Articles | Volume 17, issue 12
https://doi.org/10.5194/acp-17-7345-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-17-7345-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
20 Jun 2017
Research article |
| 20 Jun 2017
Global-scale combustion sources of organic aerosols: sensitivity to formation and removal mechanisms
Alexandra P. Tsimpidi
CORRESPONDING AUTHOR
Department of Atmospheric Chemistry, Max Planck Institute for
Chemistry, Mainz, Germany
Vlassis A. Karydis
Department of Atmospheric Chemistry, Max Planck Institute for
Chemistry, Mainz, Germany
Spyros N. Pandis
Department of Chemical Engineering, University of Patras, Patras,
Greece
Department of Chemical Engineering, Carnegie Mellon University,
Pittsburgh, PA, USA
Jos Lelieveld
Department of Atmospheric Chemistry, Max Planck Institute for
Chemistry, Mainz, Germany
Energy, Environment and Water Research Center, Cyprus Institute,
Nicosia, Cyprus
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Latest update: 29 Jun 2024
Short summary
We analyzed the sensitivity of model-predicted global-scale OA to parameters and assumptions that control primary emissions, photochemical aging, and the scavenging efficiency of LVOCs, SVOCs, and IVOCs. The simulated OA concentrations were evaluated against a global dataset of AMS measurements. According to our analysis, a combination of increased IVOCs and decreased hygroscopicity of the freshly emitted IVOCs can help reduce discrepancies between simulated SOA and observed OOA concentrations.
We analyzed the sensitivity of model-predicted global-scale OA to parameters and assumptions...
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