Articles | Volume 16, issue 2
https://doi.org/10.5194/acp-16-1105-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-1105-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
01 Feb 2016
Research article |
| 01 Feb 2016
Cloud condensation nuclei activity, droplet growth kinetics, and hygroscopicity of biogenic and anthropogenic secondary organic aerosol (SOA)
D. F. Zhao
Institute for Energy and Climate Research, IEK-8: Troposphere,
Forschungszentrum Jülich, 52425 Jülich, Germany
A. Buchholz
Institute for Energy and Climate Research, IEK-8: Troposphere,
Forschungszentrum Jülich, 52425 Jülich, Germany
now at: Department of Applied Physics, University of Eastern Finland,
70211 Kuopio, Finland
B. Kortner
Institute for Energy and Climate Research, IEK-8: Troposphere,
Forschungszentrum Jülich, 52425 Jülich, Germany
P. Schlag
Institute for Energy and Climate Research, IEK-8: Troposphere,
Forschungszentrum Jülich, 52425 Jülich, Germany
F. Rubach
Institute for Energy and Climate Research, IEK-8: Troposphere,
Forschungszentrum Jülich, 52425 Jülich, Germany
now at: Max-Planck-Institute for Chemistry, Mainz, Germany
Institute for Energy and Climate Research, IEK-8: Troposphere,
Forschungszentrum Jülich, 52425 Jülich, Germany
A. Kiendler-Scharr
Institute for Energy and Climate Research, IEK-8: Troposphere,
Forschungszentrum Jülich, 52425 Jülich, Germany
R. Tillmann
Institute for Energy and Climate Research, IEK-8: Troposphere,
Forschungszentrum Jülich, 52425 Jülich, Germany
A. Wahner
Institute for Energy and Climate Research, IEK-8: Troposphere,
Forschungszentrum Jülich, 52425 Jülich, Germany
Å. K. Watne
Department of Chemistry and Molecular Biology, University of
Gothenburg, Gothenburg, 41296, Sweden
M. Hallquist
Department of Chemistry and Molecular Biology, University of
Gothenburg, Gothenburg, 41296, Sweden
J. M. Flores
Department of Earth and Planetary Sciences, Weizmann Institute of
Science, Rehovot, 76100, Israel
Y. Rudich
Department of Earth and Planetary Sciences, Weizmann Institute of
Science, Rehovot, 76100, Israel
K. Kristensen
Department of Chemistry, Aarhus University, 8000 Aarhus, Denmark
A. M. K. Hansen
Department of Chemistry, Aarhus University, 8000 Aarhus, Denmark
M. Glasius
Department of Chemistry, Aarhus University, 8000 Aarhus, Denmark
I. Kourtchev
Department of Chemistry, University of Cambridge, Cambridge, CB2 1EW,
UK
M. Kalberer
Department of Chemistry, University of Cambridge, Cambridge, CB2 1EW,
UK
Institute for Energy and Climate Research, IEK-8: Troposphere,
Forschungszentrum Jülich, 52425 Jülich, Germany
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Cited
37 citations as recorded by crossref.
