Articles | Volume 18, issue 20
https://doi.org/10.5194/acp-18-15451-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-15451-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
26 Oct 2018
Research article |
| 26 Oct 2018
| 26 Oct 2018
Primary emissions of glyoxal and methylglyoxal from laboratory measurements of open biomass burning
Kyle J. Zarzana
NOAA Earth System Research Laboratory (ESRL) Chemical Sciences Division, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado Boulder, Boulder, CO 80309, USA
now at: Department of Chemistry and Biochemistry, University of Colorado Boulder, Boulder, CO 80309, USA
Vanessa Selimovic
Department of Chemistry and Biochemistry, University of Montana, Missoula, MT 59812, USA
Abigail R. Koss
NOAA Earth System Research Laboratory (ESRL) Chemical Sciences Division, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado Boulder, Boulder, CO 80309, USA
Department of Chemistry and Biochemistry, University of Colorado Boulder, Boulder, CO 80309, USA
now at: Department of Civil and Environmental Engineering, Massachusetts Institute of Technology, Cambridge, MA 02142, USA
Kanako Sekimoto
NOAA Earth System Research Laboratory (ESRL) Chemical Sciences Division, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado Boulder, Boulder, CO 80309, USA
Graduate School of Nanobioscience, Yokohama City University, Yokohama, Kanagawa 236-0027, Japan
Matthew M. Coggon
NOAA Earth System Research Laboratory (ESRL) Chemical Sciences Division, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado Boulder, Boulder, CO 80309, USA
NOAA Earth System Research Laboratory (ESRL) Chemical Sciences Division, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado Boulder, Boulder, CO 80309, USA
now at: Institute of Environment and Climate Research, Jinan University, Guangzhou 510632, China
William P. Dubé
NOAA Earth System Research Laboratory (ESRL) Chemical Sciences Division, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado Boulder, Boulder, CO 80309, USA
Robert J. Yokelson
Department of Chemistry and Biochemistry, University of Montana, Missoula, MT 59812, USA
Carsten Warneke
NOAA Earth System Research Laboratory (ESRL) Chemical Sciences Division, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado Boulder, Boulder, CO 80309, USA
Joost A. de Gouw
NOAA Earth System Research Laboratory (ESRL) Chemical Sciences Division, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado Boulder, Boulder, CO 80309, USA
Department of Chemistry and Biochemistry, University of Colorado Boulder, Boulder, CO 80309, USA
James M. Roberts
NOAA Earth System Research Laboratory (ESRL) Chemical Sciences Division, Boulder, CO 80305, USA
NOAA Earth System Research Laboratory (ESRL) Chemical Sciences Division, Boulder, CO 80305, USA
Department of Chemistry and Biochemistry, University of Colorado Boulder, Boulder, CO 80309, USA
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Cited
34 citations as recorded by crossref.
- Insights into the formation of secondary organic aerosols from agricultural residue burning emissions: A review of chamber-based studies S. Joshi et al. 10.1016/j.scitotenv.2024.175932
- Near-real-time detection of unexpected atmospheric events using principal component analysis on the Infrared Atmospheric Sounding Interferometer (IASI) radiances A. Vu Van et al. 10.5194/amt-16-2107-2023
- Spatiotemporal Variations and Characteristics of CO, H2CO and HCN Emissions from Biomass Burning Monitored by FTIR Spectroscopy Q. Zhu et al. 10.3390/rs16193586
- Tropical peat fire emissions: 2019 field measurements in Sumatra and Borneo and synthesis with previous studies R. Yokelson et al. 10.5194/acp-22-10173-2022
- Large contribution of in-cloud production of secondary organic aerosol from biomass burning emissions T. Wang et al. 10.1038/s41612-024-00682-6
