Articles | Volume 16, issue 18
https://doi.org/10.5194/acp-16-11773-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-11773-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Isotopic composition for source identification of mercury in atmospheric fine particles
Qiang Huang
SKLEG, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang
550081, China
SKLEG, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang
550081, China
Weilin Huang
Department of Environmental Sciences, Rutgers, The State University of
New Jersey, New Brunswick, NJ 08901, USA
Pingqing Fu
LAPC, Institute of Atmospheric Physics, Chinese Academy of Sciences,
Beijing 100029, China
Benjamin Guinot
Laboratoire d'Aérologie UMR5560 CNRS-Université Toulouse 3,
Toulouse, France
Xinbin Feng
SKLEG, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang
550081, China
Lihai Shang
SKLEG, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang
550081, China
Zhuhong Wang
SKLEG, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang
550081, China
Zhongwei Wang
SKLEG, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang
550081, China
Shengliu Yuan
SKLEG, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang
550081, China
Hongming Cai
SKLEG, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang
550081, China
Lianfang Wei
LAPC, Institute of Atmospheric Physics, Chinese Academy of Sciences,
Beijing 100029, China
Ben Yu
SKLEG, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang
550081, China
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Cited
58 citations as recorded by crossref.
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- Mercury Stable Isotope Fractionation During Coal Combustion in Coal-Fired Boilers: Reconciling Atmospheric Hg Isotope Observations with Hg Isotope Fractionation Theory R. Sun 10.1007/s00128-018-2531-1
- Ecosystem Mercury Recovery and Health Benefit Under the Minamata Convention in a Changing Climate Q. Wu et al. 10.1007/s44169-022-00016-8
- Mercury Isotopes in Earth and Environmental Chemistry A. Buchachenko 10.1134/S1990793118040048
- Seasonal Variations of the Mercury Multiple Isotopic Compositions of Subrural and Urban Aerosols Highlight an Additional Atmospheric Hg0 Oxidation Pathway D. AuYang et al. 10.3389/fenvs.2021.773327
- Diel variation in mercury stable isotope ratios records photoreduction of PM<sub>2.5</sub>-bound mercury Q. Huang et al. 10.5194/acp-19-315-2019
- Natural stable isotopic compositions of mercury in aerosols and wet precipitations around a coal-fired power plant in Xiamen, southeast China S. Huang et al. 10.1016/j.atmosenv.2017.11.003
- Mercury record of intense hydrothermal activity during the early Cambrian, South China G. Zhu et al. 10.1016/j.palaeo.2021.110294
- Domestic and Transboundary Sources of Atmospheric Particulate Bound Mercury in Remote Areas of China: Evidence from Mercury Isotopes X. Fu et al. 10.1021/acs.est.8b06736
- South-hemispheric marine aerosol Hg and S isotope compositions reveal different oxidation pathways D. AuYang et al. 10.1360/nso/20220014
- Mercury isotopes record development and attenuation of photic zone euxinia during the earliest Cambrian K. Zhao et al. 10.1016/j.gloplacha.2023.104214
- Mercury stable isotopes reveal the sources and transformations of atmospheric Hg in the high Arctic W. Zheng et al. 10.1016/j.apgeochem.2021.105002
- Stable iron isotopic composition of atmospheric aerosols: An overview Y. Wang et al. 10.1038/s41612-022-00299-7
- Environmental applications of metal stable isotopes: Silver, mercury and zinc W. Li et al. 10.1016/j.envpol.2019.06.037
- Stable isotope composition of mercury forms in flue gases from a typical coal-fired power plant, Inner Mongolia, northern China S. Tang et al. 10.1016/j.jhazmat.2017.01.014
- Atmospheric Mercury Isotope Shifts in Response to Mercury Emissions from Underground Coal Fires R. Sun et al. 10.1021/acs.est.2c08637
- Potential factors impacting PM2.5-Hg during haze evolution revealed by mercury isotope: Emission sources and photochemical processes Y. Qiu et al. 10.1016/j.atmosres.2022.106318
