Articles | Volume 18, issue 6
https://doi.org/10.5194/acp-18-4005-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue:
https://doi.org/10.5194/acp-18-4005-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Large contribution of fossil fuel derived secondary organic carbon to water soluble organic aerosols in winter haze in China
Yan-Lin Zhang
CORRESPONDING AUTHOR
Yale-NUIST Center on Atmospheric Environment, Nanjing University of
Information Science and Technology, 210044 Nanjing, China
Department of Chemistry and Biochemistry & Oeschger Centre for
Climate Change Research, University of Bern, 3012 Bern, Switzerland
Paul Scherrer Institute (PSI), 5232 Villigen, Switzerland
Key Laboratory of Meteorological Disaster, Ministry of Education (KLME)/Collaborative
Innovation Center on Forecast and Evaluation of Meteorological Disasters (CIC-FEMD),
Nanjing University of Information Science & Technology, Nanjing 210044, China
Imad El-Haddad
Paul Scherrer Institute (PSI), 5232 Villigen, Switzerland
Ru-Jin Huang
CORRESPONDING AUTHOR
Paul Scherrer Institute (PSI), 5232 Villigen, Switzerland
Key Laboratory of Aerosol Chemistry and Physics, Institute of Earth
Environment, Chinese Academy of Sciences, 710061 Xi'an China
Kin-Fai Ho
Key Laboratory of Aerosol Chemistry and Physics, Institute of Earth
Environment, Chinese Academy of Sciences, 710061 Xi'an China
School of Public Health and Primary Care, The Chinese University of
Hong Kong, Hong Kong, China
Jun-Ji Cao
CORRESPONDING AUTHOR
Key Laboratory of Aerosol Chemistry and Physics, Institute of Earth
Environment, Chinese Academy of Sciences, 710061 Xi'an China
Yongming Han
Key Laboratory of Aerosol Chemistry and Physics, Institute of Earth
Environment, Chinese Academy of Sciences, 710061 Xi'an China
Peter Zotter
Paul Scherrer Institute (PSI), 5232 Villigen, Switzerland
Carlo Bozzetti
Paul Scherrer Institute (PSI), 5232 Villigen, Switzerland
Kaspar R. Daellenbach
Paul Scherrer Institute (PSI), 5232 Villigen, Switzerland
Jay G. Slowik
Paul Scherrer Institute (PSI), 5232 Villigen, Switzerland
Gary Salazar
Department of Chemistry and Biochemistry & Oeschger Centre for
Climate Change Research, University of Bern, 3012 Bern, Switzerland
André S. H. Prévôt
CORRESPONDING AUTHOR
Paul Scherrer Institute (PSI), 5232 Villigen, Switzerland
Department of Chemistry and Biochemistry & Oeschger Centre for
Climate Change Research, University of Bern, 3012 Bern, Switzerland
Viewed
Total article views: 3,807 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 12 Dec 2017)
HTML | XML | Total | BibTeX | EndNote | |
---|---|---|---|---|---|
2,406 | 1,314 | 87 | 3,807 | 75 | 120 |
- HTML: 2,406
- PDF: 1,314
- XML: 87
- Total: 3,807
- BibTeX: 75
- EndNote: 120
Total article views: 3,124 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 22 Mar 2018)
HTML | XML | Total | BibTeX | EndNote | |
---|---|---|---|---|---|
2,022 | 1,027 | 75 | 3,124 | 66 | 104 |
- HTML: 2,022
- PDF: 1,027
- XML: 75
- Total: 3,124
- BibTeX: 66
- EndNote: 104
Total article views: 683 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 12 Dec 2017)
HTML | XML | Total | BibTeX | EndNote | |
---|---|---|---|---|---|
384 | 287 | 12 | 683 | 9 | 16 |
- HTML: 384
- PDF: 287
- XML: 12
- Total: 683
- BibTeX: 9
- EndNote: 16
Viewed (geographical distribution)
Total article views: 3,807 (including HTML, PDF, and XML)
Thereof 3,774 with geography defined
and 33 with unknown origin.
Total article views: 3,124 (including HTML, PDF, and XML)
Thereof 3,107 with geography defined
and 17 with unknown origin.
Total article views: 683 (including HTML, PDF, and XML)
Thereof 667 with geography defined
and 16 with unknown origin.