- Emission characteristics of carbonyl compounds from open burning of typical subtropical biomass in South China C. Zhang et al. 10.1016/j.chemosphere.2023.140979
- The nitrogen budget of laboratory-simulated western US wildfires during the FIREX 2016 Fire Lab study J. Roberts et al. 10.5194/acp-20-8807-2020
- Emission Factors for Crop Residue and Prescribed Fires in the Eastern US During FIREX‐AQ K. Travis et al. 10.1029/2023JD039309
- Airborne glyoxal measurements in the marine and continental atmosphere: comparison with TROPOMI observations and EMAC simulations F. Kluge et al. 10.5194/acp-23-1369-2023
- Sulfate-associated liquid water amplifies the formation of oxalic acid at a semi-arid tropical location over peninsular India during winter S. Boreddy et al. 10.1016/j.scitotenv.2023.162365
- Evolution of Reactive Organic Compounds and Their Potential Health Risk in Wildfire Smoke H. Pye et al. 10.1021/acs.est.4c06187
- An IBBCEAS system for atmospheric measurements of glyoxal and methylglyoxal in the presence of high NO<sub>2</sub> concentrations J. Liu et al. 10.5194/amt-12-4439-2019
- Atmospheric fate of two relevant unsaturated ketoethers: kinetics, products and mechanisms for the reaction of hydroxyl radicals with (<i>E</i>)-4-methoxy-3-buten-2-one and (1<i>E</i>)-1-methoxy-2-methyl-1-penten-3-one R. Gibilisco et al. 10.5194/acp-20-8939-2020
- Open biomass burning emissions and their contribution to ambient formaldehyde in Guangdong province, China C. Zhang et al. 10.1016/j.scitotenv.2022.155904
- Aging of mineral dusts and proxies by uptake of methylglyoxal: A Knudsen cell study A. Lostier et al. 10.1016/j.atmosenv.2024.120876
- OH chemistry of non-methane organic gases (NMOGs) emitted from laboratory and ambient biomass burning smoke: evaluating the influence of furans and oxygenated aromatics on ozone and secondary NMOG formation M. Coggon et al. 10.5194/acp-19-14875-2019
- Fire Influence on Regional to Global Environments and Air Quality (FIREX‐AQ) C. Warneke et al. 10.1029/2022JD037758
- Direct emissions of particulate glyoxal and methylglyoxal from biomass burning and coal combustion T. Wang et al. 10.1016/j.scitotenv.2022.160757
- Reversible and irreversible gas–particle partitioning of dicarbonyl compounds observed in the real atmosphere J. Hu et al. 10.5194/acp-22-6971-2022
- Importance of Wintertime Anthropogenic Glyoxal and Methylglyoxal Emissions in Beijing and Implications for Secondary Organic Aerosol Formation in Megacities X. Qiu et al. 10.1021/acs.est.0c02822
- Assessing the Ratios of Formaldehyde and Glyoxal to NO2 as Indicators of O3–NOx–VOC Sensitivity J. Liu et al. 10.1021/acs.est.0c07506
- Satellite Evidence for Glyoxal Depletion in Elevated Fire Plumes C. Lerot et al. 10.1029/2022GL102195
- Broadband Cavity-Enhanced Absorption Spectroscopy (BBCEAS) Coupled with an Interferometer for On-Band and Off-Band Detection of Glyoxal C. Flowerday et al. 10.3390/toxics12010026
- Parameterizations of US wildfire and prescribed fire emission ratios and emission factors based on FIREX-AQ aircraft measurements G. Gkatzelis et al. 10.5194/acp-24-929-2024
- Absorption spectra of pyruvic acid in water: insights from calculations for small hydrates and comparison to experiment D. Shemesh et al. 10.1039/D0CP01810D
- Rapid increase in atmospheric glyoxal and methylglyoxal concentrations in Lhasa, Tibetan Plateau: Potential sources and implications Q. Li et al. 10.1016/j.scitotenv.2022.153782
- Investigating vertical distributions and photochemical indications of formaldehyde, glyoxal, and NO2 from MAX-DOAS observations in four typical cities of China Q. Hong et al. 10.1016/j.scitotenv.2024.176447
- Field observational constraints on the controllers in glyoxal (CHOCHO) reactive uptake to aerosol D. Kim et al. 10.5194/acp-22-805-2022
