Articles | Volume 16, issue 4
https://doi.org/10.5194/acp-16-2083-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-2083-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
24 Feb 2016
Research article |
| 24 Feb 2016
Analysis of isothermal and cooling-rate-dependent immersion freezing by a unifying stochastic ice nucleation model
Peter A. Alpert
CORRESPONDING AUTHOR
Institute for Terrestrial and Planetary Atmospheres/School of
Marine and Atmospheric Sciences, Stony Brook University, Stony Brook,
NY 11794-5000, USA
now at: Institut de Recherches sur la Catalyse
et l'Environnement de Lyon, Centre National de la Recherche Scientifique,
Université Claude Bernard Lyon 1, 69626 Villeurbanne, France
Daniel A. Knopf
CORRESPONDING AUTHOR
Institute for Terrestrial and Planetary Atmospheres/School of
Marine and Atmospheric Sciences, Stony Brook University, Stony Brook,
NY 11794-5000, USA
Viewed
Total article views: 3,671 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 05 May 2015)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 2,135 | 1,379 | 157 | 3,671 | 394 | 113 | 126 |
- HTML: 2,135
- PDF: 1,379
- XML: 157
- Total: 3,671
- Supplement: 394
- BibTeX: 113
- EndNote: 126
Total article views: 2,956 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 24 Feb 2016)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 1,776 | 1,081 | 99 | 2,956 | 394 | 88 | 95 |
- HTML: 1,776
- PDF: 1,081
- XML: 99
- Total: 2,956
- Supplement: 394
- BibTeX: 88
- EndNote: 95
Total article views: 715 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 05 May 2015)
| HTML | XML | Total | BibTeX | EndNote | |
|---|---|---|---|---|---|
| 359 | 298 | 58 | 715 | 25 | 31 |
- HTML: 359
- PDF: 298
- XML: 58
- Total: 715
- BibTeX: 25
- EndNote: 31
Cited
46 citations as recorded by crossref.
- Atmospheric ice nucleation D. Knopf & P. Alpert 10.1038/s42254-023-00570-7
- Modeling of Aircraft Measurements of Ice Crystal Concentration in the Arctic and a Parameterization for Mixed-Phase Cloud S. Fan et al. 10.1175/JAS-D-17-0037.1
- Analysis of the Failure Modes in the Polymer Electrolyte Fuel Cell Cold-Start Process—Anode Dehydration or Cathode Pore Blockage L. Yao et al. 10.3390/en13010256
- Bias‐Free Estimation of Ice Nucleation Efficiencies D. Barahona 10.1029/2019GL086033
- Micro-spectroscopic and freezing characterization of ice-nucleating particles collected in the marine boundary layer in the eastern North Atlantic D. Knopf et al. 10.5194/acp-22-5377-2022
- Decreased dust particles amplify the cloud cooling effect by regulating cloud ice formation over the Tibetan Plateau J. Chen et al. 10.1126/sciadv.ado0885
- Stochastic nucleation processes and substrate abundance explain time-dependent freezing in supercooled droplets D. Knopf et al. 10.1038/s41612-020-0106-4
- Diverse sources and aging change the mixing state and ice nucleation properties of aerosol particles over the western Pacific and Southern Ocean J. Xue et al. 10.5194/acp-24-7731-2024
- Interfacial supercooling and the precipitation of hydrohalite in frozen NaCl solutions as seen by X-ray absorption spectroscopy T. Bartels-Rausch et al. 10.5194/tc-15-2001-2021
- The Role of Secondary Ice Processes in Midlatitude Continental Clouds A. Zipori et al. 10.1029/2018JD029146
- Time dependence of heterogeneous ice nucleation by ambient aerosols: laboratory observations and a formulation for models J. Jakobsson et al. 10.5194/acp-22-6717-2022
- Ice-nucleating agents in sea spray aerosol identified and quantified with a holistic multimodal freezing model P. Alpert et al. 10.1126/sciadv.abq6842
- A universally applicable method of calculating confidence bands for ice nucleation spectra derived from droplet freezing experiments W. Fahy et al. 10.5194/amt-15-6819-2022
- Classical nucleation theory of immersion freezing: sensitivity of contact angle schemes to thermodynamic and kinetic parameters L. Ickes et al. 10.5194/acp-17-1713-2017
- Physicochemical characterization of free troposphere and marine boundary layer ice-nucleating particles collected by aircraft in the eastern North Atlantic D. Knopf et al. 10.5194/acp-23-8659-2023
- Not all feldspars are equal: a survey of ice nucleating properties across the feldspar group of minerals A. Harrison et al. 10.5194/acp-16-10927-2016
- Measurements of Immersion Freezing and Heterogeneous Chemistry of Atmospherically Relevant Single Particles with Micro-Raman Spectroscopy L. Mael et al. 10.1021/acs.analchem.9b01819
