Articles | Volume 17, issue 21
https://doi.org/10.5194/acp-17-13417-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-17-13417-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
10 Nov 2017
Research article |
| 10 Nov 2017
Ethene, propene, butene and isoprene emissions from a ponderosa pine forest measured by relaxed eddy accumulation
Department of Geography and Berkeley Atmospheric Sciences Center, University of California Berkeley, Berkeley, CA 94720-4740, USA
Malte Julian Deventer
Department of Geography and Berkeley Atmospheric Sciences Center, University of California Berkeley, Berkeley, CA 94720-4740, USA
Andrew A. Turnipseed
2B Technologies, Boulder CO 80301, USA
Carsten Warneke
Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado Boulder, Boulder CO 80309, USA
NOAA Earth System Research Laboratory, Boulder, CO 80305, USA
John Ortega
Atmospheric Chemistry Observations and Modeling (ACOM), National Center for Atmospheric Research, Boulder, CO 80301, USA
Steve Shen
Department of Geography and Berkeley Atmospheric Sciences Center, University of California Berkeley, Berkeley, CA 94720-4740, USA
Luis Martinez
Ernest F. Hollings Undergraduate Scholarship program, NOAA, Boulder, CO 80305, USA
Abigail Koss
Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado Boulder, Boulder CO 80309, USA
NOAA Earth System Research Laboratory, Boulder, CO 80305, USA
Brian M. Lerner
Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado Boulder, Boulder CO 80309, USA
NOAA Earth System Research Laboratory, Boulder, CO 80305, USA
now at: Aerodyne Research Inc., Billerica, MA 01821-3976, USA
Jessica B. Gilman
Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado Boulder, Boulder CO 80309, USA
NOAA Earth System Research Laboratory, Boulder, CO 80305, USA
James N. Smith
Atmospheric Chemistry Observations and Modeling (ACOM), National Center for Atmospheric Research, Boulder, CO 80301, USA
now at: Department of Chemistry, University of California Irvine, Irvine, CA 92697-2025, USA
Alex B. Guenther
Department of Earth System Science, University of California Irvine, Irvine, CA 92697-3100, USA
Joost A. de Gouw
Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado Boulder, Boulder CO 80309, USA
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- Closing the Reactive Carbon Flux Budget: Observations From Dual Mass Spectrometers Over a Coniferous Forest M. Vermeuel et al. 10.1029/2023JD038753
- Determination and Characteristic Analysis of Atmospheric Non-Methane Hydrocarbons in a Regional Hub City of North China Plain J. Wang et al. 10.1088/1755-1315/223/1/012052
- Long-term trend in surface ozone in Houston-Galveston-Brazoria: Sectoral contributions based on changes in volatile organic compounds E. Soleimanian et al. 10.1016/j.envpol.2022.119647
- Changes in source apportioned VOCs during high O3 periods using initial VOC-concentration-dispersion normalized PMF Y. Wu et al. 10.1016/j.scitotenv.2023.165182
- Acyl Peroxy Nitrates Link Oil and Natural Gas Emissions to High Ozone Abundances in the Colorado Front Range During Summer 2015 J. Lindaas et al. 10.1029/2018JD028825
- Observations of Volatile Organic Compounds in the Los Angeles Basin during COVID-19 P. Van Rooy et al. 10.1021/acsearthspacechem.1c00248
- Seasonal Variations of Vocs in Houston: Source Apportionment and Spatial Distribution of Source Origins in Summertime and Wintertime B. Sadeghi et al. 10.2139/ssrn.3972065
- Potential Factors Contributing to Ozone Production in AQUAS–Kyoto Campaign in Summer 2020: Natural Source-Related Missing OH Reactivity and Heterogeneous HO2/RO2 Loss J. Li et al. 10.1021/acs.est.2c03628
- A portable, low-cost relaxed eddy accumulation (REA) system for quantifying ecosystem-level fluxes of volatile organics C. Sarkar et al. 10.1016/j.atmosenv.2020.117764
- Seasonality and Source Apportionment of Nonmethane Volatile Organic Compounds at Boulder Reservoir, Colorado, Between 2017 and 2019 I. Pollack et al. 10.1029/2020JD034234
- The Interplay Between Ozone and Urban Vegetation—BVOC Emissions, Ozone Deposition, and Tree Ecophysiology A. Fitzky et al. 10.3389/ffgc.2019.00050
- Experimental chemical budgets of OH, HO2, and RO2 radicals in rural air in western Germany during the JULIAC campaign 2019 C. Cho et al. 10.5194/acp-23-2003-2023
- Current Status and Future Directions of Tropospheric Photochemical Ozone Studies in Korea G. Lee et al. 10.5572/KOSAE.2020.36.4.419
- A comprehensive approach combining positive matrix factorization modeling, meteorology, and machine learning for source apportionment of surface ozone precursors: Underlying factors contributing to ozone formation in Houston, Texas D. Nelson et al. 10.1016/j.envpol.2023.122223
- Emissions of non-methane volatile organic compounds from a landfill site in a major city of India: impact on local air quality P. Dave et al. 10.1016/j.heliyon.2020.e04537
- Identifying the Drivers of Modeling Uncertainties in Isoprene Emissions: Schemes Versus Meteorological Forcings Y. Cao et al. 10.1029/2020JD034242
- A detailed study of the ion chemistry of alkenes focusing on heptenes aimed at their SIFT-MS quantification R. Brůhová Michalčíková et al. 10.1016/j.ijms.2017.12.004
- Ambient air characteristics of biogenic volatile organic compounds at a tropical evergreen forest site in Central Western Ghats of India N. Tripathi et al. 10.1007/s10874-021-09415-y
- Influence of seasonal variability on source characteristics of VOCs at Houston industrial area B. Sadeghi et al. 10.1016/j.atmosenv.2022.119077
- Low-level summertime isoprene observed at a forested mountaintop site in southern China: implications for strong regional atmospheric oxidative capacity D. Gong et al. 10.5194/acp-18-14417-2018
- Absorption cross sections in the CH stretching region for propene broadened by helium and nitrogen R. Dodangodage et al. 10.1016/j.jqsrt.2021.107738
- Measurements of Volatile Organic Compounds at a rural site in India: Variability and sources during the seasonal transition S. Sindhu et al. 10.1016/j.scitotenv.2023.165493
- Changes in ozone and precursors during two aged wildfire smoke events in the Colorado Front Range in summer 2015 J. Lindaas et al. 10.5194/acp-17-10691-2017
23 citations as recorded by crossref.
