Articles | Volume 16, issue 6
https://doi.org/10.5194/acp-16-4081-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-4081-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Understanding sources of organic aerosol during CalNex-2010 using the CMAQ-VBS
Matthew C. Woody
U.S. Environmental Protection Agency, Research Triangle Park, NC, USA
Kirk R. Baker
U.S. Environmental Protection Agency, Research Triangle Park, NC, USA
Patrick L. Hayes
Université de Montréal, Department of Chemistry, Montreal, QC, Canada
Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado, Boulder, CO, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder, CO, USA
Jose L. Jimenez
Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado, Boulder, CO, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder, CO, USA
Bonyoung Koo
Ramboll Environ International Corporation, Novato, CA, USA
U.S. Environmental Protection Agency, Research Triangle Park, NC, USA
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Cited
80 citations as recorded by crossref.
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- Airborne and ground-based observations of ammonium-nitrate-dominated aerosols in a shallow boundary layer during intense winter pollution episodes in northern Utah A. Franchin et al. 10.5194/acp-18-17259-2018
- Status and quality evaluation of precursor emission inventories for PM<sub>2.5</sub> and ozone in China Z. Huang et al. 10.1360/TB-2021-0783
- A method to predict PM 2.5 resulting from compliance with national ambient air quality standards J. Kelly et al. 10.1016/j.atmosenv.2017.05.009
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- Toxicological effects of fresh and aged gasoline exhaust particles in Hong Kong Y. Lau et al. 10.1016/j.jhazmat.2022.129846
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- Simulating secondary organic aerosol in a regional air quality model using the statistical oxidation model – Part 3: Assessing the influence of semi-volatile and intermediate-volatility organic compounds and NO<sub><i>x</i></sub> A. Akherati et al. 10.5194/acp-19-4561-2019
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- Chemical transport model simulations of organic aerosol in southern California: model evaluation and gasoline and diesel source contributions S. Jathar et al. 10.5194/acp-17-4305-2017
- Emissions of intermediate-volatility and semi-volatile organic compounds from domestic fuels used in Delhi, India G. Stewart et al. 10.5194/acp-21-2407-2021
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- Machine Learning-Based Integration of High-Resolution Wildfire Smoke Simulations and Observations for Regional Health Impact Assessment Y. Zou et al. 10.3390/ijerph16122137
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- Influence of Oil and Gas End-Use on Summertime Particulate Matter and Ozone Pollution in the Eastern US K. Vohra et al. 10.1021/acs.est.4c10032
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- Quantification of the sources and composition of particulate matter by field-deployable mass spectrometry: implications for air quality and public health P. Hayes 10.1039/C6AN02378A
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- Contribution of regional-scale fire events to ozone and PM2.5 air quality estimated by photochemical modeling approaches K. Baker et al. 10.1016/j.atmosenv.2016.06.032
- Simulation of organic aerosol formation during the CalNex study: updated mobile emissions and secondary organic aerosol parameterization for intermediate-volatility organic compounds Q. Lu et al. 10.5194/acp-20-4313-2020
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- Novel Approach for Evaluating Secondary Organic Aerosol from Aromatic Hydrocarbons: Unified Method for Predicting Aerosol Composition and Formation L. Li et al. 10.1021/acs.est.5b05778
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- The influence of ocean halogen and sulfur emissions in the air quality of a coastal megacity: The case of Los Angeles M. Muñiz-Unamunzaga et al. 10.1016/j.scitotenv.2017.06.098
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80 citations as recorded by crossref.