Country | # | Views | % |
---|
Country | # | Views | % |
---|
Country | # | Views | % |
---|
Total: | 0 |
HTML: | 0 |
PDF: | 0 |
XML: | 0 |
- 1
1
Total: | 0 |
HTML: | 0 |
PDF: | 0 |
XML: | 0 |
- 1
1
Total: | 0 |
HTML: | 0 |
PDF: | 0 |
XML: | 0 |
- 1
1
Cited
46 citations as recorded by crossref.
- Integration of field observation and air quality modeling to characterize Beijing aerosol in different seasons J. Liu et al. 10.1016/j.chemosphere.2019.125195
- Seasonal variation of dicarboxylic acids in PM2.5 in Beijing: Implications for the formation and aging processes of secondary organic aerosols Q. Yu et al. 10.1016/j.scitotenv.2020.142964
- Impacts of severe residential wood burning on atmospheric processing, water-soluble organic aerosol and light absorption, in an inland city of Southeastern Europe D. Kaskaoutis et al. 10.1016/j.atmosenv.2022.119139
- Haze Pollution in the Unstable Atmospheric Boundary Layer Over the West Bank of Taiwan Strait Induced by Regional Transport of PM2.5 Y. Jiang et al. 10.1029/2022EA002505
- Research progress on the characteristics, sources, and environmental and potential health effects of water-soluble organic compounds in atmospheric particulate matter L. Wang et al. 10.1007/s11356-023-31723-x
- pH-Responsive Fluorescence EEM to Titrate the Interaction between Fluorophores and Acid/Base Groups in Water-Soluble Organic Compounds of PM2.5 Y. Qin et al. 10.1021/acs.estlett.0c00645
- High time-resolved measurement of stable carbon isotope composition in water-soluble organic aerosols: method optimization and a case study during winter haze in eastern China W. Zhang et al. 10.5194/acp-19-11071-2019
- Water-soluble organic aerosols over South Asia – Seasonal changes and source characteristics C. Ramya et al. 10.1016/j.scitotenv.2023.165644
- Aqueous production of secondary organic aerosol from fossil-fuel emissions in winter Beijing haze J. Wang et al. 10.1073/pnas.2022179118
- Source apportionment of carbonaceous aerosols in diverse atmospheric environments of China by dual-carbon isotope method M. Li et al. 10.1016/j.scitotenv.2021.150654
- Brown carbon absorption and radiative effects under intense residential wood burning conditions in Southeastern Europe: New insights into the abundance and absorptivity of methanol-soluble organic aerosols D. Paraskevopoulou et al. 10.1016/j.scitotenv.2022.160434
- Quantifying the relative contributions of aqueous phase and photochemical processes to water-soluble organic carbon formation in winter in a megacity of South China J. Tao et al. 10.1016/j.chemosphere.2022.134598
- Measurement report: Molecular composition, optical properties, and radiative effects of water-soluble organic carbon in snowpack samples from northern Xinjiang, China Y. Zhou et al. 10.5194/acp-21-8531-2021
- The interaction laws of atmospheric heavy metal ions and water-soluble organic compounds in PM2.5 based on the excitation-emission matrix fluorescence spectroscopy X. Wang et al. 10.1016/j.jhazmat.2020.123497
- Sensitivity and uncertainties assessment in radiative forcing due to aerosol optical properties in diverse locations in China F. Lu et al. 10.1016/j.scitotenv.2022.160447
- Haze formation indicator based on observation of critical carbonaceous species in the atmosphere S. Yang et al. 10.1016/j.envpol.2018.10.006
- Characteristics, primary sources and secondary formation of water-soluble organic aerosols in downtown Beijing Q. Yu et al. 10.5194/acp-21-1775-2021
- Size-resolved water-soluble organic carbon and its significant contribution to aerosol liquid water M. Xu et al. 10.1016/j.scitotenv.2024.172396
- Seasonal light absorption properties of water-soluble brown carbon in atmospheric fine particles in Nanjing, China Y. Chen et al. 10.1016/j.atmosenv.2018.06.002
- Trans‐Regional Transport of Haze Particles From the North China Plain to Yangtze River Delta During Winter J. Zhang et al. 10.1029/2020JD033778
- Optical properties, molecular characterizations, and oxidative potentials of different polarity levels of water-soluble organic matters in winter PM2.5 in six China's megacities T. Zhang et al. 10.1016/j.scitotenv.2022.158600
