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Volume 17, issue 10
Atmos. Chem. Phys., 17, 6373–6391, 2017
https://doi.org/10.5194/acp-17-6373-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
Atmos. Chem. Phys., 17, 6373–6391, 2017
https://doi.org/10.5194/acp-17-6373-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 29 May 2017

Research article | 29 May 2017

Chemical and isotopic composition of secondary organic aerosol generated by α-pinene ozonolysis

Carl Meusinger et al.

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Status: closed
Status: closed
AC: Author comment | RC: Referee comment | SC: Short comment | EC: Editor comment
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Peer review completion

AR: Author's response | RR: Referee report | ED: Editor decision
AR by Carl Meusinger on behalf of the Authors (02 Aug 2016)  Author's response    Manuscript
ED: Referee Nomination & Report Request started (22 Aug 2016) by Maria Cristina Facchini
RR by Anonymous Referee #2 (02 Sep 2016)
RR by Anonymous Referee #1 (12 Sep 2016)
ED: Reconsider after major revisions (13 Sep 2016) by Maria Cristina Facchini
AR by Anna Wenzel on behalf of the Authors (09 Nov 2016)  Author's response
ED: Referee Nomination & Report Request started (11 Nov 2016) by Maria Cristina Facchini
RR by Anonymous Referee #1 (24 Nov 2016)
ED: Reconsider after major revisions (04 Dec 2016) by Maria Cristina Facchini
AR by Anna Wenzel on behalf of the Authors (16 Jan 2017)  Author's response
ED: Referee Nomination & Report Request started (16 Jan 2017) by Maria Cristina Facchini
RR by Anonymous Referee #3 (10 Feb 2017)
ED: Reconsider after major revisions (10 Feb 2017) by Maria Cristina Facchini
AR by Carl Meusinger on behalf of the Authors (21 Mar 2017)  Author's response    Manuscript
ED: Referee Nomination & Report Request started (22 Mar 2017) by Maria Cristina Facchini
RR by Anonymous Referee #3 (18 Apr 2017)
ED: Publish subject to technical corrections (20 Apr 2017) by Maria Cristina Facchini
AR by Carl Meusinger on behalf of the Authors (28 Apr 2017)  Author's response    Manuscript
Publications Copernicus
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Short summary
Isotope studies can constrain budgets of secondary organic aerosol (SOA) that is pivotal to air pollution and climate. SOA from α-pinene ozonolysis was found to be enriched in 13C relative to the precursor. The observed difference in 13C between the gas and particle phases may arise from isotope-dependent changes in branching ratios. Alternatively, some gas-phase products involve carbon atoms from highly enriched and depleted sites, giving a non-kinetic origin to the observed fractionations.
Isotope studies can constrain budgets of secondary organic aerosol (SOA) that is pivotal to air...
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