- Contribution of Organic Nitrates to Organic Aerosol over South Korea during KORUS-AQ H. Kenagy et al. 10.1021/acs.est.1c05521
- Evaluation of Secondary Organic Aerosol (SOA) Simulations for Seoul, Korea Y. Oak et al. 10.1029/2021MS002760
- Evaluation of European air quality modelled by CAMx including the volatility basis set scheme G. Ciarelli et al. 10.5194/acp-16-10313-2016
- Criteria pollutant impacts of volatile chemical products informed by near-field modelling M. Qin et al. 10.1038/s41893-020-00614-1
- EURODELTA III exercise: An evaluation of air quality models’ capacity to reproduce the carbonaceous aerosol M. Mircea et al. 10.1016/j.aeaoa.2019.100018
- Evaluating SOA formation from different sources of semi- and intermediate-volatility organic compounds from the Athabasca oil sands J. Sommers et al. 10.1039/D1EA00053E
- Multidecadal Analysis of Meteorological and Emissions Regimes for PM2.5 Across California D. Quevedo et al. 10.1021/acsestair.3c00019
- Volatile Chemical Product Enhancements to Criteria Pollutants in the United States K. Seltzer et al. 10.1021/acs.est.1c04298
- Air pollutant exposure field modeling using air quality model-data fusion methods and comparison with satellite AOD-derived fields: application over North Carolina, USA R. Huang et al. 10.1007/s11869-017-0511-y
- Investigation of factors controlling PM2.5 variability across the South Korean Peninsula during KORUS-AQ C. Jordan et al. 10.1525/elementa.424
- Impacts of water partitioning and polarity of organic compounds on secondary organic aerosol over eastern China J. Li et al. 10.5194/acp-20-7291-2020
- Airborne and ground-based observations of ammonium-nitrate-dominated aerosols in a shallow boundary layer during intense winter pollution episodes in northern Utah A. Franchin et al. 10.5194/acp-18-17259-2018
- Status and quality evaluation of precursor emission inventories for PM<sub>2.5</sub> and ozone in China Z. Huang et al. 10.1360/TB-2021-0783
- A method to predict PM 2.5 resulting from compliance with national ambient air quality standards J. Kelly et al. 10.1016/j.atmosenv.2017.05.009
- Sensitivity of northeastern US surface ozone predictions to the representation of atmospheric chemistry in the Community Regional Atmospheric Chemistry Multiphase Mechanism (CRACMMv1.0) B. Place et al. 10.5194/acp-23-9173-2023
- Improvement in Modeling of OH and HO2 Radical Concentrations during Toluene and Xylene Oxidation with RACM2 Using MCM/GECKO-A V. Lannuque et al. 10.3390/atmos12060732
- Description and evaluation of the Community Multiscale Air Quality (CMAQ) modeling system version 5.1 K. Appel et al. 10.5194/gmd-10-1703-2017
- Semivolatile POA and parameterized total combustion SOA in CMAQv5.2: impacts on source strength and partitioning B. Murphy et al. 10.5194/acp-17-11107-2017
- Chemical transport models often underestimate inorganic aerosol acidity in remote regions of the atmosphere B. Nault et al. 10.1038/s43247-021-00164-0
- Strong influence of deposition and vertical mixing on secondary organic aerosol concentrations in CMAQ and CAMx Q. Shu et al. 10.1016/j.atmosenv.2017.10.035
- Secondary organic aerosols from anthropogenic volatile organic compounds contribute substantially to air pollution mortality B. Nault et al. 10.5194/acp-21-11201-2021
- Influence of semi- and intermediate-volatile organic compounds (S/IVOC) parameterizations, volatility distributions and aging schemes on organic aerosol modelling in winter conditions P. Giani et al. 10.1016/j.atmosenv.2019.05.061
- Assessment of the effects of straw burning bans in China: Emissions, air quality, and health impacts L. Huang et al. 10.1016/j.scitotenv.2021.147935
- Secondary organic aerosol production from local emissions dominates the organic aerosol budget over Seoul, South Korea, during KORUS-AQ B. Nault et al. 10.5194/acp-18-17769-2018
- Atmospheric Chemistry in a Box or a Bag G. Hidy 10.3390/atmos10070401
- Estimating the Contribution of Local Primary Emissions to Particulate Pollution Using High‐Density Station Observations C. Zhao et al. 10.1029/2018JD028888
- Toxicological effects of fresh and aged gasoline exhaust particles in Hong Kong Y. Lau et al. 10.1016/j.jhazmat.2022.129846
- Modelling winter organic aerosol at the European scale with CAMx: evaluation and source apportionment with a VBS parameterization based on novel wood burning smog chamber experiments G. Ciarelli et al. 10.5194/acp-17-7653-2017
