Research article 23 Nov 2016
Research article | 23 Nov 2016
Detection of atmospheric gaseous amines and amides by a high-resolution time-of-flight chemical ionization mass spectrometer with protonated ethanol reagent ions
Lei Yao et al.
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Cited
50 citations as recorded by crossref.
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- Probing key organic substances driving new particle growth initiated by iodine nucleation in coastal atmosphere Y. Wan et al. 10.5194/acp-20-9821-2020
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- Determination of atmospheric alkylamines by ion chromatography using 18-crown-6 as mobile phase additive S. Zhou et al. 10.1016/j.chroma.2018.05.074
- High-resolution modeling of gaseous methylamines over a polluted region in China: source-dependent emissions and implications of spatial variations J. Mao et al. 10.5194/acp-18-7933-2018
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- Indoor acids and bases W. Nazaroff & C. Weschler 10.1111/ina.12670
- Atmospheric Sulfuric Acid‐Dimethylamine Nucleation Enhanced by Trifluoroacetic Acid Y. Lu et al. 10.1029/2019GL085627
- A density functional theory study of the molecular interactions between a series of amides and sulfuric acid X. Ma et al. 10.1016/j.chemosphere.2018.08.152
- Integrated experimental and theoretical approach to probe the synergistic effect of ammonia in methanesulfonic acid reactions with small alkylamines V. Perraud et al. 10.1039/C9EM00431A
- Autoxidation mechanism for atmospheric oxidation of tertiary amines: Implications for secondary organic aerosol formation F. Ma et al. 10.1016/j.chemosphere.2020.129207
- A dual-emitting Tb(iii)&Yb(iii)-functionalized coordination polymer: a “turn-on” sensor forN-methylformamide in urine and a “turn-off” sensor for methylglyoxal in serum X. Zheng et al. 10.1039/C9DT02643F
- Computational Study of the Reactions of Chlorine Radicals with Atmospheric Organic Compounds Featuring NHx–π-Bond (x = 1, 2) Structures H. Xie et al. 10.1021/acs.jpca.6b11418
- New Particle Formation and Growth Mechanisms in Highly Polluted Environments H. Yu et al. 10.1007/s40726-017-0067-3
- Detection of gaseous dimethylamine using vocus proton-transfer-reaction time-of-flight mass spectrometry Y. Wang et al. 10.1016/j.atmosenv.2020.117875
- Atmospheric new particle formation in China B. Chu et al. 10.5194/acp-19-115-2019
- Kinetic Understanding of the Ultrahigh Ionization Efficiencies (up to 28%) of Excited-State CH2Cl2-Induced Associative Ionization: A Case Study with Nitro Compounds J. Huang et al. 10.1021/acs.analchem.8b04813
- New Particle Formation in the Atmosphere: From Molecular Clusters to Global Climate S. Lee et al. 10.1029/2018JD029356
- Fluorescence detection of urinary N-methylformamide for biomonitoring of human occupational exposure to N,N-dimethylformamide by Eu(III) functionalized MOFs N. Sun & B. Yan 10.1016/j.snb.2018.01.087
- Gas-to-particle partitioning of atmospheric amines observed at a mountain site in southern China F. Liu et al. 10.1016/j.atmosenv.2018.09.038
- A theoretical study of hydrogen-bonded molecular clusters of sulfuric acid and organic acids with amides C. Zuo et al. 10.1016/j.jes.2020.07.022
- Particle acidity and sulfate production during severe haze events in China cannot be reliably inferred by assuming a mixture of inorganic salts G. Wang et al. 10.5194/acp-18-10123-2018
- Role of oleic acid coating in the heterogeneous uptake of dimethylamine by ammonium sulfate particles Y. Chu & C. Chan 10.1080/02786826.2017.1323072
- Formation and growth of sub-3-nm aerosol particles in experimental chambers L. Dada et al. 10.1038/s41596-019-0274-z
