Articles | Volume 16, issue 18
https://doi.org/10.5194/acp-16-11563-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-11563-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
19 Sep 2016
Research article |
| 19 Sep 2016
Volatility and lifetime against OH heterogeneous reaction of ambient isoprene-epoxydiols-derived secondary organic aerosol (IEPOX-SOA)
Cooperative Institute for Research in Environmental Sciences, University
of Colorado, Boulder, CO 80309, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder,
CO 80309, USA
Brett B. Palm
Cooperative Institute for Research in Environmental Sciences, University
of Colorado, Boulder, CO 80309, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder,
CO 80309, USA
Douglas A. Day
Cooperative Institute for Research in Environmental Sciences, University
of Colorado, Boulder, CO 80309, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder,
CO 80309, USA
Pedro Campuzano-Jost
Cooperative Institute for Research in Environmental Sciences, University
of Colorado, Boulder, CO 80309, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder,
CO 80309, USA
Jordan E. Krechmer
Cooperative Institute for Research in Environmental Sciences, University
of Colorado, Boulder, CO 80309, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder,
CO 80309, USA
Cooperative Institute for Research in Environmental Sciences, University
of Colorado, Boulder, CO 80309, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder,
CO 80309, USA
Suzane S. de Sá
John A. Paulson School of Engineering and Applied Sciences Harvard
University, Cambridge, MA 01742, USA
Scot T. Martin
John A. Paulson School of Engineering and Applied Sciences Harvard
University, Cambridge, MA 01742, USA
Department of Earth and Planetary Sciences, Harvard University, Cambridge,
MA 01742, USA
M. Lizabeth Alexander
Environmental Molecular Sciences Laboratory, Pacific Northwest National
Laboratory, Richland, WA 99352, USA
Karsten Baumann
Atmospheric Research and Analysis Inc., Morrisville, NC 27560, USA
Lina Hacker
Institute for Energy and Climate Research – Troposphere (IEK-8),
Forschungszentrum Jülich, 52425 Jülich, Germany
Astrid Kiendler-Scharr
Institute for Energy and Climate Research – Troposphere (IEK-8),
Forschungszentrum Jülich, 52425 Jülich, Germany
Abigail R. Koss
Cooperative Institute for Research in Environmental Sciences, University
of Colorado, Boulder, CO 80309, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder,
CO 80309, USA
Earth System Research Laboratory, NOAA, Boulder, CO 80305, USA
Joost A. de Gouw
Cooperative Institute for Research in Environmental Sciences, University
of Colorado, Boulder, CO 80309, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder,
CO 80309, USA
Earth System Research Laboratory, NOAA, Boulder, CO 80305, USA
Allen H. Goldstein
Department of Environmental Science, Policy, and Management, University of
California, Berkeley, CA 94720, USA
Department of Civil and Environmental Engineering, University of
California, Berkeley, CA 94720, USA
Roger Seco
Department of Earth System Science, University of California,
Irvine, CA 92697, USA
Steven J. Sjostedt
Earth System Research Laboratory, NOAA, Boulder, CO 80305, USA
Jeong-Hoo Park
National Institute of Environmental Research, Incheon 22689, Republic of Korea
Alex B. Guenther
Department of Earth System Science, University of California,
Irvine, CA 92697, USA
Saewung Kim
Department of Earth System Science, University of California,
Irvine, CA 92697, USA
Francesco Canonaco
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI), 5232
Villigen, Switzerland
André S. H. Prévôt
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI), 5232
Villigen, Switzerland
William H. Brune
Department of Meteorology, Pennsylvania State University, University
Park, PA 16802, USA
Jose L. Jimenez
Cooperative Institute for Research in Environmental Sciences, University
of Colorado, Boulder, CO 80309, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder,
CO 80309, USA
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- Secondary organic aerosol formation from ambient air in an oxidation flow reactor in central Amazonia B. Palm et al. 10.5194/acp-18-467-2018
- Impact of Aerosol-Cloud Cycling on Aqueous Secondary Organic Aerosol Formation W. Tsui et al. 10.3390/atmos10110666
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- Recent advances in understanding secondary organic aerosol: Implications for global climate forcing M. Shrivastava et al. 10.1002/2016RG000540
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- Observational evidence for pollution‐influenced selective uptake contributing to biogenic secondary organic aerosols in the southeastern U.S. J. Liu et al. 10.1002/2017GL074665
- KinSim: A Research-Grade, User-Friendly, Visual Kinetics Simulator for Chemical-Kinetics and Environmental-Chemistry Teaching Z. Peng & J. Jimenez 10.1021/acs.jchemed.9b00033
- Evaluating SOA formation from different sources of semi- and intermediate-volatility organic compounds from the Athabasca oil sands J. Sommers et al. 10.1039/D1EA00053E
- Hygroscopicity and Volatility of Biomass Burning Aromatic and Nitroaromatic Compounds M. Amugoda et al. 10.1021/acsestair.3c00071
- Predictions of the glass transition temperature and viscosity of organic aerosols from volatility distributions Y. Li et al. 10.5194/acp-20-8103-2020
- Joint Impacts of Acidity and Viscosity on the Formation of Secondary Organic Aerosol from Isoprene Epoxydiols (IEPOX) in Phase Separated Particles Y. Zhang et al. 10.1021/acsearthspacechem.9b00209
- Modeling the Impact of the Organic Aerosol Phase State on Multiphase OH Reactive Uptake Kinetics and the Resultant Heterogeneous Oxidation Timescale of Organic Aerosol in the Amazon Rainforest Q. Rasool et al. 10.1021/acsearthspacechem.2c00366
- Measurement report: Effects of anthropogenic emissions and environmental factors on the formation of biogenic secondary organic aerosol (BSOA) in a coastal city of southeastern China Y. Hong et al. 10.5194/acp-22-7827-2022
- Modeling Volatility-Based Aerosol Phase State Predictions in the Amazon Rainforest Q. Rasool et al. 10.1021/acsearthspacechem.1c00255
- Changes in Physicochemical Properties of Organic Aerosol During Photochemical Aging of Cooking and Burning Emissions W. Xu et al. 10.1029/2022JD037911
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Latest update: 18 Apr 2024
Short summary
IEPOX-SOA is biogenically derived secondary organic aerosol under anthropogenic influence, which has been shown to comprise a substantial fraction of OA globally. We investigated the lifetime of ambient IEPOX-SOA in the SE US and Amazonia, with an oxidation flow reactor and thermodenuder coupled with MS-based instrumentation. The low volatility and long lifetime of IEPOX-SOA against OH radicals' oxidation (> 2 weeks) was observed, which can help to constrain OA impact on air quality and climate.
IEPOX-SOA is biogenically derived secondary organic aerosol under anthropogenic influence, which...
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