Articles | Volume 15, issue 13
https://doi.org/10.5194/acp-15-7537-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-15-7537-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
13 Jul 2015
Research article |
| 13 Jul 2015
The role of blowing snow in the activation of bromine over first-year Antarctic sea ice
R. M. Lieb-Lappen
CORRESPONDING AUTHOR
14 Engineering Drive, Thayer School of Engineering, Dartmouth College, Hanover, NH, USA
R. W. Obbard
14 Engineering Drive, Thayer School of Engineering, Dartmouth College, Hanover, NH, USA
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Cited
24 citations as recorded by crossref.
- Fragmentation of wind‐blown snow crystals F. Comola et al. 10.1002/2017GL073039
- Environmental drivers of tropospheric bromine and mercury variability in coastal East Antarctica N. Page et al. 10.1016/j.atmosenv.2024.120918
- Frost flowers and sea-salt aerosols over seasonal sea-ice areas in northwestern Greenland during winter–spring K. Hara et al. 10.5194/acp-17-8577-2017
- Possible role of electric forces in bromine activation during polar boundary layer ozone depletion and aerosol formation events E. Tkachenko 10.1016/j.atmosres.2017.05.012
- Ocean-atmosphere interactions: Different organic components across Pacific and Southern Oceans J. Jang et al. 10.1016/j.scitotenv.2023.162969
- Evaporating brine from frost flowers with electron microscopy and implications for atmospheric chemistry and sea-salt aerosol formation X. Yang et al. 10.5194/acp-17-6291-2017
- Multiyear study of the dependence of sea salt aerosol on wind speed and sea ice conditions in the coastal Arctic N. May et al. 10.1002/2016JD025273
- Spatial Distribution of Atmospheric Mercury Species in the Southern Ocean F. Yue et al. 10.1029/2021JD034651
- Canadian Arctic sea ice reconstructed from bromine in the Greenland NEEM ice core A. Spolaor et al. 10.1038/srep33925
- The importance of blowing snow to halogen-containing aerosol in coastal Antarctica: influence of source region versus wind speed M. Giordano et al. 10.5194/acp-18-16689-2018
- Seasonal variation of tropospheric bromine monoxide over the Rann of Kutch salt marsh seen from space C. Hörmann et al. 10.5194/acp-16-13015-2016
- A network model for characterizing brine channels in sea ice R. Lieblappen et al. 10.5194/tc-12-1013-2018
- Measurements of Tropospheric Bromine Monoxide Over Four Halogen Activation Seasons in the Canadian High Arctic K. Bognar et al. 10.1029/2020JD033015
- Variability and change in the west Antarctic Peninsula marine system: Research priorities and opportunities S. Henley et al. 10.1016/j.pocean.2019.03.003
- Synchrotron X‐ray fluorescence spectroscopy of salts in natural sea ice R. Obbard et al. 10.1002/2016EA000172
- First-year sea ice leads to an increase in dimethyl sulfide-induced particle formation in the Antarctic Peninsula E. Jang et al. 10.1016/j.scitotenv.2021.150002
- Year-long ground-based observations of bromine oxide over Bharati Station, Antarctica S. Wagh et al. 10.1016/j.polar.2023.100977
- First direct observation of sea salt aerosol production from blowing snow above sea ice M. Frey et al. 10.5194/acp-20-2549-2020
- Link Between Arctic Tropospheric BrO Explosion Observed From Space and Sea‐Salt Aerosols From Blowing Snow Investigated Using Ozone Monitoring Instrument BrO Data and GEOS‐5 Data Assimilation System S. Choi et al. 10.1029/2017JD026889
- A modelling study of the atmospheric chemistry of DMS using the global model, STOCHEM-CRI M. Khan et al. 10.1016/j.atmosenv.2015.12.028
- Metrics for interpreting the microstructure of sea ice using X-ray micro-computed tomography R. Lieb-Lappen et al. 10.1016/j.coldregions.2017.03.001
- Year‐round records of sea salt, gaseous, and particulate inorganic bromine in the atmospheric boundary layer at coastal (Dumont d'Urville) and central (Concordia) East Antarctic sites M. Legrand et al. 10.1002/2015JD024066
- Atmospheric sea-salt and halogen cycles in the Antarctic K. Hara et al. 10.1039/D0EM00092B
- Simulating tropospheric BrO in the Arctic using an artificial neural network I. Bougoudis et al. 10.1016/j.atmosenv.2022.119032
24 citations as recorded by crossref.
