Articles | Volume 17, issue 24
https://doi.org/10.5194/acp-17-14975-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-17-14975-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
19 Dec 2017
Research article |
| 19 Dec 2017
| 19 Dec 2017
The single-particle mixing state and cloud scavenging of black carbon: a case study at a high-altitude mountain site in southern China
Guohua Zhang
State Key Laboratory of Organic Geochemistry and Guangdong Key Laboratory of Environmental Resources Utilization and
Protection, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, PR China
Qinhao Lin
State Key Laboratory of Organic Geochemistry and Guangdong Key Laboratory of Environmental Resources Utilization and
Protection, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, PR China
University of Chinese Academy of Sciences, Beijing 100039, PR China
Long Peng
State Key Laboratory of Organic Geochemistry and Guangdong Key Laboratory of Environmental Resources Utilization and
Protection, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, PR China
University of Chinese Academy of Sciences, Beijing 100039, PR China
State Key Laboratory of Organic Geochemistry and Guangdong Key Laboratory of Environmental Resources Utilization and
Protection, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, PR China
Duohong Chen
State Environmental Protection Key Laboratory of Regional
Air Quality Monitoring, Guangdong Environmental Monitoring Center, Guangzhou 510308, PR China
Mei Li
Institute of Mass Spectrometer and Atmospheric Environment, Jinan University, Guangzhou 510632, PR China
Guangdong Engineering Research Center for Online Atmospheric Pollution Source Apportionment, Guangzhou 510632, PR China
Institute of Mass Spectrometer and Atmospheric Environment, Jinan University, Guangzhou 510632, PR China
Guangdong Engineering Research Center for Online Atmospheric Pollution Source Apportionment, Guangzhou 510632, PR China
Fred J. Brechtel
Brechtel Manufacturing Inc., Hayward, 94544, CA, USA
Jianxin Chen
Shaoguan Environmental Monitoring Center, Shaoguan 512026, PR China
Weijun Yan
Shaoguan Environmental Monitoring Center, Shaoguan 512026, PR China
Xinming Wang
State Key Laboratory of Organic Geochemistry and Guangdong Key Laboratory of Environmental Resources Utilization and
Protection, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, PR China
Ping'an Peng
State Key Laboratory of Organic Geochemistry and Guangdong Key Laboratory of Environmental Resources Utilization and
Protection, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, PR China
Guoying Sheng
State Key Laboratory of Organic Geochemistry and Guangdong Key Laboratory of Environmental Resources Utilization and
Protection, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, PR China
Zhen Zhou
Institute of Mass Spectrometer and Atmospheric Environment, Jinan University, Guangzhou 510632, PR China
Guangdong Engineering Research Center for Online Atmospheric Pollution Source Apportionment, Guangzhou 510632, PR China
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31 citations as recorded by crossref.
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- In-cloud scavenging of chemically segregated particle types by individual particle observation Y. Yang et al. 10.1016/j.apgeochem.2023.105657
- Reconstructing Elemental Carbon Long-Term Trend in the Po Valley (Italy) from Fog Water Samples S. Gilardoni et al. 10.3390/atmos11060580
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- Organic Coating Reduces Hygroscopic Growth of Phase-Separated Aerosol Particles W. Li et al. 10.1021/acs.est.1c05901
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- In-cloud formation of secondary species in iron-containing particles Q. Lin et al. 10.5194/acp-19-1195-2019
