Multiphase composition changes and reactive oxygen species formation during limonene oxidation in the new Cambridge Atmospheric Simulation Chamber (CASC)

Gallimore, Peter J.; Mahon, Brendan M.; Wragg, Francis P. H.; Fuller, Stephen J.; Giorio, Chiara; Kourtchev, Ivan; Kalberer, Markus

doi:10.5194/acp-17-9853-2017

Articles | Volume 17, issue 16

https://doi.org/10.5194/acp-17-9853-2017

© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.

https://doi.org/10.5194/acp-17-9853-2017

© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.

Articles | Volume 17, issue 16

Research article

|

22 Aug 2017

Research article |

| 22 Aug 2017

Multiphase composition changes and reactive oxygen species formation during limonene oxidation in the new Cambridge Atmospheric Simulation Chamber (CASC)

Peter J. Gallimore, Brendan M. Mahon, Francis P. H. Wragg, Stephen J. Fuller, Chiara Giorio, Ivan Kourtchev, and Markus Kalberer

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Mar 2017	141	51	17	209
Apr 2017	64	51	12	127
May 2017	41	9	11	61
Jun 2017	35	2	11	48
Jul 2017	7	11	0	18
Aug 2017	188	84	5	277
Sep 2017	79	68	4	151
Oct 2017	24	30	1	55
Nov 2017	42	38	2	82
Dec 2017	22	21	0	43
Jan 2018	18	18	0	36
Feb 2018	10	10	0	20
Mar 2018	14	15	0	29
Apr 2018	14	13	0	27
May 2018	19	18	1	38
Jun 2018	14	12	0	26
Jul 2018	7	10	0	17
Aug 2018	17	11	0	28
Sep 2018	9	12	0	21
Oct 2018	13	13	1	27
Nov 2018	16	17	2	35
Dec 2018	4	11	1	16
Jan 2019	8	6	0	14
Feb 2019	5	4	0	9
Mar 2019	11	3	0	14
Apr 2019	6	5	0	11
May 2019	9	9	1	19
Jun 2019	6	9	0	15
Jul 2019	5	12	0	17
Aug 2019	3	1	0	4
Sep 2019	4	8	0	12
Oct 2019	10	6	2	18
Nov 2019	5	6	0	11
Dec 2019	4	4	1	9
Jan 2020	4	6	0	10
Feb 2020	12	6	0	18
Mar 2020	3	3	0	6
Apr 2020	8	9	0	17
May 2020	8	7	0	15
Jun 2020	11	9	0	20
Jul 2020	9	16	3	28
Aug 2020	14	5	2	21
Sep 2020	14	11	0	25
Oct 2020	5	11	0	16
Nov 2020	11	10	0	21
Dec 2020	12	6	0	18
Jan 2021	17	7	0	24
Feb 2021	9	10	2	21
Mar 2021	14	15	0	29
Apr 2021	10	14	2	26
May 2021	9	12	1	22
Jun 2021	7	12	0	19
Jul 2021	10	5	0	15
Aug 2021	8	15	0	23
Sep 2021	13	16	0	29
Oct 2021	9	39	0	48
Nov 2021	12	35	3	50
Dec 2021	13	17	1	31
Jan 2022	11	14	2	27
Feb 2022	14	6	1	21
Mar 2022	43	14	1	58
Apr 2022	11	16	1	28
May 2022	12	5	0	17
Jun 2022	16	13	2	31
Jul 2022	1	4	1	6
Aug 2022	12	10	0	22
Sep 2022	10	8	0	18
Oct 2022	14	4	4	22
Nov 2022	12	12	1	25
Dec 2022	16	12	1	29
Jan 2023	15	15	1	31
Feb 2023	18	9	0	27
Mar 2023	16	9	1	26
Apr 2023	5	8	0	13
May 2023	32	18	0	50
Jun 2023	40	12	4	56
Jul 2023	39	17	1	57
Aug 2023	32	14	2	48
Sep 2023	37	13	0	50
Oct 2023	46	15	3	64
Nov 2023	29	4	0	33
Dec 2023	40	9	2	51
Jan 2024	48	14	1	63
Feb 2024	32	12	0	44
Mar 2024	48	21	4	73
Apr 2024	46	10	3	59
May 2024	21	16	3	40
Jun 2024	12	19	2	33
Jul 2024	19	11	2	32
Aug 2024	23	8	1	32
Sep 2024	11	4	0	15
Oct 2024	13	12	0	25
Nov 2024	10	3	5	18
Dec 2024	16	6	1	23
Jan 2025	14	13	0	27
Feb 2025	35	14	1	50
Mar 2025	14	23	3	40
Apr 2025	29	16	0	45
May 2025	17	9	0	26
Jun 2025	55	6	3	64
Jul 2025	34	21	2	57
Aug 2025	27	20	4	51
Sep 2025	28	22	3	53
Oct 2025	35	30	1	66
Nov 2025	27	17	2	46

