Impacts of heterogeneous uptake of dinitrogen pentoxide and chlorine activation on ozone and reactive nitrogen partitioning: improvement and application of the WRF-Chem model in southern China

Li, Qinyi; Zhang, Li; Wang, Tao; Tham, Yee Jun; Ahmadov, Ravan; Xue, Likun; Zhang, Qiang; Zheng, Junyu

doi:https://doi.org/10.5194/acp-16-14875-2016

Articles | Volume 16, issue 23

https://doi.org/10.5194/acp-16-14875-2016

© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.

Special issue:

The community version of the Weather Research and Forecasting...

https://doi.org/10.5194/acp-16-14875-2016

© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.

Articles | Volume 16, issue 23

Research article

|

01 Dec 2016

Research article |

| 01 Dec 2016

Impacts of heterogeneous uptake of dinitrogen pentoxide and chlorine activation on ozone and reactive nitrogen partitioning: improvement and application of the WRF-Chem model in southern China

Qinyi Li, Li Zhang, Tao Wang, Yee Jun Tham, Ravan Ahmadov, Likun Xue, Qiang Zhang, and Junyu Zheng

Viewed

Total article views: 4,738 (including HTML, PDF, and XML)

HTML	PDF	XML	Total	Supplement	BibTeX	EndNote
2,939	1,644	155	4,738	640	144	223

HTML: 2,939
PDF: 1,644
XML: 155
Total: 4,738
Supplement: 640
BibTeX: 144
EndNote: 223

Views and downloads (calculated since 01 Jun 2016)

Month	HTML	PDF	XML	Total
Jun 2016	111	44	1	156
Jul 2016	19	7	0	26
Aug 2016	11	4	2	17
Sep 2016	14	1	0	15
Oct 2016	8	8	5	21
Nov 2016	6	3	7	16
Dec 2016	105	67	1	173
Jan 2017	28	32	2	62
Feb 2017	23	31	3	57
Mar 2017	28	33	3	64
Apr 2017	38	26	4	68
May 2017	40	25	4	69
Jun 2017	34	15	7	56
Jul 2017	26	17	0	43
Aug 2017	24	18	2	44
Sep 2017	15	12	3	30
Oct 2017	25	21	2	48
Nov 2017	11	20	2	33
Dec 2017	19	16	0	35
Jan 2018	12	13	1	26
Feb 2018	14	9	1	24
Mar 2018	19	20	1	40
Apr 2018	19	18	0	37
May 2018	14	19	0	33
Jun 2018	18	13	0	31
Jul 2018	15	14	1	30
Aug 2018	20	12	1	33
Sep 2018	18	14	0	32
Oct 2018	15	14	2	31
Nov 2018	27	22	0	49
Dec 2018	14	9	1	24
Jan 2019	8	15	2	25
Feb 2019	11	9	1	21
Mar 2019	11	21	0	32
Apr 2019	19	9	0	28
May 2019	15	13	0	28
Jun 2019	14	10	0	24
Jul 2019	12	11	0	23
Aug 2019	12	11	0	23
Sep 2019	11	9	1	21
Oct 2019	10	9	1	20
Nov 2019	7	14	0	21
Dec 2019	9	9	0	18
Jan 2020	10	10	0	20
Feb 2020	15	7	1	23
Mar 2020	7	4	1	12
Apr 2020	10	14	0	24
May 2020	9	7	2	18
Jun 2020	20	16	0	36
Jul 2020	17	22	4	43
Aug 2020	16	20	2	38
Sep 2020	14	7	3	24
Oct 2020	16	12	1	29
Nov 2020	16	12	2	30
Dec 2020	15	14	0	29
Jan 2021	24	14	1	39
Feb 2021	19	13	0	32
Mar 2021	23	12	2	37
Apr 2021	15	14	0	29
May 2021	17	14	2	33
Jun 2021	5	4	0	9
Jul 2021	14	13	0	27
Aug 2021	13	13	0	26
Sep 2021	17	9	1	27
Oct 2021	17	40	1	58
Nov 2021	33	41	0	74
Dec 2021	31	16	1	48
Jan 2022	17	13	1	31
Feb 2022	34	14	1	49
Mar 2022	33	26	0	59
Apr 2022	25	15	1	41
May 2022	26	14	0	40
Jun 2022	30	14	0	44
Jul 2022	27	10	1	38
Aug 2022	29	8	0	37
Sep 2022	22	10	1	33
Oct 2022	20	5	1	26
Nov 2022	35	7	0	42
Dec 2022	16	11	1	28
Jan 2023	16	10	0	26
Feb 2023	24	12	0	36
Mar 2023	27	19	0	46
Apr 2023	10	8	0	18
May 2023	43	13	0	56
Jun 2023	63	9	2	74
Jul 2023	50	13	1	64
Aug 2023	42	13	3	58
Sep 2023	55	15	1	71
Oct 2023	58	17	4	79
Nov 2023	42	7	0	49
Dec 2023	48	13	2	63
Jan 2024	57	11	1	69
Feb 2024	46	9	0	55
Mar 2024	59	16	2	77
Apr 2024	53	15	3	71
May 2024	34	19	4	57
Jun 2024	29	8	2	39
Jul 2024	31	19	4	54
Aug 2024	40	14	8	62
Sep 2024	19	11	5	35
Oct 2024	39	6	1	46
Nov 2024	11	3	2	16
Dec 2024	24	5	1	30
Jan 2025	28	6	2	36
Feb 2025	37	9	6	52
Mar 2025	29	17	0	46
Apr 2025	24	17	1	42
May 2025	27	6	0	33
Jun 2025	63	8	2	73
Jul 2025	27	15	2	44
Aug 2025	55	20	0	75
Sep 2025	46	17	4	67
Oct 2025	37	29	0	66
Nov 2025	10	3	0	13