- Sources and formation of carbonaceous aerosols in Xi'an, China: primary emissions and secondary formation constrained by radiocarbon H. Ni et al. 10.5194/acp-19-15609-2019
- Non‐Fossil Origin Explains the Large Seasonal Variation of Highly Processed Organic Aerosol in the Northeastern Tibetan Plateau (3,200 m a.s.l.) H. Ni et al. 10.1029/2023GL104710
- Determining the Sources and Transport of Brown Carbon Using Radionuclide Tracers and Modeling H. Jiang et al. 10.1029/2021JD034616
- The complexation between transition metals and water-soluble organic compounds (WSOC) and its effect on reactive oxygen species (ROS) formation Y. Yan et al. 10.1016/j.atmosenv.2022.119247
- Large contribution of fossil-derived components to aqueous secondary organic aerosols in China B. Xu et al. 10.1038/s41467-022-32863-3
- Oxidative potential associated with water-soluble components of PM2.5 in Beijing: The important role of anthropogenic organic aerosols Q. Yu et al. 10.1016/j.jhazmat.2022.128839
- Measurement report: Changes in light absorption and molecular composition of water-soluble humic-like substances during a winter haze bloom-decay process in Guangzhou, China C. Zou et al. 10.5194/acp-23-963-2023
- High Contribution of South Asian Biomass Burning to Southeastern Tibetan Plateau Air: New Evidence from Radiocarbon Measurement J. Liu et al. 10.1021/acs.estlett.1c00860
- Molecular Characterization of Water-Soluble Brown Carbon Chromophores in Snowpack from Northern Xinjiang, China Y. Zhou et al. 10.1021/acs.est.1c07972
- Characterization and sources of water-soluble organic species in PM2.5 in a remote mountain environment in Southeastern China J. Tao et al. 10.1016/j.atmosenv.2023.120057
- 14C characteristics of organic carbon in the atmosphere and at glacier region of the Tibetan Plateau C. Li et al. 10.1016/j.scitotenv.2022.155020
- Characterization of the organic functional group composition and sources of summertime aerosols in an eastern city of China K. Xia et al. 10.1016/j.atmosenv.2022.119078
- Abundant Biogenic Oxygenated Organic Aerosol in Atmospheric Coarse Particles: Plausible Sources and Atmospheric Implications X. Huang et al. 10.1021/acs.est.9b06311
- Significant Contribution of Primary Sources to Water-Soluble Organic Carbon During Spring in Beijing, China Y. Jin et al. 10.3390/atmos11040395
- Molecular chemodiversity of water-soluble organic matter in atmospheric particulate matter and their associations with atmospheric conditions C. Ning et al. 10.1016/j.scitotenv.2021.151171
- Estimation and Uncertainty Analysis of Secondary Organic Carbon Using 1 Year of Hourly Organic and Elemental Carbon Data C. Wu et al. 10.1029/2018JD029290
- Dual Carbon Isotope‐Based Source Apportionment and Light Absorption Properties of Water‐Soluble Organic Carbon in PM2.5 Over China Y. Mo et al. 10.1029/2020JD033920
- Sources and processes of water-soluble and water-insoluble organic aerosol in cold season in Beijing, China Z. Zhang et al. 10.5194/acp-22-10409-2022
- Vertical Characterization and Source Apportionment of Water-Soluble Organic Aerosol with High-resolution Aerosol Mass Spectrometry in Beijing, China Y. Qiu et al. 10.1021/acsearthspacechem.8b00155
- Carbon isotope seasonal characteristics of fine carbonaceous aerosol in Jinzhong City, Shanxi Province, China H. Bai et al. 10.1016/j.atmosenv.2020.118164
- Identification of Pollution Characteristics of PM2.5 Using a Geographic Information System and Statistical Tools: A Case Study of the Southeastern and Southern Regions of South Korea J. Ju et al. 10.5572/KOSAE.2023.39.4.478
- Phenomenology of the Composition of PM2.5 at an Urban Site in Northern France Y. Allouche et al. 10.3390/atmos15050603
- Chemical characteristics and sources of water-soluble organic aerosol in southwest suburb of Beijing R. Hu et al. 10.1016/j.jes.2020.04.004
- Source apportionment of carbonaceous aerosols in Beijing with radiocarbon and organic tracers: insight into the differences between urban and rural sites S. Hou et al. 10.5194/acp-21-8273-2021
- Characterizing water-soluble brown carbon in fine particles in four typical cities in northwestern China during wintertime: integrating optical properties with chemical processes M. Zhong et al. 10.5194/acp-23-12609-2023
46 citations as recorded by crossref.
