Articles | Volume 18, issue 5
https://doi.org/10.5194/acp-18-3641-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-3641-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
13 Mar 2018
Research article |
| 13 Mar 2018
| 13 Mar 2018
Modeling reactive ammonia uptake by secondary organic aerosol in CMAQ: application to the continental US
Shupeng Zhu
Computational Environmental Sciences Laboratory, Department of Mechanical and Aerospace Engineering, University of California, Irvine, Irvine, CA, 92697-3975, USA
Jeremy R. Horne
Computational Environmental Sciences Laboratory, Department of Mechanical and Aerospace Engineering, University of California, Irvine, Irvine, CA, 92697-3975, USA
Julia Montoya-Aguilera
Department of Chemistry, University of California, Irvine, Irvine, CA, 92697-3975, USA
Mallory L. Hinks
Department of Chemistry, University of California, Irvine, Irvine, CA, 92697-3975, USA
Sergey A. Nizkorodov
Department of Chemistry, University of California, Irvine, Irvine, CA, 92697-3975, USA
Computational Environmental Sciences Laboratory, Department of Mechanical and Aerospace Engineering, University of California, Irvine, Irvine, CA, 92697-3975, USA
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Cited
20 citations as recorded by crossref.
- Occurrence, distribution and human exposure of phthalic esters in road dust samples across China B. Li et al. 10.1016/j.envres.2020.110222
- Decarbonization will lead to more equitable air quality in California S. Zhu et al. 10.1038/s41467-022-33295-9
- Emissions and air quality implications of decarbonizing the natural gas system with renewable hydrogen M. Mac Kinnon et al. 10.1016/j.fuel.2025.134702
- Effect of Humidity on the Reactive Uptake of Ammonia and Dimethylamine by Nitrogen-Containing Secondary Organic Aerosol N. Smith et al. 10.3390/atmos12111502
- Modeling the Sources and Transport Processes During Extreme Ammonia Episodes in the U.S. Corn Belt C. Hu et al. 10.1029/2019JD031207
- Direct contribution of ammonia to α-pinene secondary organic aerosol formation L. Hao et al. 10.5194/acp-20-14393-2020
- An Episodic Assessment of Vehicle Emission Regulations on Saving Lives in California S. Samuelsen et al. 10.1021/acs.est.0c04060
- Quantifying the air quality and health benefits of greening freight movements L. Minet et al. 10.1016/j.envres.2020.109193
- A review of the CAMx, CMAQ, WRF-Chem and NAQPMS models: Application, evaluation and uncertainty factors Z. Gao & X. Zhou 10.1016/j.envpol.2023.123183
- The first application of a numerically exact, higher-order sensitivity analysis approach for atmospheric modelling: implementation of the hyperdual-step method in the Community Multiscale Air Quality Model (CMAQ) version 5.3.2 J. Liu et al. 10.5194/gmd-17-567-2024
- Effectiveness of ammonia reduction on control of fine particle nitrate H. Guo et al. 10.5194/acp-18-12241-2018
- Modeling Ammonia and Its Uptake by Secondary Organic Aerosol Over China K. Wu et al. 10.1029/2020JD034109
- Modeling Reactive Ammonia Uptake by Secondary Organic Aerosol in a Changing Climate: A WRF-CMAQ Evaluation S. Zhu et al. 10.3389/fenvs.2022.867908
- Benefits of near-zero freight: The air quality and health impacts of low-NOx compressed natural gas trucks M. Mac Kinnon et al. 10.1080/10962247.2021.1957727
- A comparative study on the formation of nitrogen-containing organic compounds in cloud droplets and aerosol particles G. Zhang et al. 10.1016/j.jes.2024.01.026
- Dust emission reduction enhanced gas-to-particle conversion of ammonia in the North China Plain Y. Liu et al. 10.1038/s41467-022-34733-4
- An uncertainty for clean air: Air quality modeling implications of underestimating VOC emissions in urban inventories S. Zhu et al. 10.1016/j.atmosenv.2019.05.019
- Aging of Atmospheric Brown Carbon Aerosol R. Hems et al. 10.1021/acsearthspacechem.0c00346
- Overprediction of aerosol nitrate by chemical transport models: The role of grid resolution M. Zakoura & S. Pandis 10.1016/j.atmosenv.2018.05.066
- High secondary formation of nitrogen-containing organics (NOCs) and its possible link to oxidized organics and ammonium G. Zhang et al. 10.5194/acp-20-1469-2020
20 citations as recorded by crossref.
