Articles | Volume 17, issue 11
https://doi.org/10.5194/acp-17-6907-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-17-6907-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
13 Jun 2017
Research article |
| 13 Jun 2017
Diurnal fluxes of HONO above a crop rotation
Sebastian Laufs
Physikalische und Theoretische Chemie, Fakultät 4, Bergische
Universität Wuppertal, Gaußstraße 20, 42119 Wuppertal, Germany
Mathieu Cazaunau
ICARE-CNRS, 1 C Av. de la Recherche Scientifique, 45071 Orléans
CEDEX 2, France
LISA, UMR7583, CNRS, Universités Paris Est Créteil et Paris
Diderot, 94010 Créteil, France
Patrick Stella
UMR ECOSYS, INRA, AgroParisTech, Université Paris-Saclay, 78850,
Thiverval-Grignon, France
UMR SADAPT, AgroParisTech, INRA, Université Paris-Saclay, 75005,
Paris, France
Ralf Kurtenbach
Physikalische und Theoretische Chemie, Fakultät 4, Bergische
Universität Wuppertal, Gaußstraße 20, 42119 Wuppertal, Germany
Pierre Cellier
UMR ECOSYS, INRA, AgroParisTech, Université Paris-Saclay, 78850,
Thiverval-Grignon, France
Abdelwahid Mellouki
ICARE-CNRS, 1 C Av. de la Recherche Scientifique, 45071 Orléans
CEDEX 2, France
Benjamin Loubet
UMR ECOSYS, INRA, AgroParisTech, Université Paris-Saclay, 78850,
Thiverval-Grignon, France
Jörg Kleffmann
CORRESPONDING AUTHOR
Physikalische und Theoretische Chemie, Fakultät 4, Bergische
Universität Wuppertal, Gaußstraße 20, 42119 Wuppertal, Germany
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Cited
41 citations as recorded by crossref.
- An automated dynamic chamber system for exchange flux measurement of reactive nitrogen oxides (HONO and NOX) in farmland ecosystems of the Huaihe River Basin, China K. Tang et al. 10.1016/j.scitotenv.2020.140867
- Evidence for Strong HONO Emission from Fertilized Agricultural Fields and its Remarkable Impact on Regional O3 Pollution in the Summer North China Plain C. Xue et al. 10.1021/acsearthspacechem.0c00314
- Emissions of atmospherically important nitrous acid (HONO) gas from northern grassland soil increases in the presence of nitrite (NO2−) H. Bhattarai et al. 10.1016/j.agee.2018.01.017
- Unveiling the effect of O2 on the photochemical reaction of NO2 with polycyclic aromatic hydrocarbons W. Yang et al. 10.1007/s11356-023-30289-y
- Impact of soil–atmosphere HONO exchange on concentrations of HONO and O3 in the North China Plain H. Ran et al. 10.1016/j.scitotenv.2024.172336
- Photochemical emissions of HONO, NO2 and NO from the soil surface under simulated sunlight W. Yang et al. 10.1016/j.atmosenv.2020.117596
- Insights into HONO sources from observations during a solar eclipse A. Singh et al. 10.1039/D1EA00010A
- Key Role of Equilibrium HONO Concentration over Soil in Quantifying Soil–Atmosphere HONO Fluxes F. Bao et al. 10.1021/acs.est.1c06716
- Nitrous acid formation in a snow-free wintertime polluted rural area C. Tsai et al. 10.5194/acp-18-1977-2018
- High-resolution vertical distribution and sources of HONO and NO<sub>2</sub> in the nocturnal boundary layer in urban Beijing, China F. Meng et al. 10.5194/acp-20-5071-2020
- HONO Budget and Its Role in Nitrate Formation in the Rural North China Plain C. Xue et al. 10.1021/acs.est.0c01832
- Measurement of HONO flux using the aerodynamic gradient method over an agricultural field in the Huaihe River Basin, China F. Meng et al. 10.1016/j.jes.2021.09.005
- Assessment of Daytime HONO Emission Source from Asphalt Surface to Urban Air D. Kim et al. 10.3390/app11041930
- Global and Regional Patterns of Soil Nitrous Acid Emissions and Their Acceleration of Rural Photochemical Reactions D. Wu et al. 10.1029/2021JD036379
- Heterogeneous photochemical uptake of NO2 on the soil surface as an important ground-level HONO source W. Yang et al. 10.1016/j.envpol.2020.116289
- Development and application of a twin open-top chambers method to measure soil HONO emission in the North China Plain C. Xue et al. 10.1016/j.scitotenv.2018.12.245
