Articles | Volume 17, issue 3
https://doi.org/10.5194/acp-17-1759-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-17-1759-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
06 Feb 2017
Research article |
| 06 Feb 2017
Anthropogenic influences on the physical state of submicron particulate matter over a tropical forest
Adam P. Bateman
School of Engineering and Applied Sciences, Harvard University, Cambridge, MA, USA
Zhaoheng Gong
School of Engineering and Applied Sciences, Harvard University, Cambridge, MA, USA
Tristan H. Harder
Chemical Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA, USA
now at: Physikalisches Institut, Universität Würzburg, Am Hubland, 97074 Würzburg, Germany
Suzane S. de Sá
School of Engineering and Applied Sciences, Harvard University, Cambridge, MA, USA
Bingbing Wang
William R. Wiley Environmental Molecular Sciences Laboratory, Pacific Northwest National Laboratory, Richland, WA, USA
State Key Laboratory of Marine Environmental Science, College of Ocean and Earth Sciences, Xiamen University, Xiamen, China
Paulo Castillo
Environmental and Climate Sciences Department, Brookhaven National Laboratory, Upton, NY, USA
Swarup China
William R. Wiley Environmental Molecular Sciences Laboratory, Pacific Northwest National Laboratory, Richland, WA, USA
Yingjun Liu
School of Engineering and Applied Sciences, Harvard University, Cambridge, MA, USA
Rachel E. O'Brien
Chemical Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA, USA
now at: Department of Civil and Environmental Engineering, Massachusetts Institute of Technology, Cambridge, MA, USA
Brett B. Palm
Department of Chemistry and Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado, Boulder, CO, USA
Hung-Wei Shiu
William R. Wiley Environmental Molecular Sciences Laboratory, Pacific Northwest National Laboratory, Richland, WA, USA
now at: Scientific Research Division, National Synchrotron Radiation Research Center, Hsinchu, Taiwan 30076
Glauber G. Cirino
National Institute of Amazonian Research, Manaus, Amazonas, Brazil
Ryan Thalman
Environmental and Climate Sciences Department, Brookhaven National Laboratory, Upton, NY, USA
now at: Departments of Chemistry and Natural Resources, Snow College, Richfield, UT, USA
Kouji Adachi
Atmospheric Environment and Applied Meteorology Research Department, Meteorological Research Institute, Tsukuba, Ibaraki, Japan
M. Lizabeth Alexander
William R. Wiley Environmental Molecular Sciences Laboratory, Pacific Northwest National Laboratory, Richland, WA, USA
Paulo Artaxo
Departamento de Física Aplicada, University of São Paulo, São Paulo, Brazil
Allan K. Bertram
Department of Chemistry, University of British Columbia, Vancouver, BC, Canada
Peter R. Buseck
School of Earth and Space Exploration & School of Molecular Sciences, Arizona State University, Tempe, AZ, USA
Mary K. Gilles
Chemical Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA, USA
Jose L. Jimenez
Department of Chemistry and Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado, Boulder, CO, USA
Alexander Laskin
William R. Wiley Environmental Molecular Sciences Laboratory, Pacific Northwest National Laboratory, Richland, WA, USA
Antonio O. Manzi
National Institute of Amazonian Research, Manaus, Amazonas, Brazil
Arthur Sedlacek
Environmental and Climate Sciences Department, Brookhaven National Laboratory, Upton, NY, USA
Rodrigo A. F. Souza
Amazonas State University, Manaus, Amazonas, Brazil
Jian Wang
Environmental and Climate Sciences Department, Brookhaven National Laboratory, Upton, NY, USA
Rahul Zaveri
William R. Wiley Environmental Molecular Sciences Laboratory, Pacific Northwest National Laboratory, Richland, WA, USA
Scot T. Martin
CORRESPONDING AUTHOR
School of Engineering and Applied Sciences, Harvard University, Cambridge, MA, USA
Department of Earth and Planetary Sciences, Harvard University, Cambridge, MA, USA
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Short summary
The occurrence of nonliquid and liquid physical states of submicron atmospheric particulate matter (PM) downwind of an urban region in central Amazonia was investigated. Air masses representing background conditions, urban pollution, and regional- and continental-scale biomass were measured. Anthropogenic influences contributed to the presence of nonliquid PM in the atmospheric particle population, while liquid PM dominated during periods of biogenic influence.
The occurrence of nonliquid and liquid physical states of submicron atmospheric particulate...
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