- Atmospheric Mercury Concentrations and Isotopic Compositions Impacted by Typical Anthropogenic Mercury Emissions Sources C. Wang et al. 10.1021/acs.est.4c07649
- Levels, sources, isotope signatures, and health risks of mercury in street dust across China G. Sun et al. 10.1016/j.jhazmat.2020.122276
- Katabatic Wind and Sea–Ice Dynamics Drive Isotopic Variations of Total Gaseous Mercury on the Antarctic Coast B. Yu et al. 10.1021/acs.est.0c07474
- Stable Mercury Isotopes Revealing Photochemical Processes in the Marine Boundary Layer Y. Qiu et al. 10.1029/2021JD034630
- Mercury Isotope Variations in Lake Sediment Cores in Response to Direct Mercury Emissions from Non-Ferrous Metal Smelters and Legacy Mercury Remobilization R. Sun et al. 10.1021/acs.est.2c02692
- Denitrification devices in urban boilers change mercury isotope fractionation signatures of coal combustion products J. Yuan et al. 10.1016/j.envpol.2020.115753
- Stable Isotopes Reveal Photoreduction of Particle-Bound Mercury Driven by Water-Soluble Organic Carbon during Severe Haze K. Zhang et al. 10.1021/acs.est.2c01933
- Variation in the mercury concentration and stable isotope composition of atmospheric total suspended particles in Beijing, China Q. Huang et al. 10.1016/j.jhazmat.2019.121131
- Photochemical Reduction of Particle Bound Mercury in Atmospheric Aerosol Water D. Han et al. 10.1021/acsestair.3c00070
- Stable sulfur isotope ratios and chemical compositions of fine aerosols (PM2.5) in Beijing, China L. Wei et al. 10.1016/j.scitotenv.2018.03.153
- Study of mercury transport and transformation in mangrove forests using stable mercury isotopes S. Huang et al. 10.1016/j.scitotenv.2019.135928
- Identification of potential sources of elevated PM2.5-Hg using mercury isotopes during haze events Y. Qiu et al. 10.1016/j.atmosenv.2021.118203
- Isotopic investigation of sources and processes affecting gaseous and particulate bound mercury in the east coast, South Korea H. Lee et al. 10.1016/j.scitotenv.2023.164404
- Mercury stable isotopes for monitoring the effectiveness of the Minamata Convention on Mercury S. Kwon et al. 10.1016/j.earscirev.2020.103111
- Sources of Particulate Bound Mercury in the Northwest Pacific Constrained by Hg Isotopes S. Huang et al. 10.1021/acsearthspacechem.3c00365
- Spatiotemporal Distributions and Source Apportionment of PM2.5‐Bound Antimony in Beijing, China C. Yang et al. 10.1029/2021JD036401
- Sampling and determination of antimony isotopes in airborne particles: an assessment of membrane filter materials C. Zhang et al. 10.1039/D2JA00242F
- Fate and Transport of Mercury through Waterflows in a Tropical Rainforest W. Yuan et al. 10.1021/acs.est.3c09265
- Sources and Transformation Mechanisms of Atmospheric Particulate Bound Mercury Revealed by Mercury Stable Isotopes C. Liu et al. 10.1021/acs.est.1c08065
- Mercury stable isotopes revealing the atmospheric mercury circulation: A review of particulate bound mercury in China X. Qin et al. 10.1016/j.earscirev.2024.104681
- Analysis of Isotopic Compositions of Mercury Species in Atmospheric Particulates Based on Thermo-Desorption Technique Y. SU et al. 10.3724/EE.1672-9250.2024.52.024
- Isotope Data Constrains Redox Chemistry of Atmospheric Mercury Z. Song et al. 10.1021/acs.est.4c02600
- New evidence for atmospheric mercury transformations in the marine boundary layer from stable mercury isotopes B. Yu et al. 10.5194/acp-20-9713-2020
- Mercury stable isotope fractionation during gaseous elemental mercury adsorption onto coal fly ash particles: Experimental and field observations B. Fu et al. 10.1016/j.jhazmat.2020.124280
- Molecular Characterization and Seasonal Variation in Primary and Secondary Organic Aerosols in Beijing, China L. Li et al. 10.1029/2018JD028527
- Seasonal Variation of Mercury and Its Isotopes in Atmospheric Particles at the Coastal Zhongshan Station, Eastern Antarctica C. Li et al. 10.1021/acs.est.0c04462
