Articles | Volume 16, issue 8
https://doi.org/10.5194/acp-16-5399-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-5399-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
29 Apr 2016
Research article |
| 29 Apr 2016
Size distribution and mixing state of black carbon particles during a heavy air pollution episode in Shanghai
Xianda Gong
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention,
Department of Environmental Science and Engineering, Fudan University,
Shanghai 200433, China
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention,
Department of Environmental Science and Engineering, Fudan University,
Shanghai 200433, China
Hong Chen
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention,
Department of Environmental Science and Engineering, Fudan University,
Shanghai 200433, China
Sergey A. Nizkorodov
Department of Chemistry, University of California, Irvine, California
92697, USA
Jianmin Chen
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention,
Department of Environmental Science and Engineering, Fudan University,
Shanghai 200433, China
Fudan-Tyndall Center, Fudan University, Shanghai 200433, China
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention,
Department of Environmental Science and Engineering, Fudan University,
Shanghai 200433, China
Fudan-Tyndall Center, Fudan University, Shanghai 200433, China
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Cited
80 citations as recorded by crossref.
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- Real-time physiochemistry of urban aerosols during a regional haze episode by a single-particle aerosol mass spectrometer: Mixing state, size distribution and source apportionment L. Shen et al. 10.1016/j.apr.2020.05.010
- Insights into the formation of secondary organic carbon in the summertime in urban Shanghai C. Zhang et al. 10.1016/j.jes.2017.12.018
- Research on the Attenuation Characteristics of LiDAR Transmission Energy in Different Atmospheric Environments X. Yang et al. 10.3390/atmos16020210
- Size‐resolved measurements of mixing state and cloud‐nucleating ability of aerosols in Nanjing, China Y. Ma et al. 10.1002/2017JD026583
- Size Distributions, Mixing State, and Morphology of Refractory Black Carbon in an Urban Atmosphere of Northeast Asia During Summer S. Lim et al. 10.2139/ssrn.4121032
- Understanding the Origin of Wet Deposition Black Carbon in North America During the Fall Season P. Sricharoenvech et al. 10.3390/environments12020058
- Recent Advances in Quantifying Wet Scavenging Efficiency of Black Carbon Aerosol Y. Yang et al. 10.3390/atmos10040175
- Aerosol optical properties and the mixing state of black carbon at a background mountainous site in Eastern China L. Yuan et al. 10.1016/j.jes.2019.03.013
- Amplification of light absorption of black carbon associated with air pollution Y. Zhang et al. 10.5194/acp-18-9879-2018
- Size distributions, mixing state, and morphology of refractory black carbon in an urban atmosphere of northeast Asia during summer S. Lim et al. 10.1016/j.scitotenv.2022.158436
- Distribution, Sources, and Hazards of Ambient Carbonaceous Particulates in Central India N. Jaiswal et al. 10.1061/(ASCE)HZ.2153-5515.0000447
- Absorption closure in highly aged biomass burning smoke J. Taylor et al. 10.5194/acp-20-11201-2020
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- Seasonal contrast in size distributions and mixing state of black carbon and its association with PM1.0 chemical composition from the eastern coast of India S. Kompalli et al. 10.5194/acp-20-3965-2020
- The characteristics of particulate matter during an air pollution process revealed by joint observation of multiple equipments S. Wang et al. 10.1016/j.apr.2022.101487
- Particle Size and Mixing State of Freshly Emitted Black Carbon from Different Combustion Sources in China Y. Zhang et al. 10.1021/acs.est.9b07373