- Characterization of Total OH Reactivity in a Rapeseed Field: Results from the COV3ER Experiment in April 2017 S. Bsaibes et al. 10.3390/atmos11030261
- Unveiling the underestimated direct emissions of nitrous acid (HONO) Q. Zhang et al. 10.1073/pnas.2302048120
- Emission fluxes of nitrous acid (HONO) from livestock and poultry wastes W. Zhang et al. 10.1016/j.jes.2024.09.025
- Observations by Ground-Based MAX-DOAS of the Vertical Characters of Winter Pollution and the Influencing Factors of HONO Generation in Shanghai, China S. Xu et al. 10.3390/rs13173518
- A dual dynamic chamber system based on IBBCEAS for measuring fluxes of nitrous acid in agricultural fields in the North China Plain K. Tang et al. 10.1016/j.atmosenv.2018.09.059
- Surface–atmosphere exchange of inorganic water-soluble gases and associated ions in bulk aerosol above agricultural grassland pre- and postfertilisation R. Ramsay et al. 10.5194/acp-18-16953-2018
- Nitrous acid production and uptake by Zea mays plants in growth chambers in the presence of nitrogen dioxide A. Marion et al. 10.1016/j.scitotenv.2021.150696
- Dynamic chamber as a more reliable technique for measuring methane emissions from aquatic ecosystems J. Mu et al. 10.1016/j.scitotenv.2022.158147
- Nitrous acid (HONO) emissions under real-world driving conditions from vehicles in a UK road tunnel L. Kramer et al. 10.5194/acp-20-5231-2020
- Volatile organic compound fluxes over a winter wheat field by PTR-Qi-TOF-MS and eddy covariance B. Loubet et al. 10.5194/acp-22-2817-2022
- Measurement report: Exchange fluxes of HONO over agricultural fields in the North China Plain Y. Song et al. 10.5194/acp-23-15733-2023
- Simultaneous detection of atmospheric HONO and NO<sub>2</sub> utilising an IBBCEAS system based on an iterative algorithm K. Tang et al. 10.5194/amt-13-6487-2020
- Quantifying Nitrous Acid Formation Mechanisms Using Measured Vertical Profiles During the CalNex 2010 Campaign and 1D Column Modeling K. Tuite et al. 10.1029/2021JD034689
- Nitrous acid formation on Zea mays leaves by heterogeneous reaction of nitrogen dioxide in the laboratory A. Marion et al. 10.1016/j.envres.2020.110543
- Validating HONO as an Intermediate Tracer of the External Cycling of Reactive Nitrogen in the Background Atmosphere J. Wang et al. 10.1021/acs.est.2c06731
- Comparative study of biogenic volatile organic compounds fluxes by wheat, maize and rapeseed with dynamic chambers over a short period in northern France L. Gonzaga Gomez et al. 10.1016/j.atmosenv.2019.116855
- Spatiotemporal Distribution, Sources, and Impact on Atmospheric Oxidation of Reactive Nitrogen Oxides in the North China Plain Agricultural Regions in Summer S. Wei et al. 10.3390/rs16173192
- Concentrations and biosphere–atmosphere fluxes of inorganic trace gases and associated ionic aerosol counterparts over the Amazon rainforest R. Ramsay et al. 10.5194/acp-20-15551-2020
- Aging of pollution air parcels acts as the dominant source for nocturnal HONO W. Zhang et al. 10.1016/j.scitotenv.2023.163438
- A relaxed eddy accumulation (REA) LOPAP system for flux measurements of nitrous acid (HONO) L. von der Heyden et al. 10.5194/amt-15-1983-2022
- Large Contribution of Nitrous Acid to Soil-Emitted Reactive Oxidized Nitrogen and Its Effect on Air Quality Y. Wang et al. 10.1021/acs.est.2c07793
- Emission of nitrous acid from soil and biological soil crusts represents an important source of HONO in the remote atmosphere in Cyprus H. Meusel et al. 10.5194/acp-18-799-2018
- Effect of senescence on biogenic volatile organic compound fluxes in wheat plants L. Gomez et al. 10.1016/j.atmosenv.2021.118665
- Surface exchange of HONO over paddy fields in the Pearl River Delta, China B. Han et al. 10.1016/j.atmosenv.2024.120853
- Origins of atmospheric nitrous acid and their contributions to OH radical from ship plumes, marine atmosphere, and continental air masses over South China Sea X. Ni et al. 10.1016/j.scitotenv.2024.175841
41 citations as recorded by crossref.