- Mercury concentration and isotopic composition on different atmospheric particles (PM10 and PM2.5) in the subtropical coastal suburb of Xiamen Bay, Southern China L. Sun et al. 10.1016/j.atmosenv.2021.118604
- Mercury isotope signatures of a pre-calciner cement plant in Southwest China X. Li et al. 10.1016/j.jhazmat.2020.123384
- Stable Iron Isotopic Signature Reveals Multiple Sources of Magnetic Particulate Matter in the 2021 Beijing Sandstorms P. Zuo et al. 10.1021/acs.estlett.2c00144
- Tracing the transboundary transport of atmospheric Particulate Bound Mercury driven by the East Asian monsoon X. Qin et al. 10.1016/j.jhazmat.2022.130678
- A specific role of magnetic isotopes in biological and ecological systems. Physics and biophysics beyond A. Buchachenko et al. 10.1016/j.pbiomolbio.2020.02.007
- Mercury isotopic compositions in fine particles and offshore surface seawater in a coastal area of East China: implications for Hg sources and atmospheric transformations L. Xu et al. 10.5194/acp-21-18543-2021
- Mass-Independent Fractionation of Mercury Isotopes during Photoreduction of Soot Particle Bound Hg(II) Q. Huang et al. 10.1021/acs.est.1c02679
- Non-traditional stable isotopic analysis for source tracing of atmospheric particulate matter P. Zuo et al. 10.1016/j.trac.2022.116866
- Atomic spectrometry update – a review of advances in environmental analysis O. Butler et al. 10.1039/C7JA90059G
- Soil and ambient air mercury as an indicator of coal-fired power plant emissions: a case study in North China Z. Li et al. 10.1007/s11356-021-12842-9
- A Review of Metal Levels in Urban Dust, Their Methods of Determination, and Risk Assessment C. Kaonga et al. 10.3390/atmos12070891
- The Causes and Effects of Mercury and Methylmercury Contamination in the Marine Environment: A Review M. Al-Sulaiti et al. 10.1007/s40726-022-00226-7
- Mercury stable isotope compositions of Chinese urban fine particulates in winter haze days: Implications for Hg sources and transformations H. Xu et al. 10.1016/j.chemgeo.2018.11.018
- New Insights into Unexpected Severe PM2.5 Pollution during the SARS and COVID-19 Pandemic Periods in Beijing P. Zuo et al. 10.1021/acs.est.1c05383
- Event-Based Atmospheric Precipitation Uncovers Significant Even and Odd Hg Isotope Anomalies Associated with the Circumpolar Vortex S. Yuan et al. 10.1021/acs.est.2c02613
58 citations as recorded by crossref.
- Hg isotope ratio measurements of methylmercury in fish tissues using HPLC with off line cold vapour generation MC-ICPMS J. Entwisle et al. 10.1039/C8JA00099A
- Mercury Stable Isotope Fractionation During Coal Combustion in Coal-Fired Boilers: Reconciling Atmospheric Hg Isotope Observations with Hg Isotope Fractionation Theory R. Sun 10.1007/s00128-018-2531-1
- Ecosystem Mercury Recovery and Health Benefit Under the Minamata Convention in a Changing Climate Q. Wu et al. 10.1007/s44169-022-00016-8
- Mercury Isotopes in Earth and Environmental Chemistry A. Buchachenko 10.1134/S1990793118040048
- Seasonal Variations of the Mercury Multiple Isotopic Compositions of Subrural and Urban Aerosols Highlight an Additional Atmospheric Hg0 Oxidation Pathway D. AuYang et al. 10.3389/fenvs.2021.773327
- Diel variation in mercury stable isotope ratios records photoreduction of PM<sub>2.5</sub>-bound mercury Q. Huang et al. 10.5194/acp-19-315-2019
- Natural stable isotopic compositions of mercury in aerosols and wet precipitations around a coal-fired power plant in Xiamen, southeast China S. Huang et al. 10.1016/j.atmosenv.2017.11.003
- Mercury record of intense hydrothermal activity during the early Cambrian, South China G. Zhu et al. 10.1016/j.palaeo.2021.110294
- Domestic and Transboundary Sources of Atmospheric Particulate Bound Mercury in Remote Areas of China: Evidence from Mercury Isotopes X. Fu et al. 10.1021/acs.est.8b06736
- South-hemispheric marine aerosol Hg and S isotope compositions reveal different oxidation pathways D. AuYang et al. 10.1360/nso/20220014