- Temporal variations in the hygroscopicity and mixing state of black carbon aerosols in a polluted megacity area K. Li et al. 10.5194/acp-18-15201-2018
- Influence of Black Carbon on Measurement Errors in Scattering-Based Visibility Meters Z. Yang et al. 10.3390/atmos16040467
- Existence of Crystalline Ammonium Sulfate Nuclei Affects Chemical Reactivity of Oleic Acid Particles Through Heterogeneous Nucleation W. Liu et al. 10.1029/2023JD038675
- Mixing characteristics of refractory black carbon aerosols at an urban site in Beijing H. Liu et al. 10.5194/acp-20-5771-2020
- Seasonal size distribution and mixing state of black carbon aerosols in a polluted urban environment of the Yangtze River Delta region, China Y. Yang et al. 10.1016/j.scitotenv.2018.11.087
- Quantifying the effects of the microphysical properties of black carbon on the determination of brown carbon using measurements at multiple wavelengths J. Luo et al. 10.5194/acp-24-427-2024
- Moisture-induced secondary inorganic aerosol formation dominated the light absorption enhancement of refractory black carbon at an urban site in northwest China Z. Chen et al. 10.1016/j.atmosenv.2023.120113
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- Significant restructuring and light absorption enhancement of black carbon particles by ammonium nitrate coating C. Yuan et al. 10.1016/j.envpol.2020.114172
- Quantifying black carbon light absorption enhancement with a novel statistical approach C. Wu et al. 10.5194/acp-18-289-2018
- Variations in Black Carbon concentration and sources during COVID-19 lockdown in Delhi V. Goel et al. 10.1016/j.chemosphere.2020.129435
- Characteristics and source apportionment of black carbon aerosol in the North China Plain Z. Yang et al. 10.1016/j.atmosres.2022.106246
- Size distribution and source of black carbon aerosol in urban Beijing during winter haze episodes Y. Wu et al. 10.5194/acp-17-7965-2017
- Optical carbon analysis on Teflon filters from the FRM network in New York O. Rattigan et al. 10.1016/j.apr.2021.101163
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- Sources and vertical distribution of PM2.5 over Shanghai during the winter of 2017 K. Zhang et al. 10.1016/j.scitotenv.2019.135683
- Relationship between Long-range Transport of Ammonia and Ammonium in Wintertime in Suburban Area M. Song et al. 10.5572/KOSAE.2020.36.4.543
- Mixing state of refractory black carbon in fog and haze at rural sites in winter on the North China Plain Y. Zhang et al. 10.5194/acp-21-17631-2021
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- Optimized instrument configurations for tandem particle mass analyzer and single particle-soot photometer experiments A. Naseri et al. 10.1016/j.jaerosci.2021.105897
- Aerodynamic size-resolved composition and cloud condensation nuclei properties of aerosols in a Beijing suburban region C. Yu et al. 10.5194/acp-22-4375-2022
- Chemical Characteristics of Size-Resolved Aerosols in Coastal Areas during KORUS-AQ Campaign; Comparison of Ion Neutralization Model M. Bae et al. 10.1007/s13143-018-00099-1
- Pre-monsoon submicron aerosol composition and source contribution in the Kathmandu Valley, Nepal B. Werden et al. 10.1039/D2EA00008C
- Temporal evolution of submicron particles during extreme fireworks S. Yadav et al. 10.1007/s10661-019-7735-2
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- Submicron Aerosol Composition and Source Contribution across the Kathmandu Valley, Nepal, in Winter B. Werden et al. 10.1021/acsearthspacechem.2c00226
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- Absorption enhancement of black carbon and the contribution of brown carbon to light absorption in the summer of Nanjing, China F. Cui et al. 10.1016/j.apr.2020.12.008