- Occurrence, distribution and human exposure of phthalic esters in road dust samples across China B. Li et al. 10.1016/j.envres.2020.110222
- Decarbonization will lead to more equitable air quality in California S. Zhu et al. 10.1038/s41467-022-33295-9
- Emissions and air quality implications of decarbonizing the natural gas system with renewable hydrogen M. Mac Kinnon et al. 10.1016/j.fuel.2025.134702
- Effect of Humidity on the Reactive Uptake of Ammonia and Dimethylamine by Nitrogen-Containing Secondary Organic Aerosol N. Smith et al. 10.3390/atmos12111502
- Modeling the Sources and Transport Processes During Extreme Ammonia Episodes in the U.S. Corn Belt C. Hu et al. 10.1029/2019JD031207
- Direct contribution of ammonia to α-pinene secondary organic aerosol formation L. Hao et al. 10.5194/acp-20-14393-2020
- An Episodic Assessment of Vehicle Emission Regulations on Saving Lives in California S. Samuelsen et al. 10.1021/acs.est.0c04060
- Quantifying the air quality and health benefits of greening freight movements L. Minet et al. 10.1016/j.envres.2020.109193
- A review of the CAMx, CMAQ, WRF-Chem and NAQPMS models: Application, evaluation and uncertainty factors Z. Gao & X. Zhou 10.1016/j.envpol.2023.123183
- The first application of a numerically exact, higher-order sensitivity analysis approach for atmospheric modelling: implementation of the hyperdual-step method in the Community Multiscale Air Quality Model (CMAQ) version 5.3.2 J. Liu et al. 10.5194/gmd-17-567-2024
- Effectiveness of ammonia reduction on control of fine particle nitrate H. Guo et al. 10.5194/acp-18-12241-2018
- Modeling Ammonia and Its Uptake by Secondary Organic Aerosol Over China K. Wu et al. 10.1029/2020JD034109
- Modeling Reactive Ammonia Uptake by Secondary Organic Aerosol in a Changing Climate: A WRF-CMAQ Evaluation S. Zhu et al. 10.3389/fenvs.2022.867908
- Benefits of near-zero freight: The air quality and health impacts of low-NOx compressed natural gas trucks M. Mac Kinnon et al. 10.1080/10962247.2021.1957727
- A comparative study on the formation of nitrogen-containing organic compounds in cloud droplets and aerosol particles G. Zhang et al. 10.1016/j.jes.2024.01.026
- Dust emission reduction enhanced gas-to-particle conversion of ammonia in the North China Plain Y. Liu et al. 10.1038/s41467-022-34733-4
- An uncertainty for clean air: Air quality modeling implications of underestimating VOC emissions in urban inventories S. Zhu et al. 10.1016/j.atmosenv.2019.05.019
- Aging of Atmospheric Brown Carbon Aerosol R. Hems et al. 10.1021/acsearthspacechem.0c00346
- Overprediction of aerosol nitrate by chemical transport models: The role of grid resolution M. Zakoura & S. Pandis 10.1016/j.atmosenv.2018.05.066
- High secondary formation of nitrogen-containing organics (NOCs) and its possible link to oxidized organics and ammonium G. Zhang et al. 10.5194/acp-20-1469-2020
Latest update: 31 May 2025
Short summary
For the first time, the interaction between ammonia and secondary organic aerosol (SOA) is integrated in an air quality model and investigated on a national scale. Our original analysis from simulation results indicates that a significant reduction in gas-phase ammonia is possible due to its uptake onto SOA. Significant impact is also observed in the concentration of particulate matter, with a distinct spatial pattern over different seasons.
For the first time, the interaction between ammonia and secondary organic aerosol (SOA) is...
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