- Mercury isotopes record development and attenuation of photic zone euxinia during the earliest Cambrian K. Zhao et al. 10.1016/j.gloplacha.2023.104214
- Mercury stable isotopes reveal the sources and transformations of atmospheric Hg in the high Arctic W. Zheng et al. 10.1016/j.apgeochem.2021.105002
- Stable iron isotopic composition of atmospheric aerosols: An overview Y. Wang et al. 10.1038/s41612-022-00299-7
- Environmental applications of metal stable isotopes: Silver, mercury and zinc W. Li et al. 10.1016/j.envpol.2019.06.037
- Stable isotope composition of mercury forms in flue gases from a typical coal-fired power plant, Inner Mongolia, northern China S. Tang et al. 10.1016/j.jhazmat.2017.01.014
- Atmospheric Mercury Isotope Shifts in Response to Mercury Emissions from Underground Coal Fires R. Sun et al. 10.1021/acs.est.2c08637
- Potential factors impacting PM2.5-Hg during haze evolution revealed by mercury isotope: Emission sources and photochemical processes Y. Qiu et al. 10.1016/j.atmosres.2022.106318
- Atmospheric Mercury Concentrations and Isotopic Compositions Impacted by Typical Anthropogenic Mercury Emissions Sources C. Wang et al. 10.1021/acs.est.4c07649
- Levels, sources, isotope signatures, and health risks of mercury in street dust across China G. Sun et al. 10.1016/j.jhazmat.2020.122276
- Katabatic Wind and Sea–Ice Dynamics Drive Isotopic Variations of Total Gaseous Mercury on the Antarctic Coast B. Yu et al. 10.1021/acs.est.0c07474
- Stable Mercury Isotopes Revealing Photochemical Processes in the Marine Boundary Layer Y. Qiu et al. 10.1029/2021JD034630
- Mercury Isotope Variations in Lake Sediment Cores in Response to Direct Mercury Emissions from Non-Ferrous Metal Smelters and Legacy Mercury Remobilization R. Sun et al. 10.1021/acs.est.2c02692
- Denitrification devices in urban boilers change mercury isotope fractionation signatures of coal combustion products J. Yuan et al. 10.1016/j.envpol.2020.115753
- Stable Isotopes Reveal Photoreduction of Particle-Bound Mercury Driven by Water-Soluble Organic Carbon during Severe Haze K. Zhang et al. 10.1021/acs.est.2c01933
- Variation in the mercury concentration and stable isotope composition of atmospheric total suspended particles in Beijing, China Q. Huang et al. 10.1016/j.jhazmat.2019.121131
- Photochemical Reduction of Particle Bound Mercury in Atmospheric Aerosol Water D. Han et al. 10.1021/acsestair.3c00070
- Stable sulfur isotope ratios and chemical compositions of fine aerosols (PM2.5) in Beijing, China L. Wei et al. 10.1016/j.scitotenv.2018.03.153
- Study of mercury transport and transformation in mangrove forests using stable mercury isotopes S. Huang et al. 10.1016/j.scitotenv.2019.135928
- Identification of potential sources of elevated PM2.5-Hg using mercury isotopes during haze events Y. Qiu et al. 10.1016/j.atmosenv.2021.118203
- Isotopic investigation of sources and processes affecting gaseous and particulate bound mercury in the east coast, South Korea H. Lee et al. 10.1016/j.scitotenv.2023.164404
- Mercury stable isotopes for monitoring the effectiveness of the Minamata Convention on Mercury S. Kwon et al. 10.1016/j.earscirev.2020.103111
- Sources of Particulate Bound Mercury in the Northwest Pacific Constrained by Hg Isotopes S. Huang et al. 10.1021/acsearthspacechem.3c00365
- Spatiotemporal Distributions and Source Apportionment of PM2.5‐Bound Antimony in Beijing, China C. Yang et al. 10.1029/2021JD036401
- Sampling and determination of antimony isotopes in airborne particles: an assessment of membrane filter materials C. Zhang et al. 10.1039/D2JA00242F
- Fate and Transport of Mercury through Waterflows in a Tropical Rainforest W. Yuan et al. 10.1021/acs.est.3c09265
- Sources and Transformation Mechanisms of Atmospheric Particulate Bound Mercury Revealed by Mercury Stable Isotopes C. Liu et al. 10.1021/acs.est.1c08065
- Mercury stable isotopes revealing the atmospheric mercury circulation: A review of particulate bound mercury in China X. Qin et al. 10.1016/j.earscirev.2024.104681