- Size Dependence of the Physical Characteristics of Particles Containing Refractory Black Carbon in Diesel Vehicle Exhaust C. Han et al. 10.1021/acs.est.8b04603
- Impacts of variations in aerosol refractive index on the retrieving of the light-absorption and hygroscopicity of ambient black carbon-containing aerosols using SP2 G. Zhao et al. 10.1016/j.atmosenv.2024.120359
- Perturbation of Background Atmospheric Black Carbon/PM1 Ratio during Firecracker Bursting Episode D. Majumdar & A. Gavane 10.5572/ajae.2017.11.4.322
- Selective capture of PM2.5 by urban trees: The role of leaf wax composition and physiological traits in air quality enhancement D. Chen et al. 10.1016/j.jhazmat.2024.135428
- Enhanced Light Absorption and Radiative Forcing by Black Carbon Agglomerates G. Kelesidis et al. 10.1021/acs.est.2c00428
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- Heterogeneous characteristics and absorption enhancement of refractory black carbon in an urban city of China S. Chen et al. 10.1016/j.scitotenv.2023.162997
- Vertical characteristics of black carbon physical properties over Beijing region in warm and cold seasons D. Zhao et al. 10.1016/j.atmosenv.2019.06.007
- Mixing state of refractory black carbon aerosol in the South Asian outflow over the northern Indian Ocean during winter S. Kompalli et al. 10.5194/acp-21-9173-2021
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- Characterising mass-resolved mixing state of black carbon in Beijing using a morphology-independent measurement method C. Yu et al. 10.5194/acp-20-3645-2020
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- Measurements of nonvolatile size distribution and its link to traffic soot in urban Shanghai S. Jiang et al. 10.1016/j.scitotenv.2017.09.176
- Atmospheric aerosol and black carbon optical properties and associated radiative forcing under haze conditions M. Zhang et al. 10.1016/j.jqsrt.2020.107390
- Analysis of the Effect of Optical Properties of Black Carbon on Ozone in an Urban Environment at the Yangtze River Delta, China J. An et al. 10.1007/s00376-021-0367-9
78 citations as recorded by crossref.
- Size distribution and mixing state of refractory black carbon aerosol from a coastal city in South China Q. Wang et al. 10.1016/j.atmosres.2016.06.022
- Real-time physiochemistry of urban aerosols during a regional haze episode by a single-particle aerosol mass spectrometer: Mixing state, size distribution and source apportionment L. Shen et al. 10.1016/j.apr.2020.05.010
- Insights into the formation of secondary organic carbon in the summertime in urban Shanghai C. Zhang et al. 10.1016/j.jes.2017.12.018
- Research on the Attenuation Characteristics of LiDAR Transmission Energy in Different Atmospheric Environments X. Yang et al. 10.3390/atmos16020210
- Size‐resolved measurements of mixing state and cloud‐nucleating ability of aerosols in Nanjing, China Y. Ma et al. 10.1002/2017JD026583
- Size Distributions, Mixing State, and Morphology of Refractory Black Carbon in an Urban Atmosphere of Northeast Asia During Summer S. Lim et al. 10.2139/ssrn.4121032
- Understanding the Origin of Wet Deposition Black Carbon in North America During the Fall Season P. Sricharoenvech et al. 10.3390/environments12020058
- Recent Advances in Quantifying Wet Scavenging Efficiency of Black Carbon Aerosol Y. Yang et al. 10.3390/atmos10040175
- Aerosol optical properties and the mixing state of black carbon at a background mountainous site in Eastern China L. Yuan et al. 10.1016/j.jes.2019.03.013
- Amplification of light absorption of black carbon associated with air pollution Y. Zhang et al. 10.5194/acp-18-9879-2018
- Size distributions, mixing state, and morphology of refractory black carbon in an urban atmosphere of northeast Asia during summer S. Lim et al. 10.1016/j.scitotenv.2022.158436
