Articles | Volume 18, issue 20
https://doi.org/10.5194/acp-18-15201-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-15201-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
23 Oct 2018
Research article |
| 23 Oct 2018
| 23 Oct 2018
Temporal variations in the hygroscopicity and mixing state of black carbon aerosols in a polluted megacity area
Kangning Li
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention, Department of Environmental Science and Engineering, Fudan University, Shanghai 200433, China
Xingnan Ye
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention, Department of Environmental Science and Engineering, Fudan University, Shanghai 200433, China
Hongwei Pang
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention, Department of Environmental Science and Engineering, Fudan University, Shanghai 200433, China
Xiaohui Lu
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention, Department of Environmental Science and Engineering, Fudan University, Shanghai 200433, China
Hong Chen
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention, Department of Environmental Science and Engineering, Fudan University, Shanghai 200433, China
Xiaofei Wang
CORRESPONDING AUTHOR
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention, Department of Environmental Science and Engineering, Fudan University, Shanghai 200433, China
Shanghai Institute of Pollution Control and Ecological Security, Shanghai 200092, China
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention, Department of Environmental Science and Engineering, Fudan University, Shanghai 200433, China
Shanghai Institute of Pollution Control and Ecological Security, Shanghai 200092, China
Jianmin Chen
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention, Department of Environmental Science and Engineering, Fudan University, Shanghai 200433, China
Yingjun Chen
Shanghai Institute of Pollution Control and Ecological Security, Shanghai 200092, China
College of Environmental Science and Engineering, Tongji University, Shanghai 200092, China
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- Tropospheric aerosol hygroscopicity in China C. Peng et al. 10.5194/acp-20-13877-2020
- Relationship between cloud condensation nuclei (CCN) concentration and aerosol optical depth in the Arctic region S. Ahn et al. 10.1016/j.atmosenv.2021.118748
- Estimation of real-time brown carbon absorption: An observationally constrained Mie theory-based optimization method T. Kapoor et al. 10.1016/j.jaerosci.2022.106047
- Contrasting mixing state of black carbon-containing particles in summer and winter in Beijing C. Xie et al. 10.1016/j.envpol.2020.114455
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- Enhanced mixing state of black carbon with nitrate in single particles during haze periods in Zhengzhou, China Q. Zhou et al. 10.1016/j.jes.2021.03.031
- Real-time, single-particle chemical composition, volatility and mixing state measurements of urban aerosol particles in southwest China L. Chen et al. 10.1016/j.jes.2022.12.014
- Black Carbon Involved Photochemistry Enhances the Formation of Sulfate in the Ambient Atmosphere: Evidence From In Situ Individual Particle Investigation G. Zhang et al. 10.1029/2021JD035226
- A study on the influence of inorganic ions, organic carbon and microstructure on the hygroscopic property of soot Z. Su et al. 10.5194/acp-24-993-2024
- Liquid-liquid phase separation reduces radiative absorption by aged black carbon aerosols J. Zhang et al. 10.1038/s43247-022-00462-1
- Impact of Cloud Process in the Mixing State and Microphysical Properties of Soot Particles: Implications in Light Absorption Enhancement Y. Fu et al. 10.1029/2022JD037169
- New insights into black carbon light absorption enhancement: A comprehensive analysis of two differential behaviors R. Fan et al. 10.1016/j.envpol.2024.124175
- A review of experimental techniques for aerosol hygroscopicity studies M. Tang et al. 10.5194/acp-19-12631-2019
- Amplification of black carbon light absorption induced by atmospheric aging: temporal variation at seasonal and diel scales in urban Guangzhou J. Sun et al. 10.5194/acp-20-2445-2020
- Vertical profile of particle hygroscopicity and CCN effectiveness during winter in Beijing: insight into the hygroscopicity transition threshold of black carbon D. Hu et al. 10.1039/D0FD00077A
- Single particle diversity and mixing state of carbonaceous aerosols in Guangzhou, China C. Cheng et al. 10.1016/j.scitotenv.2020.142182
- Source Apportionment of Ambient Aerosols during a Winter Pollution Episode in Yinchuan by Using Single-Particle Mass Spectrometry K. Li et al. 10.3390/atmos13081174
- Significant impact of water-soluble organic matter on hygroscopicity of fine particles under low relative humidity condition J. Tao et al. 10.1016/j.scitotenv.2023.167980
- Correlations of PM metrics with human respiratory system deposited PM mass determined from ambient particle size distributions and effective densities Y. Lin et al. 10.1080/02786826.2019.1690630
- Size distributions, mixing state, and morphology of refractory black carbon in an urban atmosphere of northeast Asia during summer S. Lim et al. 10.1016/j.scitotenv.2022.158436
22 citations as recorded by crossref.