Cumulative views and downloads (calculated since 07 Mar 2017)

Month	HTML	PDF	XML	Total
Mar 2017	141	51	17	209
Apr 2017	64	51	12	127
May 2017	41	9	11	61
Jun 2017	35	2	11	48
Jul 2017	7	11	0	18
Aug 2017	188	84	5	277
Sep 2017	79	68	4	151
Oct 2017	24	30	1	55
Nov 2017	42	38	2	82
Dec 2017	22	21	0	43
Jan 2018	18	18	0	36
Feb 2018	10	10	0	20
Mar 2018	14	15	0	29
Apr 2018	14	13	0	27
May 2018	19	18	1	38
Jun 2018	14	12	0	26
Jul 2018	7	10	0	17
Aug 2018	17	11	0	28
Sep 2018	9	12	0	21
Oct 2018	13	13	1	27
Nov 2018	16	17	2	35
Dec 2018	4	11	1	16
Jan 2019	8	6	0	14
Feb 2019	5	4	0	9
Mar 2019	11	3	0	14
Apr 2019	6	5	0	11
May 2019	9	9	1	19
Jun 2019	6	9	0	15
Jul 2019	5	12	0	17
Aug 2019	3	1	0	4
Sep 2019	4	8	0	12
Oct 2019	10	6	2	18
Nov 2019	5	6	0	11
Dec 2019	4	4	1	9
Jan 2020	4	6	0	10
Feb 2020	12	6	0	18
Mar 2020	3	3	0	6
Apr 2020	8	9	0	17
May 2020	8	7	0	15
Jun 2020	11	9	0	20
Jul 2020	9	16	3	28
Aug 2020	14	5	2	21
Sep 2020	14	11	0	25
Oct 2020	5	11	0	16
Nov 2020	11	10	0	21
Dec 2020	12	6	0	18
Jan 2021	17	7	0	24
Feb 2021	9	10	2	21
Mar 2021	14	15	0	29
Apr 2021	10	14	2	26
May 2021	9	12	1	22
Jun 2021	7	12	0	19
Jul 2021	10	5	0	15
Aug 2021	8	15	0	23
Sep 2021	13	16	0	29
Oct 2021	9	39	0	48
Nov 2021	12	35	3	50
Dec 2021	13	17	1	31
Jan 2022	11	14	2	27
Feb 2022	14	6	1	21
Mar 2022	43	14	1	58
Apr 2022	11	16	1	28
May 2022	12	5	0	17
Jun 2022	16	13	2	31
Jul 2022	1	4	1	6
Aug 2022	12	10	0	22
Sep 2022	10	8	0	18
Oct 2022	14	4	4	22
Nov 2022	12	12	1	25
Dec 2022	16	12	1	29
Jan 2023	15	15	1	31
Feb 2023	18	9	0	27
Mar 2023	16	9	1	26
Apr 2023	5	8	0	13
May 2023	32	18	0	50
Jun 2023	40	12	4	56
Jul 2023	39	17	1	57
Aug 2023	32	14	2	48
Sep 2023	37	13	0	50
Oct 2023	46	15	3	64
Nov 2023	29	4	0	33
Dec 2023	40	9	2	51
Jan 2024	48	14	1	63
Feb 2024	32	12	0	44
Mar 2024	48	21	4	73
Apr 2024	46	10	3	59
May 2024	21	16	3	40
Jun 2024	12	19	2	33
Jul 2024	19	11	2	32
Aug 2024	23	8	1	32
Sep 2024	11	4	0	15
Oct 2024	13	12	0	25
Nov 2024	10	3	5	18
Dec 2024	16	6	1	23
Jan 2025	14	13	0	27
Feb 2025	35	14	1	50
Mar 2025	14	23	3	40
Apr 2025	29	16	0	45
May 2025	17	9	0	26
Jun 2025	55	6	3	64
Jul 2025	34	21	2	57
Aug 2025	27	20	4	51
Sep 2025	28	22	3	53
Oct 2025	35	30	1	66
Nov 2025	27	17	2	46

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Short summary

Limonene is emitted in substantial quantities by plants, and also has indoor sources from air fresheners and cleaning products. We studied particle formation from the oxidation of limonene and found substantial quantities of oxidising components which are thought to be associated with the negative health effects of particulates. State-of-the-art measurements of the products of limonene–ozone chemistry were also presented.


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