- A molecular-scale study on the hydration of sulfuric acid-amide complexes and the atmospheric implication P. Ge et al. 10.1016/j.chemosphere.2018.09.068
- High Concentrations of Atmospheric Isocyanic Acid (HNCO) Produced from Secondary Sources in China Z. Wang et al. 10.1021/acs.est.0c02843
- A review of measurements of air-surface exchange of reactive nitrogen in natural ecosystems across North America J. Walker et al. 10.1016/j.scitotenv.2019.133975
- Nontargeted Tandem Mass Spectrometry Analysis Reveals Diversity and Variability in Aerosol Functional Groups across Multiple Sites, Seasons, and Times of Day J. Ditto et al. 10.1021/acs.estlett.9b00702
- Rapid and highly sensitive measurement of trimethylamine in seawater using dynamic purge-release and dopant-assisted atmospheric pressure photoionization mass spectrometry C. Wu et al. 10.1016/j.aca.2020.08.060
- Mechanism of atmospheric organic amines reacted with ozone and implications for the formation of secondary organic aerosols D. Tong et al. 10.1016/j.scitotenv.2020.139830
- Piperazine Enhancing Sulfuric Acid-Based New Particle Formation: Implications for the Atmospheric Fate of Piperazine F. Ma et al. 10.1021/acs.est.9b02117
- Spatial and temporal distribution characteristics and ozone formation potentials of volatile organic compounds from three typical functional areas in China H. Luo et al. 10.1016/j.envres.2020.109141
- Atmospheric Oxidation of Piperazine Initiated by ·Cl: Unexpected High Nitrosamine Yield F. Ma et al. 10.1021/acs.est.8b02510
- Unprecedented Ambient Sulfur Trioxide (SO3) Detection: Possible Formation Mechanism and Atmospheric Implications L. Yao et al. 10.1021/acs.estlett.0c00615
- Uptake of Gaseous Alkylamides by Suspended Sulfuric Acid Particles: Formation of Ammonium/Aminium Salts H. Chen et al. 10.1021/acs.est.7b03175
- Size‐Resolved Mixing States and Sources of Amine‐Containing Particles in the East China Sea Z. Liu et al. 10.1029/2020JD033162
- Real-time chemical characterization of atmospheric particulate matter in China: A review Y. Li et al. 10.1016/j.atmosenv.2017.02.027
- Interactions of sulfuric acid with common atmospheric bases and organic acids: Thermodynamics and implications to new particle formation Y. Li et al. 10.1016/j.jes.2020.03.033
- Composition of Ultrafine Particles in Urban Beijing: Measurement Using a Thermal Desorption Chemical Ionization Mass Spectrometer X. Li et al. 10.1021/acs.est.0c06053
- Chemical Characteristics of Organic Aerosols in Shanghai: A Study by Ultrahigh-Performance Liquid Chromatography Coupled With Orbitrap Mass Spectrometry X. Wang et al. 10.1002/2017JD026930
- Characteristics and sources of aerosol aminiums over the eastern coast of China: insights from the integrated observations in a coastal city, adjacent island and surrounding marginal seas S. Zhou et al. 10.5194/acp-19-10447-2019
- Ammonolysis of ketene as a potential source of acetamide in the troposphere: a quantum chemical investigation S. Sarkar et al. 10.1039/C8CP01650J
- Sulfuric acid–amine nucleation in urban Beijing R. Cai et al. 10.5194/acp-21-2457-2021
- Quantitation of 11 alkylamines in atmospheric samples: separating structural isomers by ion chromatography B. Place et al. 10.5194/amt-10-1061-2017
- New particle formation in the sulfuric acid–dimethylamine–water system: reevaluation of CLOUD chamber measurements and comparison to an aerosol nucleation and growth model A. Kürten et al. 10.5194/acp-18-845-2018
- Concentration, size distribution and dry deposition of amines in atmospheric particles of urban Guangzhou, China F. Liu et al. 10.1016/j.atmosenv.2017.10.016
- Mechanism and predictive model development of reaction rate constants for N-center radicals with O2 C. Liu et al. 10.1016/j.chemosphere.2019.124411
50 citations as recorded by crossref.