- Isotopic characterization of nitrogen oxides (NO<sub><i>x</i></sub>), nitrous acid (HONO), and nitrate (<i>p</i>NO<sub>3</sub><sup>−</sup>) from laboratory biomass burning during FIREX J. Chai et al. 10.5194/amt-12-6303-2019
- Impacts of urbanization on land use, air quality, and temperature dynamics in Dehradun district of Uttarakhand, India: a comprehensive analysis S. Dhankar et al. 10.3389/fenvs.2024.1324186
- Enhanced Sulfate Formation through Synergistic Effects of Chlorine Chemistry and Photosensitization in Atmospheric Particles R. Zhang & C. Chan 10.1021/acsestair.3c00030
- Profiling of formaldehyde, glyoxal, methylglyoxal, and CO over the Amazon: normalized excess mixing ratios and related emission factors in biomass burning plumes F. Kluge et al. 10.5194/acp-20-12363-2020
- Role of aerosol liquid water content on the production of dicarboxylic acids in the dust-laden air masses over the Arabian Sea: Implications for heterogeneous chemistry P. Bikkina et al. 10.1016/j.atmosres.2023.106743
- Elevated levels of glyoxal and methylglyoxal at a remote mountain site in southern China: Prompt in-situ formation combined with strong regional transport S. Lv et al. 10.1016/j.scitotenv.2019.04.020
33 citations as recorded by crossref.
- Insights into the formation of secondary organic aerosols from agricultural residue burning emissions: A review of chamber-based studies S. Joshi et al. 10.1016/j.scitotenv.2024.175932
- Near-real-time detection of unexpected atmospheric events using principal component analysis on the Infrared Atmospheric Sounding Interferometer (IASI) radiances A. Vu Van et al. 10.5194/amt-16-2107-2023
- Spatiotemporal Variations and Characteristics of CO, H2CO and HCN Emissions from Biomass Burning Monitored by FTIR Spectroscopy Q. Zhu et al. 10.3390/rs16193586
- Tropical peat fire emissions: 2019 field measurements in Sumatra and Borneo and synthesis with previous studies R. Yokelson et al. 10.5194/acp-22-10173-2022
- Large contribution of in-cloud production of secondary organic aerosol from biomass burning emissions T. Wang et al. 10.1038/s41612-024-00682-6
- Emission characteristics of carbonyl compounds from open burning of typical subtropical biomass in South China C. Zhang et al. 10.1016/j.chemosphere.2023.140979
- The nitrogen budget of laboratory-simulated western US wildfires during the FIREX 2016 Fire Lab study J. Roberts et al. 10.5194/acp-20-8807-2020
- Emission Factors for Crop Residue and Prescribed Fires in the Eastern US During FIREX‐AQ K. Travis et al. 10.1029/2023JD039309
- Airborne glyoxal measurements in the marine and continental atmosphere: comparison with TROPOMI observations and EMAC simulations F. Kluge et al. 10.5194/acp-23-1369-2023
- Sulfate-associated liquid water amplifies the formation of oxalic acid at a semi-arid tropical location over peninsular India during winter S. Boreddy et al. 10.1016/j.scitotenv.2023.162365
- Evolution of Reactive Organic Compounds and Their Potential Health Risk in Wildfire Smoke H. Pye et al. 10.1021/acs.est.4c06187
- An IBBCEAS system for atmospheric measurements of glyoxal and methylglyoxal in the presence of high NO<sub>2</sub> concentrations J. Liu et al. 10.5194/amt-12-4439-2019
- Atmospheric fate of two relevant unsaturated ketoethers: kinetics, products and mechanisms for the reaction of hydroxyl radicals with (<i>E</i>)-4-methoxy-3-buten-2-one and (1<i>E</i>)-1-methoxy-2-methyl-1-penten-3-one R. Gibilisco et al. 10.5194/acp-20-8939-2020
- Open biomass burning emissions and their contribution to ambient formaldehyde in Guangdong province, China C. Zhang et al. 10.1016/j.scitotenv.2022.155904
- Aging of mineral dusts and proxies by uptake of methylglyoxal: A Knudsen cell study A. Lostier et al. 10.1016/j.atmosenv.2024.120876