- HUB: a method to model and extract the distribution of ice nucleation temperatures from drop-freezing experiments I. de Almeida Ribeiro et al. 10.5194/acp-23-5623-2023
- Thermodynamics Explains How Solution Composition Affects the Kinetics of Stochastic Ice Nucleation L. Deck et al. 10.1021/acs.jpclett.3c01371
- Tropospheric and stratospheric wildfire smoke profiling with lidar: mass, surface area, CCN, and INP retrieval A. Ansmann et al. 10.5194/acp-21-9779-2021
- Aerosol Composition, Mixing State, and Phase State of Free Tropospheric Particles and Their Role in Ice Cloud Formation N. Lata et al. 10.1021/acsearthspacechem.1c00315
- Optical trapping and light scattering in atmospheric aerosol science A. Rafferty et al. 10.1039/D2CP05301B
- Refreeze experiments with water droplets containing different types of ice nuclei interpreted by classical nucleation theory L. Kaufmann et al. 10.5194/acp-17-3525-2017
- Long-term variability in immersion-mode marine ice-nucleating particles from climate model simulations and observations A. Raman et al. 10.5194/acp-23-5735-2023
- Single particle characteristics and ice nucleation potential of particles collected during Asian dust storms in 2021 L. Zhao et al. 10.1016/j.scitotenv.2024.174829
- Toward Improved Cloud-Phase Simulation with a Mineral Dust and Temperature-Dependent Parameterization for Ice Nucleation in Mixed-Phase Clouds S. Fan et al. 10.1175/JAS-D-18-0287.1
- Ice cloud formation potential by free tropospheric particles from long‐range transport over the Northern Atlantic Ocean S. China et al. 10.1002/2016JD025817
- Microscopic mechanism of the interaction between water and formic acid-sodium chloride aerosol C. Zhang et al. 10.1016/j.powtec.2018.11.105
- Comparative study on immersion freezing utilizing single-droplet levitation methods M. Szakáll et al. 10.5194/acp-21-3289-2021
- Development of Heterogeneous Ice Nucleation Rate Coefficient Parameterizations From Ambient Measurements G. Cornwell et al. 10.1029/2021GL095359
- Faster Nucleation of Ice at the Three-Phase Contact Line: Influence of Interfacial Chemistry A. Kar et al. 10.1021/acs.langmuir.1c02044
- Study of the Immersion Freezing Theory Using the Classical Nucleation Framework M. Lazaridis 10.3390/atmos13111812
- Bioaerosols are the dominant source of warm-temperature immersion-mode INPs and drive uncertainties in INP predictability G. Cornwell et al. 10.1126/sciadv.adg3715
- Effect of particle surface area on ice active site densities retrieved from droplet freezing spectra H. Beydoun et al. 10.5194/acp-16-13359-2016
- Modeling homogeneous ice nucleation from drop-freezing experiments: impact of droplet volume dispersion and cooling rates R. Addula et al. 10.5194/acp-24-10833-2024
- Ice nucleation imaged with X-ray spectro-microscopy P. Alpert et al. 10.1039/D1EA00077B
- Sensitivity of ice nucleation parameterizations to the variability in underlying ice nucleation rate coefficients I. Steinke & S. Burrows 10.1039/D2EA00019A
- The Role of Organic Aerosol in Atmospheric Ice Nucleation: A Review D. Knopf et al. 10.1021/acsearthspacechem.7b00120
- New developments in PySDM and PySDM-examples v2: collisional breakup, immersion freezing, dry aerosol initialization, and adaptive time-stepping E. de Jong et al. 10.21105/joss.04968
- Marine and terrestrial influences on ice nucleating particles during continuous springtime measurements in an Arctic oilfield location J. Creamean et al. 10.5194/acp-18-18023-2018
- Ice‐Nucleating Particles That Impact Clouds and Climate: Observational and Modeling Research Needs S. Burrows et al. 10.1029/2021RG000745
- Annual cycle of aerosol properties over the central Arctic during MOSAiC 2019–2020 – light-extinction, CCN, and INP levels from the boundary layer to the tropopause A. Ansmann et al. 10.5194/acp-23-12821-2023
- Direct observation of ice nucleation events on individual atmospheric particles B. Wang et al. 10.1039/C6CP05253C
- A 1D Model for Nucleation of Ice From Aerosol Particles: An Application to a Mixed‐Phase Arctic Stratus Cloud Layer D. Knopf et al. 10.1029/2023MS003663
- Surface fractal dimension, water adsorption efficiency and cloud nucleation activity of insoluble aerosol A. Laaksonen et al. 10.1038/srep25504
- Engulfment Avalanches and Thermal Hysteresis for Antifreeze Proteins on Supercooled Ice H. Farag & B. Peters 10.1021/acs.jpcb.3c01089
46 citations as recorded by crossref.