- Atmospheric new particle formation from sulfuric acid and amines in a Chinese megacity L. Yao et al. 10.1126/science.aao4839
- Influence of atmospheric conditions on sulfuric acid-dimethylamine-ammonia-based new particle formation H. Li et al. 10.1016/j.chemosphere.2019.125554
- Probing key organic substances driving new particle growth initiated by iodine nucleation in coastal atmosphere Y. Wan et al. 10.5194/acp-20-9821-2020
- Measurement of ammonia, amines and iodine compounds using protonated water cluster chemical ionization mass spectrometry J. Pfeifer et al. 10.5194/amt-13-2501-2020
- Determination of atmospheric alkylamines by ion chromatography using 18-crown-6 as mobile phase additive S. Zhou et al. 10.1016/j.chroma.2018.05.074
- High-resolution modeling of gaseous methylamines over a polluted region in China: source-dependent emissions and implications of spatial variations J. Mao et al. 10.5194/acp-18-7933-2018
- Laser Ablation-Aerosol Mass Spectrometry-Chemical Ionization Mass Spectrometry for Ambient Surface Imaging J. Berry et al. 10.1021/acs.analchem.7b05255
- Role of Gas-Phase Halogen Bonding in Ambient Chemical Ionization Mass Spectrometry Utilizing Iodine J. Ganske et al. 10.1021/acsearthspacechem.9b00030
- Characteristics and sources of water-soluble organic aerosol in a heavily polluted environment in Northern China H. Li et al. 10.1016/j.scitotenv.2020.143970
- Indoor acids and bases W. Nazaroff & C. Weschler 10.1111/ina.12670
- Atmospheric Sulfuric Acid‐Dimethylamine Nucleation Enhanced by Trifluoroacetic Acid Y. Lu et al. 10.1029/2019GL085627
- A density functional theory study of the molecular interactions between a series of amides and sulfuric acid X. Ma et al. 10.1016/j.chemosphere.2018.08.152
- Integrated experimental and theoretical approach to probe the synergistic effect of ammonia in methanesulfonic acid reactions with small alkylamines V. Perraud et al. 10.1039/C9EM00431A
- Autoxidation mechanism for atmospheric oxidation of tertiary amines: Implications for secondary organic aerosol formation F. Ma et al. 10.1016/j.chemosphere.2020.129207
- A dual-emitting Tb(iii)&Yb(iii)-functionalized coordination polymer: a “turn-on” sensor forN-methylformamide in urine and a “turn-off” sensor for methylglyoxal in serum X. Zheng et al. 10.1039/C9DT02643F
- Computational Study of the Reactions of Chlorine Radicals with Atmospheric Organic Compounds Featuring NHx–π-Bond (x = 1, 2) Structures H. Xie et al. 10.1021/acs.jpca.6b11418
- New Particle Formation and Growth Mechanisms in Highly Polluted Environments H. Yu et al. 10.1007/s40726-017-0067-3
- Detection of gaseous dimethylamine using vocus proton-transfer-reaction time-of-flight mass spectrometry Y. Wang et al. 10.1016/j.atmosenv.2020.117875
- Atmospheric new particle formation in China B. Chu et al. 10.5194/acp-19-115-2019
- Kinetic Understanding of the Ultrahigh Ionization Efficiencies (up to 28%) of Excited-State CH2Cl2-Induced Associative Ionization: A Case Study with Nitro Compounds J. Huang et al. 10.1021/acs.analchem.8b04813
- New Particle Formation in the Atmosphere: From Molecular Clusters to Global Climate S. Lee et al. 10.1029/2018JD029356
- Fluorescence detection of urinary N-methylformamide for biomonitoring of human occupational exposure to N,N-dimethylformamide by Eu(III) functionalized MOFs N. Sun & B. Yan 10.1016/j.snb.2018.01.087
- Gas-to-particle partitioning of atmospheric amines observed at a mountain site in southern China F. Liu et al. 10.1016/j.atmosenv.2018.09.038
- A theoretical study of hydrogen-bonded molecular clusters of sulfuric acid and organic acids with amides C. Zuo et al. 10.1016/j.jes.2020.07.022
- Particle acidity and sulfate production during severe haze events in China cannot be reliably inferred by assuming a mixture of inorganic salts G. Wang et al. 10.5194/acp-18-10123-2018
- Role of oleic acid coating in the heterogeneous uptake of dimethylamine by ammonium sulfate particles Y. Chu & C. Chan 10.1080/02786826.2017.1323072
- Formation and growth of sub-3-nm aerosol particles in experimental chambers L. Dada et al. 10.1038/s41596-019-0274-z
- A molecular-scale study on the hydration of sulfuric acid-amide complexes and the atmospheric implication P. Ge et al. 10.1016/j.chemosphere.2018.09.068