- Liquid–liquid phase separation in particles containing secondary organic material free of inorganic salts M. Song et al. 10.5194/acp-17-11261-2017
- Cloud droplet activation of secondary organic aerosol is mainly controlled by molecular weight, not water solubility J. Wang et al. 10.5194/acp-19-941-2019
- Molecular and spatial distributions of dicarboxylic acids, oxocarboxylic acids, and <i>α</i>-dicarbonyls in marine aerosols from the South China Sea to the eastern Indian Ocean J. Yang et al. 10.5194/acp-20-6841-2020
- Contrasting effects of secondary organic aerosol formations on organic aerosol hygroscopicity Y. Kuang et al. 10.5194/acp-21-10375-2021
- Effect of solubility limitation on hygroscopic growth and cloud drop activation of SOA particles produced from traffic exhausts C. Wittbom et al. 10.1007/s10874-018-9380-5
- Tropical and Boreal Forest – Atmosphere Interactions: A Review P. Artaxo et al. 10.16993/tellusb.34
- Hygroscopicity and CCN potential of DMS-derived aerosol particles B. Rosati et al. 10.5194/acp-22-13449-2022
- The Interplay Between Hydrogen Bonding and Coulombic Forces in Determining the Structure of Sulfuric Acid-Amine Clusters S. Waller et al. 10.1021/acs.jpclett.8b00161
- Impacts of water partitioning and polarity of organic compounds on secondary organic aerosol over eastern China J. Li et al. 10.5194/acp-20-7291-2020
- Measurement report: Distinct size dependence and diurnal variation in organic aerosol hygroscopicity, volatility, and cloud condensation nuclei activity at a rural site in the Pearl River Delta (PRD) region, China M. Cai et al. 10.5194/acp-22-8117-2022
- Hygroscopicity of Secondary Brown Carbon Aerosol from Aqueous Photo-Oxidation of Phenolic Precursors K. Betz et al. 10.1021/acsearthspacechem.2c00132
- Recent advances in understanding secondary organic aerosol: Implications for global climate forcing M. Shrivastava et al. 10.1002/2016RG000540
- Organosulfates in aerosols downwind of an urban region in central Amazon M. Glasius et al. 10.1039/C8EM00413G
- Effects of NO<sub><i>x</i></sub> and SO<sub>2</sub> on the secondary organic aerosol formation from photooxidation of <i>α</i>-pinene and limonene D. Zhao et al. 10.5194/acp-18-1611-2018
- Utilizing an electrical low-pressure impactor to indirectly probe water uptake via particle bounce measurements K. Fischer & G. Petrucci 10.5194/amt-14-7565-2021
- Accounting for Cloud Nucleation Activation Mechanism of Secondary Organic Matter from α-Pinene Oxidation Using Experimentally Retrieved Water Solubility Distributions W. Lee et al. 10.1021/acs.est.3c03039
- Introductory lecture: atmospheric chemistry in the Anthropocene B. Finlayson-Pitts 10.1039/C7FD00161D
- Gas-phase kinetics modifies the CCN activity of a biogenic SOA A. Vizenor & A. Asa-Awuku 10.1039/C8CP00075A
- Modeling of hygroscopicity parameter kappa of organic aerosols using quantitative structure-property relationships J. Markelj et al. 10.1007/s10874-016-9347-3
- The effects of morphology, mobility size, and secondary organic aerosol (SOA) material coating on the ice nucleation activity of black carbon in the cirrus regime C. Zhang et al. 10.5194/acp-20-13957-2020
- Water uptake of subpollen aerosol particles: hygroscopic growth, cloud condensation nuclei activation, and liquid–liquid phase separation E. Mikhailov et al. 10.5194/acp-21-6999-2021
- Hygroscopic growth and CCN activity of secondary organic aerosol produced from dark ozonolysis of γ-terpinene H. Bouzidi et al. 10.1016/j.scitotenv.2022.153010
- Long-term (2001–2012) trends of carbonaceous aerosols from a remote island in the western North Pacific: an outflow region of Asian pollutants S. Boreddy et al. 10.5194/acp-18-1291-2018
- Reconsideration of surface tension and phase state effects on cloud condensation nuclei activity based on the atomic force microscopy measurement C. Xiong et al. 10.5194/acp-22-16123-2022
- Hygroscopicity of internally mixed ammonium sulfate and secondary organic aerosol particles formed at low and high relative humidity P. Razafindrambinina et al. 10.1039/D1EA00069A
- Parameterizing cloud condensation nuclei concentrations during HOPE L. Hande et al. 10.5194/acp-16-12059-2016
- On the evolution of sub- and super-saturated water uptake of secondary organic aerosol in chamber experiments from mixed precursors Y. Wang et al. 10.5194/acp-22-4149-2022
- Contrasting Influence of Nitrogen Oxides on the Cloud Condensation Nuclei Activity of Monoterpene‐Derived Secondary Organic Aerosol in Daytime and Nighttime Oxidation C. Zhang et al. 10.1029/2022GL102110
- A review of experimental techniques for aerosol hygroscopicity studies M. Tang et al. 10.5194/acp-19-12631-2019
- Partitioning of secondary organic aerosol onto nanoplastics leading to hygroscopic partially-engulfed particles K. Raincrow et al. 10.1039/D3EA00103B
- Secondary aerosol formation promotes water uptake by organic-rich wildfire haze particles in equatorial Asia J. Chen et al. 10.5194/acp-18-7781-2018
- Modeling the molecular composition of secondary organic aerosol under highly polluted conditions: A case study in the Yangtze River Delta Region in China Q. Huang et al. 10.1016/j.scitotenv.2024.173327
- Environmental conditions regulate the impact of plants on cloud formation D. Zhao et al. 10.1038/ncomms14067
- Review of Smog Chamber Research Trends J. Kim et al. 10.5572/KOSAE.2023.39.5.866
- Dataset on aerosol loading and deposition over Nouakchott-Mauritania M. Emetere & G. Adeyemi 10.1016/j.dib.2018.07.018
- Size‐dependent hygroscopicity parameter (κ) and chemical composition of secondary organic cloud condensation nuclei D. Zhao et al. 10.1002/2015GL066497
- Environmental Data Retrieval and Prediction Using the Auto-regression Moving Average and Polynomial Experimentation M. Emetere 10.1007/s41810-018-0027-3
34 citations as recorded by crossref.
