Articles | Volume 18, issue 4
https://doi.org/10.5194/acp-18-2749-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Special issue:
https://doi.org/10.5194/acp-18-2749-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Molecular distribution and compound-specific stable carbon isotopic composition of dicarboxylic acids, oxocarboxylic acids and α-dicarbonyls in PM2.5 from Beijing, China
Wanyu Zhao
State Key Laboratory of Atmospheric Boundary Layer Physics and
Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of
Sciences, Beijing 100029, China
Institute of Low Temperature Science, Hokkaido University, Sapporo
060-0819, Japan
College of Earth Sciences, University of Chinese Academy of Sciences,
Beijing 100049, China
Kimitaka Kawamura
Institute of Low Temperature Science, Hokkaido University, Sapporo
060-0819, Japan
Chubu Institute for Advanced Studies, Chubu University, Kasugai
487-8501, Japan
Siyao Yue
State Key Laboratory of Atmospheric Boundary Layer Physics and
Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of
Sciences, Beijing 100029, China
College of Earth Sciences, University of Chinese Academy of Sciences,
Beijing 100049, China
Lianfang Wei
State Key Laboratory of Atmospheric Boundary Layer Physics and
Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of
Sciences, Beijing 100029, China
College of Earth Sciences, University of Chinese Academy of Sciences,
Beijing 100049, China
Hong Ren
State Key Laboratory of Atmospheric Boundary Layer Physics and
Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of
Sciences, Beijing 100029, China
College of Earth Sciences, University of Chinese Academy of Sciences,
Beijing 100049, China
Yu Yan
State Key Laboratory of Atmospheric Boundary Layer Physics and
Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of
Sciences, Beijing 100029, China
Mingjie Kang
State Key Laboratory of Atmospheric Boundary Layer Physics and
Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of
Sciences, Beijing 100029, China
Linjie Li
State Key Laboratory of Atmospheric Boundary Layer Physics and
Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of
Sciences, Beijing 100029, China
College of Earth Sciences, University of Chinese Academy of Sciences,
Beijing 100049, China
Lujie Ren
Institute of Surface-Earth System Science, Tianjin University, Tianjin
300072, China
Senchao Lai
Guangdong Provincial Engineering and Technology Research Center for
Environmental Risk Prevention and Emergency Disposal, School of Environment
and Energy, South China University of Technology, Guangzhou, China
Jie Li
State Key Laboratory of Atmospheric Boundary Layer Physics and
Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of
Sciences, Beijing 100029, China
State Key Laboratory of Atmospheric Boundary Layer Physics and
Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of
Sciences, Beijing 100029, China
College of Earth Sciences, University of Chinese Academy of Sciences,
Beijing 100049, China
Zifa Wang
State Key Laboratory of Atmospheric Boundary Layer Physics and
Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of
Sciences, Beijing 100029, China
College of Earth Sciences, University of Chinese Academy of Sciences,
Beijing 100049, China
Pingqing Fu
CORRESPONDING AUTHOR
Institute of Surface-Earth System Science, Tianjin University, Tianjin
300072, China
State Key Laboratory of Atmospheric Boundary Layer Physics and
Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of
Sciences, Beijing 100029, China
College of Earth Sciences, University of Chinese Academy of Sciences,
Beijing 100049, China
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- Excitation-emission matrix fluorescence, molecular characterization and compound-specific stable carbon isotopic composition of dissolved organic matter in cloud water over Mt. Tai W. Zhao et al. 10.1016/j.atmosenv.2019.06.034
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56 citations as recorded by crossref.
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- Water-soluble low molecular weight organics in cloud water at Mt. Tai Mo Shan, Hong Kong W. Zhao et al. 10.1016/j.scitotenv.2019.134095
- Seasonal distributions and possible sources of low molecular weight organic acids in PM2.5 from a typical mining city after decade green mining developing in Southeastern Hubei, Central China S. Liu et al. 10.1016/j.atmosenv.2024.120455
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- Primary and Secondary Emissions of Carboxylic Acids from Solid Fuel Combustion: Insight into the Source Markers and Secondary Formation Mechanism B. Zhang et al. 10.1021/acs.estlett.4c00339
- Distribution and 13C Signature of Dicarboxylic Acids and Related Compounds in Fine Aerosols Near Underground Coal Fires in North China: Implications for Fossil Origin of Azelaic Acid Z. Xu et al. 10.1029/2023JD038748
- Precursors and Pathways Leading to Enhanced Secondary Organic Aerosol Formation during Severe Haze Episodes Y. Zheng et al. 10.1021/acs.est.1c04255
- Molecular characterization and spatial distribution of dicarboxylic acids and related compounds in fresh snow in China Z. Zhang et al. 10.1016/j.envpol.2021.118114
- Mixing state and evolutionary mechanism of oxalic acid homologs in Liaocheng, East China: Insights from seasonal and hourly observations J. Ma et al. 10.1016/j.partic.2024.09.011
- Enhanced aqueous-phase formation of secondary organic aerosols due to the regional biomass burning over North China Plain J. Wang et al. 10.1016/j.envpol.2019.113401
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- Measurement Report: Investigation on the sources and formation processes of dicarboxylic acids and related species in urban aerosols before and during the COVID-19 lockdown in Jinan, East China J. Meng et al. 10.5194/acp-23-14481-2023
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- Characteristics and source apportionment of PM2.5-bound saccharides and carboxylic acids in Central Shanghai, China G. Ren et al. 10.1016/j.atmosres.2019.104817
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- Influence of vertical transport on chemical evolution of dicarboxylic acids and related secondary organic aerosol from surface emission to the top of Mount Hua, Northwest China M. Shen et al. 10.1016/j.scitotenv.2022.159892
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- Clustering mechanism of oxocarboxylic acids involving hydration reaction: Implications for the atmospheric models L. Liu et al. 10.1063/1.5030665
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- Excitation-emission matrix fluorescence, molecular characterization and compound-specific stable carbon isotopic composition of dissolved organic matter in cloud water over Mt. Tai W. Zhao et al. 10.1016/j.atmosenv.2019.06.034
- Molecular distribution and stable carbon isotopic compositions of dicarboxylic acids and related SOA from biogenic sources in the summertime atmosphere of Mt. Tai in the North China Plain J. Meng et al. 10.5194/acp-18-15069-2018
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- Technical note: Estimating aqueous solubilities and activity coefficients of mono- and <i>α</i>,<i>ω</i>-dicarboxylic acids using COSMO<i>therm</i> N. Hyttinen et al. 10.5194/acp-20-13131-2020
- Indoor acids and bases W. Nazaroff & C. Weschler 10.1111/ina.12670
Latest update: 19 Nov 2024
Short summary
In this paper, we investigate the seasonal trends in concentrations and compound-specific stable carbon isotope ratios of low molecular weight dicarboxylic acids (C2–C12) and related compounds in fine aerosols (PM2.5) in Beijing. Our study demonstrates that, in addition to the production via photo-oxidation, high abundances of diacids and related compounds in Beijing are largely associated with anthropogenic primary emissions such as biomass burning, fossil fuel combustion and plastic burning.
In this paper, we investigate the seasonal trends in concentrations and compound-specific stable...
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