- Distribution, Sources, and Hazards of Ambient Carbonaceous Particulates in Central India N. Jaiswal et al. 10.1061/(ASCE)HZ.2153-5515.0000447
- Absorption closure in highly aged biomass burning smoke J. Taylor et al. 10.5194/acp-20-11201-2020
- Speciated online PM1 from South Asian combustion sources – Part 1: Fuel-based emission factors and size distributions J. Goetz et al. 10.5194/acp-18-14653-2018
- Seasonal contrast in size distributions and mixing state of black carbon and its association with PM1.0 chemical composition from the eastern coast of India S. Kompalli et al. 10.5194/acp-20-3965-2020
- The characteristics of particulate matter during an air pollution process revealed by joint observation of multiple equipments S. Wang et al. 10.1016/j.apr.2022.101487
- Particle Size and Mixing State of Freshly Emitted Black Carbon from Different Combustion Sources in China Y. Zhang et al. 10.1021/acs.est.9b07373
- Temporal variations in the hygroscopicity and mixing state of black carbon aerosols in a polluted megacity area K. Li et al. 10.5194/acp-18-15201-2018
- Influence of Black Carbon on Measurement Errors in Scattering-Based Visibility Meters Z. Yang et al. 10.3390/atmos16040467
- Existence of Crystalline Ammonium Sulfate Nuclei Affects Chemical Reactivity of Oleic Acid Particles Through Heterogeneous Nucleation W. Liu et al. 10.1029/2023JD038675
- Mixing characteristics of refractory black carbon aerosols at an urban site in Beijing H. Liu et al. 10.5194/acp-20-5771-2020
- Seasonal size distribution and mixing state of black carbon aerosols in a polluted urban environment of the Yangtze River Delta region, China Y. Yang et al. 10.1016/j.scitotenv.2018.11.087
- Quantifying the effects of the microphysical properties of black carbon on the determination of brown carbon using measurements at multiple wavelengths J. Luo et al. 10.5194/acp-24-427-2024
- Moisture-induced secondary inorganic aerosol formation dominated the light absorption enhancement of refractory black carbon at an urban site in northwest China Z. Chen et al. 10.1016/j.atmosenv.2023.120113
- Relationships between fixed-site ambient measurements of nitrogen dioxide, ozone, and particulate matter and personal exposures in Grand Paris, France: the MobiliSense study S. Bista et al. 10.1186/s12942-025-00393-y
- Significant restructuring and light absorption enhancement of black carbon particles by ammonium nitrate coating C. Yuan et al. 10.1016/j.envpol.2020.114172
- Quantifying black carbon light absorption enhancement with a novel statistical approach C. Wu et al. 10.5194/acp-18-289-2018
- Variations in Black Carbon concentration and sources during COVID-19 lockdown in Delhi V. Goel et al. 10.1016/j.chemosphere.2020.129435
- Characteristics and source apportionment of black carbon aerosol in the North China Plain Z. Yang et al. 10.1016/j.atmosres.2022.106246
- Size distribution and source of black carbon aerosol in urban Beijing during winter haze episodes Y. Wu et al. 10.5194/acp-17-7965-2017
- Optical carbon analysis on Teflon filters from the FRM network in New York O. Rattigan et al. 10.1016/j.apr.2021.101163
- Black Carbon over Wuhan, China: Seasonal Variations in Its Optical Properties, Radiative Forcing and Contribution to Atmospheric Aerosols Y. Ma et al. 10.3390/rs13183620
- Black carbon emissions in the rural Indian households: Sources, exposure, and associated threats A. Hussain et al. 10.1002/gj.4775
- Measurements to determine the mixing state of black carbon emitted from the 2017–2018 California wildfires and urban Los Angeles J. Ko et al. 10.5194/acp-20-15635-2020
- Vertical Distributions of Refractory Black Carbon over the Yellow Sea during the Spring 2020 Y. Kang et al. 10.5572/KOSAE.2021.37.5.710
- Sources and vertical distribution of PM2.5 over Shanghai during the winter of 2017 K. Zhang et al. 10.1016/j.scitotenv.2019.135683