- OH chemistry of non-methane organic gases (NMOGs) emitted from laboratory and ambient biomass burning smoke: evaluating the influence of furans and oxygenated aromatics on ozone and secondary NMOG formation M. Coggon et al. 10.5194/acp-19-14875-2019
- Fire Influence on Regional to Global Environments and Air Quality (FIREX‐AQ) C. Warneke et al. 10.1029/2022JD037758
- Direct emissions of particulate glyoxal and methylglyoxal from biomass burning and coal combustion T. Wang et al. 10.1016/j.scitotenv.2022.160757
- Reversible and irreversible gas–particle partitioning of dicarbonyl compounds observed in the real atmosphere J. Hu et al. 10.5194/acp-22-6971-2022
- Importance of Wintertime Anthropogenic Glyoxal and Methylglyoxal Emissions in Beijing and Implications for Secondary Organic Aerosol Formation in Megacities X. Qiu et al. 10.1021/acs.est.0c02822
- Assessing the Ratios of Formaldehyde and Glyoxal to NO2 as Indicators of O3–NOx–VOC Sensitivity J. Liu et al. 10.1021/acs.est.0c07506
- Satellite Evidence for Glyoxal Depletion in Elevated Fire Plumes C. Lerot et al. 10.1029/2022GL102195
- Broadband Cavity-Enhanced Absorption Spectroscopy (BBCEAS) Coupled with an Interferometer for On-Band and Off-Band Detection of Glyoxal C. Flowerday et al. 10.3390/toxics12010026
- Parameterizations of US wildfire and prescribed fire emission ratios and emission factors based on FIREX-AQ aircraft measurements G. Gkatzelis et al. 10.5194/acp-24-929-2024
- Absorption spectra of pyruvic acid in water: insights from calculations for small hydrates and comparison to experiment D. Shemesh et al. 10.1039/D0CP01810D
- Rapid increase in atmospheric glyoxal and methylglyoxal concentrations in Lhasa, Tibetan Plateau: Potential sources and implications Q. Li et al. 10.1016/j.scitotenv.2022.153782
- Investigating vertical distributions and photochemical indications of formaldehyde, glyoxal, and NO2 from MAX-DOAS observations in four typical cities of China Q. Hong et al. 10.1016/j.scitotenv.2024.176447
- Field observational constraints on the controllers in glyoxal (CHOCHO) reactive uptake to aerosol D. Kim et al. 10.5194/acp-22-805-2022
- Isotopic characterization of nitrogen oxides (NO<sub><i>x</i></sub>), nitrous acid (HONO), and nitrate (<i>p</i>NO<sub>3</sub><sup>−</sup>) from laboratory biomass burning during FIREX J. Chai et al. 10.5194/amt-12-6303-2019
- Impacts of urbanization on land use, air quality, and temperature dynamics in Dehradun district of Uttarakhand, India: a comprehensive analysis S. Dhankar et al. 10.3389/fenvs.2024.1324186
- Enhanced Sulfate Formation through Synergistic Effects of Chlorine Chemistry and Photosensitization in Atmospheric Particles R. Zhang & C. Chan 10.1021/acsestair.3c00030
- Profiling of formaldehyde, glyoxal, methylglyoxal, and CO over the Amazon: normalized excess mixing ratios and related emission factors in biomass burning plumes F. Kluge et al. 10.5194/acp-20-12363-2020
- Role of aerosol liquid water content on the production of dicarboxylic acids in the dust-laden air masses over the Arabian Sea: Implications for heterogeneous chemistry P. Bikkina et al. 10.1016/j.atmosres.2023.106743
Latest update: 14 Dec 2024
Short summary
Emissions of glyoxal and methylglyoxal from fuels common to the western United States were measured using cavity-enhanced spectroscopy, which provides a more selective measurement of those compounds than was previously available. Primary emissions of glyoxal were lower than previously reported and showed variability between the different fuel groups. However, emissions of glyoxal relative to formaldehyde were constant across almost all the fuel groups at 6 %–7 %.
Emissions of glyoxal and methylglyoxal from fuels common to the western United States were...
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