Articles | Volume 17, issue 19
Atmos. Chem. Phys., 17, 11991–12010, 2017
https://doi.org/10.5194/acp-17-11991-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Atmos. Chem. Phys., 17, 11991–12010, 2017
https://doi.org/10.5194/acp-17-11991-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article 10 Oct 2017
Research article | 10 Oct 2017
Modeling of the chemistry in oxidation flow reactors with high initial NO
Zhe Peng and Jose L. Jimenez
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Cited
27 citations as recorded by crossref.
- Evaluation of the Oxidation Flow Reactor for particulate matter emission limit certification J. Cao et al. 10.1016/j.atmosenv.2019.117086
- Influence of the NO/NO2 Ratio on Oxidation Product Distributions under High-NO Conditions K. Nihill et al. 10.1021/acs.est.0c07621
- Photochemical transformation of residential wood combustion emissions: dependence of organic aerosol composition on OH exposure A. Hartikainen et al. 10.5194/acp-20-6357-2020
- Modeling the formation and composition of secondary organic aerosol from diesel exhaust using parameterized and semi-explicit chemistry and thermodynamic models S. Eluri et al. 10.5194/acp-18-13813-2018
- Model Evaluation of New Techniques for Maintaining High-NO Conditions in Oxidation Flow Reactors for the Study of OH-Initiated Atmospheric Chemistry Z. Peng et al. 10.1021/acsearthspacechem.7b00070
- Gas-phase composition and secondary organic aerosol formation from standard and particle filter-retrofitted gasoline direct injection vehicles investigated in a batch and flow reactor S. Pieber et al. 10.5194/acp-18-9929-2018
- Radical chemistry in oxidation flow reactors for atmospheric chemistry research Z. Peng & J. Jimenez 10.1039/C9CS00766K
- Nitrate radical generation via continuous generation of dinitrogen pentoxide in a laminar flow reactor coupled to an oxidation flow reactor A. Lambe et al. 10.5194/amt-13-2397-2020
- Changes in PM<sub>2.5</sub> peat combustion source profiles with atmospheric aging in an oxidation flow reactor J. Chow et al. 10.5194/amt-12-5475-2019
- A novel high-volume Photochemical Emission Aging flow tube Reactor (PEAR) M. Ihalainen et al. 10.1080/02786826.2018.1559918
- Mitigation of Secondary Organic Aerosol Formation from Log Wood Burning Emissions by Catalytic Removal of Aromatic Hydrocarbons S. Pieber et al. 10.1021/acs.est.8b04124
- Cyclic Ion Mobility Spectrometry Coupled to High-Resolution Time-of-Flight Mass Spectrometry Equipped with Atmospheric Solid Analysis Probe for the Molecular Characterization of Combustion Particulate Matter C. Rüger et al. 10.1021/jasms.0c00274
- Technical Note: Effect of varying the <i>λ</i> = 185 and 254 nm photon flux ratio on radical generation in oxidation flow reactors J. Rowe et al. 10.5194/acp-20-13417-2020
- Evolution of OH reactivity in NO-free volatile organic compound photooxidation investigated by the fully explicit GECKO-A model Z. Peng et al. 10.5194/acp-21-14649-2021
- HO<sub><i>x</i></sub> and NO<sub><i>x</i></sub> production in oxidation flow reactors via photolysis of isopropyl nitrite, isopropyl nitrite-d<sub>7</sub>, and 1,3-propyl dinitrite at <i>λ</i> = 254, 350, and 369 nm A. Lambe et al. 10.5194/amt-12-299-2019
- OH chemistry of non-methane organic gases (NMOGs) emitted from laboratory and ambient biomass burning smoke: evaluating the influence of furans and oxygenated aromatics on ozone and secondary NMOG formation M. Coggon et al. 10.5194/acp-19-14875-2019
- Comparison of secondary organic aerosol formation from toluene on initially wet and dry ammonium sulfate particles at moderate relative humidity T. Liu et al. 10.5194/acp-18-5677-2018