- Relationship between Long-range Transport of Ammonia and Ammonium in Wintertime in Suburban Area M. Song et al. 10.5572/KOSAE.2020.36.4.543
- Mixing state of refractory black carbon in fog and haze at rural sites in winter on the North China Plain Y. Zhang et al. 10.5194/acp-21-17631-2021
- Metrological traceability of black carbon measurement based on optical methods and its challenges in China: A review Y. Liu et al. 10.1016/j.atmosres.2023.106854
- Effect of source variation on the size and mixing state of black carbon aerosol in urban Beijing from 2013 to 2019: Implication on light absorption Y. Wu et al. 10.1016/j.envpol.2020.116089
- Characteristics and Sources of Black Carbon Aerosol in a Mega-City in the Western Yangtze River Delta, China J. Li et al. 10.3390/atmos11040315
- The Simulated Source Apportionment of Light Absorbing Aerosols: Effects of Microphysical Properties of Partially‐Coated Black Carbon J. Luo et al. 10.1029/2022JD037291
- Mixing state and light absorption enhancement of black carbon aerosols in summertime Nanjing, China Y. Ma et al. 10.1016/j.atmosenv.2019.117141
- A Major Combustion Aerosol Event Had a Negligible Impact on the Atmospheric Ice‐Nucleating Particle Population M. Adams et al. 10.1029/2020JD032938
- Influence of Emissions and Aqueous Processing on Particles Containing Black Carbon in a Polluted Urban Environment: Insights From a Soot Particle‐Aerosol Mass Spectrometer S. Collier et al. 10.1002/2017JD027851
- Contrasting mixing state of black carbon-containing particles in summer and winter in Beijing C. Xie et al. 10.1016/j.envpol.2020.114455
- Chemical properties, sources and size-resolved hygroscopicity of submicron black-carbon-containing aerosols in urban Shanghai S. Cui et al. 10.5194/acp-22-8073-2022
- Optimized instrument configurations for tandem particle mass analyzer and single particle-soot photometer experiments A. Naseri et al. 10.1016/j.jaerosci.2021.105897
- Aerodynamic size-resolved composition and cloud condensation nuclei properties of aerosols in a Beijing suburban region C. Yu et al. 10.5194/acp-22-4375-2022
- Chemical Characteristics of Size-Resolved Aerosols in Coastal Areas during KORUS-AQ Campaign; Comparison of Ion Neutralization Model M. Bae et al. 10.1007/s13143-018-00099-1
- Pre-monsoon submicron aerosol composition and source contribution in the Kathmandu Valley, Nepal B. Werden et al. 10.1039/D2EA00008C
- Temporal evolution of submicron particles during extreme fireworks S. Yadav et al. 10.1007/s10661-019-7735-2
- Black carbon aerosols over urban and high altitude remote regions: Characteristics and radiative implications T. Rajesh & S. Ramachandran 10.1016/j.atmosenv.2018.09.023
- Ice‐Nucleating Particle Concentrations and Sources in Rainwater Over the Third Pole, Tibetan Plateau J. Chen et al. 10.1029/2020JD033864
- Sensitivity of black carbon concentrations and climate impact to aging and scavenging in OsloCTM2–M7 M. Lund et al. 10.5194/acp-17-6003-2017
- Characteristics and Source Apportionment of Black Carbon in the North China Plain Z. Yang et al. 10.2139/ssrn.4052416
- Deposition of ambient particles in the human respiratory system based on single particle analysis: A case study in the Pearl River Delta, China S. Jia et al. 10.1016/j.envpol.2021.117056
- Submicron Aerosol Composition and Source Contribution across the Kathmandu Valley, Nepal, in Winter B. Werden et al. 10.1021/acsearthspacechem.2c00226
- The spatio-temporal evolution of black carbon in the North-West European ‘air pollution hotspot’ K. Wyche et al. 10.1016/j.atmosenv.2020.117874
- Personal exposure to concentrations and inhalation of black carbon according to transport mode use: The MobiliSense sensor-based study S. Bista et al. 10.1016/j.envint.2021.106990
- Atmospheric black carbon aerosol: Long-term characteristics, source apportionment, and trends T. Rajesh & S. Ramachandran 10.1016/j.scitotenv.2024.172928