- Fragmentation of wind‐blown snow crystals F. Comola et al. 10.1002/2017GL073039
- Environmental drivers of tropospheric bromine and mercury variability in coastal East Antarctica N. Page et al. 10.1016/j.atmosenv.2024.120918
- Frost flowers and sea-salt aerosols over seasonal sea-ice areas in northwestern Greenland during winter–spring K. Hara et al. 10.5194/acp-17-8577-2017
- Possible role of electric forces in bromine activation during polar boundary layer ozone depletion and aerosol formation events E. Tkachenko 10.1016/j.atmosres.2017.05.012
- Ocean-atmosphere interactions: Different organic components across Pacific and Southern Oceans J. Jang et al. 10.1016/j.scitotenv.2023.162969
- Evaporating brine from frost flowers with electron microscopy and implications for atmospheric chemistry and sea-salt aerosol formation X. Yang et al. 10.5194/acp-17-6291-2017
- Multiyear study of the dependence of sea salt aerosol on wind speed and sea ice conditions in the coastal Arctic N. May et al. 10.1002/2016JD025273
- Spatial Distribution of Atmospheric Mercury Species in the Southern Ocean F. Yue et al. 10.1029/2021JD034651
- Canadian Arctic sea ice reconstructed from bromine in the Greenland NEEM ice core A. Spolaor et al. 10.1038/srep33925
- The importance of blowing snow to halogen-containing aerosol in coastal Antarctica: influence of source region versus wind speed M. Giordano et al. 10.5194/acp-18-16689-2018
- Seasonal variation of tropospheric bromine monoxide over the Rann of Kutch salt marsh seen from space C. Hörmann et al. 10.5194/acp-16-13015-2016
- A network model for characterizing brine channels in sea ice R. Lieblappen et al. 10.5194/tc-12-1013-2018
- Measurements of Tropospheric Bromine Monoxide Over Four Halogen Activation Seasons in the Canadian High Arctic K. Bognar et al. 10.1029/2020JD033015
- Variability and change in the west Antarctic Peninsula marine system: Research priorities and opportunities S. Henley et al. 10.1016/j.pocean.2019.03.003
- Synchrotron X‐ray fluorescence spectroscopy of salts in natural sea ice R. Obbard et al. 10.1002/2016EA000172
- First-year sea ice leads to an increase in dimethyl sulfide-induced particle formation in the Antarctic Peninsula E. Jang et al. 10.1016/j.scitotenv.2021.150002
- Year-long ground-based observations of bromine oxide over Bharati Station, Antarctica S. Wagh et al. 10.1016/j.polar.2023.100977
- First direct observation of sea salt aerosol production from blowing snow above sea ice M. Frey et al. 10.5194/acp-20-2549-2020
- Link Between Arctic Tropospheric BrO Explosion Observed From Space and Sea‐Salt Aerosols From Blowing Snow Investigated Using Ozone Monitoring Instrument BrO Data and GEOS‐5 Data Assimilation System S. Choi et al. 10.1029/2017JD026889
- A modelling study of the atmospheric chemistry of DMS using the global model, STOCHEM-CRI M. Khan et al. 10.1016/j.atmosenv.2015.12.028
- Metrics for interpreting the microstructure of sea ice using X-ray micro-computed tomography R. Lieb-Lappen et al. 10.1016/j.coldregions.2017.03.001
- Year‐round records of sea salt, gaseous, and particulate inorganic bromine in the atmospheric boundary layer at coastal (Dumont d'Urville) and central (Concordia) East Antarctic sites M. Legrand et al. 10.1002/2015JD024066
- Atmospheric sea-salt and halogen cycles in the Antarctic K. Hara et al. 10.1039/D0EM00092B
- Simulating tropospheric BrO in the Arctic using an artificial neural network I. Bougoudis et al. 10.1016/j.atmosenv.2022.119032
Saved (final revised paper)
Latest update: 19 Nov 2024
Short summary
This work analyzes the chemical composition of blowing snow collected over first-year Antarctic sea ice to assess its role in bromine activation during the polar sunrise. We found lofted snow to be depleted in Br- relative to Cl- by proportionally increasing amounts with height. This is the first study to use field data to substantiate modeling results implicating blowing snow as the location for initial halogen activation. We also found lofted snow to be depleted in SO4 and enriched in NO3.
This work analyzes the chemical composition of blowing snow collected over first-year Antarctic...
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