- An automated dynamic chamber system for exchange flux measurement of reactive nitrogen oxides (HONO and NOX) in farmland ecosystems of the Huaihe River Basin, China K. Tang et al. 10.1016/j.scitotenv.2020.140867
- Evidence for Strong HONO Emission from Fertilized Agricultural Fields and its Remarkable Impact on Regional O3 Pollution in the Summer North China Plain C. Xue et al. 10.1021/acsearthspacechem.0c00314
- Emissions of atmospherically important nitrous acid (HONO) gas from northern grassland soil increases in the presence of nitrite (NO2−) H. Bhattarai et al. 10.1016/j.agee.2018.01.017
- Unveiling the effect of O2 on the photochemical reaction of NO2 with polycyclic aromatic hydrocarbons W. Yang et al. 10.1007/s11356-023-30289-y
- Impact of soil–atmosphere HONO exchange on concentrations of HONO and O3 in the North China Plain H. Ran et al. 10.1016/j.scitotenv.2024.172336
- Photochemical emissions of HONO, NO2 and NO from the soil surface under simulated sunlight W. Yang et al. 10.1016/j.atmosenv.2020.117596
- Insights into HONO sources from observations during a solar eclipse A. Singh et al. 10.1039/D1EA00010A
- Key Role of Equilibrium HONO Concentration over Soil in Quantifying Soil–Atmosphere HONO Fluxes F. Bao et al. 10.1021/acs.est.1c06716
- Nitrous acid formation in a snow-free wintertime polluted rural area C. Tsai et al. 10.5194/acp-18-1977-2018
- High-resolution vertical distribution and sources of HONO and NO<sub>2</sub> in the nocturnal boundary layer in urban Beijing, China F. Meng et al. 10.5194/acp-20-5071-2020
- HONO Budget and Its Role in Nitrate Formation in the Rural North China Plain C. Xue et al. 10.1021/acs.est.0c01832
- Measurement of HONO flux using the aerodynamic gradient method over an agricultural field in the Huaihe River Basin, China F. Meng et al. 10.1016/j.jes.2021.09.005
- Assessment of Daytime HONO Emission Source from Asphalt Surface to Urban Air D. Kim et al. 10.3390/app11041930
- Global and Regional Patterns of Soil Nitrous Acid Emissions and Their Acceleration of Rural Photochemical Reactions D. Wu et al. 10.1029/2021JD036379
- Heterogeneous photochemical uptake of NO2 on the soil surface as an important ground-level HONO source W. Yang et al. 10.1016/j.envpol.2020.116289
- Development and application of a twin open-top chambers method to measure soil HONO emission in the North China Plain C. Xue et al. 10.1016/j.scitotenv.2018.12.245
- Characterization of Total OH Reactivity in a Rapeseed Field: Results from the COV3ER Experiment in April 2017 S. Bsaibes et al. 10.3390/atmos11030261
- Unveiling the underestimated direct emissions of nitrous acid (HONO) Q. Zhang et al. 10.1073/pnas.2302048120
- Emission fluxes of nitrous acid (HONO) from livestock and poultry wastes W. Zhang et al. 10.1016/j.jes.2024.09.025
- Observations by Ground-Based MAX-DOAS of the Vertical Characters of Winter Pollution and the Influencing Factors of HONO Generation in Shanghai, China S. Xu et al. 10.3390/rs13173518
- A dual dynamic chamber system based on IBBCEAS for measuring fluxes of nitrous acid in agricultural fields in the North China Plain K. Tang et al. 10.1016/j.atmosenv.2018.09.059
- Surface–atmosphere exchange of inorganic water-soluble gases and associated ions in bulk aerosol above agricultural grassland pre- and postfertilisation R. Ramsay et al. 10.5194/acp-18-16953-2018
- Nitrous acid production and uptake by Zea mays plants in growth chambers in the presence of nitrogen dioxide A. Marion et al. 10.1016/j.scitotenv.2021.150696
