Articles | Volume 16, issue 4
https://doi.org/10.5194/acp-16-2309-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-2309-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
26 Feb 2016
Research article |
| 26 Feb 2016
Simulating secondary organic aerosol in a regional air quality model using the statistical oxidation model – Part 1: Assessing the influence of constrained multi-generational ageing
S. H. Jathar
Mechanical Engineering, Colorado State University, Fort Collins CO, USA
Civil and Environmental Engineering, University of California, Davis CA, USA
Civil and Environmental Engineering, University of California, Davis CA, USA
A. S. Wexler
Civil and Environmental Engineering, University of California, Davis CA, USA
J. H. Seinfeld
Chemical Engineering, California Institute of Technology, Pasadena CA, USA
M. J. Kleeman
CORRESPONDING AUTHOR
Civil and Environmental Engineering, University of California, Davis CA, USA
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Cited
30 citations as recorded by crossref.
- A computationally efficient model to represent the chemistry, thermodynamics, and microphysics of secondary organic aerosols (simpleSOM): model development and application to α-pinene SOA S. Jathar et al. 10.1039/D1EA00014D
- Semivolatile POA and parameterized total combustion SOA in CMAQv5.2: impacts on source strength and partitioning B. Murphy et al. 10.5194/acp-17-11107-2017
- Secondary organic aerosol formation from evaporated biofuels: comparison to gasoline and correction for vapor wall losses Y. He et al. 10.1039/D0EM00103A
- Evaluating Organic Aerosol Sources and Evolution with a Combined Molecular Composition and Volatility Framework Using the Filter Inlet for Gases and Aerosols (FIGAERO) J. Thornton et al. 10.1021/acs.accounts.0c00259
- Rethinking the global secondary organic aerosol (SOA) budget: stronger production, faster removal, shorter lifetime A. Hodzic et al. 10.5194/acp-16-7917-2016
- Simulating secondary organic aerosol from anthropogenic and biogenic precursors: comparison to outdoor chamber experiments, effect of oligomerization on SOA formation and reactive uptake of aldehydes F. Couvidat et al. 10.5194/acp-18-15743-2018
- Simulating secondary organic aerosol in a regional air quality model using the statistical oxidation model – Part 3: Assessing the influence of semi-volatile and intermediate-volatility organic compounds and NOx A. Akherati et al. 10.5194/acp-19-4561-2019
- Air pollutant exposure field modeling using air quality model-data fusion methods and comparison with satellite AOD-derived fields: application over North Carolina, USA R. Huang et al. 10.1007/s11869-017-0511-y
- Secondary organic aerosol and ozone formation from photo-oxidation of unburned diesel fuel in a surrogate atmospheric environment W. Li & D. Cocker 10.1016/j.atmosenv.2018.03.059
- Simulating secondary organic aerosol in a regional air quality model using the statistical oxidation model – Part 2: Assessing the influence of vapor wall losses C. Cappa et al. 10.5194/acp-16-3041-2016
- Measurement report: Bio-physicochemistry of tropical clouds at Maïdo (Réunion, Indian Ocean): overview of results from the BIO-MAÏDO campaign M. Leriche et al. 10.5194/acp-24-4129-2024
- Chemical transport model simulations of organic aerosol in southern California: model evaluation and gasoline and diesel source contributions S. Jathar et al. 10.5194/acp-17-4305-2017
- Modeling the formation and composition of secondary organic aerosol from diesel exhaust using parameterized and semi-explicit chemistry and thermodynamic models S. Eluri et al. 10.5194/acp-18-13813-2018
- Dilution and photooxidation driven processes explain the evolution of organic aerosol in wildfire plumes A. Akherati et al. 10.1039/D1EA00082A
- Molecular composition and volatility of isoprene photochemical oxidation secondary organic aerosol under low- and high-NOx conditions E. D'Ambro et al. 10.5194/acp-17-159-2017
- Simulated sensitivity of secondary organic aerosol in the South Coast Air Basin of California to nitrogen oxides and other chemical parameters R. Griffin et al. 10.1080/02786826.2018.1446507
- Simulation of SOA formation from the photooxidation of monoalkylbenzenes in the presence of aqueous aerosols containing electrolytes under various NOx levels C. Zhou et al. 10.5194/acp-19-5719-2019