- Atmospheric ice nucleation D. Knopf & P. Alpert 10.1038/s42254-023-00570-7
- Modeling of Aircraft Measurements of Ice Crystal Concentration in the Arctic and a Parameterization for Mixed-Phase Cloud S. Fan et al. 10.1175/JAS-D-17-0037.1
- Analysis of the Failure Modes in the Polymer Electrolyte Fuel Cell Cold-Start Process—Anode Dehydration or Cathode Pore Blockage L. Yao et al. 10.3390/en13010256
- Bias‐Free Estimation of Ice Nucleation Efficiencies D. Barahona 10.1029/2019GL086033
- Micro-spectroscopic and freezing characterization of ice-nucleating particles collected in the marine boundary layer in the eastern North Atlantic D. Knopf et al. 10.5194/acp-22-5377-2022
- Decreased dust particles amplify the cloud cooling effect by regulating cloud ice formation over the Tibetan Plateau J. Chen et al. 10.1126/sciadv.ado0885
- Stochastic nucleation processes and substrate abundance explain time-dependent freezing in supercooled droplets D. Knopf et al. 10.1038/s41612-020-0106-4
- Diverse sources and aging change the mixing state and ice nucleation properties of aerosol particles over the western Pacific and Southern Ocean J. Xue et al. 10.5194/acp-24-7731-2024
- Interfacial supercooling and the precipitation of hydrohalite in frozen NaCl solutions as seen by X-ray absorption spectroscopy T. Bartels-Rausch et al. 10.5194/tc-15-2001-2021
- The Role of Secondary Ice Processes in Midlatitude Continental Clouds A. Zipori et al. 10.1029/2018JD029146
- Time dependence of heterogeneous ice nucleation by ambient aerosols: laboratory observations and a formulation for models J. Jakobsson et al. 10.5194/acp-22-6717-2022
- Ice-nucleating agents in sea spray aerosol identified and quantified with a holistic multimodal freezing model P. Alpert et al. 10.1126/sciadv.abq6842
- A universally applicable method of calculating confidence bands for ice nucleation spectra derived from droplet freezing experiments W. Fahy et al. 10.5194/amt-15-6819-2022
- Classical nucleation theory of immersion freezing: sensitivity of contact angle schemes to thermodynamic and kinetic parameters L. Ickes et al. 10.5194/acp-17-1713-2017
- Physicochemical characterization of free troposphere and marine boundary layer ice-nucleating particles collected by aircraft in the eastern North Atlantic D. Knopf et al. 10.5194/acp-23-8659-2023
- Not all feldspars are equal: a survey of ice nucleating properties across the feldspar group of minerals A. Harrison et al. 10.5194/acp-16-10927-2016
- Measurements of Immersion Freezing and Heterogeneous Chemistry of Atmospherically Relevant Single Particles with Micro-Raman Spectroscopy L. Mael et al. 10.1021/acs.analchem.9b01819
- HUB: a method to model and extract the distribution of ice nucleation temperatures from drop-freezing experiments I. de Almeida Ribeiro et al. 10.5194/acp-23-5623-2023
- Thermodynamics Explains How Solution Composition Affects the Kinetics of Stochastic Ice Nucleation L. Deck et al. 10.1021/acs.jpclett.3c01371
- Tropospheric and stratospheric wildfire smoke profiling with lidar: mass, surface area, CCN, and INP retrieval A. Ansmann et al. 10.5194/acp-21-9779-2021
- Aerosol Composition, Mixing State, and Phase State of Free Tropospheric Particles and Their Role in Ice Cloud Formation N. Lata et al. 10.1021/acsearthspacechem.1c00315
- Optical trapping and light scattering in atmospheric aerosol science A. Rafferty et al. 10.1039/D2CP05301B
- Refreeze experiments with water droplets containing different types of ice nuclei interpreted by classical nucleation theory L. Kaufmann et al. 10.5194/acp-17-3525-2017
- Long-term variability in immersion-mode marine ice-nucleating particles from climate model simulations and observations A. Raman et al. 10.5194/acp-23-5735-2023
- Single particle characteristics and ice nucleation potential of particles collected during Asian dust storms in 2021 L. Zhao et al. 10.1016/j.scitotenv.2024.174829