- Dynamic chamber as a more reliable technique for measuring methane emissions from aquatic ecosystems J. Mu et al. 10.1016/j.scitotenv.2022.158147
- Nitrous acid (HONO) emissions under real-world driving conditions from vehicles in a UK road tunnel L. Kramer et al. 10.5194/acp-20-5231-2020
- Volatile organic compound fluxes over a winter wheat field by PTR-Qi-TOF-MS and eddy covariance B. Loubet et al. 10.5194/acp-22-2817-2022
- Measurement report: Exchange fluxes of HONO over agricultural fields in the North China Plain Y. Song et al. 10.5194/acp-23-15733-2023
- Simultaneous detection of atmospheric HONO and NO<sub>2</sub> utilising an IBBCEAS system based on an iterative algorithm K. Tang et al. 10.5194/amt-13-6487-2020
- Quantifying Nitrous Acid Formation Mechanisms Using Measured Vertical Profiles During the CalNex 2010 Campaign and 1D Column Modeling K. Tuite et al. 10.1029/2021JD034689
- Nitrous acid formation on Zea mays leaves by heterogeneous reaction of nitrogen dioxide in the laboratory A. Marion et al. 10.1016/j.envres.2020.110543
- Validating HONO as an Intermediate Tracer of the External Cycling of Reactive Nitrogen in the Background Atmosphere J. Wang et al. 10.1021/acs.est.2c06731
- Comparative study of biogenic volatile organic compounds fluxes by wheat, maize and rapeseed with dynamic chambers over a short period in northern France L. Gonzaga Gomez et al. 10.1016/j.atmosenv.2019.116855
- Spatiotemporal Distribution, Sources, and Impact on Atmospheric Oxidation of Reactive Nitrogen Oxides in the North China Plain Agricultural Regions in Summer S. Wei et al. 10.3390/rs16173192
- Concentrations and biosphere–atmosphere fluxes of inorganic trace gases and associated ionic aerosol counterparts over the Amazon rainforest R. Ramsay et al. 10.5194/acp-20-15551-2020
- Aging of pollution air parcels acts as the dominant source for nocturnal HONO W. Zhang et al. 10.1016/j.scitotenv.2023.163438
- A relaxed eddy accumulation (REA) LOPAP system for flux measurements of nitrous acid (HONO) L. von der Heyden et al. 10.5194/amt-15-1983-2022
- Large Contribution of Nitrous Acid to Soil-Emitted Reactive Oxidized Nitrogen and Its Effect on Air Quality Y. Wang et al. 10.1021/acs.est.2c07793
- Emission of nitrous acid from soil and biological soil crusts represents an important source of HONO in the remote atmosphere in Cyprus H. Meusel et al. 10.5194/acp-18-799-2018
- Effect of senescence on biogenic volatile organic compound fluxes in wheat plants L. Gomez et al. 10.1016/j.atmosenv.2021.118665
- Surface exchange of HONO over paddy fields in the Pearl River Delta, China B. Han et al. 10.1016/j.atmosenv.2024.120853
- Origins of atmospheric nitrous acid and their contributions to OH radical from ship plumes, marine atmosphere, and continental air masses over South China Sea X. Ni et al. 10.1016/j.scitotenv.2024.175841
Latest update: 20 Nov 2024
Short summary
Sources of nitrous acid (HONO), a major precursor of the OH radical, are still under controversial discussion. Since mainly ground surface sources have been proposed, HONO fluxes were measured above an agricultural field. Positive daytime fluxes were observed which showed strong correlation with the product of the NO2 concentration and J(NO2). These results indicate HONO formation by photosensitized heterogeneous conversion of NO2 on soil surfaces as observed in recent laboratory studies.
Sources of nitrous acid (HONO), a major precursor of the OH radical, are still under...
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