School of Molecular Sciences, The University of Western Australia, Crawley WA 6009, Australia
Tengyu Liu
State Key Laboratory of Organic Geochemistry and Guangdong Key Laboratory of Environmental Protection and Resources Utilization, Guangzhou Institute of
Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
University of Chinese Academy of Sciences, Beijing 100049, China
now at: School of Energy and Environment, City University of Hong Kong, Hong Kong, China
State Key Laboratory of Organic Geochemistry and Guangdong Key Laboratory of Environmental Protection and Resources Utilization, Guangzhou Institute of
Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
University of Chinese Academy of Sciences, Beijing 100049, China
Sandra M. Saunders
School of Molecular Sciences, The University of Western Australia, Crawley WA 6009, Australia
Zheng Fang
State Key Laboratory of Organic Geochemistry and Guangdong Key Laboratory of Environmental Protection and Resources Utilization, Guangzhou Institute of
Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
University of Chinese Academy of Sciences, Beijing 100049, China
State Key Laboratory of Organic Geochemistry and Guangdong Key Laboratory of Environmental Protection and Resources Utilization, Guangzhou Institute of
Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
Center for Excellence in Regional Atmospheric Environment, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen 361021, China
State Key Laboratory of Organic Geochemistry and Guangdong Key Laboratory of Environmental Protection and Resources Utilization, Guangzhou Institute of
Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
Center for Excellence in Regional Atmospheric Environment, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen 361021, China
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The atmospheric decomposition of the biogenic α-phellandrene with ozone is characterised by conducting carefully controlled experiments in a smog chamber. Major gas-phase products are identified based on theoretical/mechanism insight, with yields quantified. Meanwhile, a significant amount of aerosol is formed and characterised, with Criegee intermediates found to be important for new particle formation. It is concluded that α-phellandrene contributes to aerosol formation/growth where emitted.
The atmospheric decomposition of the biogenic α-phellandrene with ozone is characterised by...
