Articles | Volume 18, issue 19
https://doi.org/10.5194/acp-18-14175-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue:
https://doi.org/10.5194/acp-18-14175-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Atmospheric processing of iron in mineral and combustion aerosols: development of an intermediate-complexity mechanism suitable for Earth system models
Rachel A. Scanza
CORRESPONDING AUTHOR
Department of Earth and Atmospheric Sciences, Cornell University,
Ithaca, New York, USA
Atmospheric Sciences and Global Change Division, Pacific Northwest
National Laboratory, Richland, Washington, USA
Douglas S. Hamilton
Department of Earth and Atmospheric Sciences, Cornell University,
Ithaca, New York, USA
Carlos Perez Garcia-Pando
Earth Sciences Department, Barcelona Supercomputing Center, Barcelona,
Spain
Clifton Buck
Department of Marine Sciences, University of Georgia, Athens, Georgia,
USA
Alex Baker
School of Environmental Sciences, University of East Anglia, Norwich,
UK
Natalie M. Mahowald
Department of Earth and Atmospheric Sciences, Cornell University,
Ithaca, New York, USA
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40 citations as recorded by crossref.
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- Physicochemical Characterization and Oxidative Potential of Iron-Containing Particles Emitted from Xuanwei Coal Combustion S. Lu et al. 10.3390/toxics11110921
- Climate-driven oscillation of phosphorus and iron limitation in the North Pacific Subtropical Gyre R. Letelier et al. 10.1073/pnas.1900789116
- Ice nucleation imaged with X-ray spectro-microscopy P. Alpert et al. 10.1039/D1EA00077B
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- Fully Dynamic High–Resolution Model for Dispersion of Icelandic Airborne Mineral Dust B. Cvetkovic et al. 10.3390/atmos13091345
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- Responses of ocean biogeochemistry to atmospheric supply of lithogenic and pyrogenic iron-containing aerosols A. Ito et al. 10.1017/S0016756819001080
- Photo-oxidation of particle phase iron species dominates the generation of reactive oxygen species in secondary aerosol S. Jiang et al. 10.1016/j.scitotenv.2020.137994
- Aerosol Iron from Metal Production as a Secondary Source of Bioaccessible Iron A. Ito & T. Miyakawa 10.1021/acs.est.2c06472
- An aerosol odyssey: Navigating nutrient flux changes to marine ecosystems D. Hamilton et al. 10.1525/elementa.2023.00037
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- High Production of Soluble Iron Promoted by Aerosol Acidification in Fog J. Shi et al. 10.1029/2019GL086124
- The underappreciated role of anthropogenic sources in atmospheric soluble iron flux to the Southern Ocean M. Liu et al. 10.1038/s41612-022-00250-w
- Global-scale constraints on light-absorbing anthropogenic iron oxide aerosols K. Lamb et al. 10.1038/s41612-021-00171-0
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- Pyrogenic iron: The missing link to high iron solubility in aerosols A. Ito et al. 10.1126/sciadv.aau7671
- Recent (1980 to 2015) Trends and Variability in Daily‐to‐Interannual Soluble Iron Deposition from Dust, Fire, and Anthropogenic Sources D. Hamilton et al. 10.1029/2020GL089688
- Impact of Changes to the Atmospheric Soluble Iron Deposition Flux on Ocean Biogeochemical Cycles in the Anthropocene D. Hamilton et al. 10.1029/2019GB006448
- Laboratory study of iron isotope fractionation during dissolution of mineral dust and industrial ash in simulated cloud water E. Maters et al. 10.1016/j.chemosphere.2022.134472
- GNOM v1.0: an optimized steady-state model of the modern marine neodymium cycle B. Pasquier et al. 10.5194/gmd-15-4625-2022
40 citations as recorded by crossref.
- African biomass burning is a substantial source of phosphorus deposition to the Amazon, Tropical Atlantic Ocean, and Southern Ocean A. Barkley et al. 10.1073/pnas.1906091116
- Aerosol Iron Solubility Specification in the Global Marine Atmosphere with Machine Learning J. Shi et al. 10.1021/acs.est.2c05266
- Anthropogenic Asian aerosols provide Fe to the North Pacific Ocean P. Pinedo-González et al. 10.1073/pnas.2010315117
- Oxidation of low-molecular-weight organic compounds in cloud droplets: global impact on tropospheric oxidants S. Rosanka et al. 10.5194/acp-21-9909-2021
- A Mineralogy‐Based Anthropogenic Combustion‐Iron Emission Inventory S. Rathod et al. 10.1029/2019JD032114
- Abundance and Fractional Solubility of Aerosol Iron During Winter at a Coastal City in Northern China: Similarities and Contrasts Between Fine and Coarse Particles H. Zhang et al. 10.1029/2021JD036070
- Modeling dust mineralogical composition: sensitivity to soil mineralogy atlases and their expected climate impacts M. Gonçalves Ageitos et al. 10.5194/acp-23-8623-2023
- Atmospheric Trace Metal Deposition near the Great Barrier Reef, Australia M. Strzelec et al. 10.3390/atmos11040390
- Multiphase processes in the EC-Earth model and their relevance to the atmospheric oxalate, sulfate, and iron cycles S. Myriokefalitakis et al. 10.5194/gmd-15-3079-2022
- Physicochemical Characterization and Oxidative Potential of Iron-Containing Particles Emitted from Xuanwei Coal Combustion S. Lu et al. 10.3390/toxics11110921