- Different characteristics of individual particles from light-duty diesel vehicle at the launching and idling state by AAC-SPAMS B. Su et al. 10.1016/j.jhazmat.2021.126304
- Recent Advances in Quantifying Wet Scavenging Efficiency of Black Carbon Aerosol Y. Yang et al. 10.3390/atmos10040175
- Tropospheric aerosol hygroscopicity in China C. Peng et al. 10.5194/acp-20-13877-2020
- Relationship between cloud condensation nuclei (CCN) concentration and aerosol optical depth in the Arctic region S. Ahn et al. 10.1016/j.atmosenv.2021.118748
- Estimation of real-time brown carbon absorption: An observationally constrained Mie theory-based optimization method T. Kapoor et al. 10.1016/j.jaerosci.2022.106047
- Contrasting mixing state of black carbon-containing particles in summer and winter in Beijing C. Xie et al. 10.1016/j.envpol.2020.114455
- Mixing state and effective density of aerosol particles during the Beijing 2022 Olympic Winter Games A. Du et al. 10.5194/acp-23-13597-2023
- Enhanced mixing state of black carbon with nitrate in single particles during haze periods in Zhengzhou, China Q. Zhou et al. 10.1016/j.jes.2021.03.031
- Real-time, single-particle chemical composition, volatility and mixing state measurements of urban aerosol particles in southwest China L. Chen et al. 10.1016/j.jes.2022.12.014
- Black Carbon Involved Photochemistry Enhances the Formation of Sulfate in the Ambient Atmosphere: Evidence From In Situ Individual Particle Investigation G. Zhang et al. 10.1029/2021JD035226
- A study on the influence of inorganic ions, organic carbon and microstructure on the hygroscopic property of soot Z. Su et al. 10.5194/acp-24-993-2024
- Liquid-liquid phase separation reduces radiative absorption by aged black carbon aerosols J. Zhang et al. 10.1038/s43247-022-00462-1
- Impact of Cloud Process in the Mixing State and Microphysical Properties of Soot Particles: Implications in Light Absorption Enhancement Y. Fu et al. 10.1029/2022JD037169
- New insights into black carbon light absorption enhancement: A comprehensive analysis of two differential behaviors R. Fan et al. 10.1016/j.envpol.2024.124175
- A review of experimental techniques for aerosol hygroscopicity studies M. Tang et al. 10.5194/acp-19-12631-2019
- Amplification of black carbon light absorption induced by atmospheric aging: temporal variation at seasonal and diel scales in urban Guangzhou J. Sun et al. 10.5194/acp-20-2445-2020
- Vertical profile of particle hygroscopicity and CCN effectiveness during winter in Beijing: insight into the hygroscopicity transition threshold of black carbon D. Hu et al. 10.1039/D0FD00077A
- Single particle diversity and mixing state of carbonaceous aerosols in Guangzhou, China C. Cheng et al. 10.1016/j.scitotenv.2020.142182
- Source Apportionment of Ambient Aerosols during a Winter Pollution Episode in Yinchuan by Using Single-Particle Mass Spectrometry K. Li et al. 10.3390/atmos13081174
- Significant impact of water-soluble organic matter on hygroscopicity of fine particles under low relative humidity condition J. Tao et al. 10.1016/j.scitotenv.2023.167980
- Correlations of PM metrics with human respiratory system deposited PM mass determined from ambient particle size distributions and effective densities Y. Lin et al. 10.1080/02786826.2019.1690630
- Size distributions, mixing state, and morphology of refractory black carbon in an urban atmosphere of northeast Asia during summer S. Lim et al. 10.1016/j.scitotenv.2022.158436
Latest update: 19 Nov 2024
Short summary
Temporal variation in the hygroscopicity and its correlation with the mixing state of ambient BC particles were studied using a HTDMA–SP2 system. Secondary organic carbon formation and condensation of nitrates were mainly responsible for the changes of hygroscopicity of BC particles during daytime and nighttime, respectively. Different atmospheric aging processes led to the change of BC particles' mixing states, which play a fundamental role in determining their hygroscopicity.
Temporal variation in the hygroscopicity and its correlation with the mixing state of ambient BC...
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