Articles | Volume 18, issue 20
https://doi.org/10.5194/acp-18-14965-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-14965-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
18 Oct 2018
Research article |
| 18 Oct 2018
| 18 Oct 2018
The quasi-liquid layer of ice revisited: the role of temperature gradients and tip chemistry in AFM studies
Julián Gelman Constantin
CORRESPONDING AUTHOR
Departamento de Física de la Materia Condensada, Centro Atómico Constituyentes,
Comisión Nacional de Energía Atómica, San Martín, B1650KNA, Buenos Aires, Argentina
Instituto de Química Física de los Materiales, Medio Ambiente y
Energía (UBA-CONICET), Facultad de Ciencias Exactas y Naturales, Universidad
de Buenos Aires, Pabellón II, Ciudad Universitaria, C1428EGA, Buenos Aires, Argentina
current address: División de Química Atmosférica, Centro Atómico
Constituyentes, Comisión Nacional de Energía Atómica, San Martín, B1650KNA, Buenos Aires, Argentina
Melisa M. Gianetti
Instituto de Química Física de los Materiales, Medio Ambiente y
Energía (UBA-CONICET), Facultad de Ciencias Exactas y Naturales, Universidad
de Buenos Aires, Pabellón II, Ciudad Universitaria, C1428EGA, Buenos Aires, Argentina
María P. Longinotti
CORRESPONDING AUTHOR
Instituto de Química Física de los Materiales, Medio Ambiente y
Energía (UBA-CONICET), Facultad de Ciencias Exactas y Naturales, Universidad
de Buenos Aires, Pabellón II, Ciudad Universitaria, C1428EGA, Buenos Aires, Argentina
Horacio R. Corti
Departamento de Física de la Materia Condensada, Centro Atómico Constituyentes,
Comisión Nacional de Energía Atómica, San Martín, B1650KNA, Buenos Aires, Argentina
Instituto de Química Física de los Materiales, Medio Ambiente y
Energía (UBA-CONICET), Facultad de Ciencias Exactas y Naturales, Universidad
de Buenos Aires, Pabellón II, Ciudad Universitaria, C1428EGA, Buenos Aires, Argentina
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- Topology-Based Phase Identification of Bulk, Interface, and Confined Water Using an Edge-Conditioned Convolutional Graph Neural Network A. Moradzadeh et al. 10.1021/acs.jpcc.2c07423
- Probing the instability of surface structure on solid Hydrates: A microscopic perspective through experiment and simulation W. Li et al. 10.1016/j.apsusc.2023.158971
- Perspective on sum frequency generation spectroscopy of ice surfaces and interfaces S. Yamaguchi et al. 10.1016/j.chemphys.2019.03.005
- Appearance and Disappearance of Quasi-Liquid Layers on Ice Crystals in the Presence of Nitric Acid Gas K. Nagashima et al. 10.3390/cryst10020072
- Environmental chamber with controlled temperature and relative humidity for ice crystallization kinetic measurements by atomic force microscopy M. Gianetti et al. 10.1063/1.5132537
- Atomistic Simulation of Nanoindentation of Ice Ih P. Santos-Flórez et al. 10.1021/acs.jpcc.0c00255
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- HCl Droplets Induced Bunched Steps on Ice Crystal Surfaces under Atmospheric-Concentration HCl Gas K. Nagashima et al. 10.1021/acs.cgd.1c00172
- Intermolecular forces at ice and water interfaces: Premelting, surface freezing, and regelation J. Luengo-Márquez et al. 10.1063/5.0097378
- Atomic force microscopy imaging of ice crystal surfaces formed in aqueous solutions containing ice-binding proteins M. Chasnitsky et al. 10.1016/j.jcrysgro.2022.126961
- A novel hybrid anti-icing surface combining an aqueous self-lubricating coating and phase-change materials M. Shamshiri et al. 10.1016/j.porgcoat.2023.107414
Latest update: 14 Dec 2024
Short summary
Numerous studies have shown that ice surface is actually coated by a thin layer of water even for temperatures below melting temperature. This quasi-liquid layer is relevant in the atmospheric chemistry of clouds, polar regions, glaciers, and other cold regions. We present new results of atomic force microscopy on pure ice, which suggests a thickness for this layer below 1 nm between -7 ºC and -2 ºC. We propose that in many cases previous authors have overestimated this thickness.
Numerous studies have shown that ice surface is actually coated by a thin layer of water even...
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