Articles | Volume 16, issue 13
https://doi.org/10.5194/acp-16-8095-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-8095-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
04 Jul 2016
Research article |
| 04 Jul 2016
Evidence for ambient dark aqueous SOA formation in the Po Valley, Italy
Amy P. Sullivan
CORRESPONDING AUTHOR
Colorado State University, Department of Atmospheric Science, Fort
Collins, Colorado 80523, USA
Natasha Hodas
California Institute of Technology, Division of Chemical Engineering,
Pasadena, California 91125, USA
Barbara J. Turpin
Rutgers University, Department of Environmental Sciences, New
Brunswick, New Jersey 08901, USA
Kate Skog
University of Wisconsin – Madison, Department of Chemistry, Madison,
Wisconsin 53706, USA
Frank N. Keutsch
University of Wisconsin – Madison, Department of Chemistry, Madison,
Wisconsin 53706, USA
Harvard University, Department of Chemistry and Chemical Biology,
Cambridge, Massachusetts 02138, USA
Stefania Gilardoni
Istituto di Scienze dell'Atmosfera e del Clima, Consiglio Nazionale
delle Ricerche, 40129 Bologna, Italy
Marco Paglione
Istituto di Scienze dell'Atmosfera e del Clima, Consiglio Nazionale
delle Ricerche, 40129 Bologna, Italy
Matteo Rinaldi
Istituto di Scienze dell'Atmosfera e del Clima, Consiglio Nazionale
delle Ricerche, 40129 Bologna, Italy
Stefano Decesari
Istituto di Scienze dell'Atmosfera e del Clima, Consiglio Nazionale
delle Ricerche, 40129 Bologna, Italy
Maria Cristina Facchini
Istituto di Scienze dell'Atmosfera e del Clima, Consiglio Nazionale
delle Ricerche, 40129 Bologna, Italy
Laurent Poulain
Leibniz Institute for Tropospheric Research, 04318 Leipzig, Germany
Hartmut Herrmann
Leibniz Institute for Tropospheric Research, 04318 Leipzig, Germany
Alfred Wiedensohler
Leibniz Institute for Tropospheric Research, 04318 Leipzig, Germany
Eiko Nemitz
Centre for Ecology and Hydrology, Bush Estate, Penicuik, EH26QB,
UK
Marsailidh M. Twigg
Centre for Ecology and Hydrology, Bush Estate, Penicuik, EH26QB,
UK
Jeffrey L. Collett Jr.
Colorado State University, Department of Atmospheric Science, Fort
Collins, Colorado 80523, USA
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34 citations as recorded by crossref.
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33 citations as recorded by crossref.
- Is there an aerosol signature of chemical cloud processing? B. Ervens et al. 10.5194/acp-18-16099-2018
- Multiple pathways for the formation of secondary organic aerosol in the North China Plain in summer Y. Gu et al. 10.5194/acp-23-5419-2023
- Day-night variability of PM10 components at a Mediterranean urban site during winter N. Galindo et al. 10.1007/s11869-018-0627-8
- Recent advances in understanding secondary organic aerosol: Implications for global climate forcing M. Shrivastava et al. 10.1002/2016RG000540
- Significant Contribution of Primary Sources to Water-Soluble Organic Carbon During Spring in Beijing, China Y. Jin et al. 10.3390/atmos11040395
- Insights into the origin and evolution of carbonaceous aerosols in a mediterranean urban environment N. Galindo et al. 10.1016/j.chemosphere.2019.06.202
- Identifying forecast uncertainties for biogenic gases in the Po Valley related to model configuration in EURAD-IM during PEGASOS 2012 A. Vogel & H. Elbern 10.5194/acp-21-4039-2021
- Dynamics of residential indoor gas- and particle-phase water-soluble organic carbon: measurements during the CASA experiment M. Webb et al. 10.1039/D4EM00340C
- Photochemical Aqueous-Phase Reactions Induce Rapid Daytime Formation of Oxygenated Organic Aerosol on the North China Plain Y. Kuang et al. 10.1021/acs.est.9b06836
- Large contribution of in-cloud production of secondary organic aerosol from biomass burning emissions T. Wang et al. 10.1038/s41612-024-00682-6
- Modeling the partitioning of organic chemical species in cloud phases with CLEPS (1.1) C. Rose et al. 10.5194/acp-18-2225-2018
- Real-time assessment of wintertime organic aerosol characteristics and sources at a suburban site in northern France R. Roig Rodelas et al. 10.1016/j.atmosenv.2019.01.035
- Wintertime characteristics of water-soluble organic carbon in PM2.5 during haze and non-haze days in Jinan in the North China Plain X. Shi et al. 10.1016/j.atmosenv.2023.119985
