Articles | Volume 16, issue 18
https://doi.org/10.5194/acp-16-11563-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-11563-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
19 Sep 2016
Research article |
| 19 Sep 2016
Volatility and lifetime against OH heterogeneous reaction of ambient isoprene-epoxydiols-derived secondary organic aerosol (IEPOX-SOA)
Cooperative Institute for Research in Environmental Sciences, University
of Colorado, Boulder, CO 80309, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder,
CO 80309, USA
Brett B. Palm
Cooperative Institute for Research in Environmental Sciences, University
of Colorado, Boulder, CO 80309, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder,
CO 80309, USA
Douglas A. Day
Cooperative Institute for Research in Environmental Sciences, University
of Colorado, Boulder, CO 80309, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder,
CO 80309, USA
Pedro Campuzano-Jost
Cooperative Institute for Research in Environmental Sciences, University
of Colorado, Boulder, CO 80309, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder,
CO 80309, USA
Jordan E. Krechmer
Cooperative Institute for Research in Environmental Sciences, University
of Colorado, Boulder, CO 80309, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder,
CO 80309, USA
Cooperative Institute for Research in Environmental Sciences, University
of Colorado, Boulder, CO 80309, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder,
CO 80309, USA
Suzane S. de Sá
John A. Paulson School of Engineering and Applied Sciences Harvard
University, Cambridge, MA 01742, USA
Scot T. Martin
John A. Paulson School of Engineering and Applied Sciences Harvard
University, Cambridge, MA 01742, USA
Department of Earth and Planetary Sciences, Harvard University, Cambridge,
MA 01742, USA
M. Lizabeth Alexander
Environmental Molecular Sciences Laboratory, Pacific Northwest National
Laboratory, Richland, WA 99352, USA
Karsten Baumann
Atmospheric Research and Analysis Inc., Morrisville, NC 27560, USA
Lina Hacker
Institute for Energy and Climate Research – Troposphere (IEK-8),
Forschungszentrum Jülich, 52425 Jülich, Germany
Astrid Kiendler-Scharr
Institute for Energy and Climate Research – Troposphere (IEK-8),
Forschungszentrum Jülich, 52425 Jülich, Germany
Abigail R. Koss
Cooperative Institute for Research in Environmental Sciences, University
of Colorado, Boulder, CO 80309, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder,
CO 80309, USA
Earth System Research Laboratory, NOAA, Boulder, CO 80305, USA
Joost A. de Gouw
Cooperative Institute for Research in Environmental Sciences, University
of Colorado, Boulder, CO 80309, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder,
CO 80309, USA
Earth System Research Laboratory, NOAA, Boulder, CO 80305, USA
Allen H. Goldstein
Department of Environmental Science, Policy, and Management, University of
California, Berkeley, CA 94720, USA
Department of Civil and Environmental Engineering, University of
California, Berkeley, CA 94720, USA
Roger Seco
Department of Earth System Science, University of California,
Irvine, CA 92697, USA
Steven J. Sjostedt
Earth System Research Laboratory, NOAA, Boulder, CO 80305, USA
Jeong-Hoo Park
National Institute of Environmental Research, Incheon 22689, Republic of Korea
Alex B. Guenther
Department of Earth System Science, University of California,
Irvine, CA 92697, USA
Saewung Kim
Department of Earth System Science, University of California,
Irvine, CA 92697, USA
Francesco Canonaco
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI), 5232
Villigen, Switzerland
André S. H. Prévôt
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI), 5232
Villigen, Switzerland
William H. Brune
Department of Meteorology, Pennsylvania State University, University
Park, PA 16802, USA
Jose L. Jimenez
Cooperative Institute for Research in Environmental Sciences, University
of Colorado, Boulder, CO 80309, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder,
CO 80309, USA
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- Secondary aerosol formation from mixtures of marine volatile organic compounds in a potential aerosol mass oxidative flow reactor A. Moore et al. 10.1039/D3EA00169E
- Impact of aging on the sources, volatility, and viscosity of organic aerosols in Chinese outflows T. Feng et al. 10.5194/acp-23-611-2023
- A comprehensive evaluation of enhanced temperature influence on gas and aerosol chemistry in the lamp-enclosed oxidation flow reactor (OFR) system T. Pan et al. 10.5194/amt-17-4915-2024
- More Than Emissions and Chemistry: Fire Size, Dilution, and Background Aerosol Also Greatly Influence Near‐Field Biomass Burning Aerosol Aging A. Hodshire et al. 10.1029/2018JD029674
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- Organic aerosol in the summertime southeastern United States: components and their link to volatility distribution, oxidation state and hygroscopicity E. Kostenidou et al. 10.5194/acp-18-5799-2018
- Biogenic emissions and land–atmosphere interactions as drivers of the daytime evolution of secondary organic aerosol in the southeastern US J. Nagori et al. 10.5194/acp-19-701-2019
- Determining the Relative Reactivity of Sulfate, Bisulfate, and Organosulfates with Epoxides on Secondary Organic Aerosol E. Aoki et al. 10.1021/acsearthspacechem.0c00178
- Atmospheric Acetaldehyde: Importance of Air‐Sea Exchange and a Missing Source in the Remote Troposphere S. Wang et al. 10.1029/2019GL082034
- Secondary organic aerosol formation from ambient air in an oxidation flow reactor in central Amazonia B. Palm et al. 10.5194/acp-18-467-2018
- Impact of Aerosol-Cloud Cycling on Aqueous Secondary Organic Aerosol Formation W. Tsui et al. 10.3390/atmos10110666
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- Ambient Measurements of Highly Oxidized Gas-Phase Molecules during the Southern Oxidant and Aerosol Study (SOAS) 2013 P. Massoli et al. 10.1021/acsearthspacechem.8b00028
- Long-term observational constraints of organic aerosol dependence on inorganic species in the southeast US Y. Zheng et al. 10.5194/acp-20-13091-2020
- Quantifying the volatility of organic aerosol in the southeastern US P. Saha et al. 10.5194/acp-17-501-2017
- Recent advances in understanding secondary organic aerosol: Implications for global climate forcing M. Shrivastava et al. 10.1002/2016RG000540
- Organic peroxy radical chemistry in oxidation flow reactors and environmental chambers and their atmospheric relevance Z. Peng et al. 10.5194/acp-19-813-2019
- Resolving Ambient Organic Aerosol Formation and Aging Pathways with Simultaneous Molecular Composition and Volatility Observations B. Lee et al. 10.1021/acsearthspacechem.9b00302
- Observational evidence for pollution‐influenced selective uptake contributing to biogenic secondary organic aerosols in the southeastern U.S. J. Liu et al. 10.1002/2017GL074665
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Short summary
IEPOX-SOA is biogenically derived secondary organic aerosol under anthropogenic influence, which has been shown to comprise a substantial fraction of OA globally. We investigated the lifetime of ambient IEPOX-SOA in the SE US and Amazonia, with an oxidation flow reactor and thermodenuder coupled with MS-based instrumentation. The low volatility and long lifetime of IEPOX-SOA against OH radicals' oxidation (> 2 weeks) was observed, which can help to constrain OA impact on air quality and climate.
IEPOX-SOA is biogenically derived secondary organic aerosol under anthropogenic influence, which...
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