Articles | Volume 16, issue 3
https://doi.org/10.5194/acp-16-1417-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-1417-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Impact of chamber wall loss of gaseous organic compounds on secondary organic aerosol formation: explicit modeling of SOA formation from alkane and alkene oxidation
Y. S. La
LISA, UMR CNRS 7583, Université Paris Est Créteil et
Université Paris Diderot, 94010 Créteil CEDEX, France
M. Camredon
LISA, UMR CNRS 7583, Université Paris Est Créteil et
Université Paris Diderot, 94010 Créteil CEDEX, France
P. J. Ziemann
Department of Chemistry and Biochemistry and Cooperative Institute for
Research in Environmental Sciences (CIRES), University of Colorado, Boulder,
Colorado, USA
R. Valorso
LISA, UMR CNRS 7583, Université Paris Est Créteil et
Université Paris Diderot, 94010 Créteil CEDEX, France
A. Matsunaga
Air Pollution Research Center, University of California,
Riverside, California, USA
V. Lannuque
LISA, UMR CNRS 7583, Université Paris Est Créteil et
Université Paris Diderot, 94010 Créteil CEDEX, France
J. Lee-Taylor
Department of Chemistry and Biochemistry and Cooperative Institute for
Research in Environmental Sciences (CIRES), University of Colorado, Boulder,
Colorado, USA
National Center for Atmospheric Research,
Boulder, Colorado, USA
A. Hodzic
National Center for Atmospheric Research,
Boulder, Colorado, USA
S. Madronich
National Center for Atmospheric Research,
Boulder, Colorado, USA
LISA, UMR CNRS 7583, Université Paris Est Créteil et
Université Paris Diderot, 94010 Créteil CEDEX, France
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- Estimation of secondary organic aerosol viscosity from explicit modeling of gas-phase oxidation of isoprene and <i>α</i>-pinene T. Galeazzo et al. 10.5194/acp-21-10199-2021
- Secondary organic aerosol formation from propylene irradiations in a chamber study S. Ge et al. 10.1016/j.atmosenv.2017.03.019
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Short summary
The potential impact of chamber walls on the loss of gaseous organic species and secondary organic aerosol (SOA) formation has been explored using the GECKO-A modeling tool, which explicitly represents SOA formation and gas-wall partitioning. The model was compared with 41 smog chamber experiments of SOA formation under OH oxidation of alkane and alkene serie. The organic vapor loss to the chamber walls is found to affect SOA yields as well as the composition of the gas and the particle phase.
The potential impact of chamber walls on the loss of gaseous organic species and secondary...
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