- Absorption enhancement of black carbon and the contribution of brown carbon to light absorption in the summer of Nanjing, China F. Cui et al. 10.1016/j.apr.2020.12.008
- Size Dependence of the Physical Characteristics of Particles Containing Refractory Black Carbon in Diesel Vehicle Exhaust C. Han et al. 10.1021/acs.est.8b04603
- Impacts of variations in aerosol refractive index on the retrieving of the light-absorption and hygroscopicity of ambient black carbon-containing aerosols using SP2 G. Zhao et al. 10.1016/j.atmosenv.2024.120359
- Perturbation of Background Atmospheric Black Carbon/PM1 Ratio during Firecracker Bursting Episode D. Majumdar & A. Gavane 10.5572/ajae.2017.11.4.322
- Selective capture of PM2.5 by urban trees: The role of leaf wax composition and physiological traits in air quality enhancement D. Chen et al. 10.1016/j.jhazmat.2024.135428
- Enhanced Light Absorption and Radiative Forcing by Black Carbon Agglomerates G. Kelesidis et al. 10.1021/acs.est.2c00428
- Role of black carbon mass size distribution in the direct aerosol radiative forcing G. Zhao et al. 10.5194/acp-19-13175-2019
- Enhanced mixing state of black carbon with nitrate in single particles during haze periods in Zhengzhou, China Q. Zhou et al. 10.1016/j.jes.2021.03.031
- Emission characteristics of refractory black carbon aerosols from fresh biomass burning: a perspective from laboratory experiments X. Pan et al. 10.5194/acp-17-13001-2017
- Technical note: Mismeasurement of the core-shell structure of black carbon-containing ambient aerosols by SP2 measurements G. Zhao et al. 10.1016/j.atmosenv.2020.117885
- Heterogeneous characteristics and absorption enhancement of refractory black carbon in an urban city of China S. Chen et al. 10.1016/j.scitotenv.2023.162997
- Vertical characteristics of black carbon physical properties over Beijing region in warm and cold seasons D. Zhao et al. 10.1016/j.atmosenv.2019.06.007
- Mixing state of refractory black carbon aerosol in the South Asian outflow over the northern Indian Ocean during winter S. Kompalli et al. 10.5194/acp-21-9173-2021
- Internally mixed black carbon in the Indo-Gangetic Plain and its effect on absorption enhancement N. Thamban et al. 10.1016/j.atmosres.2017.07.007
- Characterising mass-resolved mixing state of black carbon in Beijing using a morphology-independent measurement method C. Yu et al. 10.5194/acp-20-3645-2020
- Characterizing Black Carbon and Gaseous Pollutants on the Yangtze River Across Eastern China Continent Y. Ting et al. 10.1029/2020JD033488
- Measurements of nonvolatile size distribution and its link to traffic soot in urban Shanghai S. Jiang et al. 10.1016/j.scitotenv.2017.09.176
2 citations as recorded by crossref.
- Atmospheric aerosol and black carbon optical properties and associated radiative forcing under haze conditions M. Zhang et al. 10.1016/j.jqsrt.2020.107390
- Analysis of the Effect of Optical Properties of Black Carbon on Ozone in an Urban Environment at the Yangtze River Delta, China J. An et al. 10.1007/s00376-021-0367-9
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Short summary
In this study, we used a Single Particle Aerosol Mass Spectrometer and a Single Particle Soot Photometer to investigate the chemical and physical properties of black carbon (BC) aerosols during a regional air pollution episode in urban Shanghai. BC containing particles were mainly attributed to biomass burning and traffic emissions. We observed a group of highly aged traffic emitted particles with a relatively small BC core (~ 60–80 nm) and a very thick absolute coating thickness (~ 130–300 nm).
In this study, we used a Single Particle Aerosol Mass Spectrometer and a Single Particle Soot...
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