Articles | Volume 15, issue 13
https://doi.org/10.5194/acp-15-7203-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Special issue:
https://doi.org/10.5194/acp-15-7203-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Experimental investigation of ion–ion recombination under atmospheric conditions
A. Franchin
CORRESPONDING AUTHOR
Department of Physics, P.O. Box 64, 00014 University of Helsinki, Helsinki, Finland
S. Ehrhart
CERN, 1211 Geneva, Switzerland
Institute for Atmospheric and Environmental Sciences, Goethe University Frankfurt, Altenhöferallee 1, 60438 Frankfurt am Main, Germany
J. Leppä
Finnish Meteorological Institute, Atmospheric Composition Research, P.O. Box 503, 00101 Helsinki, Finland
California Institute of Technology, Department of Chemical Engineering, 1200 E. California Blvd., Mail Code 101-20, Pasadena, CA 91125, US
T. Nieminen
Department of Physics, P.O. Box 64, 00014 University of Helsinki, Helsinki, Finland
Helsinki Institute of Physics, Helsinki, Finland
Department of Physics and Atmospheric Science, Dalhousie University, Halifax, B3H 3J5, Canada
Environment Canada, Downsview, Toronto, M3H 5T4, Canada
S. Schobesberger
Department of Physics, P.O. Box 64, 00014 University of Helsinki, Helsinki, Finland
D. Wimmer
Department of Physics, P.O. Box 64, 00014 University of Helsinki, Helsinki, Finland
J. Duplissy
Helsinki Institute of Physics, Helsinki, Finland
F. Riccobono
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232 Villigen, Switzerland
E. M. Dunne
Finnish Meteorological Institute, Kuopio Unit, P.O. Box 1627, 70211 Kuopio, Finland
L. Rondo
Institute for Atmospheric and Environmental Sciences, Goethe University Frankfurt, Altenhöferallee 1, 60438 Frankfurt am Main, Germany
A. Downard
California Institute of Technology, Department of Chemical Engineering, 1200 E. California Blvd., Mail Code 101-20, Pasadena, CA 91125, US
F. Bianchi
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232 Villigen, Switzerland
Institute for Atmospheric and Climate Science, ETH Zurich, 8092 Zurich, Switzerland
University of Vienna, Universitätsring 1, 1010 Vienna, Austria
G. Tsagkogeorgas
Leibniz Institute for Tropospheric Research, Permoserstr. 15, 04318 Leipzig, Germany
K. Lehtipalo
Department of Physics, P.O. Box 64, 00014 University of Helsinki, Helsinki, Finland
H. E. Manninen
Department of Physics, P.O. Box 64, 00014 University of Helsinki, Helsinki, Finland
J. Almeida
CERN, 1211 Geneva, Switzerland
A. Amorim
CENTRA-SIM, F.C.U. Lisboa and U. Beira Interior, Portugal
P. E. Wagner
University of Vienna, Universitätsring 1, 1010 Vienna, Austria
A. Hansel
Ionicon Analytik GmbH and University of Innsbruck, Institute for Ion and Applied Physics, 6020 Innsbruck, Austria
J. Kirkby
CERN, 1211 Geneva, Switzerland
Institute for Atmospheric and Environmental Sciences, Goethe University Frankfurt, Altenhöferallee 1, 60438 Frankfurt am Main, Germany
A. Kürten
Institute for Atmospheric and Environmental Sciences, Goethe University Frankfurt, Altenhöferallee 1, 60438 Frankfurt am Main, Germany
N. M. Donahue
Carnegie Mellon University, Center for Atmospheric Particle Studies, 5000 Forbes Avenue, Pittsburgh, PA 15213, USA
V. Makhmutov
Lebedev Physical Institute, Leninsky Prospect 53, 119991 Moscow, Russia
S. Mathot
CERN, 1211 Geneva, Switzerland
A. Metzger
Ionicon Analytik GmbH and University of Innsbruck, Institute for Ion and Applied Physics, 6020 Innsbruck, Austria
T. Petäjä
Department of Physics, P.O. Box 64, 00014 University of Helsinki, Helsinki, Finland
R. Schnitzhofer
Ionicon Analytik GmbH and University of Innsbruck, Institute for Ion and Applied Physics, 6020 Innsbruck, Austria
M. Sipilä
Department of Physics, P.O. Box 64, 00014 University of Helsinki, Helsinki, Finland
Y. Stozhkov
Lebedev Physical Institute, Leninsky Prospect 53, 119991 Moscow, Russia
CENTRA-SIM, F.C.U. Lisboa and U. Beira Interior, Portugal
V.-M. Kerminen
Department of Physics, P.O. Box 64, 00014 University of Helsinki, Helsinki, Finland
Finnish Meteorological Institute, Atmospheric Composition Research, P.O. Box 503, 00101 Helsinki, Finland
K. Carslaw
School of Earth and Environment, University of Leeds, LS2 9JT, Leeds, UK
J. Curtius
Institute for Atmospheric and Environmental Sciences, Goethe University Frankfurt, Altenhöferallee 1, 60438 Frankfurt am Main, Germany
U. Baltensperger
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232 Villigen, Switzerland
M. Kulmala
Department of Physics, P.O. Box 64, 00014 University of Helsinki, Helsinki, Finland
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- Final revised paper (published on 01 Jul 2015)
- Preprint (discussion started on 09 Feb 2015)
Interactive discussion
Status: closed
Status: closed
AC: Author comment | RC: Referee comment | SC: Short comment | EC: Editor comment
- Printer-friendly version
- Supplement
-
RC C829: 'Revision', Anonymous Referee #1, 16 Mar 2015
- AC C2638: 'Answer to Referee#1', A. Franchin, 15 May 2015
-
RC C1033: 'Review comments', Anonymous Referee #2, 24 Mar 2015
- AC C2639: 'Answer to Referee#2', A. Franchin, 15 May 2015
Peer-review completion
AR: Author's response | RR: Referee report | ED: Editor decision
AR by A. Franchin on behalf of the Authors (18 May 2015)
Author's response
ED: Publish as is (26 May 2015) by John H. Seinfeld
AR by A. Franchin on behalf of the Authors (26 May 2015)
Manuscript
Short summary
The ion-ion recombination coefficient was measured at different temperatures, relative humidities and concentrations of ozone and sulfur dioxide. The experiments were carried out using the CLOUD chamber at CERN.
We observed a strong dependency on temperature and on relative humidity, which has not been reported previously. No dependency of the ion-ion recombination coefficient on ozone concentration was observed and a weak variation with sulfur dioxide concentration was also observed.
The ion-ion recombination coefficient was measured at different temperatures, relative...
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