- A comprehensive evaluation of enhanced temperature influence on gas and aerosol chemistry in the lamp-enclosed oxidation flow reactor (OFR) system T. Pan et al. 10.5194/amt-17-4915-2024
- Comprehensive Assessment for the Impacts of S/IVOC Emissions from Mobile Sources on SOA Formation in China J. Zhao et al. 10.1021/acs.est.2c07265
- A Scheme for Representing Aromatic Secondary Organic Aerosols in Chemical Transport Models: Application to Source Attribution of Organic Aerosols Over South Korea During the KORUS‐AQ Campaign J. Brewer et al. 10.1029/2022JD037257
- Parameterized Yields of Semivolatile Products from Isoprene Oxidation under Different NOx Levels: Impacts of Chemical Aging and Wall-Loss of Reactive Gases L. Xing et al. 10.1021/acs.est.8b00373
- Ozonolysis of α-phellandrene – Part 1: Gas- and particle-phase characterisation F. Mackenzie-Rae et al. 10.5194/acp-17-6583-2017
- Exploring Volatility Properties of Discrete Secondary Organic Aerosol Constituents of α-Pinene and Polycyclic Aromatic Hydrocarbons Z. Babar et al. 10.1021/acsearthspacechem.0c00210
- Influence of semi- and intermediate-volatile organic compounds (S/IVOC) parameterizations, volatility distributions and aging schemes on organic aerosol modelling in winter conditions P. Giani et al. 10.1016/j.atmosenv.2019.05.061
- Oxygenated Aromatic Compounds are Important Precursors of Secondary Organic Aerosol in Biomass-Burning Emissions A. Akherati et al. 10.1021/acs.est.0c01345
- Modeling biogenic secondary organic aerosol (BSOA) formation from monoterpene reactions with NO3: A case study of the SOAS campaign using CMAQ M. Qin et al. 10.1016/j.atmosenv.2018.03.042
- Anthropogenic Effects on Biogenic Secondary Organic Aerosol Formation L. Xu et al. 10.1007/s00376-020-0284-3
- The effects of isoprene and NOx on secondary organic aerosols formed through reversible and irreversible uptake to aerosol water M. El-Sayed et al. 10.5194/acp-18-1171-2018
- Mass accommodation and gas–particle partitioning in secondary organic aerosols: dependence on diffusivity, volatility, particle-phase reactions, and penetration depth M. Shiraiwa & U. Pöschl 10.5194/acp-21-1565-2021
- Quantifying the effect of organic aerosol aging and intermediate-volatility emissions on regional-scale aerosol pollution in China B. Zhao et al. 10.1038/srep28815
29 citations as recorded by crossref.
- A computationally efficient model to represent the chemistry, thermodynamics, and microphysics of secondary organic aerosols (simpleSOM): model development and application to α-pinene SOA S. Jathar et al. 10.1039/D1EA00014D
- Semivolatile POA and parameterized total combustion SOA in CMAQv5.2: impacts on source strength and partitioning B. Murphy et al. 10.5194/acp-17-11107-2017
- Secondary organic aerosol formation from evaporated biofuels: comparison to gasoline and correction for vapor wall losses Y. He et al. 10.1039/D0EM00103A
- Evaluating Organic Aerosol Sources and Evolution with a Combined Molecular Composition and Volatility Framework Using the Filter Inlet for Gases and Aerosols (FIGAERO) J. Thornton et al. 10.1021/acs.accounts.0c00259
- Rethinking the global secondary organic aerosol (SOA) budget: stronger production, faster removal, shorter lifetime A. Hodzic et al. 10.5194/acp-16-7917-2016
- Simulating secondary organic aerosol from anthropogenic and biogenic precursors: comparison to outdoor chamber experiments, effect of oligomerization on SOA formation and reactive uptake of aldehydes F. Couvidat et al. 10.5194/acp-18-15743-2018
- Simulating secondary organic aerosol in a regional air quality model using the statistical oxidation model – Part 3: Assessing the influence of semi-volatile and intermediate-volatility organic compounds and NOx A. Akherati et al. 10.5194/acp-19-4561-2019
- Air pollutant exposure field modeling using air quality model-data fusion methods and comparison with satellite AOD-derived fields: application over North Carolina, USA R. Huang et al. 10.1007/s11869-017-0511-y
- Secondary organic aerosol and ozone formation from photo-oxidation of unburned diesel fuel in a surrogate atmospheric environment W. Li & D. Cocker 10.1016/j.atmosenv.2018.03.059