- Simulating secondary organic aerosol in a regional air quality model using the statistical oxidation model – Part 3: Assessing the influence of semi-volatile and intermediate-volatility organic compounds and NO<sub><i>x</i></sub> A. Akherati et al. 10.5194/acp-19-4561-2019
- Full-volatility emission framework corrects missing and underestimated secondary organic aerosol sources X. Chang et al. 10.1016/j.oneear.2022.03.015
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- Process-based and observation-constrained SOA simulations in China: the role of semivolatile and intermediate-volatility organic compounds and OH levels R. Miao et al. 10.5194/acp-21-16183-2021
- Prediction of secondary organic aerosol from the multiphase reaction of gasoline vapor by using volatility–reactivity base lumping S. Han & M. Jang 10.5194/acp-22-625-2022
- Simulations of Organic Aerosol with CAMx over the Po Valley during the Summer Season B. Basla et al. 10.3390/atmos13121996
- Modeling organic aerosol over Europe in summer conditions with the VBS-GECKO parameterization: sensitivity to secondary organic compound properties and IVOC (intermediate-volatility organic compound) emissions V. Lannuque et al. 10.5194/acp-20-4905-2020
- Impacts of shipping emissions on PM<sub>2.5</sub> pollution in China Z. Lv et al. 10.5194/acp-18-15811-2018
- Reactive organic carbon air emissions from mobile sources in the United States B. Murphy et al. 10.5194/acp-23-13469-2023
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- Contrast in Secondary Organic Aerosols between the Present Day and the Preindustrial Period: The Importance of Nontraditional Sources and the Changed Atmospheric Oxidation Capability Y. Yang et al. 10.1007/s00376-024-3281-0
- Comprehensive organic emission profiles, secondary organic aerosol production potential, and OH reactivity of domestic fuel combustion in Delhi, India G. Stewart et al. 10.1039/D0EA00009D
- Modeling of wintertime regional formation of secondary organic aerosols around Beijing: sensitivity analysis and anthropogenic contributions Y. Zhang et al. 10.1007/s44246-023-00040-w
- The impact of US wildland fires on ozone and particulate matter: a comparison of measurements and CMAQ model predictions from 2008 to 2012 J. Wilkins et al. 10.1071/WF18053
- Modeling organic aerosol concentrations and properties during winter 2014 in the northwestern Mediterranean region M. Chrit et al. 10.5194/acp-18-18079-2018
- Impact of wildfires on particulate matter in the Euro-Mediterranean in 2007: sensitivity to some parameterizations of emissions in air quality models M. Majdi et al. 10.5194/acp-19-785-2019
- Detailed Inventory of the Evaporative Emissions from Parked Gasoline Vehicles and an Evaluation of Their Atmospheric Impact in Japan H. Hata et al. 10.1021/acs.est.9b06539
- Larger Submicron Particles for Emissions With Residential Burning in Wintertime San Joaquin Valley (Fresno) than for Vehicle Combustion in Summertime South Coast Air Basin (Fontana) R. Betha et al. 10.1029/2017JD026730
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- Emissions of intermediate-volatility and semi-volatile organic compounds from domestic fuels used in Delhi, India G. Stewart et al. 10.5194/acp-21-2407-2021
- Comparative Assessment of Cooking Emission Contributions to Urban Organic Aerosol Using Online Molecular Tracers and Aerosol Mass Spectrometry Measurements D. Huang et al. 10.1021/acs.est.1c03280
- Machine Learning-Based Integration of High-Resolution Wildfire Smoke Simulations and Observations for Regional Health Impact Assessment Y. Zou et al. 10.3390/ijerph16122137
- Sources of organic aerosols in Europe: a modeling study using CAMx with modified volatility basis set scheme J. Jiang et al. 10.5194/acp-19-15247-2019
- Influence of Oil and Gas End-Use on Summertime Particulate Matter and Ozone Pollution in the Eastern US K. Vohra et al. 10.1021/acs.est.4c10032
- Assessing Model Characterization of Single Source Secondary Pollutant Impacts Using 2013 SENEX Field Study Measurements K. Baker & M. Woody 10.1021/acs.est.6b05069
- Source–Receptor Relationship Revealed by the Halted Traffic and Aggravated Haze in Beijing during the COVID-19 Lockdown Z. Lv et al. 10.1021/acs.est.0c04941
- Origin of Fine Particulate Carbon in the Rural United States B. Schichtel et al. 10.1021/acs.est.7b00645