- Constraining nucleation, condensation, and chemistry in oxidation flow reactors using size-distribution measurements and aerosol microphysical modeling A. Hodshire et al. 10.5194/acp-18-12433-2018
- Exposure of Lung Epithelial Cells to Photochemically Aged Secondary Organic Aerosol Shows Increased Toxic Effects P. Chowdhury et al. 10.1021/acs.estlett.8b00256
- Dynamic changes in optical and chemical properties of tar ball aerosols by atmospheric photochemical aging C. Li et al. 10.5194/acp-19-139-2019
- Impact of photochemical ageing on Polycyclic Aromatic Hydrocarbons (PAH) and oxygenated PAH (Oxy-PAH/OH-PAH) in logwood stove emissions T. Miersch et al. 10.1016/j.scitotenv.2019.05.412
- Photochemical aging and secondary organic aerosols generated from limonene in an oxidation flow reactor S. Sbai & B. Farida 10.1007/s11356-019-05012-5
- Understanding the Impact of High-NOx Conditions on the Formation of Secondary Organic Aerosol in the Photooxidation of Oil Sand-Related Precursors K. Li et al. 10.1021/acs.est.9b05404
- Assessing the degree of plug flow in oxidation flow reactors (OFRs): a study on a potential aerosol mass (PAM) reactor D. Mitroo et al. 10.5194/amt-11-1741-2018
- Organic peroxy radical chemistry in oxidation flow reactors and environmental chambers and their atmospheric relevance Z. Peng et al. 10.5194/acp-19-813-2019
- Secondary Organic Aerosol Formation Potential from Ambient Air in Beijing: Effects of Atmospheric Oxidation Capacity at Different Pollution Levels J. Liu et al. 10.1021/acs.est.1c00890
- Rate constant and secondary organic aerosol formation from the gas-phase reaction of eugenol with hydroxyl radicals C. Liu et al. 10.5194/acp-19-2001-2019
27 citations as recorded by crossref.
- Evaluation of the Oxidation Flow Reactor for particulate matter emission limit certification J. Cao et al. 10.1016/j.atmosenv.2019.117086
- Influence of the NO/NO2 Ratio on Oxidation Product Distributions under High-NO Conditions K. Nihill et al. 10.1021/acs.est.0c07621
- Photochemical transformation of residential wood combustion emissions: dependence of organic aerosol composition on OH exposure A. Hartikainen et al. 10.5194/acp-20-6357-2020
- Modeling the formation and composition of secondary organic aerosol from diesel exhaust using parameterized and semi-explicit chemistry and thermodynamic models S. Eluri et al. 10.5194/acp-18-13813-2018
- Model Evaluation of New Techniques for Maintaining High-NO Conditions in Oxidation Flow Reactors for the Study of OH-Initiated Atmospheric Chemistry Z. Peng et al. 10.1021/acsearthspacechem.7b00070
- Gas-phase composition and secondary organic aerosol formation from standard and particle filter-retrofitted gasoline direct injection vehicles investigated in a batch and flow reactor S. Pieber et al. 10.5194/acp-18-9929-2018
- Radical chemistry in oxidation flow reactors for atmospheric chemistry research Z. Peng & J. Jimenez 10.1039/C9CS00766K
- Nitrate radical generation via continuous generation of dinitrogen pentoxide in a laminar flow reactor coupled to an oxidation flow reactor A. Lambe et al. 10.5194/amt-13-2397-2020
- Changes in PM<sub>2.5</sub> peat combustion source profiles with atmospheric aging in an oxidation flow reactor J. Chow et al. 10.5194/amt-12-5475-2019
- A novel high-volume Photochemical Emission Aging flow tube Reactor (PEAR) M. Ihalainen et al. 10.1080/02786826.2018.1559918
- Mitigation of Secondary Organic Aerosol Formation from Log Wood Burning Emissions by Catalytic Removal of Aromatic Hydrocarbons S. Pieber et al. 10.1021/acs.est.8b04124