- Simulating secondary organic aerosol in a regional air quality model using the statistical oxidation model – Part 2: Assessing the influence of vapor wall losses C. Cappa et al. 10.5194/acp-16-3041-2016
- Measurement report: Bio-physicochemistry of tropical clouds at Maïdo (Réunion, Indian Ocean): overview of results from the BIO-MAÏDO campaign M. Leriche et al. 10.5194/acp-24-4129-2024
- Chemical transport model simulations of organic aerosol in southern California: model evaluation and gasoline and diesel source contributions S. Jathar et al. 10.5194/acp-17-4305-2017
- Modeling the formation and composition of secondary organic aerosol from diesel exhaust using parameterized and semi-explicit chemistry and thermodynamic models S. Eluri et al. 10.5194/acp-18-13813-2018
- Dilution and photooxidation driven processes explain the evolution of organic aerosol in wildfire plumes A. Akherati et al. 10.1039/D1EA00082A
- Molecular composition and volatility of isoprene photochemical oxidation secondary organic aerosol under low- and high-NOx conditions E. D'Ambro et al. 10.5194/acp-17-159-2017
- Simulated sensitivity of secondary organic aerosol in the South Coast Air Basin of California to nitrogen oxides and other chemical parameters R. Griffin et al. 10.1080/02786826.2018.1446507
- Simulation of SOA formation from the photooxidation of monoalkylbenzenes in the presence of aqueous aerosols containing electrolytes under various NOx levels C. Zhou et al. 10.5194/acp-19-5719-2019
- A comprehensive evaluation of enhanced temperature influence on gas and aerosol chemistry in the lamp-enclosed oxidation flow reactor (OFR) system T. Pan et al. 10.5194/amt-17-4915-2024
- Comprehensive Assessment for the Impacts of S/IVOC Emissions from Mobile Sources on SOA Formation in China J. Zhao et al. 10.1021/acs.est.2c07265
- A Scheme for Representing Aromatic Secondary Organic Aerosols in Chemical Transport Models: Application to Source Attribution of Organic Aerosols Over South Korea During the KORUS‐AQ Campaign J. Brewer et al. 10.1029/2022JD037257
- Parameterized Yields of Semivolatile Products from Isoprene Oxidation under Different NOx Levels: Impacts of Chemical Aging and Wall-Loss of Reactive Gases L. Xing et al. 10.1021/acs.est.8b00373
- Ozonolysis of α-phellandrene – Part 1: Gas- and particle-phase characterisation F. Mackenzie-Rae et al. 10.5194/acp-17-6583-2017
- Exploring Volatility Properties of Discrete Secondary Organic Aerosol Constituents of α-Pinene and Polycyclic Aromatic Hydrocarbons Z. Babar et al. 10.1021/acsearthspacechem.0c00210
- Influence of semi- and intermediate-volatile organic compounds (S/IVOC) parameterizations, volatility distributions and aging schemes on organic aerosol modelling in winter conditions P. Giani et al. 10.1016/j.atmosenv.2019.05.061
- Oxygenated Aromatic Compounds are Important Precursors of Secondary Organic Aerosol in Biomass-Burning Emissions A. Akherati et al. 10.1021/acs.est.0c01345
- Modeling biogenic secondary organic aerosol (BSOA) formation from monoterpene reactions with NO3: A case study of the SOAS campaign using CMAQ M. Qin et al. 10.1016/j.atmosenv.2018.03.042
- Anthropogenic Effects on Biogenic Secondary Organic Aerosol Formation L. Xu et al. 10.1007/s00376-020-0284-3
- The effects of isoprene and NOx on secondary organic aerosols formed through reversible and irreversible uptake to aerosol water M. El-Sayed et al. 10.5194/acp-18-1171-2018
- Mass accommodation and gas–particle partitioning in secondary organic aerosols: dependence on diffusivity, volatility, particle-phase reactions, and penetration depth M. Shiraiwa & U. Pöschl 10.5194/acp-21-1565-2021
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Short summary
Multi-generational chemistry schemes applied in regional models do not increase secondary organic aerosol (SOA) mass production relative to traditional "two-product" schemes when both models are fitted to the same chamber data. The multi-generational chemistry schemes do change the predicted composition of SOA and the source attribution of SOA.
Multi-generational chemistry schemes applied in regional models do not increase secondary...
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