- High Concentrations of Atmospheric Isocyanic Acid (HNCO) Produced from Secondary Sources in China Z. Wang et al. 10.1021/acs.est.0c02843
- A review of measurements of air-surface exchange of reactive nitrogen in natural ecosystems across North America J. Walker et al. 10.1016/j.scitotenv.2019.133975
- Nontargeted Tandem Mass Spectrometry Analysis Reveals Diversity and Variability in Aerosol Functional Groups across Multiple Sites, Seasons, and Times of Day J. Ditto et al. 10.1021/acs.estlett.9b00702
- Rapid and highly sensitive measurement of trimethylamine in seawater using dynamic purge-release and dopant-assisted atmospheric pressure photoionization mass spectrometry C. Wu et al. 10.1016/j.aca.2020.08.060
- Mechanism of atmospheric organic amines reacted with ozone and implications for the formation of secondary organic aerosols D. Tong et al. 10.1016/j.scitotenv.2020.139830
- Piperazine Enhancing Sulfuric Acid-Based New Particle Formation: Implications for the Atmospheric Fate of Piperazine F. Ma et al. 10.1021/acs.est.9b02117
- Spatial and temporal distribution characteristics and ozone formation potentials of volatile organic compounds from three typical functional areas in China H. Luo et al. 10.1016/j.envres.2020.109141
- Atmospheric Oxidation of Piperazine Initiated by ·Cl: Unexpected High Nitrosamine Yield F. Ma et al. 10.1021/acs.est.8b02510
- Unprecedented Ambient Sulfur Trioxide (SO3) Detection: Possible Formation Mechanism and Atmospheric Implications L. Yao et al. 10.1021/acs.estlett.0c00615
- Uptake of Gaseous Alkylamides by Suspended Sulfuric Acid Particles: Formation of Ammonium/Aminium Salts H. Chen et al. 10.1021/acs.est.7b03175
- Size‐Resolved Mixing States and Sources of Amine‐Containing Particles in the East China Sea Z. Liu et al. 10.1029/2020JD033162
- Real-time chemical characterization of atmospheric particulate matter in China: A review Y. Li et al. 10.1016/j.atmosenv.2017.02.027
- Interactions of sulfuric acid with common atmospheric bases and organic acids: Thermodynamics and implications to new particle formation Y. Li et al. 10.1016/j.jes.2020.03.033
- Composition of Ultrafine Particles in Urban Beijing: Measurement Using a Thermal Desorption Chemical Ionization Mass Spectrometer X. Li et al. 10.1021/acs.est.0c06053
- Chemical Characteristics of Organic Aerosols in Shanghai: A Study by Ultrahigh-Performance Liquid Chromatography Coupled With Orbitrap Mass Spectrometry X. Wang et al. 10.1002/2017JD026930
- Characteristics and sources of aerosol aminiums over the eastern coast of China: insights from the integrated observations in a coastal city, adjacent island and surrounding marginal seas S. Zhou et al. 10.5194/acp-19-10447-2019
- Ammonolysis of ketene as a potential source of acetamide in the troposphere: a quantum chemical investigation S. Sarkar et al. 10.1039/C8CP01650J
- Sulfuric acid–amine nucleation in urban Beijing R. Cai et al. 10.5194/acp-21-2457-2021
- Quantitation of 11 alkylamines in atmospheric samples: separating structural isomers by ion chromatography B. Place et al. 10.5194/amt-10-1061-2017
- New particle formation in the sulfuric acid–dimethylamine–water system: reevaluation of CLOUD chamber measurements and comparison to an aerosol nucleation and growth model A. Kürten et al. 10.5194/acp-18-845-2018
- Concentration, size distribution and dry deposition of amines in atmospheric particles of urban Guangzhou, China F. Liu et al. 10.1016/j.atmosenv.2017.10.016
- Mechanism and predictive model development of reaction rate constants for N-center radicals with O2 C. Liu et al. 10.1016/j.chemosphere.2019.124411
Latest update: 28 Feb 2021
Short summary
We present the development of a high-resolution time-of-flight chemical ionization mass spectrometer (HR-ToF-CIMS) method, utilizing protonated ethanol as reagent ions to simultaneously detect atmospheric gaseous amines (C1 to C6) and amides (C1 to C6). Deployment of this ethanol HR-ToF-CIMS has been demonstrated in a field campaign in urban Shanghai, China, detecting amines (from a few pptv to hundreds of pptv) and amides (from tens of pptv to a few ppbv).
We present the development of a high-resolution time-of-flight chemical ionization mass...
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