Cumulative views and downloads (calculated since 01 Jun 2016)

Month	HTML	PDF	XML	Total
Jun 2016	111	44	1	156
Jul 2016	19	7	0	26
Aug 2016	11	4	2	17
Sep 2016	14	1	0	15
Oct 2016	8	8	5	21
Nov 2016	6	3	7	16
Dec 2016	105	67	1	173
Jan 2017	28	32	2	62
Feb 2017	23	31	3	57
Mar 2017	28	33	3	64
Apr 2017	38	26	4	68
May 2017	40	25	4	69
Jun 2017	34	15	7	56
Jul 2017	26	17	0	43
Aug 2017	24	18	2	44
Sep 2017	15	12	3	30
Oct 2017	25	21	2	48
Nov 2017	11	20	2	33
Dec 2017	19	16	0	35
Jan 2018	12	13	1	26
Feb 2018	14	9	1	24
Mar 2018	19	20	1	40
Apr 2018	19	18	0	37
May 2018	14	19	0	33
Jun 2018	18	13	0	31
Jul 2018	15	14	1	30
Aug 2018	20	12	1	33
Sep 2018	18	14	0	32
Oct 2018	15	14	2	31
Nov 2018	27	22	0	49
Dec 2018	14	9	1	24
Jan 2019	8	15	2	25
Feb 2019	11	9	1	21
Mar 2019	11	21	0	32
Apr 2019	19	9	0	28
May 2019	15	13	0	28
Jun 2019	14	10	0	24
Jul 2019	12	11	0	23
Aug 2019	12	11	0	23
Sep 2019	11	9	1	21
Oct 2019	10	9	1	20
Nov 2019	7	14	0	21
Dec 2019	9	9	0	18
Jan 2020	10	10	0	20
Feb 2020	15	7	1	23
Mar 2020	7	4	1	12
Apr 2020	10	14	0	24
May 2020	9	7	2	18
Jun 2020	20	16	0	36
Jul 2020	17	22	4	43
Aug 2020	16	20	2	38
Sep 2020	14	7	3	24
Oct 2020	16	12	1	29
Nov 2020	16	12	2	30
Dec 2020	15	14	0	29
Jan 2021	24	14	1	39
Feb 2021	19	13	0	32
Mar 2021	23	12	2	37
Apr 2021	15	14	0	29
May 2021	17	14	2	33
Jun 2021	5	4	0	9
Jul 2021	14	13	0	27
Aug 2021	13	13	0	26
Sep 2021	17	9	1	27
Oct 2021	17	40	1	58
Nov 2021	33	41	0	74
Dec 2021	31	16	1	48
Jan 2022	17	13	1	31
Feb 2022	34	14	1	49
Mar 2022	33	26	0	59
Apr 2022	25	15	1	41
May 2022	26	14	0	40
Jun 2022	30	14	0	44
Jul 2022	27	10	1	38
Aug 2022	29	8	0	37
Sep 2022	22	10	1	33
Oct 2022	20	5	1	26
Nov 2022	35	7	0	42
Dec 2022	16	11	1	28
Jan 2023	16	10	0	26
Feb 2023	24	12	0	36
Mar 2023	27	19	0	46
Apr 2023	10	8	0	18
May 2023	43	13	0	56
Jun 2023	63	9	2	74
Jul 2023	50	13	1	64
Aug 2023	42	13	3	58
Sep 2023	55	15	1	71
Oct 2023	58	17	4	79
Nov 2023	42	7	0	49
Dec 2023	48	13	2	63
Jan 2024	57	11	1	69
Feb 2024	46	9	0	55
Mar 2024	59	16	2	77
Apr 2024	53	15	3	71
May 2024	34	19	4	57
Jun 2024	29	8	2	39
Jul 2024	31	19	4	54
Aug 2024	40	14	8	62
Sep 2024	19	11	5	35
Oct 2024	39	6	1	46
Nov 2024	11	3	2	16
Dec 2024	24	5	1	30
Jan 2025	28	6	2	36
Feb 2025	37	9	6	52
Mar 2025	29	17	0	46
Apr 2025	24	17	1	42
May 2025	27	6	0	33
Jun 2025	63	8	2	73
Jul 2025	27	15	2	44
Aug 2025	55	20	0	75
Sep 2025	46	17	4	67
Oct 2025	37	29	0	66
Nov 2025	10	3	0	13

Latest update: 07 Nov 2025

Download

Article (9846 KB)
Full-text XML

Short summary

The regional distributions and impacts of N₂O₅ and ClNO₂ remain poorly understood. To address the problem, we developed a chemical transport model further and conducted the first high-resolution simulation of the distributions of the two species. Our research demonstrated the significant impacts of the two gases on the lifetime of nitrogen oxides, secondary nitrate production and ozone formation in southern China and highlighted the necessity of considering this chemistry in air quality models.