- Ecosystem‐Scale Measurements of Methyl Halide Fluxes From a Brackish Tidal Marsh Invaded With Perennial Pepperweed (Lepidium latifolium) M. Deventer et al. 10.1029/2018JG004536
- Closing the Reactive Carbon Flux Budget: Observations From Dual Mass Spectrometers Over a Coniferous Forest M. Vermeuel et al. 10.1029/2023JD038753
- Determination and Characteristic Analysis of Atmospheric Non-Methane Hydrocarbons in a Regional Hub City of North China Plain J. Wang et al. 10.1088/1755-1315/223/1/012052
- Long-term trend in surface ozone in Houston-Galveston-Brazoria: Sectoral contributions based on changes in volatile organic compounds E. Soleimanian et al. 10.1016/j.envpol.2022.119647
- Changes in source apportioned VOCs during high O3 periods using initial VOC-concentration-dispersion normalized PMF Y. Wu et al. 10.1016/j.scitotenv.2023.165182
- Acyl Peroxy Nitrates Link Oil and Natural Gas Emissions to High Ozone Abundances in the Colorado Front Range During Summer 2015 J. Lindaas et al. 10.1029/2018JD028825
- Observations of Volatile Organic Compounds in the Los Angeles Basin during COVID-19 P. Van Rooy et al. 10.1021/acsearthspacechem.1c00248
- Seasonal Variations of Vocs in Houston: Source Apportionment and Spatial Distribution of Source Origins in Summertime and Wintertime B. Sadeghi et al. 10.2139/ssrn.3972065
- Potential Factors Contributing to Ozone Production in AQUAS–Kyoto Campaign in Summer 2020: Natural Source-Related Missing OH Reactivity and Heterogeneous HO2/RO2 Loss J. Li et al. 10.1021/acs.est.2c03628
- A portable, low-cost relaxed eddy accumulation (REA) system for quantifying ecosystem-level fluxes of volatile organics C. Sarkar et al. 10.1016/j.atmosenv.2020.117764
- Seasonality and Source Apportionment of Nonmethane Volatile Organic Compounds at Boulder Reservoir, Colorado, Between 2017 and 2019 I. Pollack et al. 10.1029/2020JD034234
- The Interplay Between Ozone and Urban Vegetation—BVOC Emissions, Ozone Deposition, and Tree Ecophysiology A. Fitzky et al. 10.3389/ffgc.2019.00050
- Experimental chemical budgets of OH, HO2, and RO2 radicals in rural air in western Germany during the JULIAC campaign 2019 C. Cho et al. 10.5194/acp-23-2003-2023
- Current Status and Future Directions of Tropospheric Photochemical Ozone Studies in Korea G. Lee et al. 10.5572/KOSAE.2020.36.4.419
- A comprehensive approach combining positive matrix factorization modeling, meteorology, and machine learning for source apportionment of surface ozone precursors: Underlying factors contributing to ozone formation in Houston, Texas D. Nelson et al. 10.1016/j.envpol.2023.122223
- Emissions of non-methane volatile organic compounds from a landfill site in a major city of India: impact on local air quality P. Dave et al. 10.1016/j.heliyon.2020.e04537
- Identifying the Drivers of Modeling Uncertainties in Isoprene Emissions: Schemes Versus Meteorological Forcings Y. Cao et al. 10.1029/2020JD034242
- A detailed study of the ion chemistry of alkenes focusing on heptenes aimed at their SIFT-MS quantification R. Brůhová Michalčíková et al. 10.1016/j.ijms.2017.12.004
- Ambient air characteristics of biogenic volatile organic compounds at a tropical evergreen forest site in Central Western Ghats of India N. Tripathi et al. 10.1007/s10874-021-09415-y
- Influence of seasonal variability on source characteristics of VOCs at Houston industrial area B. Sadeghi et al. 10.1016/j.atmosenv.2022.119077
- Low-level summertime isoprene observed at a forested mountaintop site in southern China: implications for strong regional atmospheric oxidative capacity D. Gong et al. 10.5194/acp-18-14417-2018
- Absorption cross sections in the CH stretching region for propene broadened by helium and nitrogen R. Dodangodage et al. 10.1016/j.jqsrt.2021.107738
- Measurements of Volatile Organic Compounds at a rural site in India: Variability and sources during the seasonal transition S. Sindhu et al. 10.1016/j.scitotenv.2023.165493
Latest update: 26 Sep 2023
Short summary
Alkenes emanate from both natural and anthropogenic sources and can contribute to atmospheric ozone production. This study measured
lightalkene (ethene, propene and butene) fluxes from a ponderosa pine forest using a novel relaxed eddy accumulation method, revealing much larger emissions than previously estimated and accounting for a significant fraction of OH reactivity. Emissions have a diurnal cycle related to sunlight and temperature, and the forest canopy appears to be the source.
Alkenes emanate from both natural and anthropogenic sources and can contribute to atmospheric...
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