Articles | Volume 18, issue 6
https://doi.org/10.5194/acp-18-4005-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue:
https://doi.org/10.5194/acp-18-4005-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Large contribution of fossil fuel derived secondary organic carbon to water soluble organic aerosols in winter haze in China
Yan-Lin Zhang
CORRESPONDING AUTHOR
Yale-NUIST Center on Atmospheric Environment, Nanjing University of
Information Science and Technology, 210044 Nanjing, China
Department of Chemistry and Biochemistry & Oeschger Centre for
Climate Change Research, University of Bern, 3012 Bern, Switzerland
Paul Scherrer Institute (PSI), 5232 Villigen, Switzerland
Key Laboratory of Meteorological Disaster, Ministry of Education (KLME)/Collaborative
Innovation Center on Forecast and Evaluation of Meteorological Disasters (CIC-FEMD),
Nanjing University of Information Science & Technology, Nanjing 210044, China
Imad El-Haddad
Paul Scherrer Institute (PSI), 5232 Villigen, Switzerland
Ru-Jin Huang
CORRESPONDING AUTHOR
Paul Scherrer Institute (PSI), 5232 Villigen, Switzerland
Key Laboratory of Aerosol Chemistry and Physics, Institute of Earth
Environment, Chinese Academy of Sciences, 710061 Xi'an China
Kin-Fai Ho
Key Laboratory of Aerosol Chemistry and Physics, Institute of Earth
Environment, Chinese Academy of Sciences, 710061 Xi'an China
School of Public Health and Primary Care, The Chinese University of
Hong Kong, Hong Kong, China
Jun-Ji Cao
CORRESPONDING AUTHOR
Key Laboratory of Aerosol Chemistry and Physics, Institute of Earth
Environment, Chinese Academy of Sciences, 710061 Xi'an China
Yongming Han
Key Laboratory of Aerosol Chemistry and Physics, Institute of Earth
Environment, Chinese Academy of Sciences, 710061 Xi'an China
Peter Zotter
Paul Scherrer Institute (PSI), 5232 Villigen, Switzerland
Carlo Bozzetti
Paul Scherrer Institute (PSI), 5232 Villigen, Switzerland
Kaspar R. Daellenbach
Paul Scherrer Institute (PSI), 5232 Villigen, Switzerland
Jay G. Slowik
Paul Scherrer Institute (PSI), 5232 Villigen, Switzerland
Gary Salazar
Department of Chemistry and Biochemistry & Oeschger Centre for
Climate Change Research, University of Bern, 3012 Bern, Switzerland
André S. H. Prévôt
CORRESPONDING AUTHOR
Paul Scherrer Institute (PSI), 5232 Villigen, Switzerland
Department of Chemistry and Biochemistry & Oeschger Centre for
Climate Change Research, University of Bern, 3012 Bern, Switzerland
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Latest update: 14 Dec 2024
Short summary
Here we present a quantitative source apportionment of WSOC, isolated from aerosols in China using radiocarbon (14C) and offline high-resolution time of flight aerosol mass spectrometer measurements. We demonstrate a dominant contribution of non-fossil emissions to WSOC aerosols in the Northern Hemisphere. However, the fossil fraction is substantially larger in aerosols from East Asia and the east Asian pollution outflow, especially during winter, due to increasing coal combustion.
Here we present a quantitative source apportionment of WSOC, isolated from aerosols in China...
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