- Climate-driven oscillation of phosphorus and iron limitation in the North Pacific Subtropical Gyre R. Letelier et al. 10.1073/pnas.1900789116
- Ice nucleation imaged with X-ray spectro-microscopy P. Alpert et al. 10.1039/D1EA00077B
- Importance of different parameterization changes for the updated dust cycle modeling in the Community Atmosphere Model (version 6.1) L. Li et al. 10.5194/gmd-15-8181-2022
- Pre‐Industrial, Present and Future Atmospheric Soluble Iron Deposition and the Role of Aerosol Acidity and Oxalate Under CMIP6 Emissions E. Bergas‐Massó et al. 10.1029/2022EF003353
- Evaluating the potential of iron-based interventions in methane reduction and climate mitigation D. Meidan et al. 10.1088/1748-9326/ad3d72
- Fully Dynamic High–Resolution Model for Dispersion of Icelandic Airborne Mineral Dust B. Cvetkovic et al. 10.3390/atmos13091345
- Glacially sourced dust as a potentially significant source of ice nucleating particles Y. Tobo et al. 10.1038/s41561-019-0314-x
- Responses of ocean biogeochemistry to atmospheric supply of lithogenic and pyrogenic iron-containing aerosols A. Ito et al. 10.1017/S0016756819001080
- Photo-oxidation of particle phase iron species dominates the generation of reactive oxygen species in secondary aerosol S. Jiang et al. 10.1016/j.scitotenv.2020.137994
- Aerosol Iron from Metal Production as a Secondary Source of Bioaccessible Iron A. Ito & T. Miyakawa 10.1021/acs.est.2c06472
- An aerosol odyssey: Navigating nutrient flux changes to marine ecosystems D. Hamilton et al. 10.1525/elementa.2023.00037
- Quantifying anthropogenic emission of iron in marine aerosol in the Northwest Pacific with shipborne online measurements T. Zhang et al. 10.1016/j.scitotenv.2023.169158
- High Production of Soluble Iron Promoted by Aerosol Acidification in Fog J. Shi et al. 10.1029/2019GL086124
- The underappreciated role of anthropogenic sources in atmospheric soluble iron flux to the Southern Ocean M. Liu et al. 10.1038/s41612-022-00250-w
- Global-scale constraints on light-absorbing anthropogenic iron oxide aerosols K. Lamb et al. 10.1038/s41612-021-00171-0
- Tracing and constraining anthropogenic aerosol iron fluxes to the North Atlantic Ocean using iron isotopes T. Conway et al. 10.1038/s41467-019-10457-w
- Improved representation of the global dust cycle using observational constraints on dust properties and abundance J. Kok et al. 10.5194/acp-21-8127-2021
- Up in Smoke: Most Aerosolized Fe From Biomass Burning Does Not Derive From Foliage L. Tegler et al. 10.1029/2023GB007796
- Sources of aeolian magnetite at a remote site in Japan: Dominantly Asian desert dust or anthropogenic emissions? N. Tsuchiya et al. 10.1016/j.atmosenv.2023.120093
- Reviews and syntheses: the GESAMP atmospheric iron deposition model intercomparison study S. Myriokefalitakis et al. 10.5194/bg-15-6659-2018
- Morphological features and water solubility of iron in aged fine aerosol particles over the Indian Ocean S. Ueda et al. 10.5194/acp-23-10117-2023
- Reversible scavenging traps hydrothermal iron in the deep ocean S. Roshan et al. 10.1016/j.epsl.2020.116297
- Atmospheric Chemistry of Oxalate: Insight Into the Role of Relative Humidity and Aerosol Acidity From High‐Resolution Observation C. Yang et al. 10.1029/2021JD035364
- Sulfur Isotope Anomalies (Δ33S) in Urban Air Pollution Linked to Mineral-Dust-Associated Sulfate S. Dasari et al. 10.1021/acs.estlett.2c00312
- Improved methodologies for Earth system modelling of atmospheric soluble iron and observation comparisons using the Mechanism of Intermediate complexity for Modelling Iron (MIMI v1.0) D. Hamilton et al. 10.5194/gmd-12-3835-2019
- Pyrogenic iron: The missing link to high iron solubility in aerosols A. Ito et al. 10.1126/sciadv.aau7671
- Recent (1980 to 2015) Trends and Variability in Daily‐to‐Interannual Soluble Iron Deposition from Dust, Fire, and Anthropogenic Sources D. Hamilton et al. 10.1029/2020GL089688
- Impact of Changes to the Atmospheric Soluble Iron Deposition Flux on Ocean Biogeochemical Cycles in the Anthropocene D. Hamilton et al. 10.1029/2019GB006448
- Laboratory study of iron isotope fractionation during dissolution of mineral dust and industrial ash in simulated cloud water E. Maters et al. 10.1016/j.chemosphere.2022.134472
- GNOM v1.0: an optimized steady-state model of the modern marine neodymium cycle B. Pasquier et al. 10.5194/gmd-15-4625-2022
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Short summary
Soluble iron input to remote oceans from dust and combustion aerosols may significantly impact the ability of the ocean to remove carbon dioxide from the atmosphere. In this paper, the processing of insoluble iron during atmospheric transport is simulated using parameterizations that can be implemented in most Earth system models. Our mechanism reasonably matches observations and is computationally efficient, enabling the study of trends and climate impacts due to the Fe–C cycle.
Soluble iron input to remote oceans from dust and combustion aerosols may significantly impact...
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