Articles | Volume 17, issue 18
https://doi.org/10.5194/acp-17-11313-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-17-11313-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
25 Sep 2017
Research article |
| 25 Sep 2017
Brominated VSLS and their influence on ozone under a changing climate
Institute of Meteorology and Climate Research, Karlsruhe Institute of Technology, Karlsruhe, Germany
Björn-Martin Sinnhuber
Institute of Meteorology and Climate Research, Karlsruhe Institute of Technology, Karlsruhe, Germany
Gisèle Krysztofiak
LPC2E, Université d'Orléans, CNRS, UMR7328, Orléans, France
Patrick Jöckel
Deutsches Zentrum für Luft- und Raumfahrt e.V., Oberpfaffenhofen, Germany
Phoebe Graf
Deutsches Zentrum für Luft- und Raumfahrt e.V., Oberpfaffenhofen, Germany
Sinikka T. Lennartz
Geomar, Helmholtz Centre for Ocean Research Kiel, Kiel, Germany
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- Bromoform, dibromochloromethane, and dibromomethane over the East China Sea and the western Pacific Ocean: Oceanic emission and spatial variation S. Liu et al. 10.1016/j.chemosphere.2020.127151
21 citations as recorded by crossref.
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- Seasonal impact of biogenic very short-lived bromocarbons on lowermost stratospheric ozone between 60° N and 60° S during the 21st century J. Barrera et al. 10.5194/acp-20-8083-2020
- Very short-lived halogens amplify ozone depletion trends in the tropical lower stratosphere J. Villamayor et al. 10.1038/s41558-023-01671-y
- Bromine from short-lived source gases in the extratropical northern hemispheric upper troposphere and lower stratosphere (UTLS) T. Keber et al. 10.5194/acp-20-4105-2020
- Organic and inorganic bromine measurements around the extratropical tropopause and lowermost stratosphere: insights into the transport pathways and total bromine M. Rotermund et al. 10.5194/acp-21-15375-2021
- A novel, balloon-borne UV–Vis spectrometer for direct sun measurements of stratospheric bromine K. Voss et al. 10.5194/amt-17-4507-2024
- Polar boundary layer bromine explosion and ozone depletion events in the chemistry–climate model EMAC v2.52: implementation and evaluation of AirSnow algorithm S. Falk & B. Sinnhuber 10.5194/gmd-11-1115-2018
- Stratospheric ozone, UV radiation, and climate interactions G. Bernhard et al. 10.1007/s43630-023-00371-y
- On the atmospheric budget of 1,2-dichloroethane and its impact on stratospheric chlorine and ozone (2002–2020) R. Hossaini et al. 10.5194/acp-24-13457-2024
- Photothermal conditions and upwelling enhance very short-lived brominated halocarbons emissions in the western tropical Pacific Ocean J. Ni et al. 10.1016/j.scitotenv.2024.173035
- Natural halogens buffer tropospheric ozone in a changing climate F. Iglesias-Suarez et al. 10.1038/s41558-019-0675-6
- Stratospheric Injection of Brominated Very Short‐Lived Substances: Aircraft Observations in the Western Pacific and Representation in Global Models P. Wales et al. 10.1029/2017JD027978
- Renewed and emerging concerns over the production and emission of ozone-depleting substances M. Chipperfield et al. 10.1038/s43017-020-0048-8
- Phototransformation of Plastic Containing Brominated Flame Retardants: Enhanced Fragmentation and Release of Photoproducts to Water and Air A. Khaled et al. 10.1021/acs.est.8b03172
- Climate change influence on the levels and trends of persistent organic pollutants (POPs) and chemicals of emerging Arctic concern (CEACs) in the Arctic physical environment – a review H. Hung et al. 10.1039/D1EM00485A
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- The Michelson Interferometer for Passive Atmospheric Sounding global climatology of BrONO2 2002–2012: a test for stratospheric bromine chemistry M. Höpfner et al. 10.5194/acp-21-18433-2021
- Bromoform, dibromochloromethane, and dibromomethane over the East China Sea and the western Pacific Ocean: Oceanic emission and spatial variation S. Liu et al. 10.1016/j.chemosphere.2020.127151
Latest update: 29 Jul 2025
Short summary
Brominated very short-lived source gases (VSLS) contribute significantly to the tropospheric and stratospheric bromine loading. We find an increase of future ocean–atmosphere flux of brominated VSLS of 8–10 % compared to present day. A decrease in the tropospheric mixing ratios of VSLS and an increase in the lower stratosphere are attributed to changes in atmospheric chemistry and transport. Bromine impact on stratospheric ozone at the end of the 21st century is reduced compared to present day.
Brominated very short-lived source gases (VSLS) contribute significantly to the tropospheric and...
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