- Integration of field observation and air quality modeling to characterize Beijing aerosol in different seasons J. Liu et al. 10.1016/j.chemosphere.2019.125195
- Seasonal variation of dicarboxylic acids in PM2.5 in Beijing: Implications for the formation and aging processes of secondary organic aerosols Q. Yu et al. 10.1016/j.scitotenv.2020.142964
- Impacts of severe residential wood burning on atmospheric processing, water-soluble organic aerosol and light absorption, in an inland city of Southeastern Europe D. Kaskaoutis et al. 10.1016/j.atmosenv.2022.119139
- Haze Pollution in the Unstable Atmospheric Boundary Layer Over the West Bank of Taiwan Strait Induced by Regional Transport of PM2.5 Y. Jiang et al. 10.1029/2022EA002505
- Research progress on the characteristics, sources, and environmental and potential health effects of water-soluble organic compounds in atmospheric particulate matter L. Wang et al. 10.1007/s11356-023-31723-x
- pH-Responsive Fluorescence EEM to Titrate the Interaction between Fluorophores and Acid/Base Groups in Water-Soluble Organic Compounds of PM2.5 Y. Qin et al. 10.1021/acs.estlett.0c00645
- High time-resolved measurement of stable carbon isotope composition in water-soluble organic aerosols: method optimization and a case study during winter haze in eastern China W. Zhang et al. 10.5194/acp-19-11071-2019
- Water-soluble organic aerosols over South Asia – Seasonal changes and source characteristics C. Ramya et al. 10.1016/j.scitotenv.2023.165644
- Aqueous production of secondary organic aerosol from fossil-fuel emissions in winter Beijing haze J. Wang et al. 10.1073/pnas.2022179118
- Source apportionment of carbonaceous aerosols in diverse atmospheric environments of China by dual-carbon isotope method M. Li et al. 10.1016/j.scitotenv.2021.150654
- Brown carbon absorption and radiative effects under intense residential wood burning conditions in Southeastern Europe: New insights into the abundance and absorptivity of methanol-soluble organic aerosols D. Paraskevopoulou et al. 10.1016/j.scitotenv.2022.160434
- Quantifying the relative contributions of aqueous phase and photochemical processes to water-soluble organic carbon formation in winter in a megacity of South China J. Tao et al. 10.1016/j.chemosphere.2022.134598
- Measurement report: Molecular composition, optical properties, and radiative effects of water-soluble organic carbon in snowpack samples from northern Xinjiang, China Y. Zhou et al. 10.5194/acp-21-8531-2021
- The interaction laws of atmospheric heavy metal ions and water-soluble organic compounds in PM2.5 based on the excitation-emission matrix fluorescence spectroscopy X. Wang et al. 10.1016/j.jhazmat.2020.123497
- Sensitivity and uncertainties assessment in radiative forcing due to aerosol optical properties in diverse locations in China F. Lu et al. 10.1016/j.scitotenv.2022.160447
- Haze formation indicator based on observation of critical carbonaceous species in the atmosphere S. Yang et al. 10.1016/j.envpol.2018.10.006
- Characteristics, primary sources and secondary formation of water-soluble organic aerosols in downtown Beijing Q. Yu et al. 10.5194/acp-21-1775-2021
- Size-resolved water-soluble organic carbon and its significant contribution to aerosol liquid water M. Xu et al. 10.1016/j.scitotenv.2024.172396
- Seasonal light absorption properties of water-soluble brown carbon in atmospheric fine particles in Nanjing, China Y. Chen et al. 10.1016/j.atmosenv.2018.06.002
- Trans‐Regional Transport of Haze Particles From the North China Plain to Yangtze River Delta During Winter J. Zhang et al. 10.1029/2020JD033778
- Optical properties, molecular characterizations, and oxidative potentials of different polarity levels of water-soluble organic matters in winter PM2.5 in six China's megacities T. Zhang et al. 10.1016/j.scitotenv.2022.158600
- Sources and formation of carbonaceous aerosols in Xi'an, China: primary emissions and secondary formation constrained by radiocarbon H. Ni et al. 10.5194/acp-19-15609-2019
- Non‐Fossil Origin Explains the Large Seasonal Variation of Highly Processed Organic Aerosol in the Northeastern Tibetan Plateau (3,200 m a.s.l.) H. Ni et al. 10.1029/2023GL104710
- Determining the Sources and Transport of Brown Carbon Using Radionuclide Tracers and Modeling H. Jiang et al. 10.1029/2021JD034616