- Cyclic Ion Mobility Spectrometry Coupled to High-Resolution Time-of-Flight Mass Spectrometry Equipped with Atmospheric Solid Analysis Probe for the Molecular Characterization of Combustion Particulate Matter C. Rüger et al. 10.1021/jasms.0c00274
- Technical Note: Effect of varying the <i>λ</i> = 185 and 254 nm photon flux ratio on radical generation in oxidation flow reactors J. Rowe et al. 10.5194/acp-20-13417-2020
- Evolution of OH reactivity in NO-free volatile organic compound photooxidation investigated by the fully explicit GECKO-A model Z. Peng et al. 10.5194/acp-21-14649-2021
- HO<sub><i>x</i></sub> and NO<sub><i>x</i></sub> production in oxidation flow reactors via photolysis of isopropyl nitrite, isopropyl nitrite-d<sub>7</sub>, and 1,3-propyl dinitrite at <i>λ</i> = 254, 350, and 369 nm A. Lambe et al. 10.5194/amt-12-299-2019
- OH chemistry of non-methane organic gases (NMOGs) emitted from laboratory and ambient biomass burning smoke: evaluating the influence of furans and oxygenated aromatics on ozone and secondary NMOG formation M. Coggon et al. 10.5194/acp-19-14875-2019
- Comparison of secondary organic aerosol formation from toluene on initially wet and dry ammonium sulfate particles at moderate relative humidity T. Liu et al. 10.5194/acp-18-5677-2018
- Constraining nucleation, condensation, and chemistry in oxidation flow reactors using size-distribution measurements and aerosol microphysical modeling A. Hodshire et al. 10.5194/acp-18-12433-2018
- Exposure of Lung Epithelial Cells to Photochemically Aged Secondary Organic Aerosol Shows Increased Toxic Effects P. Chowdhury et al. 10.1021/acs.estlett.8b00256
- Dynamic changes in optical and chemical properties of tar ball aerosols by atmospheric photochemical aging C. Li et al. 10.5194/acp-19-139-2019
- Impact of photochemical ageing on Polycyclic Aromatic Hydrocarbons (PAH) and oxygenated PAH (Oxy-PAH/OH-PAH) in logwood stove emissions T. Miersch et al. 10.1016/j.scitotenv.2019.05.412
- Photochemical aging and secondary organic aerosols generated from limonene in an oxidation flow reactor S. Sbai & B. Farida 10.1007/s11356-019-05012-5
- Understanding the Impact of High-NOx Conditions on the Formation of Secondary Organic Aerosol in the Photooxidation of Oil Sand-Related Precursors K. Li et al. 10.1021/acs.est.9b05404
- Assessing the degree of plug flow in oxidation flow reactors (OFRs): a study on a potential aerosol mass (PAM) reactor D. Mitroo et al. 10.5194/amt-11-1741-2018
- Organic peroxy radical chemistry in oxidation flow reactors and environmental chambers and their atmospheric relevance Z. Peng et al. 10.5194/acp-19-813-2019
- Secondary Organic Aerosol Formation Potential from Ambient Air in Beijing: Effects of Atmospheric Oxidation Capacity at Different Pollution Levels J. Liu et al. 10.1021/acs.est.1c00890
- Rate constant and secondary organic aerosol formation from the gas-phase reaction of eugenol with hydroxyl radicals C. Liu et al. 10.5194/acp-19-2001-2019
Latest update: 16 Oct 2021
Short summary
Oxidation flow reactors (OFRs) have been increasingly used to study atmospheric chemistry at high NO. We show that it is very difficult to obtain high-NO chemistry (in terms of RO2 fate) in OFRs by initial NO injection. Past OFR studies with combustion sources generally had too-high precursor and NOx concentrations that caused several types of experimental artifacts. A strong dilution (× 100 or larger) may be needed for such experiments to avoid undesired chemistry.
Oxidation flow reactors (OFRs) have been increasingly used to study atmospheric chemistry at...
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