- Toward Improved Cloud-Phase Simulation with a Mineral Dust and Temperature-Dependent Parameterization for Ice Nucleation in Mixed-Phase Clouds S. Fan et al. 10.1175/JAS-D-18-0287.1
- Ice cloud formation potential by free tropospheric particles from long‐range transport over the Northern Atlantic Ocean S. China et al. 10.1002/2016JD025817
- Microscopic mechanism of the interaction between water and formic acid-sodium chloride aerosol C. Zhang et al. 10.1016/j.powtec.2018.11.105
- Comparative study on immersion freezing utilizing single-droplet levitation methods M. Szakáll et al. 10.5194/acp-21-3289-2021
- Development of Heterogeneous Ice Nucleation Rate Coefficient Parameterizations From Ambient Measurements G. Cornwell et al. 10.1029/2021GL095359
- Faster Nucleation of Ice at the Three-Phase Contact Line: Influence of Interfacial Chemistry A. Kar et al. 10.1021/acs.langmuir.1c02044
- Study of the Immersion Freezing Theory Using the Classical Nucleation Framework M. Lazaridis 10.3390/atmos13111812
- Bioaerosols are the dominant source of warm-temperature immersion-mode INPs and drive uncertainties in INP predictability G. Cornwell et al. 10.1126/sciadv.adg3715
- Effect of particle surface area on ice active site densities retrieved from droplet freezing spectra H. Beydoun et al. 10.5194/acp-16-13359-2016
- Modeling homogeneous ice nucleation from drop-freezing experiments: impact of droplet volume dispersion and cooling rates R. Addula et al. 10.5194/acp-24-10833-2024
- Ice nucleation imaged with X-ray spectro-microscopy P. Alpert et al. 10.1039/D1EA00077B
- Sensitivity of ice nucleation parameterizations to the variability in underlying ice nucleation rate coefficients I. Steinke & S. Burrows 10.1039/D2EA00019A
- The Role of Organic Aerosol in Atmospheric Ice Nucleation: A Review D. Knopf et al. 10.1021/acsearthspacechem.7b00120
- New developments in PySDM and PySDM-examples v2: collisional breakup, immersion freezing, dry aerosol initialization, and adaptive time-stepping E. de Jong et al. 10.21105/joss.04968
- Marine and terrestrial influences on ice nucleating particles during continuous springtime measurements in an Arctic oilfield location J. Creamean et al. 10.5194/acp-18-18023-2018
- Ice‐Nucleating Particles That Impact Clouds and Climate: Observational and Modeling Research Needs S. Burrows et al. 10.1029/2021RG000745
- Annual cycle of aerosol properties over the central Arctic during MOSAiC 2019–2020 – light-extinction, CCN, and INP levels from the boundary layer to the tropopause A. Ansmann et al. 10.5194/acp-23-12821-2023
- Direct observation of ice nucleation events on individual atmospheric particles B. Wang et al. 10.1039/C6CP05253C
- A 1D Model for Nucleation of Ice From Aerosol Particles: An Application to a Mixed‐Phase Arctic Stratus Cloud Layer D. Knopf et al. 10.1029/2023MS003663
- Surface fractal dimension, water adsorption efficiency and cloud nucleation activity of insoluble aerosol A. Laaksonen et al. 10.1038/srep25504
- Engulfment Avalanches and Thermal Hysteresis for Antifreeze Proteins on Supercooled Ice H. Farag & B. Peters 10.1021/acs.jpcb.3c01089
Saved (preprint)
Latest update: 21 Nov 2024
Short summary
A stochastic immersion freezing model is introduced capable of reproducing laboratory data for a variety of experimental methods using a time and surface area dependent ice nucleation process. The assumption that droplets contain identical surface area is evaluated. A quantitative uncertainty analysis of the laboratory observed freezing process is presented. Our results imply that ice nuclei surface area assumptions are crucial for interpretation of experimental immersion freezing results.
A stochastic immersion freezing model is introduced capable of reproducing laboratory data for a...
Altmetrics
Final-revised paper
Preprint