- Liquid–liquid phase separation in particles containing secondary organic material free of inorganic salts M. Song et al. 10.5194/acp-17-11261-2017
- Cloud droplet activation of secondary organic aerosol is mainly controlled by molecular weight, not water solubility J. Wang et al. 10.5194/acp-19-941-2019
- Molecular and spatial distributions of dicarboxylic acids, oxocarboxylic acids, and <i>α</i>-dicarbonyls in marine aerosols from the South China Sea to the eastern Indian Ocean J. Yang et al. 10.5194/acp-20-6841-2020
- Contrasting effects of secondary organic aerosol formations on organic aerosol hygroscopicity Y. Kuang et al. 10.5194/acp-21-10375-2021
- Effect of solubility limitation on hygroscopic growth and cloud drop activation of SOA particles produced from traffic exhausts C. Wittbom et al. 10.1007/s10874-018-9380-5
- Tropical and Boreal Forest – Atmosphere Interactions: A Review P. Artaxo et al. 10.16993/tellusb.34
- Hygroscopicity and CCN potential of DMS-derived aerosol particles B. Rosati et al. 10.5194/acp-22-13449-2022
- The Interplay Between Hydrogen Bonding and Coulombic Forces in Determining the Structure of Sulfuric Acid-Amine Clusters S. Waller et al. 10.1021/acs.jpclett.8b00161
- Impacts of water partitioning and polarity of organic compounds on secondary organic aerosol over eastern China J. Li et al. 10.5194/acp-20-7291-2020
- Measurement report: Distinct size dependence and diurnal variation in organic aerosol hygroscopicity, volatility, and cloud condensation nuclei activity at a rural site in the Pearl River Delta (PRD) region, China M. Cai et al. 10.5194/acp-22-8117-2022
- Hygroscopicity of Secondary Brown Carbon Aerosol from Aqueous Photo-Oxidation of Phenolic Precursors K. Betz et al. 10.1021/acsearthspacechem.2c00132
- Recent advances in understanding secondary organic aerosol: Implications for global climate forcing M. Shrivastava et al. 10.1002/2016RG000540
- Organosulfates in aerosols downwind of an urban region in central Amazon M. Glasius et al. 10.1039/C8EM00413G
- Effects of NO<sub><i>x</i></sub> and SO<sub>2</sub> on the secondary organic aerosol formation from photooxidation of <i>α</i>-pinene and limonene D. Zhao et al. 10.5194/acp-18-1611-2018
- Utilizing an electrical low-pressure impactor to indirectly probe water uptake via particle bounce measurements K. Fischer & G. Petrucci 10.5194/amt-14-7565-2021
- Accounting for Cloud Nucleation Activation Mechanism of Secondary Organic Matter from α-Pinene Oxidation Using Experimentally Retrieved Water Solubility Distributions W. Lee et al. 10.1021/acs.est.3c03039
- Introductory lecture: atmospheric chemistry in the Anthropocene B. Finlayson-Pitts 10.1039/C7FD00161D
- Gas-phase kinetics modifies the CCN activity of a biogenic SOA A. Vizenor & A. Asa-Awuku 10.1039/C8CP00075A
- Modeling of hygroscopicity parameter kappa of organic aerosols using quantitative structure-property relationships J. Markelj et al. 10.1007/s10874-016-9347-3
- The effects of morphology, mobility size, and secondary organic aerosol (SOA) material coating on the ice nucleation activity of black carbon in the cirrus regime C. Zhang et al. 10.5194/acp-20-13957-2020
- Water uptake of subpollen aerosol particles: hygroscopic growth, cloud condensation nuclei activation, and liquid–liquid phase separation E. Mikhailov et al. 10.5194/acp-21-6999-2021