- The complexation between transition metals and water-soluble organic compounds (WSOC) and its effect on reactive oxygen species (ROS) formation Y. Yan et al. 10.1016/j.atmosenv.2022.119247
- Large contribution of fossil-derived components to aqueous secondary organic aerosols in China B. Xu et al. 10.1038/s41467-022-32863-3
- Oxidative potential associated with water-soluble components of PM2.5 in Beijing: The important role of anthropogenic organic aerosols Q. Yu et al. 10.1016/j.jhazmat.2022.128839
- Measurement report: Changes in light absorption and molecular composition of water-soluble humic-like substances during a winter haze bloom-decay process in Guangzhou, China C. Zou et al. 10.5194/acp-23-963-2023
- High Contribution of South Asian Biomass Burning to Southeastern Tibetan Plateau Air: New Evidence from Radiocarbon Measurement J. Liu et al. 10.1021/acs.estlett.1c00860
- Molecular Characterization of Water-Soluble Brown Carbon Chromophores in Snowpack from Northern Xinjiang, China Y. Zhou et al. 10.1021/acs.est.1c07972
- Characterization and sources of water-soluble organic species in PM2.5 in a remote mountain environment in Southeastern China J. Tao et al. 10.1016/j.atmosenv.2023.120057
- 14C characteristics of organic carbon in the atmosphere and at glacier region of the Tibetan Plateau C. Li et al. 10.1016/j.scitotenv.2022.155020
- Characterization of the organic functional group composition and sources of summertime aerosols in an eastern city of China K. Xia et al. 10.1016/j.atmosenv.2022.119078
- Abundant Biogenic Oxygenated Organic Aerosol in Atmospheric Coarse Particles: Plausible Sources and Atmospheric Implications X. Huang et al. 10.1021/acs.est.9b06311
- Significant Contribution of Primary Sources to Water-Soluble Organic Carbon During Spring in Beijing, China Y. Jin et al. 10.3390/atmos11040395
- Molecular chemodiversity of water-soluble organic matter in atmospheric particulate matter and their associations with atmospheric conditions C. Ning et al. 10.1016/j.scitotenv.2021.151171
- Estimation and Uncertainty Analysis of Secondary Organic Carbon Using 1 Year of Hourly Organic and Elemental Carbon Data C. Wu et al. 10.1029/2018JD029290
- Dual Carbon Isotope‐Based Source Apportionment and Light Absorption Properties of Water‐Soluble Organic Carbon in PM2.5 Over China Y. Mo et al. 10.1029/2020JD033920
- Sources and processes of water-soluble and water-insoluble organic aerosol in cold season in Beijing, China Z. Zhang et al. 10.5194/acp-22-10409-2022
- Vertical Characterization and Source Apportionment of Water-Soluble Organic Aerosol with High-resolution Aerosol Mass Spectrometry in Beijing, China Y. Qiu et al. 10.1021/acsearthspacechem.8b00155
- Carbon isotope seasonal characteristics of fine carbonaceous aerosol in Jinzhong City, Shanxi Province, China H. Bai et al. 10.1016/j.atmosenv.2020.118164
- Identification of Pollution Characteristics of PM2.5 Using a Geographic Information System and Statistical Tools: A Case Study of the Southeastern and Southern Regions of South Korea J. Ju et al. 10.5572/KOSAE.2023.39.4.478
- Phenomenology of the Composition of PM2.5 at an Urban Site in Northern France Y. Allouche et al. 10.3390/atmos15050603
- Chemical characteristics and sources of water-soluble organic aerosol in southwest suburb of Beijing R. Hu et al. 10.1016/j.jes.2020.04.004
- Source apportionment of carbonaceous aerosols in Beijing with radiocarbon and organic tracers: insight into the differences between urban and rural sites S. Hou et al. 10.5194/acp-21-8273-2021
- Characterizing water-soluble brown carbon in fine particles in four typical cities in northwestern China during wintertime: integrating optical properties with chemical processes M. Zhong et al. 10.5194/acp-23-12609-2023
Latest update: 20 Nov 2024
Short summary
Here we present a quantitative source apportionment of WSOC, isolated from aerosols in China using radiocarbon (14C) and offline high-resolution time of flight aerosol mass spectrometer measurements. We demonstrate a dominant contribution of non-fossil emissions to WSOC aerosols in the Northern Hemisphere. However, the fossil fraction is substantially larger in aerosols from East Asia and the east Asian pollution outflow, especially during winter, due to increasing coal combustion.
Here we present a quantitative source apportionment of WSOC, isolated from aerosols in China...
Altmetrics
Final-revised paper
Preprint