- Black Carbon Involved Photochemistry Enhances the Formation of Sulfate in the Ambient Atmosphere: Evidence From In Situ Individual Particle Investigation G. Zhang et al. 10.1029/2021JD035226
- Aerodynamic size-resolved composition and cloud condensation nuclei properties of aerosols in a Beijing suburban region C. Yu et al. 10.5194/acp-22-4375-2022
- Stage-resolved in-cloud scavenging of submicron and BC-containing particles: A case study Y. Yang et al. 10.1016/j.atmosenv.2020.117883
- Black carbon linked aerosol hygroscopic growth: Size and mixing state are crucial B. Sarangi et al. 10.1016/j.atmosenv.2018.12.001
- Impact of in-cloud aqueous processes on the chemical compositions and morphology of individual atmospheric aerosols Y. Fu et al. 10.5194/acp-20-14063-2020
- Efficient droplet activation of ambient black carbon particles in a suburban environment P. Tian et al. 10.5194/acp-24-5149-2024
- The optical properties and in-situ observational evidence for the formation of brown carbon in clouds Z. Guo et al. 10.5194/acp-22-4827-2022
- Mixing state and influence factors controlling diurnal variation of particulate nitrophenol compounds at a suburban area in northern China Z. Guo et al. 10.1016/j.envpol.2024.123368
- Size-segregated deposition of atmospheric elemental carbon (EC) in the human respiratory system: A case study of the Pearl River Delta, China S. Jia et al. 10.1016/j.scitotenv.2019.134932
- Source apportionment using receptor model based on aerosol mass spectra and 1 h resolution chemical dataset in Tianjin, China X. Peng et al. 10.1016/j.atmosenv.2018.11.018
- Characterization of black carbon aerosol at the summit of Mount Tai (1534 m) in central east China: Temporal variation, source appointment and transport L. Shen et al. 10.1016/j.atmosenv.2020.118152
- Enhanced mixing state of black carbon with nitrate in single particles during haze periods in Zhengzhou, China Q. Zhou et al. 10.1016/j.jes.2021.03.031
- Fog/cloud processing of atmospheric aerosols from a single particle perspective: A review of field observations G. Zhang et al. 10.1016/j.atmosenv.2024.120536
- Particle number size distribution of PM1 and PM10 in fogs and implications on fog droplet evolutions S. Wu et al. 10.1016/j.atmosenv.2022.119086
- Influence of pollution control measures on the reduction of black carbon in an urban site of megacity, Tianjin, China based on ground-monitored and MERRA-2 reanalysis data X. Cheng et al. 10.1016/j.scitotenv.2023.169466
- Impact of Cloud Process in the Mixing State and Microphysical Properties of Soot Particles: Implications in Light Absorption Enhancement Y. Fu et al. 10.1029/2022JD037169
- Black carbon content of traffic emissions significantly impacts black carbon mass size distributions and mixing states F. Li et al. 10.5194/acp-23-6545-2023
- Observation of atmospheric new particle growth events at the summit of mountain Tai (1534 m) in Central East China L. Shen et al. 10.1016/j.atmosenv.2018.12.051
- Characteristics and mixing state of aerosol at the summit of Mount Tai (1534 m) in Central East China: First measurements with SPAMS H. Wang et al. 10.1016/j.atmosenv.2019.06.021
- Extensive Soot Compaction by Cloud Processing from Laboratory and Field Observations J. Bhandari et al. 10.1038/s41598-019-48143-y
- Variation, sources and historical trend of black carbon in Beijing, China based on ground observation and MERRA-2 reanalysis data W. Qin et al. 10.1016/j.envpol.2018.11.063
- Lifecycle of light-absorbing carbonaceous aerosols in the atmosphere D. Liu et al. 10.1038/s41612-020-00145-8
- Recent Advances in Quantifying Wet Scavenging Efficiency of Black Carbon Aerosol Y. Yang et al. 10.3390/atmos10040175
- Exploring secondary aerosol formation associated with elemental carbon in the lower free troposphere L. Li et al. 10.1016/j.scitotenv.2024.172992
31 citations as recorded by crossref.