- Size-resolved aerosol composition at an urban and a rural site in the Po Valley in summertime: implications for secondary aerosol formation S. Sandrini et al. 10.5194/acp-16-10879-2016
- Insights into the formation of secondary organic carbon in the summertime in urban Shanghai C. Zhang et al. 10.1016/j.jes.2017.12.018
- Simulation of atmospheric organic aerosol using its volatility–oxygen-content distribution during the PEGASOS 2012 campaign E. Karnezi et al. 10.5194/acp-18-10759-2018
- Zeppelin-led study on the onset of new particle formation in the planetary boundary layer J. Lampilahti et al. 10.5194/acp-21-12649-2021
- Limononic Acid Oxidation by Hydroxyl Radicals and Ozone in the Aqueous Phase B. Witkowski et al. 10.1021/acs.est.7b04867
- The formation and evolution of secondary organic aerosol during summer in Xi'an: Aqueous phase processing in fog-rain days J. Duan et al. 10.1016/j.scitotenv.2020.144077
- Source profiles and contributions of biofuel combustion for PM2.5, PM10 and their compositions, in a city influenced by biofuel stoves Y. Tian et al. 10.1016/j.chemosphere.2017.09.044
- Tracking the Photomineralization Mechanism in Irradiated Lab-Generated and Field-Collected Brown Carbon Samples and Its Effect on Cloud Condensation Nuclei Abilities S. Müller et al. 10.1021/acsenvironau.2c00055
- Highly time-resolved characterization of carbonaceous aerosols using a two-wavelength Sunset thermal–optical carbon analyzer M. Bao et al. 10.5194/amt-14-4053-2021
- A three-year investigation of daily PM2.5 main chemical components in four sites: the routine measurement program of the Supersito Project (Po Valley, Italy) I. Ricciardelli et al. 10.1016/j.atmosenv.2016.12.052
- The impact of biomass burning and aqueous-phase processing on air quality: a multi-year source apportionment study in the Po Valley, Italy M. Paglione et al. 10.5194/acp-20-1233-2020
- cis-Pinonic Acid Oxidation by Hydroxyl Radicals in the Aqueous Phase under Acidic and Basic Conditions: Kinetics and Mechanism B. Witkowski & T. Gierczak 10.1021/acs.est.7b02427
- Field study of a soft X-ray aerosol neutralizer combined with electrostatic classifiers for nanoparticle size distribution measurements A. Nicosia et al. 10.1016/j.partic.2017.08.001
- Atmospheric “HULIS” in Different Environments: Polarities, Molecular Sizes, and Sources Suggest More Than 50% Are Not “Humic-like” T. Spranger et al. 10.1021/acsearthspacechem.9b00299
- Comparative major components and health risks of toxic elements and polycyclic aromatic hydrocarbons of PM2.5 in winter and summer in Zhengzhou: Based on three-year data N. Jiang et al. 10.1016/j.atmosres.2018.06.008
- Cloud Processing of Secondary Organic Aerosol from Isoprene and Methacrolein Photooxidation C. Giorio et al. 10.1021/acs.jpca.7b05933
- Increasing surface ozone and enhanced secondary organic carbon formation at a city junction site: An epitome of the Yangtze River Delta, China (2014–2017) Y. Liu et al. 10.1016/j.envpol.2020.114847
- Mass Spectrometry Analysis in Atmospheric Chemistry J. Laskin et al. 10.1021/acs.analchem.7b04249
- Seasonal differences in formation processes of oxidized organic aerosol near Houston, TX Q. Dai et al. 10.5194/acp-19-9641-2019
- Uptake of Water‐soluble Gas‐phase Oxidation Products Drives Organic Particulate Pollution in Beijing G. Gkatzelis et al. 10.1029/2020GL091351
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Latest update: 23 Nov 2024
Short summary
This paper presents the results from our measurements and approach for the investigation of aqueous secondary organic aerosol (aqSOA) formation in the ambient atmosphere. When local aqSOA formation was observed, a correlation of water-soluble organic carbon with organic aerosol, aerosol liquid water, relative humidity, and aerosol nitrate was found. Key factors of local aqSOA production include air mass stagnation, formation of local nitrate overnight, and significant amounts of ammonia.
This paper presents the results from our measurements and approach for the investigation of...
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