- Linking gas, particulate, and toxic endpoints to air emissions in the Community Regional Atmospheric Chemistry Multiphase Mechanism (CRACMM) H. Pye et al. 10.5194/acp-23-5043-2023
- Modeling Secondary Organic Aerosols in China: State of the Art and Perspectives J. Li et al. 10.1007/s40726-022-00246-3
- Emission of intermediate, semi and low volatile organic compounds from traffic and their impact on secondary organic aerosol concentrations over Greater Paris K. Sartelet et al. 10.1016/j.atmosenv.2018.02.031
- Characterization of organic aerosol across the global remote troposphere: a comparison of ATom measurements and global chemistry models A. Hodzic et al. 10.5194/acp-20-4607-2020
- Quantification of the sources and composition of particulate matter by field-deployable mass spectrometry: implications for air quality and public health P. Hayes 10.1039/C6AN02378A
- Improving spatial surrogates for area source emissions inventories in California Y. Li et al. 10.1016/j.atmosenv.2020.117665
- Contribution of regional-scale fire events to ozone and PM2.5 air quality estimated by photochemical modeling approaches K. Baker et al. 10.1016/j.atmosenv.2016.06.032
- Simulation of organic aerosol formation during the CalNex study: updated mobile emissions and secondary organic aerosol parameterization for intermediate-volatility organic compounds Q. Lu et al. 10.5194/acp-20-4313-2020
- Comprehensive organic emission profiles for gasoline, diesel, and gas-turbine engines including intermediate and semi-volatile organic compound emissions Q. Lu et al. 10.5194/acp-18-17637-2018
- Modeling secondary organic aerosol formation from volatile chemical products E. Pennington et al. 10.5194/acp-21-18247-2021
- Contribution of Particulate Nitrate Photolysis to Heterogeneous Sulfate Formation for Winter Haze in China H. Zheng et al. 10.1021/acs.estlett.0c00368
- Regional modeling of secondary organic aerosol formation over eastern China: The impact of uptake coefficients of dicarbonyls and semivolatile process of primary organic aerosol X. Chen et al. 10.1016/j.scitotenv.2021.148176
- Novel Approach for Evaluating Secondary Organic Aerosol from Aromatic Hydrocarbons: Unified Method for Predicting Aerosol Composition and Formation L. Li et al. 10.1021/acs.est.5b05778
- Evaluating the impact of new observational constraints on P-S/IVOC emissions, multi-generation oxidation, and chamber wall losses on SOA modeling for Los Angeles, CA P. Ma et al. 10.5194/acp-17-9237-2017
- SSH-Aerosol v1.1: A Modular Box Model to Simulate the Evolution of Primary and Secondary Aerosols K. Sartelet et al. 10.3390/atmos11050525
- Comprehensive chemical characterization of gaseous I/SVOC emissions from heavy-duty diesel vehicles using two-dimensional gas chromatography time-of-flight mass spectrometry X. He et al. 10.1016/j.envpol.2022.119284
- Sources and atmospheric processing of winter aerosols in Seoul, Korea: insights from real-time measurements using a high-resolution aerosol mass spectrometer H. Kim et al. 10.5194/acp-17-2009-2017
- Reactive organic carbon emissions from volatile chemical products K. Seltzer et al. 10.5194/acp-21-5079-2021
- Evaluating wildfire emissions projection methods in comparisons of simulated and observed air quality U. Shankar et al. 10.5194/acp-19-15157-2019
- Impact of Fire Emissions on U.S. Air Quality from 1997 to 2016–A Modeling Study in the Satellite Era Z. Tao et al. 10.3390/rs12060913
- Influence of biomass burning vapor wall loss correction on modeling organic aerosols in Europe by CAMx v6.50 J. Jiang et al. 10.5194/gmd-14-1681-2021
- Secondary organic aerosol formation in China from urban-lifestyle sources: Vehicle exhaust and cooking emission Z. Zhang et al. 10.1016/j.scitotenv.2022.159340
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Short summary
In this work, organic aerosol (OA) predictions from the volatility basis set (VBS) module in the CMAQ photochemical transport model were evaluated against routine monitoring data and measurements collected during the 2010 CalNex field study. We found that the VBS module more accurately reproduced the observed primary/secondary OA split and secondary OA (SOA) mass at the CalNex Pasadena ground site compared to the traditional CMAQ OA module but still underpredicted observed SOA by ~ 5.2 ×.
In this work, organic aerosol (OA) predictions from the volatility basis set (VBS) module in the...
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