- Single particle diversity and mixing state of carbonaceous aerosols in Guangzhou, China C. Cheng et al. 10.1016/j.scitotenv.2020.142182
- In-cloud scavenging of chemically segregated particle types by individual particle observation Y. Yang et al. 10.1016/j.apgeochem.2023.105657
- Reconstructing Elemental Carbon Long-Term Trend in the Po Valley (Italy) from Fog Water Samples S. Gilardoni et al. 10.3390/atmos11060580
- Cloud droplet activation properties and scavenged fraction of black carbon in liquid-phase clouds at the high-alpine research station Jungfraujoch (3580 m a.s.l.) G. Motos et al. 10.5194/acp-19-3833-2019
- Organic Coating Reduces Hygroscopic Growth of Phase-Separated Aerosol Particles W. Li et al. 10.1021/acs.est.1c05901
- Cloud scavenging of anthropogenic refractory particles at a mountain site in North China L. Liu et al. 10.5194/acp-18-14681-2018
- In-cloud formation of secondary species in iron-containing particles Q. Lin et al. 10.5194/acp-19-1195-2019
- Black Carbon Involved Photochemistry Enhances the Formation of Sulfate in the Ambient Atmosphere: Evidence From In Situ Individual Particle Investigation G. Zhang et al. 10.1029/2021JD035226
- Aerodynamic size-resolved composition and cloud condensation nuclei properties of aerosols in a Beijing suburban region C. Yu et al. 10.5194/acp-22-4375-2022
- Stage-resolved in-cloud scavenging of submicron and BC-containing particles: A case study Y. Yang et al. 10.1016/j.atmosenv.2020.117883
- Black carbon linked aerosol hygroscopic growth: Size and mixing state are crucial B. Sarangi et al. 10.1016/j.atmosenv.2018.12.001
- Impact of in-cloud aqueous processes on the chemical compositions and morphology of individual atmospheric aerosols Y. Fu et al. 10.5194/acp-20-14063-2020
- Efficient droplet activation of ambient black carbon particles in a suburban environment P. Tian et al. 10.5194/acp-24-5149-2024
- The optical properties and in-situ observational evidence for the formation of brown carbon in clouds Z. Guo et al. 10.5194/acp-22-4827-2022
- Mixing state and influence factors controlling diurnal variation of particulate nitrophenol compounds at a suburban area in northern China Z. Guo et al. 10.1016/j.envpol.2024.123368
- Size-segregated deposition of atmospheric elemental carbon (EC) in the human respiratory system: A case study of the Pearl River Delta, China S. Jia et al. 10.1016/j.scitotenv.2019.134932
- Source apportionment using receptor model based on aerosol mass spectra and 1 h resolution chemical dataset in Tianjin, China X. Peng et al. 10.1016/j.atmosenv.2018.11.018
- Characterization of black carbon aerosol at the summit of Mount Tai (1534 m) in central east China: Temporal variation, source appointment and transport L. Shen et al. 10.1016/j.atmosenv.2020.118152
- Enhanced mixing state of black carbon with nitrate in single particles during haze periods in Zhengzhou, China Q. Zhou et al. 10.1016/j.jes.2021.03.031
- Fog/cloud processing of atmospheric aerosols from a single particle perspective: A review of field observations G. Zhang et al. 10.1016/j.atmosenv.2024.120536
- Particle number size distribution of PM1 and PM10 in fogs and implications on fog droplet evolutions S. Wu et al. 10.1016/j.atmosenv.2022.119086
- Influence of pollution control measures on the reduction of black carbon in an urban site of megacity, Tianjin, China based on ground-monitored and MERRA-2 reanalysis data X. Cheng et al. 10.1016/j.scitotenv.2023.169466
- Impact of Cloud Process in the Mixing State and Microphysical Properties of Soot Particles: Implications in Light Absorption Enhancement Y. Fu et al. 10.1029/2022JD037169
- Black carbon content of traffic emissions significantly impacts black carbon mass size distributions and mixing states F. Li et al. 10.5194/acp-23-6545-2023
- Observation of atmospheric new particle growth events at the summit of mountain Tai (1534 m) in Central East China L. Shen et al. 10.1016/j.atmosenv.2018.12.051
- Characteristics and mixing state of aerosol at the summit of Mount Tai (1534 m) in Central East China: First measurements with SPAMS H. Wang et al. 10.1016/j.atmosenv.2019.06.021
- Extensive Soot Compaction by Cloud Processing from Laboratory and Field Observations J. Bhandari et al. 10.1038/s41598-019-48143-y
- Variation, sources and historical trend of black carbon in Beijing, China based on ground observation and MERRA-2 reanalysis data W. Qin et al. 10.1016/j.envpol.2018.11.063
- Lifecycle of light-absorbing carbonaceous aerosols in the atmosphere D. Liu et al. 10.1038/s41612-020-00145-8
- Recent Advances in Quantifying Wet Scavenging Efficiency of Black Carbon Aerosol Y. Yang et al. 10.3390/atmos10040175
- Exploring secondary aerosol formation associated with elemental carbon in the lower free troposphere L. Li et al. 10.1016/j.scitotenv.2024.172992
Latest update: 29 Jun 2024
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Short summary
The mixing state of black carbon (BC)-containing particles and the mass scavenging efficiency of BC in cloud were investigated at a mountain site (1690 m a.s.l.) in southern China. The measured BC-containing particles were internally mixed extensively with sulfate, and thus the number fraction of scavenged BC-containing particles is close to that of all the measured particles. BC-containing particles with higher fractions of organics were scavenged relatively less.
The mixing state of black carbon (BC)-containing particles and the mass scavenging efficiency of...
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