. 10.1016/j.envpol.2020.115477
- Understanding PFAAs exposure in a generalist seabird species breeding in the vicinity of a fluorochemical plant: Influence of maternal transfer and diet A. Lopez-Antia et al. 10.1016/j.envpol.2020.116355
- Per- and polyfluoroalkyl substances in surface water, gas and particle in open ocean and coastal environment E. Yamazaki et al. 10.1016/j.chemosphere.2021.129869
- Occurrence and toxicity of perfluoroalkyl acids along the estuarine and coastal regions under varied environmental factors R. Avellán-Llaguno et al. 10.1016/j.scitotenv.2020.144584
- A review of the pathways of human exposure to poly- and perfluoroalkyl substances (PFASs) and present understanding of health effects E. Sunderland et al. 10.1038/s41370-018-0094-1
- Snow buntings (Plectrophenax nivealis) as bio-indicators for exposure differences to legacy and emerging persistent organic pollutants from the Arctic terrestrial environment on Svalbard N. Warner et al. 10.1016/j.scitotenv.2019.02.351
- Legacy and Emerging Persistent Organic Pollutants (POPs) in Terrestrial Compartments in the High Arctic: Sorption and Secondary Sources A. Cabrerizo et al. 10.1021/acs.est.8b05011
- Atmospheric Deposition and Annual Flux of Legacy Perfluoroalkyl Substances and Replacement Perfluoroalkyl Ether Carboxylic Acids in Wilmington, NC, USA M. Shimizu et al. 10.1021/acs.estlett.1c00251
- Fluorine Mass Balance and Suspect Screening in Marine Mammals from the Northern Hemisphere K. Spaan et al. 10.1021/acs.est.9b06773
- Fate and Transport of Perfluoroalkyl Substances from Snowpacks into a Lake in the High Arctic of Canada J. MacInnis et al. 10.1021/acs.est.9b03372
- Influence of Water Concentrations of Perfluoroalkyl Acids (PFAAs) on Their Size-Resolved Enrichment in Nascent Sea Spray Aerosols B. Sha et al. 10.1021/acs.est.0c03804
- A Bad Start in Life? Maternal Transfer of Legacy and Emerging Poly- and Perfluoroalkyl Substances to Eggs in an Arctic Seabird W. Jouanneau et al. 10.1021/acs.est.1c03773
- Influence of atmospheric conditions on the role of trifluoroacetic acid in atmospheric sulfuric acid–dimethylamine nucleation L. Liu et al. 10.5194/acp-21-6221-2021
- Investigation of perfluoroalkyl substances in proglacial rivers and permafrost seep in a high Arctic watershed J. MacInnis et al. 10.1039/D1EM00349F
- A closer look into the contribution of atmospheric gas-phase pathways in the formation of perfluorocarboxylic acids M. Altarawneh 10.1016/j.apr.2021.101255
- Levels and Seasonal Trends of C1–C4 Perfluoroalkyl Acids and the Discovery of Trifluoromethane Sulfonic Acid in Surface Snow in the Arctic M. Björnsdotter et al. 10.1021/acs.est.1c04776
- Assessing the contribution of atmospheric transport and tourism activities to the occurrence of perfluoroalkyl acids (PFAAs) in an Alpine Nature Reserve C. Wang et al. 10.1016/j.scitotenv.2019.133851
- Lethal and sublethal toxicity of perfluorooctanoic acid (PFOA) in chronic tests with Hyalella azteca (amphipod) and early-life stage tests with Pimephales promelas (fathead minnow) A. Bartlett et al. 10.1016/j.ecoenv.2020.111250
- Poly- and Perfluoroalkyl Substances in Seawater and Plankton from the Northwestern Atlantic Margin X. Zhang et al. 10.1021/acs.est.9b03230
- Sea Spray Aerosol (SSA) as a Source of Perfluoroalkyl Acids (PFAAs) to the Atmosphere: Field Evidence from Long-Term Air Monitoring B. Sha et al. 10.1021/acs.est.1c04277
Discussed (final revised paper)
Discussed (final revised paper)
Discussed (preprint)
Latest update: 26 Jan 2023
Short summary
Perfluoroalkyl acids (PFAAs) are persistent, bioaccumulative compounds found in the environment far from source regions, including the remote Arctic. We collected a 15 m ice core from the Canadian High Arctic to measure a 38-year deposition record of PFAAs, proving information about major pollutant sources and production changes over time. Our results demonstrate that PFAAs have continuous and increasing deposition, despite recent North American regulations and phase-outs.
Perfluoroalkyl acids (PFAAs) are persistent, bioaccumulative compounds found in the environment...
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Final-revised paper
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