- Hygroscopic growth and CCN activity of secondary organic aerosol produced from dark ozonolysis of γ-terpinene H. Bouzidi et al. 10.1016/j.scitotenv.2022.153010
- Long-term (2001–2012) trends of carbonaceous aerosols from a remote island in the western North Pacific: an outflow region of Asian pollutants S. Boreddy et al. 10.5194/acp-18-1291-2018
- Reconsideration of surface tension and phase state effects on cloud condensation nuclei activity based on the atomic force microscopy measurement C. Xiong et al. 10.5194/acp-22-16123-2022
- Hygroscopicity of internally mixed ammonium sulfate and secondary organic aerosol particles formed at low and high relative humidity P. Razafindrambinina et al. 10.1039/D1EA00069A
- Parameterizing cloud condensation nuclei concentrations during HOPE L. Hande et al. 10.5194/acp-16-12059-2016
- On the evolution of sub- and super-saturated water uptake of secondary organic aerosol in chamber experiments from mixed precursors Y. Wang et al. 10.5194/acp-22-4149-2022
- Contrasting Influence of Nitrogen Oxides on the Cloud Condensation Nuclei Activity of Monoterpene‐Derived Secondary Organic Aerosol in Daytime and Nighttime Oxidation C. Zhang et al. 10.1029/2022GL102110
- A review of experimental techniques for aerosol hygroscopicity studies M. Tang et al. 10.5194/acp-19-12631-2019
- Partitioning of secondary organic aerosol onto nanoplastics leading to hygroscopic partially-engulfed particles K. Raincrow et al. 10.1039/D3EA00103B
- Secondary aerosol formation promotes water uptake by organic-rich wildfire haze particles in equatorial Asia J. Chen et al. 10.5194/acp-18-7781-2018
- Modeling the molecular composition of secondary organic aerosol under highly polluted conditions: A case study in the Yangtze River Delta Region in China Q. Huang et al. 10.1016/j.scitotenv.2024.173327
- Environmental conditions regulate the impact of plants on cloud formation D. Zhao et al. 10.1038/ncomms14067
- Review of Smog Chamber Research Trends J. Kim et al. 10.5572/KOSAE.2023.39.5.866
3 citations as recorded by crossref.
- Dataset on aerosol loading and deposition over Nouakchott-Mauritania M. Emetere & G. Adeyemi 10.1016/j.dib.2018.07.018
- Size‐dependent hygroscopicity parameter (κ) and chemical composition of secondary organic cloud condensation nuclei D. Zhao et al. 10.1002/2015GL066497
- Environmental Data Retrieval and Prediction Using the Auto-regression Moving Average and Polynomial Experimentation M. Emetere 10.1007/s41810-018-0027-3
Saved (final revised paper)
Saved (preprint)
Latest update: 21 Nov 2024
Short summary
This study investigated the cloud droplet activation behavior and hygroscopic growth of mixed anthropogenic and biogenic SOA (ABSOA) compared to pure biogenic SOA (BSOA) and pure anthropogenic SOA (ASOA). Cloud droplet activation behaviors of different types of SOA were similar. In contrast, the hygroscopicity of ASOA was higher than BSOA and ABSOA. ASOA components enhanced the hygroscopicity of the ABSOA. Yet this enhancement cannot be described by a linear mixing of pure SOA systems.
This study investigated the cloud droplet activation behavior and hygroscopic growth of mixed...
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