- Analysis of Isotopic Compositions of Mercury Species in Atmospheric Particulates Based on Thermo-Desorption Technique Y. SU et al. 10.3724/EE.1672-9250.2024.52.024
- Isotope Data Constrains Redox Chemistry of Atmospheric Mercury Z. Song et al. 10.1021/acs.est.4c02600
- New evidence for atmospheric mercury transformations in the marine boundary layer from stable mercury isotopes B. Yu et al. 10.5194/acp-20-9713-2020
- Mercury stable isotope fractionation during gaseous elemental mercury adsorption onto coal fly ash particles: Experimental and field observations B. Fu et al. 10.1016/j.jhazmat.2020.124280
- Molecular Characterization and Seasonal Variation in Primary and Secondary Organic Aerosols in Beijing, China L. Li et al. 10.1029/2018JD028527
- Seasonal Variation of Mercury and Its Isotopes in Atmospheric Particles at the Coastal Zhongshan Station, Eastern Antarctica C. Li et al. 10.1021/acs.est.0c04462
- Mercury concentration and isotopic composition on different atmospheric particles (PM10 and PM2.5) in the subtropical coastal suburb of Xiamen Bay, Southern China L. Sun et al. 10.1016/j.atmosenv.2021.118604
- Mercury isotope signatures of a pre-calciner cement plant in Southwest China X. Li et al. 10.1016/j.jhazmat.2020.123384
- Stable Iron Isotopic Signature Reveals Multiple Sources of Magnetic Particulate Matter in the 2021 Beijing Sandstorms P. Zuo et al. 10.1021/acs.estlett.2c00144
- Tracing the transboundary transport of atmospheric Particulate Bound Mercury driven by the East Asian monsoon X. Qin et al. 10.1016/j.jhazmat.2022.130678
- A specific role of magnetic isotopes in biological and ecological systems. Physics and biophysics beyond A. Buchachenko et al. 10.1016/j.pbiomolbio.2020.02.007
- Mercury isotopic compositions in fine particles and offshore surface seawater in a coastal area of East China: implications for Hg sources and atmospheric transformations L. Xu et al. 10.5194/acp-21-18543-2021
- Mass-Independent Fractionation of Mercury Isotopes during Photoreduction of Soot Particle Bound Hg(II) Q. Huang et al. 10.1021/acs.est.1c02679
- Non-traditional stable isotopic analysis for source tracing of atmospheric particulate matter P. Zuo et al. 10.1016/j.trac.2022.116866
- Atomic spectrometry update – a review of advances in environmental analysis O. Butler et al. 10.1039/C7JA90059G
- Soil and ambient air mercury as an indicator of coal-fired power plant emissions: a case study in North China Z. Li et al. 10.1007/s11356-021-12842-9
- A Review of Metal Levels in Urban Dust, Their Methods of Determination, and Risk Assessment C. Kaonga et al. 10.3390/atmos12070891
- The Causes and Effects of Mercury and Methylmercury Contamination in the Marine Environment: A Review M. Al-Sulaiti et al. 10.1007/s40726-022-00226-7
- Mercury stable isotope compositions of Chinese urban fine particulates in winter haze days: Implications for Hg sources and transformations H. Xu et al. 10.1016/j.chemgeo.2018.11.018
- New Insights into Unexpected Severe PM2.5 Pollution during the SARS and COVID-19 Pandemic Periods in Beijing P. Zuo et al. 10.1021/acs.est.1c05383
- Event-Based Atmospheric Precipitation Uncovers Significant Even and Odd Hg Isotope Anomalies Associated with the Circumpolar Vortex S. Yuan et al. 10.1021/acs.est.2c02613
Latest update: 14 Dec 2024
Short summary
Atmospheric airborne mercury is of particular concern because, once inhaled, both Hg and its vectors might have adverse effects on human beings. In this study, we attempted to identify the sources of PM2.5-Hg in Beijing, China, using Hg isotopic composition. Large range and seasonal variations in both mass-dependent and mass-independent fractionations of Hg isotopes in haze particles demonstrate the usefulness of Hg isotopes for directly tracing the sources and its vectors in the atmosphere.
Atmospheric airborne mercury is of particular concern because, once inhaled, both Hg and its...
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